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JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2022

Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Koike, Yuko; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; Nagai, Shinji; et al.

JAEA-Review 2023-046, 164 Pages, 2024/03

JAEA-Review-2023-046.pdf:4.2MB

The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2022 to March 2023 and the results of dose calculations for the surrounding public due to the release of radioactive materials into the atmosphere and ocean. In the results of the above environmental radiation monitoring, many items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.

Journal Articles

Development of wide range photon detection system for muonic X-ray spectroscopy

Mizuno, Rurie*; Niikura, Megumi*; Saito, Takeshi*; Matsuzaki, Teiichiro*; Sakurai, Hiroyoshi*; Amato, A.*; Asari, Shunsuke*; Biswas, S.*; Chiu, I.-H. ; Gianluca, J.*; et al.

Nuclear Instruments and Methods in Physics Research A, 1060, p.169029_1 - 169029_14, 2024/03

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

Journal Articles

Sequential loss-on-ignition as a simple method for evaluating the stability of soil organic matter under actual environmental conditions

Sato, Yuhi*; Ishizuka, Shigehiro*; Hiradate, Shuntaro*; Atarashi-Andoh, Mariko; Nagano, Hirohiko*; Koarashi, Jun

Environmental Research, 239(Part 1), p.117224_1 - 117224_9, 2023/12

 Times Cited Count:0 Percentile:0(Environmental Sciences)

The stability of soil organic matter (SOM) is important for improving our understanding of the global carbon cycle and ongoing climate change. This study examined the applicability of loss-on-ignition of soil with a stepwise increase in temperature (SIT-LOI) to evaluate the stability of the SOM using soil samples from Japan having different organic matter (OM) and mineral contents and different mean residence times (MRTs), estimated from radiocarbon analysis, for SOM. As the result of this examination, SIT-LOI data was strongly correlated with MRTs. This clearly suggests that SIT-LOI can be an indicator evaluating the stability of SOM in actual environments.

Journal Articles

Study on simulation code for transverse instabilities for the J-PARC MR

Yoshimura, Nobuyuki*; Toyama, Takeshi*; Shobuda, Yoshihiro; Nakamura, Takeshi*; Omi, Kazuhito*; Kobayashi, Aine*; Okada, Masashi*; Sato, Yoichi*; Nakaya, Tsuyoshi*

Proceedings of 20th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.260 - 264, 2023/11

The J-PARC main ring (MR) will be increased to 1.3 MW. To cope with the increase in beam intensity, the intra-bunch feedback system (IBFB) needs to be upgraded to handle higher frequencies up to about 200 MHz. To evaluate the performance and understand the optimal parameters after this upgrade, we are developing a particle tracking simulation that includes the necessary components. The recoherence period induced by chromaticity between tracking simulations and experiments are compared and it cannot be discribed by the simple simulations, and we investigate what mechanisms explain this result. The shift of synchrotron tune caused by longitudinal wakes using tracking simulations are calculated and it find that introducing the effect of longitudinal wakes only does not explain the recoherence period in the experimental results.

Journal Articles

Update of Bragg edge analysis software "GUI-RITS"

Oikawa, Kenichi; Sato, Hirotaka*; Watanabe, Kenichi*; Su, Y. H.; Shinohara, Takenao; Kai, Tetsuya; Kiyanagi, Yoshiaki*; Hasemi, Hiroyuki

Journal of Physics; Conference Series, 2605, p.012013_1 - 012013_6, 2023/10

Journal Articles

Effect of decay heat on pyrochemical reprocessing of minor actinide transmutation nitride fuels

Hayashi, Hirokazu; Tsubata, Yasuhiro; Sato, Takumi

Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 22(3), p.97 - 107, 2023/08

The Japan Atomic Energy Agency has chosen nitride fuel as the first candidate for the transmutation of long-lived minor actinides (MA) using accelerator-driven systems (ADS). The pyrochemical method has been considered for reprocessing spent MA nitride fuels, because their decay heat should be very large for aqueous reprocessing. This study was conducted to investigate the effect of decay heat on the pyrochemical reprocessing of MA nitride fuels. On the basis of the estimated decay heats and the temperature limits of the materials that are to be handled in pyrochemical reprocessing, quantities adequate for handling in argon gas atmosphere were evaluated. From these considerations, we proposed that an electrorefiner with a diameter of 26 cm comprising 12 cadmium (Cd) cathodes with a diameter of 4 cm is suitable. On the basis of the size of the electrorefiner, the number necessary to reprocess spent MA fuels from 1 ADS in 200 days was evaluated to be 25. Furthermore, the amount of Cd-actinides (An) alloy to produce An nitrides by the nitridation-distillation combined reaction process was proposed to be about one-quarter that of Cd-An cathode material. The evaluated sizes and required numbers of equipment support the feasibility of pyrochemical reprocessing for MA nitride fuels.

