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Sato, Tomonori; Hata, Kuniki; Kaji, Yoshiyuki; Ueno, Fumiyoshi; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; Abe, Hiroshi*; Akiyama, Eiji*; et al.
JAEA-Review 2021-001, 123 Pages, 2021/06
JAEA-Review-2021-001.pdf:10.33MB
In the implement of the decommissioning of Fukushima Daiichi Nuclear Power Station (1F), there are many problems to be solved. Specially, the mitigation of the aging degradation by the corrosion of the structural materials is important to implement the decommissioning safely and continuously. However, there are limited data for the environmental factors of corrosion in 1F, and the condition of 1F is continuously changing. So, the literature data for the water radiolysis and the corrosion under irradiation are listed as the database of corrosion under irradiation in this report. And the new obtained radiolysis and corrosion data, which have not been reported in the literature and will be required in the decommissioning of 1F, are reported.
Omori, Atsushi*; Akiyama, Eiji*; Abe, Hiroshi*; Hata, Kuniki; Sato, Tomonori; Kaji, Yoshiyuki; Inoue, Hiroyuki*; Taguchi, Mitsumasa*; Seito, Hajime*; Tada, Eiji*; et al.
Zairyo To Kankyo, 69(4), p.107 - 111, 2020/04
To evaluate the effect of oxidants, which are formed by radiolysis of water under gamma ray irradiation, on the corrosion of a carbon steel in humid environment, ozone was introduced as a model oxidant in to humidity-controlled air at 50
C in a thermo-hygrostat chamber. Corrosion monitoring was performed by using an Atmospheric Corrosion Monitor-type (ACM) sensor consisting of a carbon steel anode and an Ag cathode. The output current of the ACM sensor was increased with the increase in relative humidity and it was obviously increased with the increase in the introduced ozone concentration at each relative humidity. The results indicate that ozone accelerates the corrosion of the carbon steel. The effect of ozone on the corrosion acceleration is attributed to the fast reduction reaction and fast dissolution reaction in to water compared to that of oxygen.
Hata, Kuniki; Inoue, Hiroyuki*
Journal of Nuclear Science and Technology, 56(9-10), p.842 - 850, 2019/09
Times Cited Count：1 Percentile：11.15(Nuclear Science & Technology)To investigate the effect of dissolved species from steels on the radiolysis processes of Cl
, radiolysis simulations of solutions containing both Cl and Fe
were carried out. The results showed that the generation of radiolytic products (H
O, O and H) increased mainly by the addition of Fe, and a drop in the pH was caused by the hydrolysis of Fe
. This pH drop enhanced the reactivity of Cl with 
OH, which induced additional generation of HO and O. These results show that low concentrations of Cl (1 
10
mol/dm
= 35ppm) in the presence of Fe could influence the generation of HO and O during water radiolysis. However, it is considered that these effects of Fe and low concentration of Cl on water radiolysis are less important for corrosion of steels due to the low concentrations of HO and O generated. The other process, such as dissolution of iron enhanced by FeOOH, might predominantly induce corrosion under the conditions of solutions with low concentrations of HO and O.
and Br and its effect on corrosion of a low-alloy steelHata, Kuniki; Inoue, Hiroyuki*; Kojima, Takao*; Kasahara, Shigeki; Hanawa, Satoshi; Ueno, Fumiyoshi; Tsukada, Takashi; Iwase, Akihiro*
Proceedings of Symposium on Water Chemistry and Corrosion in Nuclear Power Plants in Asia 2017 (AWC 2017) (USB Flash Drive), p.304 - 314, 2017/09
A model simulation of 
radiolysis of mixed solutions of NaCl and NaBr was carried out. The simulation result agreed well with the experimental result, and Br played an important role in determining the amounts of products from water radiolysis. The simulation result also showed that, in highly pure NaCl solutions, the steady-state concentration of a radolytic product, HO, was mainly controlled by three reactions (Cl + OH 
ClOH
, ClOH Cl + OH, and ClOH + H
Cl + HO), which indicated that accurate evaluation of the rate constants of these reactions was very important in improving the radiolysis simulation of solutions containing Cl. An immersion test using a low-alloy steel, SQV2A, in the mixed solutions was also carried out under irradiation. The corrosion rate increased or decreased depending on the pH or the concentrations of the halide ions in a similar way to the change in concentration of HO produced from water radiolysis, which is affected by the presence of Cl and Br. However, at high pH values (
12), the corrosion rate was almost zero even though the concentration of HO was high. This could be attributed to enhancement of the passivity of test specimens at higher pH values.
