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Journal Articles

Study on criticality safety control of fuel debris for validation of methodology applied to the safety regulation

Suyama, Kenya; Ueki, Taro; Gunji, Satoshi; Watanabe, Tomoaki; Araki, Shohei; Fukuda, Kodai; Yamane, Yuichi; Izawa, Kazuhiko; Nagaya, Yasunobu; Kikuchi, Takeo; et al.

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 6 Pages, 2023/10

To remove and store safely the fuel debris generated by the severe accident of the Fukushima Daiichi Nuclear Power Station in 2011 is one of the most important and challenging topics for decommissioning of the damaged reactors in Fukushima. To validate the adopted method for the evaluation of criticality safety control of the fuel debris through comparison with the experimental data obtained by the criticality experiments, the Nuclear Regulation Authority (NRA) of Japan funds a research and development project which was entrusted to the Nuclear Safety Research Center (NSRC) of Japan Atomic Energy Agency (JAEA) from 2014. In this project, JAEA has been conducting such activities as i) comprehensive computation of the criticality characteristics of the fuel debris and making database (criticality map of the fuel debris), ii) development of new continuous energy Monte Carlo code, iii) evaluation of criticality accident and iv) modification of the critical assembly STACY for the experiments for validation of criticality safety control methodology. After the last ICNC2019, the project has the substantial progress in the modification of STACY which will start officially operation from May 2024 and the development of the Monte Carlo Code "Solomon" suitable for the criticality calculation for materials having spatially random distribution complies with the power spectrum. We present the whole picture of this research and development project and status of each technical topics in the session.

Journal Articles

Criticality characteristics of fuel debris mixed by fuels with different burnups based on fuel loading pattern

Watanabe, Tomoaki; Okubo, Kiyoshi*; Araki, Shohei; Tonoike, Kotaro

Proceedings of 11th International Conference on Nuclear Criticality Safety (ICNC 2019) (Internet), 8 Pages, 2019/09

Journal Articles

Criticality characteristics of MCCI products possibly produced in reactors of Fukushima Daiichi Nuclear Power Station

Tonoike, Kotaro; Okubo, Kiyoshi; Takada, Tomoyuki*

Proceedings of International Conference on Nuclear Criticality Safety (ICNC 2015) (DVD-ROM), p.292 - 300, 2015/09

The damaged Unit 1-3 reactors of the Fukushima Daiichi Nuclear Power Station may contain fuel debris of a significant amount that is in a form of molten-core-concrete-interaction (MCCI) product with porous structure. Such low density MCCI product including fissile material is a great concern for its criticality control, especially under submerged condition, due to its fairly good neutron moderation. This report shows computation results of basic criticality characteristics of the MCCI product, which will facilitate criticality risk assessments during decommissioning of the reactors. The results imply that water bound in concrete may raise the risk from the viewpoints of possibility of criticality events and of effectiveness of mitigation measures such as neutron poison injection into coolant water.

JAEA Reports

Examination of measurement method of isotopic composition of fission products in spent fuel

Fukaya, Hiroyuki; Suyama, Kenya; Sonoda, Takashi; Okubo, Kiyoshi; Umeda, Miki; Uchiyama, Gunzo

JAEA-Research 2013-020, 81 Pages, 2013/10

JAEA-Research-2013-020.pdf:3.81MB

Japan Atomic Energy Agency conducted a project "Isotopic Composition measurement of Fission Products in Spent Fuel from FY2008 to FY2011" by the entrustment of Japan Nuclear Energy Safety Organization. In that project, we measured the isotopic composition of neodymium isotopes which are important to evaluate the burnup value of spent nuclear fuel by using two different methods and obtained different results. So that we carried out the follow-up measurement in order to investigate the reason of the difference between two neodymium measurements. It was found that we needed correction to the measurement results of neodymium for two samples and a part of other fission products for all samples in total five samples. This report summarizes the all works carried out in this follow-up measurement and obtained results.

