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Journal Articles

Post irradiation experiment about SiC-coated oxidation-resistant graphite for high temperature gas-cooled reactor

Shibata, Taiju; Mizuta, Naoki; Sumita, Junya; Sakaba, Nariaki; Osaki, Takashi*; Kato, Hideki*; Izawa, Shoichi*; Muto, Takenori*; Gizatulin, S.*; Shaimerdenov, A.*; et al.

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 7 Pages, 2018/10

Graphite materials are used for the in-core components of High Temperature Gas-cooled Reactor (HTGR). Oxidation damage on the graphite components in air ingress accident is a crucial issue for the safety point of view. SiC coating on graphite surface is a possible technique to enhance oxidation resistance. However, it is important to confirm the integrity of this material against high temperature and neutron irradiation for the application of the in-core components. JAEA and Japanese graphite companies carried out the R&D to develop the oxidation-resistant graphite. JAEA and INP investigated the irradiation effects on the oxidation-resistant graphite by using a framework of ISTC partner project. This paper describes the results of post irradiation experiment about the neutron irradiated SiC-coated oxidation-resistant graphite. A brand of oxidation-resistant graphite shows excellent performance against oxidation test after the irradiation.

Journal Articles

Enhancement of oxidation tolerance of graphite materials for high temperature gas-cooled reactor

Mizuta, Naoki; Sumita, Junya; Shibata, Taiju; Osaki, Takashi*; Kato, Hideki*; Izawa, Shoichi*; Muto, Takenori*; Gizatulin, S.*; Sakaba, Nariaki

Tanso Zairyo Kagaku No Shinten; Nihon Gakutsu Shinkokai Dai-117-Iinkai 70-Shunen Kinen-Shi, p.161 - 166, 2018/10

To enhance oxidation resistance of graphite material for in-core components of HTGR, JAEA and four Japanese graphite companies; Toyo Tanso, IBIDEN, Tokai Carbon and Nippon Techno-Carbon, are carrying out for development of oxidation-resistant graphite by CVD-SiC coating. This paper describes the outline of neutron irradiation test about the oxidation-resistant graphite by WWR-K reactor of INP, Kazakhstan through an ISTC partner project. Prior to the irradiation test, the oxidation-resistant graphite by CVD-SiC coating of all specimens showed enough oxidation resistance under un-irradiation condition. The neutron irradiation test was already completed and out-of-pile oxidation test will be carried out at the hot-laboratory of WWR-K.

Journal Articles

Irradiation test about oxidation-resistant graphite in WWR-K research reactor

Shibata, Taiju; Sumita, Junya; Sakaba, Nariaki; Osaki, Takashi*; Kato, Hideki*; Izawa, Shoichi*; Muto, Takenori*; Gizatulin, S.*; Shaimerdenov, A.*; Dyussambayev, D.*; et al.

Proceedings of 8th International Topical Meeting on High Temperature Reactor Technology (HTR 2016) (CD-ROM), p.567 - 571, 2016/11

Graphite are used for the in-core components of HTGR, and it is desirable to enhance oxidation resistance to keep much safety margin. SiC coating is the candidate method for this purpose. JAEA and four Japanese graphite companies are studying to develop oxidation-resistant graphite. Neutron irradiation test was carried out by WWR-K reactor of INP of Kazakhstan through ISTC partner project. The total irradiation cycles of WWR-K operation was 10 cycles by 200 days. Irradiation temperature about 1473 K would be attained. The maximum fast neutron fluence (E $$>$$0.18 MeV) for the capsule irradiated at a central irradiation hole was preliminary calculated as 1.2$$times$$10$$^{25}$$/m$$^{-2}$$, and for the capsule at a peripheral irradiation hole as 4.2$$times$$10$$^{24}$$/m$$^{-2}$$. Dimension and weight of the irradiated specimens were measured, and outer surface of the specimens were observed by optical microscope. For the irradiated oxidation resistant graphite, out-of-pile oxidation test will be carried out at an experimental laboratory.

