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Journal Articles

Production and synthesis of a novel $$^{191}$$Pt-labeled platinum complex and evaluation of its biodistribution in healthy mice

Omokawa, Marina*; Kimura, Hiroyuki*; Hatsukawa, Yuichi*; Kawashima, Hidekazu*; Tsukada, Kazuaki; Yagi, Yusuke*; Naito, Yuki*; Yasui, Hiroyuki*

Bioorganic & Medicinal Chemistry, 97, p.117557_1 - 117557_6, 2024/01

 Times Cited Count:0 Percentile:0.01(Biochemistry & Molecular Biology)

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Star-polymer-DNA gels showing highly predictable and tunable mechanical responses

Ohira, Masashi*; Katashima, Takuya*; Naito, Mitsuru*; Aoki, Daisuke*; Yoshikawa, Yusuke*; Iwase, Hiroki*; Takata, Shinichi; Miyata, Kanjiro*; Chung, U.-I.*; Sakai, Takamasa*; et al.

Advanced Materials, 34(13), p.2108818_1 - 2108818_9, 2022/01

 Times Cited Count:13 Percentile:89.15(Chemistry, Multidisciplinary)

Journal Articles

Disk and washer coupled cavity linac design and cold-model for muon linac

Otani, Masashi*; Futatsukawa, Kenta*; Mibe, Tsutomu*; Naito, Fujio*; Hasegawa, Kazuo; Ito, Takashi; Kitamura, Ryo; Kondo, Yasuhiro; Morishita, Takatoshi; Iinuma, Hiromi*; et al.

Journal of Physics; Conference Series, 1350, p.012097_1 - 012097_7, 2019/12

 Times Cited Count:2 Percentile:72.74(Physics, Particles & Fields)

A disk and washer (DAW) coupled cavity linac (CCL) has been developed for a middle velocity part in a muon linac to measure muon anomalous magnetic moment and search for electric dipole moment. I will accelerate muons from $$v/c$$ = $$beta$$ = 0.3 to 0.7 at an operational frequency of 1.3GHz. In this poster, the cavity design, beam dynamics design, and the cold-model measurements will be presented.

Journal Articles

Development of remote sensing technique using radiation resistant optical fibers under high-radiation environment

Ito, Chikara; Naito, Hiroyuki; Ishikawa, Takashi; Ito, Keisuke; Wakaida, Ikuo

JPS Conference Proceedings (Internet), 24, p.011038_1 - 011038_6, 2019/01

A high-radiation resistant optical fiber has been developed in order to investigate the interiors of the reactor pressure vessels and the primary containment vessels at the Fukushima Daiichi Nuclear Power Station. The tentative dose rate in the reactor pressure vessels is assumed to be up to 1 kGy/h. We developed a radiation resistant optical fiber consisting of a 1000 ppm hydroxyl doped pure silica core and 4 % fluorine doped pure silica cladding. We attempted to apply the optical fiber to remote imaging technique by means of fiberscope. The number of core image fibers was increased from 2000 to 22000 for practical use. The transmissive rate of infrared images was not affected after irradiation of 1 MGy. No change in the spatial resolution of the view scope by means of image fiber was noted between pre- and post-irradiation. We confirmed the applicability of the probing system, which consists of a view scope using radiation-resistant optical fibers.

Journal Articles

Progress report of Japanese simulation research projects using the high-performance computer system Helios in the International Fusion Energy Research Centre

Ishizawa, Akihiro*; Idomura, Yasuhiro; Imadera, Kenji*; Kasuya, Naohiro*; Kanno, Ryutaro*; Satake, Shinsuke*; Tatsuno, Tomoya*; Nakata, Motoki*; Nunami, Masanori*; Maeyama, Shinya*; et al.

Purazuma, Kaku Yugo Gakkai-Shi, 92(3), p.157 - 210, 2016/03

The high-performance computer system Helios which is located at The Computational Simulation Centre (CSC) in The International Fusion Energy Research Centre (IFERC) started its operation in January 2012 under the Broader Approach (BA) agreement between Japan and the EU. The Helios system has been used for magnetised fusion related simulation studies in the EU and Japan and has kept high average usage rate. As a result, the Helios system has contributed to many research products in a wide range of research areas from core plasma physics to reactor material and reactor engineering. This project review gives a short catalogue of domestic simulation research projects. First, we outline the IFERC-CSC project. After that, shown are objectives of the research projects, numerical schemes used in simulation codes, obtained results and necessary computations in future.