Journal Articles

Infinite multiplication factor of low-enriched UO$$_2$$-concrete system

Izawa, Kazuhiko; Uchida, Yuriko; Okubo, Kiyoshi; Totsuka, Masayoshi; Sono, Hiroki; Tonoike, Kotaro

Journal of Nuclear Science and Technology, 49(11), p.1043 - 1047, 2012/11

AA2012-0375.pdf:0.63MB

 Times Cited Count:12 Percentile:66.54(Nuclear Science & Technology)

Possibility of criticality of fuel debris in a form of UO$$_2$$-concrete mixture is evaluated by calculating infinite multiplication factor ($$k_infty$$) for a study of criticality control on the fuel debris generated through the molten core concrete interaction (MCCI) in a severe accident of a light water reactor (LWR). The infinite multiplication factor can be greater than unity, which means that handling of the mixture is subject to criticality control. This paper shows that concrete have efficient slowing-down capability of neutron and points out the necessity of further investigations on the criticality of low-enriched UO$$_2$$-concrete system for actual handling of fuel debris.

Journal Articles

Study on reactivity effect of fission products for introducing burnup credit into the criticality safety evaluation of spent nuclear fuel

Okubo, Kiyoshi*; Suyama, Kenya; Uchiyama, Gunzo

Proceedings of International Conference on Toward and Over the Fukushima Daiichi Accident (GLOBAL 2011) (CD-ROM), 6 Pages, 2011/12

The amount of the spent nuclear fuel (SNF) stored at the nuclear reactor sites is increasing continuously in Japan. To correspond to such a situation, it is considered to take into account the decrease in the reactivity of SNF according to the burnup for the criticality safety control of SNF. This idea is called as burnup credit. If the negative reactivity effect of the fission product nuclides accumulated during the burnup is adopted into the burnup credit which considers only uranium and plutonium, the amount of fuel assembly that can be treated in the same facility is increased. This study reveals the reactivity effect of fission products has almost linear correlation with the increase of burnup SNF for both solution and heterogeneous systems. The negative reactivity effect of the selected fission product is equal to the increase of the burnup of approximately 20-25% for the solution system and 30-35% for the heterogeneous system respectively. It also implies that the estimation error of burnup value of 20% could be acceptable if we take the burnup credit adopting only uranium and plutonium isotopes, considering the fission products as the safety margin.

Journal Articles

Re-evaluation of assay data of spent nuclear fuel obtained at Japan Atomic Energy Research Institute for validation of burnup calculation code systems

Suyama, Kenya; Murazaki, Minoru*; Okubo, Kiyoshi; Nakahara, Yoshinori*; Uchiyama, Gunzo

Annals of Nuclear Energy, 38(5), p.930 - 941, 2011/05

 Times Cited Count:13 Percentile:69.64(Nuclear Science & Technology)

The isotopic composition of spent nuclear fuels is vital data for studies on the nuclear fuel cycle and reactor physics. The Japan Atomic Energy Agency (JAEA) has been active in obtaining such data for pressurized water reactor (PWR) and boiling water reactor (BWR) fuels, and some data has already been published. These data have been registered with the international Spent Fuel Isotopic Composition Database (SFCOMPO) and widely used as international benchmarks for burnup calculation codes and libraries. In this paper, postirradiation examination (PIE) data from two fuel assemblies irradiated in the Ohi-1 and Ohi-2 PWRs in Japan are shown. The PIE data from Ohi-2 has already been published. However, these data were not suitable for the benchmarking of calculation codes and libraries because several important specifications and data were not included. This paper summarizes the details of PIE data from Ohi-1 and Ohi-2 and shows in detail the data and specifications required for analyses of isotopic composition. For precise burnup analyses, the burnup values of PIE samples were re-evaluated in this study. These PIE data were analyzed using the SWAT2.1 code, and the calculation results showed good agreement with experimental results. This indicates that the quality of PIE data from Ohi-1 and Ohi-2 PWRs is high, and that these PIE data are suitable for the benchmarking of burnup calculation code systems.

