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Eichler, R.*; Asai, Masato; Brand, H.*; Chiera, N. M.*; Di Nitto, A.*; Dressler, R.*; D
llmann, Ch. E.*; Even, J.*; Fangli, F.*; Goetz, M.*; et al.
EPJ Web of Conferences, 131, p.07005_1 - 07005_7, 2016/12
Times Cited Count：3 Percentile：72.98(Chemistry, Inorganic & Nuclear)In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the productions and investigations of fragile single molecular species of superheavy elements. The latest highlight is the formation of very volatile hexacarbonyl compound of element 106, Sg(CO)
. Following this success, second-generation experiments were performed to measure the first bond dissociation energy between the central metal atom and the surrounding ligand. The method using a tubular decomposition reactor was developed and successfully applied to short-lived Mo(CO), W(CO), and Sg(CO).
and W(CO)Usoltsev, I.*; Eichler, R.*; Wang, Y.*; Even, J.*; Yakushev, A.*; Haba, Hiromitsu*; Asai, Masato; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; et al.
Radiochimica Acta, 104(3), p.141 - 151, 2016/03
Times Cited Count：31 Percentile：94.91(Chemistry, Inorganic & Nuclear)Conditions of the production and decomposition of hexacarbonyl complexes of short-lived Mo and W isotopes were investigated to study thermal stability of the heaviest group 6 hexacarbonyl complex Sg(CO). A tubular flow reactor was tested to decompose the hexacarbonyl complexes and to extract the first bond dissociation energies. A silver was found to be the most appropriate reaction surface to study the decomposition of the group 6 hexacarbonyl. It was found that the surface temperature at which the decomposition occurred was correlated to the first bond dissociation energy of Mo(CO) and W(CO), indicating that the first bond dissociation energy of Sg(CO) could be determined with this technique.
Kobayashi, Takayuki; Moriyama, Shinichi; Yokokura, Kenji; Sawahata, Masayuki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Sato, Yoshikatsu; Hinata, Jun; Hoshino, Katsumichi; et al.
Nuclear Fusion, 55(6), p.063008_1 - 063008_8, 2015/06
Times Cited Count：25 Percentile：77.41(Physics, Fluids & Plasmas)A gyrotron enabling high-power, long-pulse oscillations at both 110 GHz and 138 GHz has been developed for electron cyclotron heating (ECH) and current drive (CD) in JT-60SA. Oscillations of 1 MW for 100 s have been demonstrated at both frequencies, for the first time as a gyrotron operating at two frequencies. The optimization of the anode voltage, or the electron pitch factor, using a triode gun was a key to obtain high power and high efficiency at two frequencies. It was also confirmed that the internal losses in the gyrotron were sufficiently low for expected long pulse operation at the higher power level of 
1.5 MW. Another important result is that an oscillation at 82 GHz, which enables to use fundamental harmonic waves in JT-60SA while the other two frequencies are used as second harmonics waves, was demonstrated up to 0.4 MW for 2 s. These results of the gyrotron development significantly contribute to enhancing operation regime of the ECH/CD system in JT-60SA.
Kobayashi, Takayuki; Moriyama, Shinichi; Isayama, Akihiko; Sawahata, Masayuki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Sato, Yoshikatsu; Hinata, Jun; Yokokura, Kenji; et al.
EPJ Web of Conferences, 87, p.04008_1 - 04008_5, 2015/03
Times Cited Count：5 Percentile：83.48(Physics, Fluids & Plasmas)A dual-frequency gyrotron, which can generate 110 GHz and 138 GHz waves independently, is being developed in JAEA to enable electron cyclotron heating (ECH) and current drive (ECCD) in a wider range of plasma discharge conditions of JT-60SA. Operation for the gyrotron conditioning and parameter optimization toward 1 MW for 100 s, which is the target output power and pulse length for JT-60SA, is in progress without problems. Oscillations of 1 MW for 10 s and 0.51 MW for 198 s were obtained, so far, at both frequencies. In addition, an oscillation (0.3 MW for 20 ms) at 82 GHz was demonstrated as an additional frequency of the dual-frequency gyrotron which shows a possibility of the use of fundamental harmonic wave in JT-60SA.