Journal Articles

Present status of J-PARC linac

Oguri, Hidetomo; Hasegawa, Kazuo; Ito, Takashi; Chishiro, Etsuji; Hirano, Koichiro; Morishita, Takatoshi; Shinozaki, Shinichi; Ao, Hiroyuki; Okoshi, Kiyonori; Kondo, Yasuhiro; et al.

Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 393, 2014/10

no abstracts in English

Journal Articles

Development of radiation-resistant optical fiber for application to observation and laser spectroscopy under high radiation dose

Ito, Chikara; Naito, Hiroyuki; Nishimura, Akihiko; Oba, Hironori; Wakaida, Ikuo; Sugiyama, Akira; Chiyatani, Keiji

Journal of Nuclear Science and Technology, 51(7-8), p.944 - 950, 2014/07

 Times Cited Count:30 Percentile:91.28(Nuclear Science & Technology)

In the Fukushima Daiichi Nuclear Power Station, it is necessary to survey the locations and conditions of fuel debris inside reactor pressure vessels or primary containment vessels under water and radiation environment in preparation for removing fuel debris. An optical fiber is well known for features such as signal transmission, light weight, superior insulation performance, water resistance and electromagnetic noise resistance. These features allow the optical fiber to simplify the instrumentation systems for in-vessel inspection, as long as provide that the optical fiber can be used under high radiation dose environment. The radiation resistance of an optical fiber was improved by increasing the amount of hydroxyl up to 1000 ppm in pure silica fiber. The improved optical fibers were irradiated with $$gamma$$-ray up to 1 $$times$$ 10$$^{6}$$ Gy using a $$^{60}$$Co source. They indicated a large peak around 600 nm and a peak tail from ultraviolet region, but no large absorption in infrared region except a hydroxyl absorption peak of 945 nm. We have confirmed that the optical fiber containing 1000 ppm hydroxyl has enough radiation resistance for radiation induced transmission losses and the infrared imaging is effective for observation under high radiation doses.

Journal Articles

In-vessel inspection probing technique using optical fibers under high radiation dose

Ito, Chikara; Naito, Hiroyuki; Oba, Hironori; Saeki, Morihisa; Ito, Keisuke; Ishikawa, Takashi; Nishimura, Akihiko; Wakaida, Ikuo; Sekine, Takashi

Proceedings of 22nd International Conference on Nuclear Engineering (ICONE-22) (DVD-ROM), 7 Pages, 2014/07

A high-radiation resistant optical fiber has been developed in order to investigate the interiors of the reactor pressure vessels and the primary containment vessels of the Fukushima Daiichi Nuclear Power Station. The radiation resistance of an optical fiber was improved by increasing the amount of hydroxyl up to 1000 ppm in pure silica fiber. The improved image fiber consists of common cladding and a large number of fiber cores made from pure silica that contains 1000 ppm hydroxyl. The transmissive rate of an infrared image was not affected after the irradiation of 1 MGy. We have developed the fiber-coupled LIBS system to detect plasma emission efficiently in near-infrared region. In addition, we have performed a $$gamma$$ ray dose rate measurement using an optical fiber of which scintillator is attached to the tip. As a result, the concept of applicability of a probing system using the high-radiation resistant optical fibers has been confirmed.

Journal Articles

Characteristic evaluation of colloidal silica grout material developed for a high level radioactive waste geological repository

Kishi, Hirokazu; Kawaguchi, Masanao; Naito, Morimasa; Hatanaka, Koichiro; Nobuto, Jun*; Sugiyama, Hirokazu*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 19(1), p.3 - 8, 2012/06

To reduce amount of groundwater inflow into a geological repository, the grouting is expected to play a very important role because the geological environment in Japan is often characterized by many fractures and abundant groundwater. Basically, cementitious materials are used for grouting, however the resulting highly alkaline plume released from the materials could influence the long-term performance of barrier system as a consequence of alteration of both the buffer material and the host rock. To minimize such effects, JAEA has carried out research and development on three types of grout material with low-pH performance that decreases influence in the alteration. This paper focuses on the Colloidal silica grout, and presents its unique characteristics obtained from laboratory tests on pH, viscosity, leaching and so on. The results indicate that the grout has good performances in pH and viscosity. It is concluded that the grout can be greatly used for the repository.