Journal Articles

Irradiation test plan of oxidation-resistant graphite in WWR-K research reactor

Sumita, Junya; Shibata, Taiju; Sakaba, Nariaki; Osaki, Hiroki*; Kato, Hideki*; Fujitsuka, Kunihiro*; Muto, Takenori*; Gizatulin, S.*; Shaimerdenov, A.*; Dyussambayev, D.*; et al.

Proceedings of 7th International Topical Meeting on High Temperature Reactor Technology (HTR 2014) (USB Flash Drive), 7 Pages, 2014/10

Graphite materials are used for the in-core components of High Temperature Gas-cooled Reactor(HTGR)which is a graphite-moderated and helium gas-cooled reactor. In the case of air ingress accident in HTGR, SiO$$_{2}$$ protective layer is formed on the surface of SiC layer in TRISO CFP and oxidation of SiC does not proceed and fission products are retained inside the fuel particle. A new safety concept for the HTGR, called Naturally Safe HTGR, has been recently proposed. To enhance the safety of Naturally Safe HTGR ultimately, it is expected that oxidation-resistant graphite is used for graphite components to prevent the TRISO CFPs and fuel compacts from failure. SiC coating is one of candidate methods for oxidation-resistant graphite. JAEA and four graphite companies launched R&Ds to develop the oxidation-resistant graphite and the International Science and Technology Center(ISTC) partner project with JAEA and INP was launched to investigate the irradiation effects on the oxidation-resistant graphite. To determine grades of the oxidation-resistant graphite which will be adopted as irradiation test, a preliminary oxidation test was carried out. This paper described the results of the preliminary oxidation test, the plan of out-of-pile test, irradiation test and post-irradiation test(PIE)of the oxidation-resistant graphite.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2009

Sumiya, Shuichi; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Fujita, Hiroki; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; Kokubun, Yuji; et al.

JAEA-Review 2011-004, 161 Pages, 2011/03

JAEA-Review-2011-004.pdf:4.09MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2009 to March 2010. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes.

Journal Articles

Selective vibrational excitation in the resonant Auger decay following core-to-$$pi^*$$ transitions in N$$_2$$O

Travnikova, O.*; C$'e$olin, D.*; Bao, Z.*; B${o}$rve, K. J.*; Tanaka, Takahiro*; Hoshino, Masamitsu*; Kato, Hideki*; Tanaka, Hiroshi*; Harries, J.; Tamenori, Yusuke*; et al.

Journal of Electron Spectroscopy and Related Phenomena, 181(2-3), p.129 - 134, 2010/08

 Times Cited Count:1 Percentile:7.37(Spectroscopy)

In N$$_2$$O a detailed study of the vibrational distribution of the state reached after decay of core-to-$$pi^*$$ excitation of N terminal, N central and O 1s core levels is reported. We observe a change in the relative intensity of bending versus stretching modes while scanning the photon energy across all three resonances. While this effect is known to be due to the Renner-Teller splitting in the core-excited states, we could derive that the antisymmetric stretching is excited mainly in the decay of the N terminal 1s-to-$$pi^*$$ excitation. An explanation for such selectivity is provided in terms of interplay of vibrational structure on potential energy surfaces of different electronic states involved in the process.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2008

Takeishi, Minoru; Sumiya, Shuichi; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki*; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; et al.

JAEA-Review 2009-048, 177 Pages, 2009/12

JAEA-Review-2009-048.pdf:19.3MB
JAEA-Review-2009-048(errata).pdf:0.12MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV; Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2008 to March 2009. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2007

Takeishi, Minoru; Matsuura, Kenichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; Kokubun, Yuji; et al.

JAEA-Review 2008-057, 155 Pages, 2008/11

JAEA-Review-2008-057.pdf:2.15MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of JAEA, Chapter IV; Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged to the atmosphere and the sea during April 2007 to March 2008. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and its trends, meteorological data and discharged radioactive wastes.