Even, J.*; Ackermann, D.*; Asai, Masato; Block, M.*; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; Eichler, R.*; Fan, F.*; Haba, Hiromitsu*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 303(3), p.2457 - 2466, 2015/03
Times Cited Count：15 Percentile：77.35(Chemistry, Analytical)Rapid In situ synthesis of metal carbonyl complexes has been demonstrated using short-lived isotopes produced in nuclear fission and fusion reactions. The short-lived isotopes with high recoil energy directly react with carbon-monoxides and form carbonyl complexes. Only highly volatile complexes were fast transported in a gas stream to counting and chemistry devices. Short-lived Mo, Tc, Ru, Rh, W, Re, Os, and Ir were found to form volatile carbonyl complexes, while no volataile complex of Hf and Ta were detected. This technique has been applied to a chemical investigation of the superheavy element Sg (atomic number 106), and will be applicable to various fields of nuclear science with short-lived transition metal isotopes.
Even, J.*; Yakushev, A.*; Dllmann, Ch. E.*; Haba, Hiromitsu*; Asai, Masato; Sato, Tetsuya; Brand, H.*; Di Nitto, A.*; Eichler, R.*; Fan, F. L.*; et al.
Science, 345(6203), p.1491 - 1493, 2014/09
Times Cited Count：64 Percentile：83.15(Multidisciplinary Sciences)A new superheavy element complex, a seaborgium carbonyl, has been successfully synthesized, and its adsorption property has been studied using a cryo-thermochromatography and 
-detection apparatus COMPACT. Nuclear reaction products of short-lived 
Sg preseparated with a gas-filled recoil ion separator GARIS at RIKEN were directly injected into a gas cell filled with He/CO mixture gas, and chemical reaction products of volatile carbonyl complexes were trasported to COMPACT. The Sg carbonyl complex detected with COMPACT was found to be very volatile with adsorption enthalpy of 
50 kJ/mol, from which we have concluded that this complex should be a Sg hexacarbonyl Sg(CO). This is the first synthesis of organometallic compounds of transactinide elements for which only simple inorganic comounds have been synthesized so far.
Maeda, Koji; Sasaki, Shinji; Kumai, Misaki; Sato, Isamu; Suto, Mitsuo; Osaka, Masahiko; Goto, Tetsuo*; Sakai, Hitoshi*; Chigira, Takayuki*; Murata, Hirotoshi*
Journal of Nuclear Science and Technology, 51(7-8), p.1006 - 1023, 2014/07
Times Cited Count：14 Percentile：72.29(Nuclear Science & Technology)Since the start of the severe accident at the Fukushima Daiichi Nuclear Power Plant in March 2011, concrete surfaces within the reactor buildings have been exposed to radioactive contaminants. Released radiation sources still remain too high to permit entry into some areas of the RBs to allow the damage to be assessed and to allow carrying out the restoration of lost safety functions, decommissioning activities, etc. In order to clarify the situation of this contamination in the RBs, 18 samples were subjected to analyses to determine the surface radionuclide concentrations and to characterize the radionuclide distributions in the samples. Decontamination tests on the sample of Unit 2 were conducted to reduce the levels of radioactivity present near the sample surface. As a result of the tests, the level of radioactivity of the sample was reduced with the removal of 97% of the contamination present near the sample surface.
Yokokura, Kenji; Moriyama, Shinichi; Kobayashi, Takayuki; Hiranai, Shinichi; Sawahata, Masayuki; Terakado, Masayuki; Hinata, Jun; Wada, Kenji; Sato, Yoshikatsu; Hoshino, Katsumichi; et al.