irradiationYukawa, Takuji*; Inoue, Hiroyuki*; Kojima, Takao*; Iwase, Akihiro*; Taniguchi, Naoki; Tachikawa, Hirokazu*
Zairyo To Kankyo 2016 Koenshu (CD-ROM), p.359 - 362, 2016/05
The immersion tests of pure titanium were carried out in aqueous solution containing carbonate/bicarbonate with 50 mM-chloride ion under gamma irradiation. The effect of pH on general corrosion rate of titanium were studied. The experimental results showed that the concentration of hydrogen preoxide was increased with pH, and the corrosion rate increased with the hydrogen preoxide concentration. The corrosion rate in pH12 and 13 were 5 to10 times larger than those under unirradiated conditions.
radiolysis of sodium chloride solutions containing a small amount of bromide ionHata, Kuniki; Inoue, Hiroyuki*; Kojima, Takao*; Iwase, Akihiro*; Kasahara, Shigeki; Hanawa, Satoshi; Ueno, Fumiyoshi; Tsukada, Takashi
Nuclear Technology, 193(3), p.434 - 443, 2016/03
Times Cited Count：13 Percentile：77.16(Nuclear Science & Technology) ion beams for ITER NB acceleratorUmeda, Naotaka; Kashiwagi, Mieko; Taniguchi, Masaki; Tobari, Hiroyuki; Watanabe, Kazuhiro; Dairaku, Masayuki; Yamanaka, Haruhiko; Inoue, Takashi; Kojima, Atsushi; Hanada, Masaya
Review of Scientific Instruments, 85(2), p.02B304_1 - 02B304_3, 2014/02
Times Cited Count：12 Percentile：48.5(Instruments & Instrumentation)In order to realize neutral beam systems in ITER whose target is to produce D ion beam of 1 MeV, 200 A/m
during 3600s, the electrostatic five-stages negative ion accelerator has been developed at JAEA. To extend pulse length, heat load of the acceleration grids was reduced by controlling the ion beam trajectory. Namely, the beam deflection due to the residual magnetic filter in the accelerator was suppressed with the newly developed extractor with a 0.5 mm off-set aperture displacement. The use of new extractor improved the deflection angle from 6 mrad to 1 mrad, resulting in the reduction of direct interception of negative ions from 23% to 15% of the total acceleration power, respectively. As a result, the pulse length of 130 A/m, 881 keV H ion beam has been successfully extended from a previous value of 0.4s to 8.7s.
Kashiwagi, Mieko; Umeda, Naotaka; Tobari, Hiroyuki; Kojima, Atsushi; Yoshida, Masafumi; Taniguchi, Masaki; Dairaku, Masayuki; Maejima, Tetsuya; Yamanaka, Haruhiko; Watanabe, Kazuhiro; et al.
Review of Scientific Instruments, 85(2), p.02B320_1 - 02B320_3, 2014/02
Times Cited Count：29 Percentile：75.28(Instruments & Instrumentation)The negative ion extractor for high power and long-pulse operations is newly developed toward the neutral beam injector (NBI) for heating & current drive of future fusion machines such as ITER, JT-60 Super Advanced (SA) and DEMO reactor. The satisfactory cooling capability is designed in the thermal analysis. A negative ion production and a suppression of electrons are experimentally validated for this new extractor. As the results, the negative ion current shows increases by a factor of 1.3 with suppressing the electron current. The beam divergence angle is also maintained small enough, 4 mrad.
Tobari, Hiroyuki; Inoue, Takashi; Taniguchi, Masaki; Kashiwagi, Mieko; Umeda, Naotaka; Dairaku, Masayuki; Yamanaka, Haruhiko; Watanabe, Kazuhiro; Sakamoto, Keishi; Kuriyama, Masaaki*; et al.
Fusion Engineering and Design, 88(6-8), p.975 - 979, 2013/10
Times Cited Count：1 Percentile：10.69(Nuclear Science & Technology)The HV bushing, one of the ITER NB components, which is to be procured by JADA, is a multi-conductor feed through composed of five-stage double-layered insulator columns with large brazed ceramic ring and fiber reinforced plastic (FRP) ring. The HV bushing is a bulk head between insulation gas at 0.6 MPa and vacuum. The FRP ring is required to sustain the pressure load, seismic load and dead weight. Brazing area of the ceramic ring with Kovar is required to maintain vacuum leak tightness and pressure tightness against the air filled at 0.6 MPa. To design the HV bushing satisfying the safety factor of 
3.5, mechanical analyses were carried out. As for the FRP ring, it was confirmed that isotropic fiber cloth FRP rings should be used for sufficient strength against shear stress. Also, shape and fixation area of the Kovar sleeve were modified to lower the stress at the joint area. As a result, a design of the insulator for the HV bushing was established satisfying the requirement.