Journal Articles

Photoabsorption spectra of CF$$_3$$I and thermally dissociated CF$$_3$$I near the C 1s, I 3d and F 1s ionisation thresholds

Tanaka, Takahiro*; Hoshino, Masamitsu*; Kato, Hideki*; Harries, J.; Tamenori, Yusuke*; Ueda, Kiyoshi*; Tanaka, Hiroshi*

Journal of Electron Spectroscopy and Related Phenomena, 164(1-3), p.24 - 27, 2008/07

 Times Cited Count:4 Percentile:24.49(Spectroscopy)

We report soft X-ray total ion yield and angular-resolved ion yield spectra of CF$$_3$$I in the C 1s, I 3d and F 1s ionisation regions, and tentatively assign the observed electronic states. Anisotropy in ion yield is observed only for the C 1s$$rightarrowsigma^*_{C-I}$$ transition, indicating that the dipole moment for this transition is parallel to the C$$_{3v}$$. The effusive source of CF$$_3$$I is heated to 800 K to produce a mixture of CF$$_3$$ and I, and the resulting spectra are compared to those recorded at room temperature to reveal the first information on the inner-shell excitation of CF$$_3$$.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2006

Takeishi, Minoru; Miyagawa, Naoto; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; Kokubun, Yuji; Kato, Chiaki; et al.

JAEA-Review 2007-044, 155 Pages, 2008/02

JAEA-Review-2007-044.pdf:2.58MB
JAEA-Review-2007-044(errata).pdf:0.13MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of JAEA, Chapter 4; Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged to the atmosphere and the sea during April 2006 to March 2007. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and its trends, meteorological data and discharged radioactive wastes.

JAEA Reports

HTTR hydrogen production system structure and main specifications of mock-up test facility (Contract research)

Kato, Michio; Hayashi, Koji; Aita, Hideki; Ohashi, Hirofumi; Sato, Hiroyuki; Inaba, Yoshitomo; Iwatsuki, Jin; Takada, Shoji; Inagaki, Yoshiyuki

JAEA-Technology 2007-022, 209 Pages, 2007/03

JAEA-Technology-2007-022.pdf:14.46MB

The mock-up test facility was fabricated to investigate performance of the steam generator for mitigation of the temperature fluctuation of helium gas and transient behavior of the hydrogen production system for HTTR and to obtain experimental data for verification of a dynamic analysis code. The test facility has an approximate hydrogen production capacity of 120Nm$$^{3}$$/h and the steam reforming process of methane; CH$$_{4}$$+H$$_{2}$$O=3H$$_{2}$$+CO, was used for hydrogen production of the test facility. An electric heater was used as a heat source instead of the reactor in order to heat helium gas up to 880 $$^{circ}$$C (4MPa) at the chemical reactor inlet which is the same temperature as the HTTR hydrogen production system. Fabrication of the test facility was completed in February in 2002, and seven cycle operations were carried out from March in 2002 to December in 2004. This report describes the structure and main specifications of the test facility.

JAEA Reports

Annual report on the environmental radiation monitoring around Tokai Reprocessing Plant FY2005

Takeishi, Minoru; Miyagawa, Naoto; Nakano, Masanao; Takeyasu, Masanori; Isozaki, Hisaaki; Isozaki, Tokuju; Morisawa, Masato; Fujita, Hiroki; Kokubun, Yuji; Kato, Chiaki; et al.

JAEA-Review 2006-031, 155 Pages, 2006/10

JAEA-Review-2006-031.pdf:7.76MB
JAEA-Review-2006-031(errata).pdf:0.13MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of JAEA, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged to the atmosphere and the sea during April 2005 to March 2006. Appendices present comprehensive information, such as monitoring program, monitoring methods, monitoring results and its trends, meteorological data and discharged radioactive wastes.

JAEA Reports

Annual report on experimental operations and maintenances of mock-up model test facility with a full-scale reaction tube for HTTR hydrogen production system in 2004 fiscal year (Contract research)

Hayashi, Koji; Ohashi, Hirofumi; Morisaki, Norihiro; Kato, Michio; Aita, Hideki; Takeda, Tetsuaki; Nishihara, Tetsuo; Inaba, Yoshitomo; Takada, Shoji; Inagaki, Yoshiyuki

