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Saito, Takumi*; Nishi, Shusaku*; Amano, Yuki; Beppu, Hikari*; Miyakawa, Kazuya
ACS ES&T Water (Internet), 3(12), p.4103 - 4112, 2023/12
MethanoperedenaceaeNishimura, Hiroki*; Kozuka, Mariko*; Fukuda, Akari*; Ishimura, Toyoho*; Amano, Yuki; Beppu, Hikari*; Miyakawa, Kazuya; Suzuki, Yohei*
Environmental Microbiology Reports (Internet), 15(3), p.197 - 205, 2023/06
Times Cited Count：1 Percentile：59.23(Environmental Sciences)The family Methanoperedenaceae archaea mediate anaerobic oxidation of methane (AOM). We newly developed a high-pressure laboratory incubation system and investigated groundwater from 214- and 249-m deep boreholes at Horonobe Underground Research Laboratory, Japan, where the high and low abundances of Methanoperedenaceae archaea have been revealed, respectively. We incubated the samples amended with or without amorphous Fe(III) and 
C-labelled methane at an in-situ pressure of 1.6 MPa. After three to seven-day incubation, AOM activities were not detected from the 249-m sample but from the 214-m sample. The AOM rates were 93.7
40.6 and 27.737.5 nM/day with and without Fe(III) amendment. Suspended particulates were not visible in the 249-m sample on the filter, while they were abundant and contained amorphous Fe(III) and Fe(III)-bearing phyllosilicates in the 214-m sample. This supports the in-situ activity of Fe(III)-dependent AOM in the deep subsurface borehole.
Terashima, Motoki; Endo, Takashi*; Kimuro, Shingo; Beppu, Hikari*; Nemoto, Kazuaki*; Amano, Yuki
Journal of Nuclear Science and Technology, 60(4), p.374 - 384, 2023/04
Times Cited Count：2 Percentile：53.91(Nuclear Science & Technology)Nagae, Daisuke*; Abe, Yasushi*; Okada, Shunsuke*; Omika, Shuichiro*; Wakayama, Kiyoshi*; Hosoi, Shun*; Suzuki, Shinji*; Moriguchi, Tetsuro*; Amano, Masamichi*; Kamioka, Daiki*; et al.
Nuclear Instruments and Methods in Physics Research A, 986, p.164713_1 - 164713_7, 2021/01
Times Cited Count：5 Percentile：65.59(Instruments & Instrumentation)Ikebe, Yurie*; Oshima, Masumi*; Bamba, Shigeru*; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi*; Bi, C.*; Seto, Hirofumi*; Amano, Hikaru*; et al.
Applied Radiation and Isotopes, 164, p.109106_1 - 109106_7, 2020/10
Times Cited Count：2 Percentile：24.28(Chemistry, Inorganic & Nuclear)Boron Neutron Capture Therapy (BNCT) is a radiotherapy for the treatment of intractable cancer. In BNCT precise determination of 
B concentration in whole blood sample before neutron irradiation is crucial for control of the neutron irradiation time and the neutron dosimetry. We have applied the Charged Particle Activation Analysis (CPAA) to non-destructive and accurate determination of B concentration in whole blood sample. The experiment was performed at JAEA Tandem Accelerator using an 8 MeV proton beam. The 478 keV 
ray of 
Be produced in the B(p,
)Be reaction was used to quantify the B, and rays of 
Co originating from the reaction with Fe in blood was used to normalize the -ray intensity. The results demonstrated that the present CPAA method can be applied to the determination of the B concentration in the blood sample.
Cs and 
C in a Japanese forest soil profile and their implications for the fate and migration processes of Fukushima-derived CsKoarashi, Jun; Atarashi-Andoh, Mariko; Amano, Hikaru*; Matsunaga, Takeshi
Journal of Radioanalytical and Nuclear Chemistry, 311(1), p.473 - 481, 2017/01
Times Cited Count：17 Percentile：85.35(Chemistry, Analytical)Vertical distributions of global fallout Cs and C were investigated in a Japanese forest soil in 2001. Even 38 years after the fallout, Cs was still observed mostly in the uppermost 5 cm. A preferential accumulation of Cs was found in a 1-cm-thick transition layer between organic-rich A and underlying B horizons. This unique observation indicated that Cs migrated through the A horizon at a rate of 0.20% y
and the transition layer acted as a barrier for Cs migration to deeper layers. The vertical distributions of Cs and C were significantly correlated, suggesting a coupled downward migration of Cs and organic matter on a time scale of decades, along the same physical pathways.
