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Journal Articles

Isotope-selective microscale imaging of radioactive Cs without isobaric interferences using sputtered neutral mass spectrometry with two-step resonant ionization employing newly-developed Ti:Sapphire lasers

Sakamoto, Tetsuo*; Morita, Masato*; Kanenari, Keita*; Tomita, Hideki*; Sonnenschein, V.*; Saito, Kosuke*; Ohashi, Masaya*; Kato, Kotaro*; Iguchi, Tetsuo*; Kawai, Toshihide*; et al.

Analytical Sciences, 34(11), p.1265 - 1270, 2018/11

 Times Cited Count:8 Percentile:31.52(Chemistry, Analytical)

Journal Articles

Comparison of $$^{14}$$C collected by precipitation and gas-strip methods for dating groundwater

Nakata, Kotaro*; Hasegawa, Takuma*; Iwatsuki, Teruki; Kato, Toshihiro

Radiocarbon, 58(3), p.491 - 503, 2016/09

AA2015-0781.pdf:0.96MB

 Times Cited Count:5 Percentile:21.26(Geochemistry & Geophysics)

Dissolved inorganic carbon (DIC) for $$^{14}$$C analysis of groundwater is usually extracted by a gas-strip or precipitation method. In this study, the certainty of the two methods for $$^{14}$$C dating were confirmed. DIC and $$^{14}$$C concentrations obtained by the gas-strip method were close to the theoretically predicted $$^{14}$$C value. Conversely, the $$^{14}$$C value obtained by the precipitation method always showed higher values than the predicted values. The difference in $$^{14}$$C value between gas-strip and precipitation methods was assumed to arise owing to contamination of modern carbon used in the precipitation method. The applicability of the precipitation method for groundwater should be considered carefully according to the DIC, $$^{14}$$C concentration of groundwater and purpose of the study being conducted.

Oral presentation

Applicability of degassing and precipitation methods for DIC collection from groundwater

Nakata, Kotaro*; Hasegawa, Takuma*; Iwatsuki, Teruki; Kato, Toshihiro

no journal, , 

$$^{14}$$C concentration in dissolved inorganic carbon is available index to infer groundwater residence time. We confirmed precision and accuracy during DIC collection methods such as degassing and precipitation by using NaHCO$$_{3}$$ solution and natural groundwater.

Oral presentation

Hydrochemical investigation at the Mizunami Underground Research Laboratory; Development of gas-strip techniques of dissolved inorganic carbon for dating groundwater

Kato, Toshihiro; Iwatsuki, Teruki; Munemoto, Takashi; Kubota, Mitsuru; Hayashida, Kazuki; Nakata, Kotaro*; Hasegawa, Takuma*

no journal, , 

no abstracts in English

Oral presentation

Estimation of hydraulic conditions of groundwater using carbon isotope

Kato, Toshihiro; Iwatsuki, Teruki; Nakata, Kotaro*; Hasegawa, Takuma*

no journal, , 

no abstracts in English

Oral presentation

Chemical and isotopic study of the impact on groundwater environment by an large underground facility

Iwatsuki, Teruki; Kato, Toshihiro; Nakata, Kotaro*; Hasegawa, Takuma*

no journal, , 

Water chemistry, isotopes and chlorofluorocarbons in groundwater down to a depth of 500 m were monitored in the Mizunami Underground Research Laboratory (MIU), Japan. The monitoring of water chemistry for more than 10 years shows the increase of shallow water infiltration in UHFD at depths between 200 - 400 m. Based on 3H and CFCs concentrations the mixing proportion of shallow groundwater was estimated up to about 50 %. On the other hand groundwater in LSFD at the depth of 500 m was identified relatively isolated condition from the hydraulic disturbance by the facility construction. The residence time of the isolated groundwater was estimated 18 - 25 ka by $$^{14}$$C.

Oral presentation

Study of groundwater residence time in Mizunami Underground Research Laboratory

Hasegawa, Takuma*; Nakata, Kotaro*; Tomioka, Yuichi*; Ota, Tomoko*; Hama, Katsuhiro; Iwatsuki, Teruki; Kato, Toshihiro*; Hayashida, Kazuki

no journal, , 

Groundwater dating using $$^{14}$$C, $$^{4}$$He, noble gas method was conducted in Mizunami Underground Research laboratory. The availability of degassing method for $$^{14}$$, flux estimation method for He were examined. It was identified that the groundwater have been derived in glacial age. The integration of distinct dating method is available to estimate precise age of groundwater.

Oral presentation

CRIEPI-JAEA collaboration study on mass transport by groundwater in and around the Mizunami Underground Research Laboratory

Hasegawa, Takuma*; Nakata, Kotaro*; Tomioka, Yuichi*; Ota, Tomoko*; Hama, Katsuhiro; Iwatsuki, Teruki; Kato, Toshihiro*; Hayashida, Kazuki

no journal, , 

no abstracts in English

Oral presentation

Resonant laser secondary neutral mass spectrometry for micro imaging of radioactive isotopes, 2

Tomita, Hideki*; Saito, Kosuke*; Ohashi, Masaya*; Sonnenschein, V.*; Kato, Kotaro*; Suzuki, So*; Iguchi, Tetsuo*; Morita, Masato*; Sakamoto, Tetsuo*; Kanenari, Keita*; et al.

no journal, , 

no abstracts in English

Oral presentation

Groundwater dating conducted in Mizunami Underground Research Laboratory

Hasegawa, Takuma*; Nakata, Kotaro*; Tomioka, Yuichi*; Ota, Tomoko*; Hama, Katsuhiro; Iwatsuki, Teruki; Kato, Toshihiro*; Hayashida, Kazuki

no journal, , 

Groundwater dating was conducted to Mizunami Underground Research Laboratory (MIU). $$^{14}$$C age and $$^{4}$$He age were estimated about 20,000 years around MIU. The estimation of noble gas temperature is also conducted. The estimated recharge temperature is around 6$$^{circ}$$C. This temperature is about 9$$^{circ}$$C cooler than present annual average temperature, which agree with estimation of modern analog method conducted near MIU.

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