JAEA Reports

Inspection and repair techniques in the reactor vessel of the experimental fast reactor Joyo; Development of a high radiation resistance fiberscope (Joint research)

Naito, Hiroyuki; Itagaki, Wataru; Okazaki, Yoshihiro; Imaizumi, Kazuyuki; Ito, Chikara; Nagai, Akinori; Kitamura, Ryoichi; Shamoto, Naoki*; Takeshima, Yoshiyuki*

JAEA-Technology 2012-009, 100 Pages, 2012/05

JAEA-Technology-2012-009.pdf:9.89MB

The radiation characteristics of image fiber and light guide fiber were evaluated to develop a high radiation resistant fiberscope for the fast reactor in-vessel observation. It is known that a pure silica core fiber has a high radiation resistance and radiation resistance is influenced with impurities in silica. Moreover it is necessary to change the clad material of the light guide fiber because that of the current light guide fiber is acrylate, which is weak against radiation. Hence the improved fibers consist of a pure silica core with 1,000 ppm OH and fluorine-doped silica clad. As a result of a $$gamma$$ irradiation test, we confirm that OH inhibits the generation of the precursor by $$gamma$$ irradiation. About the clad material, we confirmed that the transmission loss of the fluorine-doped silica clad fiber is smaller than that of the acrylate clad fiber. About the mechanical strength of a fiber, we confirmed that there is no weakening the strength of the fiber and no exfoliation of the coating from the glass. In this study, we discovered the fiber which consists of a pure silica core with 1,000 ppm OH and fluorine-doped silica clad has a high radiation resistance and it is possible to observe using this fiber under the 200 $$^{circ}$$C after 5$$times$$10$$^{5}$$ Gy irradiation.

Journal Articles

Development of high sensitive and reliable FFD and sodium leak detection technique for fast reactor using RIMS

Ito, Chikara; Araki, Yoshio; Naito, Hiroyuki; Iwata, Yoshihiro; Aoyama, Takafumi

Proceedings of International Conference on Fast Reactors and Related Fuel Cycles (FR 2009) (CD-ROM), 12 Pages, 2012/00

no abstracts in English

Journal Articles

Mix design of low pH cement shotcrete in high level radioactive waste repositories

Noguchi, Akira; Kishi, Hirokazu; Hatanaka, Koichiro; Naito, Morimasa

Proceedings of 19th International Conference on Nuclear Engineering (ICONE-19) (CD-ROM), 6 Pages, 2011/10

A standardized method for choosing a mix design of low pH shotcrete is proposed for their intended use in the construction of a High Level Radioactive Waste (HLW) repository in order to be applied to the various geological environment of the location of the HLW repositories. There are two improvement in this method. One is estimating binder composition to satisfy low pH. The other is estimating water bender ratio to satisfy the strength of sprayed concrete. The method uses a sequential development process with consideration given to a number of physicochemical requirements, incorporates current shotcrete technology. The method is demonstrated in its entirety through a series of experiments and tests using a low pH cement binder comprised of a mixture of ordinary Portland cement, fly ash (FA) and silica fume (SF), referred to here as high-volume FA SF cement (HFSC). Moreover, the method is referred from the demonstration of HFSC shotcrete in Horonobe underground research laboratory.