Hama, Katsuhiro; Mizuno, Takashi; Sasao, Eiji; Iwatsuki, Teruki; Saegusa, Hiromitsu; Sato, Toshinori; Fujita, Tomoo; Sasamoto, Hiroshi; Matsuoka, Toshiyuki; Yokota, Hideharu; et al.
JAEA-Research 2015-007, 269 Pages, 2015/08
JAEA-Research-2015-007.pdf:68.65MBJAEA-Research-2015-007(errata).pdf:0.07MB
We have synthesised the research results from Mizunami/Horonobe URLs and geo-stability projects in the second mid-term research phase. It could be used as technical bases for NUMO/Regulator in each decision point from sitting to beginning of disposal (Principal Investigation to Detailed Investigation Phase). High quality construction techniques and field investigation methods have been developed and implemented and these will be directly applicable to the National Disposal Program (along with general assessments of hazardous natural events and processes). It will be crucial to acquire technical knowledge on decisions of partial backfilling and final closure by actual field experiments in Mizunami/Horonobe URLs as main themes for the next phases.
Kushita, Kohei; Atarashi-Andoh, Mariko; Amano, Hikaru*
Bunseki Kagaku, 63(11), p.867 - 871, 2014/11
Times Cited Count：0 Percentile：0(Chemistry, Analytical)We report here the study of activated gold for the estimation of neutron dose in the environment in the case of JCO criticality accident happened in Tokai, Japan, in 1999. We collected and analyzed 16 gold samples, such as ring, coin or necklace stored at residents houses in the range from 168 to 568 m from the accident place of JCO. They gave activities from 91.9 to 0.322 Bq/g-Au as standardized values at 06:15, Oct. 1, 1999, when the criticality reaction had ceased after 20 hours of continuation. The induced radioactivity of gold samples showed a good correlation as a power function of distance. The induced radioactivity of gold is discussed with reference data to estimate dose equivalent in the environment around JCO. This paper gives an example showing the usefulness of gold in the field of nuclear and radiation studies and applications.
Shiga, Hideaki*; Taki, Junichi*; Washiyama, Koshin*; Yamamoto, Jumpei*; Kinase, Sakae; Okuda, Koichi*; Kinuya, Seigo*; Watanabe, Naoto*; Tonami, Hisao*; Koshida, Kichiro*; et al.
PLOS ONE (Internet), 8(2), p.e57671_1 - e57671_8, 2013/02
Times Cited Count：18 Percentile：68.67(Multidisciplinary Sciences)Sugihara, Shinji*; Tanaka, Masahiro*; Tamari, Toshiya*; Shimada, Jun*; Takahashi, Tomoyuki*; Momoshima, Noriyuki*; Fukutani, Satoshi*; Atarashi-Andoh, Mariko; Sakuma, Yoichi*; Yokoyama, Sumi*; et al.
Fusion Science and Technology, 60(4), p.1300 - 1303, 2011/11
Times Cited Count：2 Percentile：18.29(Nuclear Science & Technology)The purpose of this study is to develop the technique to evaluate the environmental tritium behavior of the nuclear facility origin. Tritium concentrations of river water, precipitation and ground water around the NIFS site were determined by low background liquid scintillation measurement system combined with the electrolysis using solid polymer electrolyte. The electric conductivity and flow rate of the river and isotopic ratio of oxygen and hydrogen of water samples were also measured. The tritium concentrations in precipitation showed the seasonal variation and the range were 0.09-0.78 Bq/L. The tritium concentrations of river water and ground water were almost constant, 0.34 and 0.24 Bq/L respectively. The simple dynamic model for the site around the NIFS facilities was developed using measured data, and the behavior of tritium was simulated.
Sukegawa, Atsuhiko; Takiyoshi, Koji*; Amano, Toshio*; Kawasaki, Hiromitsu*; Okuno, Koichi*
Progress in Nuclear Science and Technology (Internet), 1, p.36 - 39, 2011/02
A complete 3D radiation shielding analysis by PHITS has been performed for the JT-60U and JT-60 superconducting tokamak device (JT-60SA) in the present study. The PHITS has been developed for high energy particles physics in Japan. The neutron and photon transport analysis less than 20 MeV with the general cross section library is the same algorism of MCNP-4C code. The monoenergetic neutron (E
= 2.45 MeV) of the DD fusion devices are used for the neutron source in the analysis. The neutron source distribution are available a toroidally symmetric source for the analysis. The toroidal source has a poloidal distribution, so that a source routine in the PHITS has been replaced a newly developed source routine. The visual nuclear responses such as the neutron flux distribution, the photon flux distribution, the nuclear heating of the coils and the dose rate around the devices has been calculated by the PHITS for the fusion tokamak devices. Initial results by the PHITS have been demonstrated.