Kojima, Atsushi; Hanada, Masaya; Yoshida, Masafumi; Inoue, Takashi; Watanabe, Kazuhiro; Taniguchi, Masaki; Kashiwagi, Mieko; Umeda, Naotaka; Tobari, Hiroyuki; Grisham, L. R.*; et al.
Fusion Engineering and Design, 88(6-8), p.918 - 921, 2013/10
Times Cited Count：6 Percentile：44.02(Nuclear Science & Technology)In this paper, the recent activities are reported toward demonstration of the long pulse production. As for the improvement of uniform beam current profile, a symmetric magnetic field configuration for the source plasma production, a so-called tent-shaped filter, was found to be effective to improve the uniformity of the beam current profile. A similar configuration is applied to the JT-60 negative ion source whose plasma size is 1220 mm 564 mm. An estimation from trajectory calculations of primary electrons with the symmetric magnetic field configuration showed that the primary electrons were distributed uniformly in a longitudinal direction. As for the temperature control of the plasma grid, a prototype of the grid with cooling/heating by circulating a high-temperature fluorinated fluid has been developed. This grid was found to have a capability to control the temperature with a time constant of 10 s by considering the physical properties of the fluid.
Kashiwagi, Mieko; Taniguchi, Masaki; Umeda, Naotaka; Dairaku, Masayuki; Tobari, Hiroyuki; Yamanaka, Haruhiko; Watanabe, Kazuhiro; Inoue, Takashi; DeEsch, H. P. L.*; Grisham, L. R.*; et al.
AIP Conference Proceedings 1515, p.227 - 236, 2013/02
Times Cited Count：12 Percentile：96.1(Physics, Applied)In a five stage multi-aperture multi-grid (MAMuG) accelerator for the ITER neutral beam injector (NBI), 1 MeV, 40 A D
ion beam is required for 1 hour. However, beamlets are deflected due to (1) magnetic field for electron suppression and (2) space charge repulsion between beamlets, and consequently, cause excess grid heat load. A three dimensional beam analysis has been carried out to compensate the beamlet deflections. This paper shows that the beamlet deflections due to (1) and (2) are compensated by an aperture offset of only 0.6 mm applied to the aperture of 17 mm in diameter in the extractor and by a metal bar attached around aperture area beneath the extractor, respectively. When the metal bar is increased to 3 mm in thickness and installed 30 mm away from the aperture area, the beamlet is steered gently by the weaker electric field distortion. The beam optics was confirmed not deteriorated by those compensations. The presentation also discusses application of these compensation techniques to the ITER design.
Shibata, Takanori; Terasaki, Ryo*; Kashiwagi, Mieko; Inoue, Takashi; Dairaku, Masayuki; Taniguchi, Masaki; Tobari, Hiroyuki; Umeda, Naotaka; Watanabe, Kazuhiro; Sakamoto, Keishi; et al.
AIP Conference Proceedings 1515, p.177 - 186, 2013/02
Times Cited Count：8 Percentile：92.97(Physics, Applied)In the neutral beam injector in JT-60SA, one of issues is that negative ion beam is partially intercepted at acceleration grids due to a spatial non-uniformity of negative ion production on large extraction area (0.90.45m). Previous experiments showed that fast electrons emitted from filament cathodes are transported in a longitudinal direction by 
drift and the spatial distribution of electron temperature (
) strongly relates with the non-uniformity. In this study, a three-dimensional electron transport analysis has been developed. Electron temperature in the analysis agreed well with measurements in JAEA 10A ion source. This study clarified that the bias of distribution are caused by the following reasons; (1) fast electrons drifted in the longitudinal direction survives near the end wall with energy up to 
= 25-60 eV and (2) they produces thermal electrons by collision with plasma particles there.
H ion beam acceleration at JAEA for the ITER neutral beam injectorTobari, Hiroyuki; Taniguchi, Masaki; Kashiwagi, Mieko; Dairaku, Masayuki; Umeda, Naotaka; Yamanaka, Haruhiko; Tsuchida, Kazuki; Takemoto, Jumpei; Watanabe, Kazuhiro; Inoue, Takashi; et al.