Journal Articles

Long term integrity of overpack closure weld for HLW geological disposal, 2; Corrosion properties under anaerobic conditions

Kobayashi, Masato*; Yokoyama, Yutaka*; Takahashi, Rieko*; Asano, Hidekazu*; Taniguchi, Naoki; Naito, Morimasa

Corrosion Engineering, Science and Technology, 46(2), p.212 - 216, 2011/04

 Times Cited Count:4 Percentile:28.93(Materials Science, Multidisciplinary)

The corrosion behaviour of a carbon steel weld joint under anaerobic conditions was investigated to estimate the long-term integrity of the carbon steel overpack. The weld specimens in this study were produced using three welding methods: GTAW, GMAW and EBW. General corrosion was observed for each immersion specimen and the weld joint corrosion rate was the same as or less than that of the base metal. The hydrogen concentration absorbed during immersion testing was less than 2.48$$times$$10$$^{-5}$$ mol kg[Fe]$$^{-1}$$(0.05 ppm) after three years, a value regarded as having little influence on hydrogen embrittlement. The susceptibility to hydrogen embrittlement was highest in the base metal, suggesting that there was little adverse effect on the weld joint from welding. The welded carbon steel overpack is assumed to maintain its resistance to corrosion as a disposal container for the expected lifetime under anaerobic underground conditions.

JAEA Reports

Measurement and analysis of in-vessel component activation and gamma dose rate distribution in Joyo

Ito, Hideaki; Maeda, Shigetaka; Naito, Hiroyuki; Akiyama, Yoichi; Miyamoto, Kazuyuki; Ashida, Takashi; Noguchi, Koichi; Ito, Chikara; Aoyama, Takafumi

JAEA-Technology 2010-049, 129 Pages, 2011/03

JAEA-Technology-2010-049.pdf:6.99MB

The in-vessel gamma dose rate was measured in the experimental fast reactor Joyo to evaluate the activation of reactor structural components and the radiation exposure of the fiber scope used for in-vessel visual inspection. The measurement system, which requires a wide sensitivity range and high durability in a high-temperature environment, was specifically developed for use in the sodium cooled fast reactor. Using this system, the in-vessel gamma dose rate with cooling times of 450 and 720 days after reactor shutdown was measured in Joyo, which has been operated for 71,000 hours over approximately 30 years. The gamma dose rate was calculated using QAD-CGGP2 code with the gamma source intensity obtained by the ORIGEN2 code. The neutron flux used as input to the ORIGEN2 was evaluated by the Joyo dosimetry method. The ratio between the calculated and experimental values ranged from 1.1 to 2.4, confirming the accuracy of gamma dose rate and component activation calculation.

JAEA Reports

Horonobe Underground Research Laboratory Project; Synthesis of phase I investigation 2001 - 2005, Volume "Geological disposal research"

Fujita, Tomoo; Taniguchi, Naoki; Matsui, Hiroya; Tanai, Kenji; Maekawa, Keisuke; Sawada, Atsushi; Makino, Hitoshi; Sasamoto, Hiroshi; Yoshikawa, Hideki; Shibata, Masahiro; et al.

JAEA-Research 2011-001, 193 Pages, 2011/03

JAEA-Research-2011-001.pdf:5.23MB

This report summarizes the progress of research and development on geological disposal during the surface-based investigation phase (2001-2005) in the Horonobe Underground Research Laboratory project, of which aims are to apply the design methods of geological disposal and mass transport analysis to actual geological conditions obtained from the surface-based investigations in the Horonobe Underground Research Laboratory project as an example of actual geological environment.

JAEA Reports

A Study on the technology for reducing cement-type materials used for tunnel supports at high-level radioactive waste disposal sites (Joint research)

Hayashi, Katsuhiko; Noguchi, Akira; Kishi, Hirokazu; Kabayashi, Yasushi*; Nakama, Shigeo; Fujita, Tomoo; Naito, Morimasa; Tada, Hiroyuki*; Kumasaka, Hiroo*; Goke, Mitsuo*; et al.

JAEA-Research 2010-057, 101 Pages, 2011/03

JAEA-Research-2010-057.pdf:7.47MB

Cement-type materials that are used for supports or grouting at high-level radioactive waste disposal facilities leach into the groundwater and create a highly alkaline environment. Of concern in highly alkaline environments are the alteration of bentonite used as buffers or backfill materials, and of surrounding rock mass, and the increased uncertainty regarding the provision of performance of the disposal system over a long period of time. In this study, to reduce the quantity of cement-type materials that cause highly alkaline environments, technical feasibility of the support structure including the materials which considered the long-term performance of the HLW disposal system are discussed by using knowledge and technology accumulated in JAEA and Shimizu Construction. Moreover, based on the results, the problems remained in the application to the future HLW disposal institution are summarized.