JAEA-Technology 2006-013, 73 Pages, 2006/03

JAEA-Technology-2006-013.pdf:6.27MB

This is annual report on the experimental test operations and maintenances of the mock-up test facility with a full-scale reaction tube for the HTTR hydrogen production system in 2004 fiscal year. The improvement work of catalyst dust filter in combustion system was performed in May 2004, and the performance was confirmed. The sixth experimental test operation was performed from June to July 2004. Periodic inspections on boiler equipment and high-pressure gas production facilities were performed from end of July to September 2004. The seventh experimental test operation was performed from October to December 2004 for chemical reaction shutdown test. From the results, a behavior of the helium-gas cooling system, consists of steam generator and radiator, during chemical reaction shutdown was confirmed. This report is summarized with the outline and the results of the test, maintenance works and inspections, and operation records in mentioned above.

JAEA Reports

Annual report on experimental operations and maintenances of mock-up model test facility with a full-scale reaction tube for HTTR hydrogen production system in 2003 fiscal year (Contract research)

Hayashi, Koji; Morisaki, Norihiro; Ohashi, Hirofumi; Kato, Michio; Aita, Hideki; Takeda, Tetsuaki; Nishihara, Tetsuo; Inaba, Yoshitomo; Takada, Shoji; Inagaki, Yoshiyuki

JAEA-Technology 2006-012, 98 Pages, 2006/03

JAEA-Technology-2006-012.pdf:7.83MB

This is a report on the experimental operations and maintenances of the mock-up test facility with a full-scale reaction tube for the HTTR hydrogen production system in 2003 fiscal year. The fourth and fifth experimental test operations were performed, from May to July and from October to December in 2003, for the following tests; (a)start-up and shutdown operation test, (b)process change test, (c)continuous hydrogen-production test and (d)chemical reaction shutdown test. From the results, a long time-range stability of the hydrogen production system was confirmed, a behavior of the helium-gas cooling system, consists of steam generator and radiator, during chemical reaction shutdown, was understanded, and so on. Periodic inspections on boiler equipment and high-pressure gas production facilities were performed from end of July 2003. This report is summarized on outlines and results of the tests, outlines and results of the periodic inspections, and operation records of the mock-up test facility.

JAEA Reports

Annual report on experimental operations and maintenances of mock-up model test facility with a full-scale reaction tube for HTTR hydrogen production system in 2002 fiscal year (Contract research)

Hayashi, Koji; Ohashi, Hirofumi; Inaba, Yoshitomo; Kato, Michio; Aita, Hideki; Morisaki, Norihiro; Takeda, Tetsuaki; Nishihara, Tetsuo; Takada, Shoji; Inagaki, Yoshiyuki

JAEA-Technology 2006-011, 132 Pages, 2006/03

JAEA-Technology-2006-011.pdf:9.47MB

This report describes 2002 fiscal-year experimental test operations of the mock-up test facility with a full-scale reaction tube for the HTTR hydrogen production system. The improvement works were performed in May 2002. The second experimental test operation was performed from June 2002 and the performances of the improved parts were confirmed. Periodic inspections on boiler equipment and high-pressure gas production facilities were performed from end of July 2002. The third experimental test operation was performed, from October 2002, for (a)start-up and shutdown test, (b)process change test, (c)chemical reaction shutdown test and (d)characteristics test on steam reformer. It was confirmed that the changes of helium gas temperature, caused at steam reformer, could be mitigated into the target range by the steam generator. Maintenance works of high-pressure gas production facilities were also performed in February 2003. This report is summarized with the outline and the results of the test, maintenance works and inspections, and operation records in mentioned above.

JAEA Reports

Annual report on experimental operation of mock-up model test facility with a full-scale reaction tube for HTTR hydrogen production system in 2001 fiscal year (Contract research)

Hayashi, Koji; Inagaki, Yoshiyuki; Kato, Michio; Fujisaki, Katsuo*; Aita, Hideki; Takeda, Tetsuaki; Nishihara, Tetsuo; Inaba, Yoshitomo; Ohashi, Hirofumi; Katanishi, Shoji; et al.

