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Journal Articles

Longitudinal spin fluctuations driving field-reinforced superconductivity in UTe$$_2$$

Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori; Kitagawa, Shunsaku*; Ishida, Kenji*; Aoki, Dai*; Knebel, G.*; et al.

Physical Review Letters, 131(22), p.226503_1 - 226503_7, 2023/12

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Superconducting spin reorientation in spin-triplet multiple superconducting phases of UTe$$_2$$

Kinjo, Katsuki*; Fujibayashi, Hiroki*; Matsumura, Hiroki*; Hori, Fumiya*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; et al.

Science Advances (Internet), 9(30), p.2736_1 - 2736_6, 2023/07

 Times Cited Count:0 Percentile:0(Multidisciplinary Sciences)

Journal Articles

Low-temperature magnetic fluctuations investigated by $$^{125}$$Te-NMR on the uranium-based superconductor UTe$$_2$$

Fujibayashi, Hiroki*; Kinjo, Katsuki*; Nakamine, Genki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; et al.

Journal of the Physical Society of Japan, 92(5), p.053702_1 - 053702_5, 2023/05

 Times Cited Count:2 Percentile:80.44(Physics, Multidisciplinary)

Journal Articles

Large reduction in the $$a$$-axis knight shift on UTe$$_2$$ with $$T_c$$ = 2.1 K

Matsumura, Hiroki*; Fujibayashi, Hiroki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; et al.

Journal of the Physical Society of Japan, 92(6), p.063701_1 - 063701_5, 2023/05

 Times Cited Count:5 Percentile:92.42(Physics, Multidisciplinary)

Journal Articles

Physics of spin-triplet superconductivity in uranium compounds studied by NMR

Tokunaga, Yo; Sakai, Hironori; Kitagawa, Shunsaku*; Ishida, Kenji*

Nihon Butsuri Gakkai-Shi, 78(5), p.267 - 272, 2023/04

no abstracts in English

Journal Articles

Change of superconducting character in UTe$$_{2}$$ induced by magnetic field

Kinjo, Katsuki*; Fujibayashi, Hiroki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; Homma, Yoshiya*; et al.

Physical Review B, 107(6), p.L060502_1 - L060502_5, 2023/02

 Times Cited Count:7 Percentile:93.16(Materials Science, Multidisciplinary)

Journal Articles

Investigation of physical properties of glove for glove-box and estimation of its life-time

Kobayashi, Daisuke; Yamamoto, Masahiko; Nishida, Naoki; Miyoshi, Ryuta; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kato, Keisuke; Nishino, Saki; Kuno, Takehiko; Kitao, Takahiko; et al.

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.237 - 240, 2022/07

All gloves attached to glove-box in Tokai Reprocessing Plant have a fixed expiration date and have to be replaced every 4-year. However, degrees of glove deterioration are different depending on its usage environment (frequency, chemicals, radiation, etc.), because of rubber products. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured, and the life-time of gloves are estimated. As a result, gloves without any defects in its appearance have enough physical property for acceptance criteria of new glove. The extrapolated physical property of glove is sufficiently larger than the reported values of damaged glove. No deterioration in physical properties of gloves, that are periodically replaced without any defects in its appearance, is observed and the usable life-time of the glove is estimated to be 8 years.

Journal Articles

Hydrogen absorption and diffusion behaviors in cube-shaped palladium nanoparticles revealed by ambient-pressure X-ray photoelectron spectroscopy

Tang, J.*; Seo, O.*; Rivera Rocabado, D. S.*; Koitaya, Takanori*; Yamamoto, Susumu*; Namba, Yusuke*; Song, C.*; Kim, J.*; Yoshigoe, Akitaka; Koyama, Michihisa*; et al.

Applied Surface Science, 587, p.152797_1 - 152797_8, 2022/06

 Times Cited Count:7 Percentile:77.62(Chemistry, Physical)

The hydrogen absorption and diffusion mechanisms on cube-shaped Pd nanoparticles (NPs) which are important hydrogen-storage materials were studied using X-ray photoelectron spectroscopy and DFT calculations. In the surface region, hydrogen absorption showed almost similar behavior regardless of the NPs size. It was found that the octahedral sites are more favorable than the tetrahedral sites for hydrogen occupation. We also clarified that the hydrogen atoms absorbing on the smaller-sized Pd NPs diffuse to the subsurface more actively because of the weakened Pd-H bond by the surface disordering, which plays an important role in hydrogen adsorption at a low H$$_{2}$$ pressure.

Journal Articles

Drastic change in magnetic anisotropy of UTe$$_2$$ under pressure revealed by $$^{125}$$Te-NMR

Kinjo, Katsuki*; Fujibayashi, Hiroki*; Nakamine, Genki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; et al.