Journal Articles

Improvement in the elution performance of an N,N,N',N-tetraoctyl diglycolamide impregnated extraction chromatography adsorbent using neodymium via micro-particle-induced X-ray emission analysis

Takahatake, Yoko; Watanabe, So; Arai, Tsuyoshi*; Sato, Takahiro*; Shibata, Atsuhiro

Applied Radiation and Isotopes, 196, p.110783_1 - 110783_5, 2023/06

 Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)

Journal Articles

Comprehensive analysis and evaluation of Fukushima Daiichi Nuclear Power Station Unit 3

Yamashita, Takuya; Honda, Takeshi*; Mizokami, Masato*; Nozaki, Kenichiro*; Suzuki, Hiroyuki*; Pellegrini, M.*; Sakai, Takeshi*; Sato, Ikken; Mizokami, Shinya*

Nuclear Technology, 209(6), p.902 - 927, 2023/06

 Times Cited Count:2 Percentile:90.12(Nuclear Science & Technology)

Journal Articles

Temperature-variable apparatus for measuring Barnett field

Umeda, Maki; Chudo, Hiroyuki; Imai, Masaki; Sato, Nana; Saito, Eiji

Review of Scientific Instruments, 94(6), p.063906_1 - 063906_8, 2023/06

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

Journal Articles

Validation of evaluation model for analysis of steam reformer in HTGR hydrogen production plant

Ishii, Katsunori; Aoki, Takeshi; Isaka, Kazuyoshi; Noguchi, Hiroki; Shimizu, Atsushi; Sato, Hiroyuki

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 9 Pages, 2023/05

Journal Articles

Development of safety design philosophy of HTTR-Heat Application Test Facility

Aoki, Takeshi; Shimizu, Atsushi; Noguchi, Hiroki; Kurahayashi, Kaoru; Yasuda, Takanori; Nomoto, Yasunobu; Iigaki, Kazuhiko; Sato, Hiroyuki; Sakaba, Nariaki

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 9 Pages, 2023/05

The safety design philosophy is developed for the HTTR (High Temperature Engineering Test Reactor) heat application test facility connecting high temperature gas-cooled reactor (HTGR) and the hydrogen production plant. The philosophy was proposed to apply proven conventional chemical plant standards to the hydrogen production facility for ensuring public safety against anticipated disasters caused by high pressure and combustible gases. The present study also proposed the safety design philosophy to meet specific safety requirements identified to the nuclear facilities with coupling to the hydrogen production facility such as measures to ensure a capability of normal operation of the nuclear facility against a fire and/or explosion of leaked combustible material, and fluctuation of amount of heat removal occurred in the hydrogen production plant. The safety design philosophy will be utilized to establish its basic and detailed designs of the HTTR-heat application test facility.

Journal Articles

Development plan for coupling technology between high temperature gas-cooled reactor HTTR and hydrogen production facility, 1; Overview of the HTTR heat application test plan to establish high safety coupling technology

Nomoto, Yasunobu; Mizuta, Naoki; Morita, Keisuke; Aoki, Takeshi; Okita, Shoichiro; Ishii, Katsunori; Kurahayashi, Kaoru; Yasuda, Takanori; Tanaka, Masato; Isaka, Kazuyoshi; et al.

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 7 Pages, 2023/05

Journal Articles

Development plan for coupling technology between high temperature gas-cooled reactor HTTR and Hydrogen Production Facility, 2; Development plan for coupling equipment between HTTR and Hydrogen Production Facility

Mizuta, Naoki; Morita, Keisuke; Aoki, Takeshi; Okita, Shoichiro; Ishii, Katsunori; Kurahayashi, Kaoru; Yasuda, Takanori; Tanaka, Masato; Isaka, Kazuyoshi; Noguchi, Hiroki; et al.

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 6 Pages, 2023/05

Journal Articles

Multiple mechanisms in proton-induced nucleon removal at $$sim$$100 MeV/nucleon

Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G$'o$mez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.

Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04

 Times Cited Count:5 Percentile:92.42(Physics, Multidisciplinary)

We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient $$^{14}$$O nucleus with large Fermi-surface asymmetry at $$sim$$100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2021

Nakada, Akira; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Futagawa, Kazuo; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; et al.

JAEA-Review 2022-078, 164 Pages, 2023/03

JAEA-Review-2022-078.pdf:2.64MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2021 to March 2022. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

High-sensitive XANES analysis at Ce L$$_{2}$$-edge for Ce in bauxites using transition-edge sensors; Implications for Ti-rich geological samples

Li, W.*; Yamada, Shinya*; Hashimoto, Tadashi; Okumura, Takuma*; Hayakawa, Ryota*; Nitta, Kiyofumi*; Sekizawa, Oki*; Suga, Hiroki*; Uruga, Tomoya*; Ichinohe, Yuto*; et al.