JAEA-Technology 2014-002, 64 Pages, 2014/03
JAEA-Technology-2014-002.pdf:6.83MB
A new instrument has been developed to measure spatial distribution of power density and total power of the millimeter wave, by measuring temperature rise of dielectric material inserted in the waveguide. For a measurement, a dielectric disk with thermally insulated support is inserted into the few millimeters gap in the waveguide. The disk is heated by the millimeter wave pulse for 0.10.2 s, and immediately after the pulse, it is pulled up and its temperature distribution is measured by an infrared camera to estimate the spatial power density distribution of the millimeter wave. In the other hand, total transmission power is estimated by the disk temperature reached equilibrium. In the measurement test, deformation of the power density distribution was successfully detected when the mirror angle was intentionally changed in the matching optics unit (MOU) at the waveguide input from the gyrotron. The test result shows that the instrument is effective for both adjustment of MOU without opening the vacuum boundary and to detect any abnormal transmission during operation of the ECH system. The test also shows high reliability of the instrument which stands with 1 MW high power transmission without any arcing or pressure rise in vacuum region. The instrument will be contributed to keep good condition of high power long pulse ECH system by detecting abnormal transmission in the waveguide in operation without open vacuum boundary.
Moriyama, Shinichi; Kobayashi, Takayuki; Isayama, Akihiko; Hoshino, Katsumichi; Suzuki, Sadaaki; Hiranai, Shinichi; Yokokura, Kenji; Sawahata, Masayuki; Terakado, Masayuki; Hinata, Jun; et al.
Fusion Engineering and Design, 88(6-8), p.935 - 939, 2013/10
Times Cited Count：4 Percentile：32.32(Nuclear Science & Technology)An antenna having a first mirror driven in the linear motion (LM) and a fixed second mirror was proposed for electron cyclotron range of frequency (ECRF) heating and current drive system, to minimize the risk of cooling-water-leakage. Basic mechanical feasibilities of the bellows covering the movable structures of the antenna were previously investigated using a mock-up. This time, a support structure of the shaft has been designed using a metallic sliding bearing with solid lubricant. The sliding bearing can support combination of linear and rotational motions while a ball bearing supports either linear or rotational motion. We have newly installed the sliding bearing into the mock-up. A vacuum pumping test has been carried out paying attention to the influence of the solid lubricant by mass analysis. To design the LM antenna for JT-60SA in detail, heating and current drive characteristics for typical experimental scenarios of JT-60SA has been investigated by calculation.
Maeda, Koji; Sasaki, Shinji; Kumai, Misaki; Sato, Isamu; Osaka, Masahiko; Fukushima, Mineo; Kawatsuma, Shinji; Goto, Tetsuo*; Sakai, Hitoshi*; Chigira, Takayuki*; et al.
Proceedings of International Nuclear Fuel Cycle Conference; Nuclear Energy at a Crossroads (GLOBAL 2013) (CD-ROM), p.272 - 277, 2013/09
Cm + 
O reactionMurakami, Masashi*; Goto, Shinichi*; Murayama, Hirofumi*; Kojima, Takayuki*; Kudo, Hisaaki*; Kaji, Daiya*; Morimoto, Koji*; Haba, Hiromitsu*; Kudo, Yuki*; Sumita, Takayuki*; et al.
Physical Review C, 88(2), p.024618_1 - 024618_8, 2013/08
Times Cited Count：16 Percentile：69.99(Physics, Nuclear)Production cross sections of Rf isotopes in the Cm + O reaction were measured at the beam energy range of 88.2 to 101.3 MeV by use of a gas-filled recoil ion separator. The excitation functions of 
Rf, 
Rf, and 
Rf were obtained together with those of spontaneously fissioning nuclides which have few-second half-lives and have been assigned to 
Rf and a longer-lived state of Rf. The excitation function of few-second spontaneously fissioning nuclide exhibited the maximum cross section at the O beam energy of 94.8 MeV. The shape of the excitation function was almost the same as that of Rf, whereas it was quite different from those of Rf and Rf. A few-second spontaneously fissioning nuclide previously reported as Rf and Rf observed inCm + O reaction was identified as Rf.
Kobayashi, Takayuki; Isayama, Akihiko; Sawahata, Masayuki; Suzuki, Sadaaki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Sato, Yoshikatsu; Hinata, Jun; Yokokura, Kenji; et al.