Plasma Science and Technology, 15(2), p.179 - 183, 2013/02
Times Cited Count：1 Percentile：4.39(Physics, Fluids & Plasmas)Vacuum insulation is a common issue for the accelerator and the HV bushing for the ITER NBI. The HV bushing has five-stage structure and each stage consists of double-layered insulators. Hence, several triple points exist around the insulators. To reduce electric field at those points simultaneously, three types of stress ring were developed. In voltage holding test of a full-scale mockup equipped with those stress rings, 120% of rated voltage was sustained and the voltage holding capability required in ITER was verified. In the MeV accelerator, voltage holding capability was not sufficient due to breakdown triggered by electric field concentration at edge and corner on grid components. By extending gap length, 1 MV was sustained in vacuum. Furthermore, with new accelerator grids which compensates beam deflection due to magnetic field and space charge repulsion between beamlets, 980 keV, 185 A/m H ion beam acceleration was demonstrated, which was close to ITER requirement.
Kojima, Atsushi; Hanada, Masaya; Hilmi, A.*; Inoue, Takashi; Watanabe, Kazuhiro; Taniguchi, Masaki; Kashiwagi, Mieko; Umeda, Naotaka; Tobari, Hiroyuki; Kobayashi, Shinichi*; et al.
Review of Scientific Instruments, 83(2), p.02B117_1 - 02B117_5, 2012/02
Times Cited Count：17 Percentile：60.55(Instruments & Instrumentation)Production of 500 keV, 3 A beams has been successfully achieved in the JT-60 negative by overcoming the low voltage holding of the accelerator. Toward the design of next ion source, database for the voltage holding capability based on experimental results is required and obtained. As a result, the voltage holding capability was found to vary with 67 N power of -0.15 and with 31.7 S power of -0.125 where N is the aperture number and S is the anode surface area. When N = 1100 and S = 2 m are applied to the design of JT-60SA ion source, the factors C are estimated to be 23 and 29, respectively. Therefore, the influence of the local electric field around the apertures is stronger than that of the surface area.
Taniguchi, Masaki; Kashiwagi, Mieko; Umeda, Naotaka; Dairaku, Masayuki; Takemoto, Jumpei; Tobari, Hiroyuki; Tsuchida, Kazuki; Yamanaka, Haruhiko; Watanabe, Kazuhiro; Kojima, Atsushi; et al.
Review of Scientific Instruments, 83(2), p.02B121_1 - 02B121_3, 2012/02
Times Cited Count：11 Percentile：46.97(Instruments & Instrumentation)JAEA has developed the MeV accelerator to demonstrate 1 MeV, 200 A/m H ion beam acceleration required for ITER NBI. A key to realize such a high power accelerator is improvement of voltage holding capability. Based on detailed investigation of the voltage holding characteristics, MeV accelerator was modified to reduce electric field concentration by extending gaps between the grid supports and increasing curvature radiuses at the support corners. After the modifications, accelerator succeeded in sustaining -1 MV in vacuum without beam acceleration. Moreover, beam deflection due to the magnetic field for electron suppression and space charge repulsion was compensated by aperture displacement technique. As the result, beam deflection was compensated and voltage holding during the beam acceleration was improved. Beam parameter of the MeV accelerator was increased to 980 keV, 185 A/m, which is close to the requirement of ITER accelerator.
Shibata, Takanori; Koga, Shojiro*; Terasaki, Ryo*; Inoue, Takashi; Dairaku, Masayuki; Kashiwagi, Mieko; Taniguchi, Masaki; Tobari, Hiroyuki; Tsuchida, Kazuki; Umeda, Naotaka; et al.
Review of Scientific Instruments, 83(2), p.02A719_1 - 02A719_3, 2012/02
Times Cited Count：2 Percentile：12.31(Instruments & Instrumentation)In the NBI for large fusion devices, production of uniform negative ion beam is one of important issues. A physical model is proposed to understand the non-uniformity. It has been qualitatively shown that the non-uniform beam intensity is due to the following process; (1) formation of non-uniform EEDF, (2) localized production of hydrogen atoms/ions (H
/H
) due to (1), (3) non-uniform flux of H/H to the PG and (4) localized surface production of negative ions. However, in the past studies, the EEDF was assumed as two temperature Maxwellian distribution from measurements. Thus effects of high energy electrons are not taken into account precisely. In the present research, local EEDF is calculated by the 3D Monte-Carlo kinetic model which takes into account the spatial and magnetic configurations of the real negative ion source. The numerical result show that high energy component of the EEDF enhances the spatial non-uniformity in the production rate of H/H.