Analytica Chimica Acta, 1240, p.340755_1 - 340755_9, 2023/02

 Times Cited Count:2 Percentile:31.9(Chemistry, Analytical)

no abstracts in English

Journal Articles

Formation of MPd$$_{3+x}$$ (M = Gd, Np) by the reaction of MN with Pd and chlorination of MPd$$_{3+x}$$ using cadmium chloride

Hayashi, Hirokazu; Shibata, Hiroki; Sato, Takumi; Otobe, Haruyoshi

Journal of Radioanalytical and Nuclear Chemistry, 332(2), p.503 - 510, 2023/02

 Times Cited Count:0 Percentile:0.01(Chemistry, Analytical)

The formation of MPd$$_{3+x}$$ (M = Gd, Np) by the reaction of MN with Pd at 1323 K in Ar gas flow was observed. Cubic AuCu$$_3$$-type GdPd$$_{3.3}$$ (${it a}$ = 0.4081 $$pm$$ 0.0001 nm) and NpPd$$_3$$ (${it a}$ = 0.4081 $$pm$$ 0.0001 nm) were identified, respectively. The product obtained from the reaction of NpN with Pd contained additional phases including the hexagonal TiNi$$_3$$-type NpPd$$_3$$. Chlorination of the MPd$$_{3+x}$$ (M = Gd, Np) samples was accomplished by the solid-state reaction using cadmium chloride at 673 K in a dynamic vacuum. Pd-rich solid solution phase saturated with Cd and an intermetallic compound PdCd were obtained as by-products of MCl$$_3$$ formation.

Journal Articles

Difference in expansion and dehydration behaviors between NH$$_4$$- and K-montmorillonite

Kawakita, Ryohei; Saito, Akito*; Sakuma, Hiroshi*; Anraku, Sohtaro; Kikuchi, Ryosuke*; Otake, Tsubasa*; Sato, Tsutomu*

Applied Clay Science, 231, p.106722_1 - 106722_7, 2023/01

 Times Cited Count:1 Percentile:21.06(Chemistry, Physical)

Journal Articles

Progress of evaluation of beam coupling impedance reduction for the Eddy-current type septum magnet in J-PARC MR

Kobayashi, Aine*; Toyama, Takeshi*; Nakamura, Takeshi*; Shobuda, Yoshihiro; Ishii, Koji*; Tomizawa, Masahito*; Takeuchi, Yasunao*; Sato, Yoichi*

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.19 - 23, 2023/01

In the J-PARC main ring, density modulation due to longitudinal beam instability occurs during the debunching process of coasting beams. This leads to the generation of an electron cloud, which in turn causes transverse beam instabilities. The transverse beam instability causes beam loss and the electron cloud is assumed to cause vacuum degradation, both of which hinder the beam intensity enhancement, so it is essential to clarify the causes and countermeasures. In particular, the longitudinal impedance of several hundred MHz has been investigated as relevant, and measures to reduce the impedance of individual devices are underway. The Eddy-current type septum magnet, newly installed this year, was found to have a large impedance by simulation. Therefore, we are investigating a method to reduce the impedance by a flange loaded with SiC radio wave absorber, which can be applied to locations where there is no spatial margin to install a taper. In this report, we will discuss the characterization of SiC to be used in actual devices, impedance simulation reflecting the results of SiC evaluation, and evaluation of the effect of impedance countermeasures by impedance measurement using the wire method, and progress in evaluating the effect on the beam by beam simulation and beam study.

Journal Articles

Present status of JAEA's R&D toward HTGR deployment

Shibata, Taiju; Nishihara, Tetsuo; Kubo, Shinji; Sato, Hiroyuki; Sakaba, Nariaki; Kunitomi, Kazuhiko

Nuclear Engineering and Design, 398, p.111964_1 - 111964_4, 2022/11

 Times Cited Count:2 Percentile:53.91(Nuclear Science & Technology)

Japan Atomic Energy Agency (JAEA) has been promoting the research and development (R&D) of High Temperature Gas-cooled Reactor (HTGR). R&D on reactor technologies is carried out by using High Temperature engineering Test Reactor (HTTR). The HTTR was resumed without significant reinforcements in 2021. On January 2022, a safety demonstration test under the OECD/NEA LOFC project was carried out. JAEA is promoting R&D on a carbon-free hydrogen production by thermochemical water splitting Iodine-Sulfur process (IS process). JAEA conducts design study for various HTGR systems toward commercialization. A new test program about demonstration of hydrogen production by the HTTR was launched. Steam methane reforming hydrogen production system was selected for the first demonstration by 2030.

1628 (Records 1-20 displayed on this page)