Physical Review B, 105(14), p.L140502_1 - L140502_5, 2022/04

 Times Cited Count:5 Percentile:67.2(Materials Science, Multidisciplinary)

Journal Articles

Slow electronic dynamics in the paramagnetic state of UTe$$_2$$

Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Haga, Yoshinori; Tokiwa, Yoshifumi; Opletal, P.; Fujibayashi, Hiroki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; et al.

Journal of the Physical Society of Japan, 91(2), p.023707_1 - 023707_5, 2022/02

 Times Cited Count:14 Percentile:93.17(Physics, Multidisciplinary)

$$^{125}$$Te NMR experiments in field ($$H$$) applied along the easy magnetization axis (the $$a$$-axis) revealed slow electronic dynamics developing in the paramagnetic state of UTe$$_2$$. The observed slow fluctuations are concerned with a successive growth of long-range electronic correlations below 30$$-$$40 K, where the spin susceptibility along the hard magnetization axis (the $$b$$-axis) shows a broad maximum. The experiments also imply that tiny amounts of disorder or defects locally disturb the long-range electronic correlations and develop an inhomogeneous electronic state at low temperatures, leading to a low temperature upturn observed in the bulk-susceptibility in $$H|a$$. We suggest that UTe$$_2$$ would be located on the paramagnetic side near an electronic phase boundary, where either the magnetic or Fermi-surface instability would be the origin of the characteristic fluctuations.

Journal Articles

Inhomogeneous superconducting state probed by $$^{125}$$Te NMR on UTe$$_2$$

Nakamine, Genki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; Homma, Yoshiya*; et al.

Journal of the Physical Society of Japan, 90(6), p.064709_1 - 064709_7, 2021/06

 Times Cited Count:17 Percentile:85.26(Physics, Multidisciplinary)

Journal Articles

Anisotropic response of spin susceptibility in the superconducting state of UTe$$_2$$ probed with $$^{125}$$Te-NMR measurement

Nakamine, Genki*; Kinjo, Katsuki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; Homma, Yoshiya*; et al.

Physical Review B, 103(10), p.L100503_1 - L100503_5, 2021/03

 Times Cited Count:32 Percentile:93.31(Materials Science, Multidisciplinary)

Journal Articles

Hydrogen absorption and desorption on Rh nanoparticles revealed by ${it in situ}$ dispersive X-ray absorption fine structure spectroscopy

Song, C.*; Seo, O.*; Matsumura, Daiju; Hiroi, Satoshi*; Cui, Y.-T.*; Kim, J.*; Chen, Y.*; Tayal, A.*; Kusada, Kohei*; Kobayashi, Hirokazu*; et al.

RSC Advances (Internet), 10(34), p.19751 - 19758, 2020/05

 Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)

Journal Articles

Superconducting properties of heavy fermion UTe$$_2$$ revealed by $$^{125}$$Te-nuclear magnetic resonance

Nakamine, Genki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Nakamura, Ai*; Shimizu, Yusei*; Homma, Yoshiya*; Li, D.*; et al.

Journal of the Physical Society of Japan, 88(11), p.113703_1 - 113703_4, 2019/11

 Times Cited Count:68 Percentile:95.42(Physics, Multidisciplinary)

Journal Articles

$$^{125}$$Te-NMR study on a single crystal of heavy fermion superconductor UTe$$_2$$

Tokunaga, Yo; Sakai, Hironori; Kambe, Shinsaku; Hattori, Taisuke; Higa, Nonoka; Nakamine, Genki*; Kitagawa, Shunsaku*; Ishida, Kenji*; Nakamura, Ai*; Shimizu, Yusei*; et al.

Journal of the Physical Society of Japan, 88(7), p.073701_1 - 073701_4, 2019/07

 Times Cited Count:58 Percentile:94.69(Physics, Multidisciplinary)

We report $$^{125}$$Te-NMR studies on a newly discovered heavy fermion superconductor UTe$$_2$$. Using a single crystal, we have measured the $$^{125}$$Te-NMR Knight shift $$K$$ and spin-lattice relaxation rate $$1/T_1$$ for fields along the three orthorhombic crystal axes. The data confirm a moderate Ising anisotropy for both the static ($$K$$) and dynamical susceptibilities ($$1/T_1$$) in the paramagnetic state above about 20 K. Around 20 K, however, we have observed a sudden loss of NMR spin-echo signal due to sudden enhancement of the NMR spin-spin relaxation rate $$1/T_2$$, when the field is applied along the easy axis of magnetization (=$$a$$ axis). This behavior suggests the development of longitudinal magnetic fluctuations along the $$a$$ axis at very low frequencies below 20 K.