Fusion Science and Technology, 63(1T), p.160 - 163, 2013/05
Times Cited Count：7 Percentile：49.06(Nuclear Science & Technology)A dual frequency electron cyclotron range of frequency system has been developed for JT-60SA, by which a second frequency (135 140 GHz) is generated in addition to the first frequency of 110 GHz. A development of a dual frequency gyrotron is a key to realize the dual frequency system. The second frequency was chosen to be 138 GHz from the above frequency range from the viewpoint of gyrotron design. In order to realize high-power (
1 MW) and long-pulse operation for both frequencies, we designed main components of the gyrotron (the diamond window, cavity resonator and quasi-optical mode converter). We found the optimum parameter set from the parameters of these components, which has discrete characteristics. It was confirmed that the output power higher than 1 MW is obtained for both frequencies as a result of numerical design. Based on the above design, a dual frequency gyrotron was newly fabricated. In the conditioning operation, an output power was obtained as we expected.
113 of the 113th elementMorita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sumita, Takayuki*; Wakabayashi, Yasuo*; Yoneda, Akira*; Tanaka, Kengo*; et al.
Journal of the Physical Society of Japan, 81(10), p.103201_1 - 103201_4, 2012/10
Times Cited Count：167 Percentile：97.31(Physics, Multidisciplinary)An isotope of the 113th element, 113, was produced in a nuclear reaction with a 
Zn beam on a 
Bi target. We observed six consecutive decays following the implantation of a heavy particle in nearly the same position in the semiconductor detector, in extremely low background condition. The fifth and sixth decays are fully consistent with the sequential decays of Db and 
Lr both in decay energies and decay times. This indicates that the present decay chain consisted of 113, 
Rg (Z = 111), 
Mt (Z = 109), 
Bh (Z = 107), Db (Z = 105), and Lr (Z = 103) with firm connections. This result, together with previously reported results from 2004 and 2007, conclusively leads the unambiguous production and identification of the isotope 113, of the 113th element.
Kobayashi, Takayuki; Isayama, Akihiko; Sawahata, Masayuki; Suzuki, Sadaaki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Sato, Yoshikatsu; Hinata, Jun; Yokokura, Kenji; et al.
Proceedings of 37th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz 2012) (USB Flash Drive), 2 Pages, 2012/09
A new dual frequency (110 GHz and 138 GHz) gyrotron development began for JT-60SA. An output power and efficiency higher than 1 MW and 30% with a peak heat load lower than 1.4 kW/cm
were obtained for both frequencies in calculation. High mode conversion efficiencies of the quasioptical mode converter (96.8% for 110 GHz and 98.3% for 138 GHz), which is higher than the previously developed 110 GHz long pulse gyrotron (96.5%), was obtained. The new gyrotron was fabricated and conditioning operation has been started from the middle of June 2012. The gyrotron output power of approximately 200 kW was obtained, so far, as we expected in the design of the gyrotron at low beam current of 10 A and low beam voltage of 75 kV.
Isayama, Akihiko; Kobayashi, Takayuki; Yokokura, Kenji; Shimono, Mitsugu; Sawahata, Masayuki; Suzuki, Sadaaki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Hinata, Jun; et al.
Plasma and Fusion Research (Internet), 7(Sp.1), p.2405029_1 - 2405029_5, 2012/05
no abstracts in English
Sg in the Cm(
Ne,5
)Sg reaction and decay properties of two isomeric states in SgHaba, Hiromitsu*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sakai, Ryutaro*; Sumita, Takayuki*; Yoneda, Akira*; Kasamatsu, Yoshitaka*; et al.
Physical Review C, 85(2), p.024611_1 - 024611_11, 2012/02
Times Cited Count：53 Percentile：91.21(Physics, Nuclear)Two isomeric states in Sg, i.e, Sg
and Sg
were produced in the Cm(Ne,5) reaction. Decay properties of Sg
were investigated with a rotating-wheel apparatus for and spontaneous fission (SF) spectrometry under low background condition attained by a gas-jet transport system coupled to the RIKEN gas-filled recoil ion separator. Based on genetically correlated - (-) and -SF decay chains, 18 and 24 events were assigned to Sg and Sg, respectively. The half-life and -particle energy of Sg were measured to be 
s and 
MeV, respectively, and those of Sg were 
s and 
MeV.
Kobayashi, Takayuki; Isayama, Akihiko; Hasegawa, Koichi; Suzuki, Sadaaki; Hiranai, Shinichi; Sato, Fumiaki; Wada, Kenji; Yokokura, Kenji; Shimono, Mitsugu; Sawahata, Masayuki; et al.