Suzuki, Takashi; Minakawa, Masayuki*; Amano, Hikaru; Togawa, Orihiko
Nuclear Instruments and Methods in Physics Research B, 268, p.1229 - 1231, 2010/04
Times Cited Count：26 Percentile：84.21(Instruments & Instrumentation)no abstracts in English
Tanaka, Takayuki; Otosaka, Shigeyoshi; Wakita, Masahide*; Amano, Hikaru*; Togawa, Orihiko
Nuclear Instruments and Methods in Physics Research B, 268(7-8), p.1219 - 1221, 2010/04
Times Cited Count：9 Percentile：54.21(Instruments & Instrumentation)Dissolved organic carbon (DOC) in seawater is one of the largest reservoirs of organic matter on the earth's surface, holding approximately as much carbon as available in atmospheric CO
. As a result of the huge carbon reservoir, the role and dynamics of DOC have become of greater interest in the global carbon cycle. It has been suggested that dissolved organic radiocarbon (
C-DOC) in seawater is a powerful tool to understand the dynamics of DOC and its researches have been carried out using AMS. However, there are very few data in the world oceans because of the difficulties of the measurement technique. Although it has been represented that the western North Pacific plays an important role in the carbon cycle from the viewpoint of a terminal of the deep water circulation in the world oceans and a high biological activity, C-DOC has not been measured yet. In this study, we obtained its vertical profile in the western North Pacific for the first time.
C concentration in tree rings of beech trees living near CO vents in the Hakkoda Cardera, Aomori, JapanHoriuchi, Kazuho*; Chiba, Takuji*; Hoshino, Yasuharu*; Oyama, Motonari*; Tanaka, Takayuki; Amano, Hikaru*
JAEA-Conf 2010-001, p.71 - 74, 2010/03
We investigated how volcanic CO emission affects the C concentrations in tree rings of beech trees in the Hakkoda Caldera in Aomori, which is one of high emission regions of volcanic CO in the world. There was a tendency that the obtained C concentrations were, surprisingly, quite near to the values of the concurrent atmospheric CO and decreased from 1991 to 2001. The C concentrations in caldera are lower than those of the control samples taken from a beech living outside of the caldera. We revealed the possibility that we can solve the local dynamics of fossil CO emission using C in tree rings. However, the maximum difference of C between inside and outside of the caldera was 14 permil. This result showed that the volcanic CO mixed with atmospheric CO by 4.4 ppm or less. As the trunk absorbing CO exist in height that is several meters higher than the volcanic CO vents, the low mixing may occur.
Tsuruta, Tadahiko; Uchida, Masahiro; Hama, Katsuhiro; Matsui, Hiroya; Takeuchi, Shinji; Amano, Kenji; Takeuchi, Ryuji; Saegusa, Hiromitsu; Matsuoka, Toshiyuki; Mizuno, Takashi
Proceedings of 12th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM '09/DECOM '09) (CD-ROM), 8 Pages, 2009/10
Takeuchi, Shinji; Mikake, Shinichiro; Nishio, Kazuhisa; Tsuruta, Tadahiko; Amano, Kenji; Matsuoka, Toshiyuki; Hayano, Akira; Takeuchi, Ryuji; Saegusa, Hiromitsu; Oyama, Takuya; et al.
JAEA-Review 2009-017, 29 Pages, 2009/08
JAEA-Review-2009-017.pdf:3.69MB
Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is developing a geoscientific research project named the Mizunami Underground Research Laboratory (MIU) project in crystalline rock environment in order to establish scientific and technological basis for geological disposal of HLW. Geoscientific research at the MIU project is planned to be carried out in three phases over a period of 20 years; Surface-based Investigation Phase (Phase 1), Construction Phase (Phase 2) and Operation Phase (Phase 3). Currently, the project is under the Construction Phase. This document presents the following 2009 fiscal year plan based on the MIU Master Plan updated in 2002, (1) Investigation Plan, (2) Construction Plan, (3) Research Collaboration Plan, etc.