JAERI-Tech 2005-032, 46 Pages, 2005/06

JAERI-Tech-2005-032.pdf:4.79MB

This is annual report on the experimental operation of the mock-up test facility with a full-scale reaction tube for the HTTR hydrogen production system in 2001 fiscal year. The first experimental operation was performed during two weeks from March 1, 2002 to March 13, 2002 to test on the thermal hydraulic performance of the steam reformer and also to train the operators. The thermal hydraulic performance test of the steam reformer was performed to evaluate the heat transfer characteristics between helium gas and process gas in the steam reformer. This report is summarized with an overview of the test, the results and its operation records.

JAEA Reports

Heat transfer characteristics evaluation of heat exchangers of mock-up test facility with full-scale reaction tube for HTTR hydrogen production system (Contract research)

Shimizu, Akira; Ohashi, Hirofumi; Kato, Michio; Hayashi, Koji; Aita, Hideki; Nishihara, Tetsuo; Inaba, Yoshitomo; Takada, Shoji; Morisaki, Norihiro; Sakaki, Akihiro*; et al.

JAERI-Tech 2005-031, 174 Pages, 2005/06

JAERI-Tech-2005-031.pdf:20.71MB

Connection of hydrogen production system by steam reforming of methane to the High Temperature Engineering Test Reactor (HTTR) of the Japan Atomic Energy Research Institute (JAERI) has been surveyed until now. Mock-up test facility of this steam reforming system with full-scale reaction tube was constructed in FY 2001, and a lot of operational test data on heat exchanges were obtained in these tests.In this report specifications, structures and heat transfer formulae of steam reformer, steam superheater, steam generator, condenser, helium gas cooler, feed gas heater and feed gas superheater were described. Evaluation codes were newly made to evaluate heat transfer characteristics from measured test data. Overall heat-transfer coefficient obtained from the experimental data were compared and evaluated with the prospective value calculated with heat transfer formulae. As a result, heat transfer performance and thermal efficiency of these heat exchangers were confirmed to be appropriate.

JAEA Reports

Improvement works report on mock-up model test facility with a full-scale reaction tube for HTTR hydrogen production system (Contract research)

Sakaki, Akihiro*; Kato, Michio; Hayashi, Koji; Fujisaki, Katsuo*; Aita, Hideki; Ohashi, Hirofumi; Takada, Shoji; Shimizu, Akira; Morisaki, Norihiro; Maeda, Yukimasa; et al.

JAERI-Tech 2005-023, 72 Pages, 2005/04

JAERI-Tech-2005-023.pdf:14.86MB

In order to establish the system integration technology to connect a hydrogen production system to a high temperature gas cooled reactor, the mock-up test facility with a full-scale reaction tube for the steam reforming HTTR hydrogen production system was constructed in fiscal year 2001 and its functional test operation was performed in the year. Seven experimental test operations were performed from fiscal year 2001 to 2004. On a period of each test operation, there happened some troubles. For each trouble, the cause was investigated and the countermeasures and the improvement works were performed to succeed the experiments. The tests were successfully achieved according to plan.This report describes the improvement works on the test facility performed from fiscal year 2001 to 2004.

Journal Articles

Elution curve of Rutherfordium (Rf) in anion-exchange chromatography with hydrofluoric acid solution

Toyoshima, Atsushi; Haba, Hiromitsu*; Tsukada, Kazuaki; Asai, Masato; Akiyama, Kazuhiko; Nishinaka, Ichiro; Nagame, Yuichiro; Saika, Daisuke*; Matsuo, Keishi*; Sato, Wataru*; et al.

Journal of Nuclear and Radiochemical Sciences, 5(2), p.45 - 48, 2004/12

no abstracts in English

JAEA Reports

Performance test results of mock-up model test facility with a full-scale reaction tube for HTTR hydrogen production system (Contract research)

Inagaki, Yoshiyuki; Hayashi, Koji; Kato, Michio; Fujisaki, Katsuo; Aita, Hideki; Takeda, Tetsuaki; Nishihara, Tetsuo; Inaba, Yoshitomo; Ohashi, Hirofumi; Katanishi, Shoji; et al.

JAERI-Tech 2003-034, 129 Pages, 2003/05

JAERI-Tech-2003-034.pdf:7.62MB

no abstracts in English

36 (Records 1-20 displayed on this page)