Journal Articles

Measurement and analysis of in-vessel component activation and $$gamma$$ dose rate distribution in Joyo

Maeda, Shigetaka; Naito, Hiroyuki; Ito, Chikara; Aoyama, Takafumi

Progress in Nuclear Science and Technology (Internet), 1, p.182 - 185, 2011/02

In-vessel $$gamma$$ rate measurements have been conducted in the experimental fast reactor Joyo to obtain experimental data and to verify the analysis method. The in-vessel $$gamma$$ dose with cooling times of 500 and 700 days after reactor shutdown was measured in Joyo which had been operated for approximately 30 years. The $$gamma$$ dose was calculated using QAD code with the $$gamma$$ source obtained by ORIGEN2 code. The ratios between the calculated and experimental value was ranged 1.3 and 2.7. The accuracy of analys method for the amount and distribution of radioactive products and $$gamma$$ ray dose inside reactor vessel was confirmed for the in-vessel inspection or repair.

Journal Articles

Development of superfine spherical silica grout as an alternative grouting material for the geological disposal of long-lived radioactive waste

Naito, Morimasa; Kishi, Hirokazu; Fukuoka, Naomi; Yamada, Tsutomu*; Ishida, Hideaki*

Proceedings of 18th International Conference on Nuclear Engineering (ICONE-18) (CD-ROM), 7 Pages, 2010/05

As an alternative grouting material for the geological repository of long-lived radioactive waste, the "Superfine Spherical silica Grout" (SFSG) material is developed using a fine spherical silica and a fine calcium hydroxide. The developed SFSG material takes an advantage of its smaller particle size distribution (max. $$sim$$1 micron or less) than those of the cementitious materials, and also provides a low alkaline environment so as to reduce unfavorable effects on the long-term performance of geological disposal system. The SFSG is a mixture of the super fine silica powder, the superfine calcium hydroxide and additives such as superplasticizer. Some preliminary laboratory experiments were carried out to characterize its fundamental properties from the viewpoint of practical use for geological disposal, which is required to be equivalent with the conventional cementitious materials in terms of penetrability, strength, pH performance and workability.

Journal Articles

Development of advanced operation scenarios in weak magnetic-shear regime on JT-60U

Suzuki, Takahiro; Oyama, Naoyuki; Isayama, Akihiko; Sakamoto, Yoshiteru; Fujita, Takaaki; Ide, Shunsuke; Kamada, Yutaka; Naito, Osamu; Sueoka, Michiharu; Moriyama, Shinichi; et al.

Nuclear Fusion, 49(8), p.085003_1 - 085003_8, 2009/08

 Times Cited Count:8 Percentile:30.67(Physics, Fluids & Plasmas)

Fully non-inductive discharge having a relaxed current profile and high bootstrap current fraction f$$_{BS}$$=0.5 has been realized in the high-$$beta$$$$_{p}$$ ELMy H-mode discharge with weak magnetic-shear having q$$_{95}$$=5.8, qmin=2.1, and q(0)=2.4, where qmin and q(0) are the safety factor q at the minimum and the plasma center, respectively. The rest of the plasma current is externally driven by neutral beams (NBs) and lower-hybrid (LH) waves. The safety factor profile evaluated by the motional Stark effect (MSE) diagnostic is kept unchanged during 0.7 s at the end of the full current drive (CD) sustainment for 2 s (1.5 times the current relaxation time $$_{tau R}$$). The loop voltage profile is spatially uniform at 0 V at the end of the sustainment. This demonstration shows, for the first time, that the steady sustainment of ful-CD plasma is possible at high f$$_{BS}$$=0.5 and reasonably low q$$_{95}$$=5.8 regime and is stably controlled by appropriate external current drivers. On the other hand, when the combination of bootstrap current and externally driven current does not match to the steady current profile, slight change in the current profile due to current relaxation resulted in appearance of magnetohydrodynamic (MHD) instability, e.g. neo-classical tearing mode (NTM), in a high beta plasma. This discharge clarifies importance of the demonstration of steady current profile developed here. These discharges contribute to the ITER steady-state operation scenario development.

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