Journal Articles

Vibrational states of atomic hydrogen in bulk and nanocrystalline palladium studied by neutron spectroscopy

Kofu, Maiko; Hashimoto, Naoki*; Akiba, Hiroshi*; Kobayashi, Hirokazu*; Kitagawa, Hiroshi*; Iida, Kazuki*; Nakamura, Mitsutaka; Yamamuro, Osamu*

Physical Review B, 96(5), p.054304_1 - 054304_7, 2017/08

 Times Cited Count:15 Percentile:58.3(Materials Science, Multidisciplinary)

The vibrational states of hydrogen atoms in bulk and nanocrystalline palladium were examined in a wide energy region $$0 le hbar omega le 300$$ meV using neutron spectroscopy. In bulk PdH$$_{0.73}$$, the vibrational excitations of H atoms were roughly reproduced by the quantum harmonic oscillator (QHO) model. In PdH$$_{0.42}$$ nanocrystals with a diameter of 8 nm, however, additional vibrational excitations were found at energies above 80 meV. The energies and intensities of the additional states were not explained by QHO but reasonably described as vibrations in a highly anharmonic trumpet-like potential. The additional excitations are attributed to the vibrations of H atoms at tetrahedral sites in the subsurface region stabilized by surface effects. This is an experimental work which clearly detects hydrogen vibration ${it inside}$ metal nanoparticles.

Journal Articles

$$^{61}$$Ni synchrotron radiation-based M$"o$ssbauer spectroscopy of nickel-based nanoparticles with hexagonal structure

Masuda, Ryo*; Kobayashi, Yasuhiro*; Kitao, Shinji*; Kurokuzu, Masayuki*; Saito, Makina*; Yoda, Yoshitaka*; Mitsui, Takaya; Hosoi, Kohei*; Kobayashi, Hirokazu*; Kitagawa, Hiroshi*; et al.

Scientific Reports (Internet), 6, p.20861_1 - 20861_8, 2016/02

 Times Cited Count:9 Percentile:40.77(Multidisciplinary Sciences)

Journal Articles

Study on chemical reactivity control of sodium by suspended nanoparticles, 1

Ara, Kuniaki; Sugiyama, Kenichiro*; Kitagawa, Hiroshi*; Nagai, Masahiko*; Yoshioka, Naoki*

Journal of Nuclear Science and Technology, 47(12), p.1165 - 1170, 2010/12

 Times Cited Count:11 Percentile:59.22(Nuclear Science & Technology)

A study on the chemical reactivity control of sodium utilizing the atomic interaction of sodium with suspended nanoparticles was carried out. The atomic interaction between nanoparticles and sodium atoms were estimated by theoretical calculations and verified by fundamental physical properties measurements. Results showed the atomic bond of the sodium atom and the nanoparticle atom was significantly larger than that of the sodium atoms, when the transition metals that have the property of large electronegativity are applied as nanoparticles. From the theoretical calculation results, it was suggested that charge transfer occurs from the sodium atom to the nanoparticle atom. The fundamental physical properties of sodium with suspended nanoparticles were examined in comparison with that of sodium to verify the change of the atomic interaction. From the experimental results, it became clear that the surface tension becomes larger and the evaporation rate becomes smaller. These changes in fundamental physical properties were measured to verify the stability of the atomic interaction under the conditions of wide temperature range and the phase transformation from solid phase to liquid phase.

Journal Articles

Study on chemical reactivity control of sodium by suspended nanoparticles, 2

Ara, Kuniaki; Sugiyama, Kenichiro*; Kitagawa, Hiroshi*; Nagai, Masahiko*; Yoshioka, Naoki*

Journal of Nuclear Science and Technology, 47(12), p.1171 - 1181, 2010/12

 Times Cited Count:10 Percentile:56.32(Nuclear Science & Technology)

A study was conducted on the control of the chemical reactivity of sodium utilizing the atomic interaction between sodium and nanoparticles. The authors reported in a previous paper that the atomic interaction between sodium and nanoparticles increases and has the potential to suppress chemical reactivity. In this paper, the authors examined the released reaction heat and the reaction behavior. As a result, it was confirmed that the released reaction heat and the reaction rate decreased. From the results of experimental studies, it is clear that the suppressions of chemical reactivity are caused by a change in the sodium evaporation rate and fundamental physical properties such as surface tension which originate in the change in the atomic interaction between sodium and nanoparticle atoms. The suppression of chemical reactivity applying to FBR coolant was estimated for the case of sodium combustion and sodium-water reaction. It was confirmed that the concept of suspending nanoparticles into sodium has high potential for the suppression of chemical reactivity. Applicability as coolant to the FBR was investigated, including not only the chemical reaction properties but also the aspects of heat transfer and operation.

Journal Articles

Study on chemical reactivity control of liquid sodium; Development of nano-fluid and its property and applicability to FBR plant

Saito, Junichi; Ara, Kuniaki; Sugiyama, Kenichiro*; Kitagawa, Hiroshi*; Nakano, Haruyuki*; Ogata, Kan*; Yoshioka, Naoki*

Proceedings of 16th International Conference on Nuclear Engineering (ICONE-16) (CD-ROM), 4 Pages, 2008/05

no abstracts in English

42 (Records 1-20 displayed on this page)