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Journal Articles

Large scale production of $$^{64}$$Cu and $$^{67}$$Cu via the $$^{64}$$Zn(n, p)$$^{64}$$Cu and $$^{68}$$Zn(n, np/d)$$^{67}$$Cu reactions using accelerator neutrons

Kawabata, Masako*; Motoishi, Shoji*; Ota, Akio*; Motomura, Arata*; Saeki, Hideya*; Tsukada, Kazuaki; Hashimoto, Shintaro; Iwamoto, Nobuyuki; Nagai, Yasuki*; Hashimoto, Kazuyuki*

Journal of Radioanalytical and Nuclear Chemistry, 330(3), p.913 - 922, 2021/12

 Times Cited Count:7 Percentile:75.99(Chemistry, Analytical)

Both $$^{64}$$Cu and $$^{67}$$Cu are promising radionuclides in nuclear medicine. Production yields of these radionuclides were quantified by irradiating 55.4 g of natural zinc with accelerator neutrons. Clinically suitable $$^{64}$$Cu and $$^{67}$$Cu yields were estimated by experimental based numerical simulations using 100 g of enriched $$^{64}$$Zn and $$^{68}$$Zn, respectively, and elevated neutron fluxes from 40 MeV, 2 mA deuterons. A combined thermal- and resin-separation method was developed to isolate $$^{64}$$Cu and $$^{67}$$Cu from zinc, resulting in 73% separation efficiency and 97% zinc recovery. Such methods can provide large scale production of $$^{64}$$Cu and $$^{67}$$Cu for clinical applications.

Journal Articles

Generation of radioisotopes with accelerator neutrons by deuterons

Nagai, Yasuki; Hashimoto, Kazuyuki; Hatsukawa, Yuichi; Saeki, Hideya; Motoishi, Shoji; Sonoda, Nozomi; Kawabata, Masako; Harada, Hideo; Kin, Tadahiro*; Tsukada, Kazuaki; et al.

Journal of the Physical Society of Japan, 82(6), p.064201_1 - 064201_7, 2013/06

 Times Cited Count:43 Percentile:85.32(Physics, Multidisciplinary)

Journal Articles

Systematic study for the shell effect in the fission fragment mass distribution reptured from neutron rich nuclei

Ota, Masahisa*; Tatsuda, Sayuki*; Yamamoto, Kazuyuki*; Asano, Tomomasa*; Wada, Takahiro*; Hashizume, Kazuaki*; Sumiyoshi, Kosuke*; Otsuki, Kaori*; Kajino, Toshitaka*; Koura, Hiroyuki; et al.

Nuclear Physics A, 805(2), p.558 - 560, 2008/02

The data base for the fission fragment mass distribution used in the r-process network calculation is constructed. The differences appeared in the final element abundance calculated with and without fission process are demonstrated and the mass region modified by the fission products is presented.

Journal Articles

Fission fragment mass distribution for nuclei in the r-process region

Tatsuda, Sayuki*; Hashizume, Kazuaki*; Wada, Takahiro*; Ota, Masahisa*; Sumiyoshi, Kosuke*; Otsuki, Kaori*; Kajino, Toshitaka*; Koura, Hiroyuki; Chiba, Satoshi; Aritomo, Yoshihiro*

AIP Conference Proceedings 891, p.423 - 426, 2007/03

We investigate the fission-fragment mass distribution on about 2000 nuclides, which should have a critical impact on the r-process nucleosynthesis through fission ($$Z>85$$). The mass distribution of fission fragment is thought to be one of the most important elements on some astrophysical conditions for the theoretical estimation of the r-process abundance pattern. We calculated the potential energy surface (PES) by means of the liquid-drop model with the shell energy correction by the Two-Center shell model in 3-dimensional parameter space. We derive fission-fragment mass distribution by considering the location and the depth of the valley of PES near the saddle point and the scission point of nuclei with the use of the Langevin calculation. We determine the fission asymmetry by examining the valley depth and its location in the deformation parameter space. The consistency of our mass asymmetry with available experimental data is discussed.

JAEA Reports

Conceptual design of backend technology R & D facility for TRU recycle in the future cycle system

Fujine, Sachio; Usuda, Shigekazu; Morita, Yasuji; Yoshida, Zenko; ; Furuta, Teruo; Tone, Tatsuzo; *; Nishimura, Kenji*; *

JAERI-M 93-211, 87 Pages, 1993/11

JAERI-M-93-211.pdf:2.42MB

no abstracts in English

Journal Articles

Construction and testing of the new multijunction LHRF launcher for JT-60 upgrade

Seki, Masami; Ikeda, Yoshitaka; *; Imai, Tsuyoshi; ; Yokokura, Kenji; Sawahata, Masayuki; Suganuma, Kazuaki; Sato, Minoru; *; et al.

Fusion Technology 1990, p.1060 - 1064, 1991/00

no abstracts in English

Oral presentation

Surrogate reaction study at JAEA, 2; Measurement of fission cross sections

Nishio, Katsuhisa; Nagayama, Tatsuro*; Nishinaka, Ichiro; Mitsuoka, Shinichi; Makii, Hiroyuki; Ota, Shuya*; Furutaka, Kazuyoshi; Tsukada, Kazuaki; Asai, Masato; Ishii, Tetsuro; et al.

no journal, , 

no abstracts in English

Oral presentation

Study of delayed-neutron yields for acculate evaluation of kinetics of high-burnup reactors, 2; Measurement of fission fragnment mass distributions for actinide nuclei by surrogate method

Nishio, Katsuhisa; Hirose, Kentaro; Nishinaka, Ichiro; Makii, Hiroyuki; Ota, Shuya; Nagayama, Tatsuro*; Chiba, Satoshi; Tsukada, Kazuaki; Asai, Masato; Ishii, Tetsuro; et al.

no journal, , 

no abstracts in English

Oral presentation

Fission study by multi-nucleon transfer reaction at JAEA

Hirose, Kentaro; Nishio, Katsuhisa; L$'e$guillon, R.; Makii, Hiroyuki; Nishinaka, Ichiro; Orlandi, R.; Smallcombe, J.; Ishii, Tetsuro; Tsukada, Kazuaki; Asai, Masato; et al.

no journal, , 

Oral presentation

Production method development of cancer therapeutic $$^{67}$$Cu using thermoseparation for cancer therapy

Ota, Akio*; Kawabata, Masako*; Motoishi, Shoji*; Saeki, Hideya*; Hashimoto, Kazuyuki*; Tsukada, Kazuaki; Hatsukawa, Yuichi*; Nagai, Yasuki*

no journal, , 

$$^{67}$$Cu and $$^{64}$$Cu are recognized to be promising radioisotopes for cancer therapy and diagnosis in nuclear medicine. It is possible to produce both $$^{67}$$Cu and $$^{64}$$Cu using accelerator neutrons from the zinc sample with different isotopic enrichment level, therefore the same separation procedure can be applied for both radioisotopes. Three-step-column separation chemistry was previously reported to separate $$^{67}$$Cu from the irradiated zinc sample. This paper reports that newly developed thermo-separation system to remove the bulk zinc from the sample using a difference in vapor pressure between Zn and Cu.

Oral presentation

Production of Sc-47 for cancer therapy using accelerator neutrons

Tsukada, Kazuaki; Hashimoto, Kazuyuki*; Hashimoto, Shintaro; Asai, Masato; Hatsukawa, Yuichi*; Saeki, Hideya*; Kawabata, Masako*; Ota, Akio*; Motomura, Arata*

no journal, , 

no abstracts in English

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