Nishio, Kazuhisa; Matsuoka, Toshiyuki; Mikake, Shinichiro; Tsuruta, Tadahiko; Amano, Kenji; Oyama, Takuya; Takeuchi, Ryuji; Saegusa, Hiromitsu; Hama, Katsuhiro; Mizuno, Takashi; et al.
JAEA-Review 2009-002, 88 Pages, 2009/03
JAEA-Review-2009-002-1.pdf:29.31MBJAEA-Review-2009-002-2.pdf:35.38MB
Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is developing a geoscientific research project named Mizunami Underground Research Laboratory (MIU) Project in crystalline rock environment in order to establish scientific and technological basis for geological disposal of HLW. Geoscientific research at MIU is planned to be carried out in three phases over a period of 20 years; Surface-based Investigation Phase (Phase I), Construction Phase (Phase II) and Operation Phase (Phase III). Currently, the project is under the Construction Phase. This document presents the following results of the research and development performed in 2007 fiscal year, as a part of the Construction Phase based on the MIU Master Plan updated in 2002, (1) Investigation at the MIU Construction Site and the Shobasama Site, (2) Construction at the MIU Construction Site, (3) Research Collaboration.
Nishio, Kazuhisa; Matsuoka, Toshiyuki; Mikake, Shinichiro; Tsuruta, Tadahiko; Amano, Kenji; Oyama, Takuya; Takeuchi, Ryuji; Saegusa, Hiromitsu; Hama, Katsuhiro; Yoshida, Haruo*; et al.
JAEA-Review 2009-001, 110 Pages, 2009/03
JAEA-Review-2009-001.pdf:49.84MB
Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is developing a geoscientific research project named Mizunami Underground Research Laboratory (MIU) project in crystalline rock environment in order to establish scientific and technological basis for geological disposal of HLW. Geoscientific research at MIU is planned to be carried out in three phases over a period of 20 years; Surface-based Investigation Phase (Phase 1), Construction Phase (Phase 2) and Operation Phase (Phase 3). Currently, the project is under the Construction Phase. This document presents the following results of the research and development performed in 2006 fiscal year, as a part of the Construction Phase based on the MIU Master Plan updated in 2002, (1) Investigation at the MIU Construction Site, (2) Construction at the MIU Construction Site, (3) Research Collaboration.
Nishio, Kazuhisa; Matsuoka, Toshiyuki; Mikake, Shinichiro; Tsuruta, Tadahiko; Amano, Kenji; Oyama, Takuya; Takeuchi, Ryuji; Saegusa, Hiromitsu; Hama, Katsuhiro; Yoshida, Haruo*; et al.
JAEA-Review 2008-073, 99 Pages, 2009/03
JAEA-Review-2008-073-1.pdf:37.33MBJAEA-Review-2008-073-2.pdf:37.16MB
Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center (TGC) is developing a geoscientific research project named Mizunami Underground Research Laboratory (MIU) project in crystalline rock environment in order to establish scientific and technological basis for geological disposal of HLW. Geoscientific research at MIU is planned to be carried out in three phases over a period of 20 years; Surface-based Investigation Phase (Phase 1), Construction Phase (Phase 2) and Operation Phase (Phase 3). Currently, the project is under the Construction Phase. This document presents the following results of the research and development performed in 2005 fiscal year, as a part of the Construction Phase based on the MIU Master Plan updated in 2002, (1) Investigation at the MIU Construction Site, (2) Construction at the MIU Construction Site, (3) Research Collaboration.
Tanaka, Takayuki; Otosaka, Shigeyoshi; Amano, Hikaru; Togawa, Orihiko
Journal of Nuclear Science and Technology, 46(3), p.289 - 294, 2009/03
Times Cited Count：2 Percentile：17.7(Nuclear Science & Technology)We developed an extraction system of carbon from dissolved organic carbon (DOC) to achieve its accurate and precision C measurement by AMS. The system was devised for reducing the blank carbon by decreasing the contamination of dead carbon mainly induced from oil products and CO in air, and for extracting it from large volume seawater. The developed system gained lower blank than the previous studies to be less than 1% of sample size. It was demonstrated that the C value extracted from organic material by the system of lower blank was agreed with that by the conventional combusted method and the precision was very low value of 5‰. Results indicated that the system achieved the high accuracy and precision for C. We tied to measure DOC in large volume seawater and confirmed the great extraction and good precision to be 8‰. Results revealed that the system attained the supreme accuracy and precision for DOC in large volume seawater.