Kashiwagi, Mieko; Taniguchi, Masaki; Umeda, Naotaka; DeEsch, H. P. L.*; Grisham, L. R.*; Boilson, D.*; Hemsworth, R. S.*; Tanaka, Masanobu*; Tobari, Hiroyuki; Watanabe, Kazuhiro; et al.
Review of Scientific Instruments, 83(2), p.02B119_1 - 02B119_3, 2012/02
Times Cited Count：11 Percentile：46.97(Instruments & Instrumentation)In a multi-aperture multi-grid (MAMuG) accelerator of the ITER neutral beam injector (NBI), 1 MeV, 40 A D ion beam is required for 3600 s. Suppression of grid power loading by the direct interception of deflected beamlets is one of the critical issues to realize this accelerator. The beamlets are deflected due to space charge repulsion among beamlets/beam groups and magnetic field. Moreover, the beamlet deflection is influenced by electric field distortion generated by grid supports. To examine such complicated beamlet deflections and design the compensating methods, a three-dimensional beam analysis has been applied to the ITER accelerator. As the simulation model, a 1/4 accelerator model including step/edge of the grid supports is constructed. As results, compensation methods of the beamlet deflection, that it, a metal bar of 1 mm thick around the aperture area, and an aperture offset of 1 mm, were designed.
Jeong, S. H.*; Chang, D. H.*; Kim, T. S.*; In, S. R.*; Lee, K. W.*; Jin, J. T.*; Chang, D. S.*; Oh, B. H.*; Bae, Y. S.*; Kim, J. S.*; et al.
Review of Scientific Instruments, 83(2), p.02B102_1 - 02B102_3, 2012/02
Times Cited Count：22 Percentile：68.03(Instruments & Instrumentation)The first NB (neutral beam) injection system of the KSTAR tokamak was partially completed in 2010 with only 1/3 of its full design capability, and NB heating experiments were carried out during the 2010 KSTAR operation campaign. The ion source is composed of a JAEA bucket plasma generator and a KAERI large multi-aperture accelerator assembly. Before the beam injection experiments, characteristics of the ion source were investigated. A minimum beam divergence angle was 0.8 . The ion species ratio was D:D:D
=75:20:5. The arc efficiency is more than 1.0 A/kW. In the 2010 KSTAR campaign, the deuterium NB power of 0.7-1.5 MW was successfully injected into the KSTAR plasma with the beam energy of 70-90 keV. L-H transitions were observed within a wide range of beam powers relative to a threshold value. In every deuterium NB injection, a burst of D-D neutrons was recorded, and increases in the ion temperature and the plasma stored energy were found.
Honda, Akira; Masuda, Kaoru*; Tateishi, Tsuyoshi*; Kato, Osamu*; Inoue, Hiroyuki*
Zairyo To Kankyo, 60(12), p.541 - 552, 2011/12
Immersion tests and rest potential measurements under hyper-alkaline and high sodium nitrate concentrations were conducted to elucidate and improve model predictions of chemical interactions between carbon steel and nitrate ion in high concentrations of nitrate salt. The modified model can estimate the tendency of time dependent variation of chemical species and of rest potentials.
Hanada, Masaya; Kojima, Atsushi; Tanaka, Yutaka; Inoue, Takashi; Watanabe, Kazuhiro; Taniguchi, Masaki; Kashiwagi, Mieko; Tobari, Hiroyuki; Umeda, Naotaka; Akino, Noboru; et al.
Fusion Engineering and Design, 86(6-8), p.835 - 838, 2011/10
Times Cited Count：13 Percentile：69.64(Nuclear Science & Technology)Neutral beam (NB) injectors for JT-60 Super Advanced (JT-60SA) have been designed and developed. Twelve positive-ion-based and one negative-ion-based NB injectors are allocated to inject 30 MW D
beams in total for 100 s. Each of the positive-ion-based NB injector is designed to inject 1.7 MW for 100s at 85 keV. A part of the power supplies and magnetic shield utilized on JT-60U are upgraded and reused on JT-60SA. To realize the negative-ion-based NB injector for JT-60SA where the injection of 500 keV, 10 MW D beams for 100s is required, R&Ds of the negative ion source have been carried out. High-energy negative ion beams of 490-500 keV have been successfully produced at a beam current of 1-2.8 A through 20% of the total ion extraction area, by improving voltage holding capability of the ion source. This is the first demonstration of a high-current negative ion acceleration of 1 A to 500 keV. The design of the power supplies and the beamline is also in progress. The procurement of the acceleration power supply starts in 2010.