Fusion Engineering and Design, 86(6-8), p.763 - 767, 2011/10
Times Cited Count：6 Percentile：44.16(Nuclear Science & Technology)Progress of antenna development of the Electron Cyclotron Range of Frequency system for JT-60 SA is presented. Capability of pulse length of 100 s, which requires active cooling for mirrors, and flexibility of beam injection angles in both poloidal and toroidal directions are required for the antenna with high reliability. Mechanical and structural design works of the launcher (antenna and its support with steering structure) based on a linear motion antenna concept are in progress. The key component is a long-stroke bellows which enables to alter poloidal injection angle and a bellows which enables to alter toroidal injection angle. Using a newly fabricated mock-up of the steering structure, it was confirmed that the antenna was mechanically realized for poloidal and toroidal injection angle ranges of -10 to +45
and -15 to +15, respectively. Those angles are consistent with angles required in JT-60SA. The results of thermal and structural analyses are also presented.
Kobayashi, Takayuki; Isayama, Akihiko; Yokokura, Kenji; Shimono, Mitsugu; Hasegawa, Koichi; Sawahata, Masayuki; Suzuki, Sadaaki; Terakado, Masayuki; Hiranai, Shinichi; Sato, Fumiaki; et al.
Nuclear Fusion, 51(10), p.103037_1 - 103037_10, 2011/10
Times Cited Count：19 Percentile：62.29(Physics, Fluids & Plasmas)A new gyrotron operation technique to increase oscillation efficiency was developed on the JT 60 ECRF system. The electron pitch factor was optimized by controlling anode voltage within 0.1 s after the start of the operation. By applying this technique, the gyrotron output power of 1.5 MW for 4 s was recorded, for the first time. The reduced collector heat load at 1.5 MW operations was reduced by 20% and it will be acceptable for longer pulse operation. A new gyrotron with an improved mode converter was developed in order to demonstrate reduction of the stray radiation which had limited the pulse length. The stray radiation was reduced to 1/3 of that of the original gyrotron. A conditioning operation of the improved gyrotron is proceeding up to 31 s at 1 MW. These progresses significantly contribute to enhancing the high power and long pulse capability of the ECRF system toward JT 60SA.
Hs and HsSato, Nozomi; Haba, Hiromitsu*; Ichikawa, Takatoshi*; Kaji, Daiya*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Ozeki, Kazutaka*; Sumita, Takayuki*; Yoneda, Akira*; et al.
Journal of the Physical Society of Japan, 80(9), p.094201_1 - 094201_7, 2011/09
Times Cited Count：15 Percentile：65.21(Physics, Multidisciplinary)Decay properties of Hs and Hs produced in the 
Pb(
Fe, 
) [
=1, 2] reactions were studied using a gas-filled recoil ion separator at the linear accelerator facility of RIKEN. A total of 6 decay chains were assigned to Hs. Cross sections for the Hs production in the 
Pb(Fe,
) and 
Pb(Fe,) reactions were measured to be 
pb and 
pb, respectively. The isotope Hs decayed with a half-life of 
ms by -particle emission and spontaneous fission. The -particle energy of Hs was observed at 10.61
0.04 and 10.800.08 MeV. The spontaneous fission branch of Hs was found to be 
.
Sato, Shoichi*; Ichimura, Makoto*; Yamaguchi, Yusuke*; Katano, Makoto*; Imai, Yasutaka*; Murakami, Tatsuya*; Miyake, Yuichiro*; Yokoyama, Takuro*; Moriyama, Shinichi; Kobayashi, Takayuki; et al.
Plasma and Fusion Research (Internet), 5, p.S2067_1 - S2067_4, 2010/12
Ion cyclotron emissions (ICEs) due to deuterium-deuterium fusion-product (FP) ions on JT-60U are studied. ICE due to H-ions is identified from the difference of the toroidal wave number of 2nd ICE(D). The parameter dependence for the appearance of ICE(H) is investigated from the experimental conditions and also is studied by using "Escape Particle Orbit analysis Code (EPOC)".