JAEA Reports

SWAT3.1; The Integrated burnup code system driving continuous energy Monte Carlo codes MVP and MCNP

Suyama, Kenya; Mochizuki, Hiroki*; Takada, Tomoyuki*; Ryufuku, Susumu*; Okuno, Hiroshi; Murazaki, Minoru; Okubo, Kiyoshi

JAEA-Data/Code 2009-002, 124 Pages, 2009/05

JAEA-Data-Code-2009-002.pdf:14.09MB

Integrated burnup calculation code system SWAT is a system that combines neutronics calculation code SRAC widely used in Japan and point burnup calculation code ORIGEN2. It has been used to evaluate the composition of the uranium, plutonium, minor actinide and the fission products in the spent nuclear fuel. Because of the ability to treat the arbitrary fuel geometry and no requirement of generating the effective cross section data, there is a great advantage to introduce continuous energy Monte Carlo Code into the burnup calculation code. Based on this idea, the integrated burnup calculation code system SWAT3.1 was developed by combining the continuous energy Monte Carlo code MVP and MCNP and ORIGEN2. This report describes the outline, input data instruction and several example of the calculation.

Journal Articles

Active reduction of the end effect by local installation of neutron absorbers

Suyama, Kenya; Murazaki, Minoru; Okubo, Kiyoshi; Okuno, Hiroshi

Annals of Nuclear Energy, 35(9), p.1628 - 1635, 2008/09

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

In the analysis of the burnup credit, it has been pointed out that the neutron multiplication factor becomes greater if we consider an axial burnup distribution of spent fuel assemblies than the case under an assumption of an average burnup through the fuel assemblies. This phenomenon is called "end effect" and it is one of the main technical issues in the burnup credit study. In this study, the reason why the end effect occurs in the criticality calculation of spent fuel assemblies is discussed by analyses of neutron flux distribution measurement both fixed source and eigenvalue calculations. These calculations show us that the end effect is induced by the solution of neutron balance equation as eigenvalue problem and an actual neutron flux increase occurs only when the neutron multiplication factor is close to unity. Based on the discussion, reducing the end effect actively by local installation of neutron absorbers (LINA) around the end regions of the fuel assemblies are proposed and its effect was confirmed based on the several criticality calculations.

Journal Articles

Reactivity effect measurement of neutron interaction between two slab cores containing 10% enriched uranyl nitrate solution without neutron isolater

Tonoike, Kotaro; Miyoshi, Yoshinori; Okubo, Kiyoshi

Journal of Nuclear Science and Technology, 40(4), p.238 - 245, 2003/04

 Times Cited Count:2 Percentile:19(Nuclear Science & Technology)

The reactivity effect of neutron interaction between two identical units containing low enriched (10% $$^{235}$$ enrichment) uranyl nitrate solution was measured in the STACY. The unit has 350mm of thickness and 690mm of width and distance between those two units was adjustable from 0mm to 1450mm. Condition of the solution was about 290gU/L in uranium concentration, about 0.8N in free nitric acid molarity, 24$$sim$$27$$^{circ}$$C in temperature and about 1.4g/cm$$^{3}$$ in solution density. The reactivity effect was estimated from variation of critical solution level from 495mm to 763mm depending on the core distance. The reactivity effect was also evaluated by the solid angle method and a computational method using the continuous energy Monte Carlo code MCNP-4C and the nuclear data library JENDL3.2. Comparison of those estimations is presented.

Oral presentation

Criticality safety evaluation of damaged burned nuclear fuel; Effect of structural materials

Okubo, Kiyoshi; Suyama, Kenya; Kashima, Takao; Tonoike, Kotaro; Takada, Tomoyuki*

no journal, , 

Criticality safety analysis is necessary for the damaged-fuel handling in the Fukushima Daiichi NPP decommissioning. This presentation show influence of structural materials such as Zry-2, Fe, concrete expected to be present in the damaged fuel. Multiplication factor (kinf) decreases most by replacing moisture, in the damaged fuel, with iron. Replacement of all moisture with Zry-2 gives the same influence as iron, although decrease rate of kinf is lower because of the smaller absorb cross section of Zry-2. Concrete has much less influence due to the neutron moderation by hydrogen contained in concrete, which calls attention on handling of the concrete-fuel mixture. Effect as reflector of the materials is also evaluated.

Oral presentation

Critical Mass estimation of MCCI products

Tonoike, Kotaro; Okubo, Kiyoshi; Takada, Tomoyuki*

no journal, , 

no abstracts in English

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