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Journal Articles

Formation of high-quality SiO$$_{2}$$/GaN interfaces with suppressed Ga-oxide interlayer via sputter deposition of SiO$$_{2}$$

Onishi, Kentaro*; Kobayashi, Takuma*; Mizobata, Hidetoshi*; Nozaki, Mikito*; Yoshigoe, Akitaka; Shimura, Takayoshi*; Watanabe, Heiji*

Japanese Journal of Applied Physics, 62(5), p.050903_1 - 050903_4, 2023/05

While the formation of an GaO$$_{x}$$ interlayer is key to achieving SiO$$_{2}$$/GaN interfaces with low defect density, it can affect the reliability and stability of metal-oxide-semiconductor (MOS) devices if the annealing conditions are not properly designed. In the present study, we aimed to minimize the growth of the GaO$$_{x}$$ layer on the basis of the sputter deposition of SiO$$_{2}$$ on GaN. Synchrotron radiation X-ray photoelectron spectrometry measurements confirmed the suppressed growth of the GaO$$_{x}$$ layer compared with a SiO$$_{2}$$/GaN structure formed by plasma-enhanced chemical vapor deposition. Negligible GaO$$_{x}$$ growth was also observed when subsequent oxygen annealing up to 600$$^{circ}$$C was performed. A MOS device with negligible capacitance-voltage hysteresis, nearly ideal flat-band voltage, and low leakage current was demonstrated by performing oxygen and forming gas annealing at temperatures of 600$$^{circ}$$C and 400$$^{circ}$$C, respectively.

Journal Articles

Magnetic orderings from spin-orbit coupled electrons on kagome lattice

Watanabe, Jin*; Araki, Yasufumi; Kobayashi, Koji*; Ozawa, Akihiro*; Nomura, Kentaro*

Journal of the Physical Society of Japan, 91(8), p.083702_1 - 083702_5, 2022/08

 Times Cited Count:3 Percentile:58.88(Physics, Multidisciplinary)

We investigate magnetic orderings on kagome lattice numerically from the tight-binding Hamiltonian of electrons, governed by the filling factor and spin-orbit coupling (SOC) of electrons. We find that even a simple kagome lattice model can host both ferromagnetic and noncollinear antiferromagnetic orderings depending on the electron filling, reflecting gap structures in the Dirac and flat bands characteristic to the kagome lattice. Kane-Mele- or Rashba-type SOC tends to stabilize noncollinear orderings, such a magnetic spirals and 120-degree antiferromagnetic orderings, due to the effective Dzyaloshinskii-Moriya interaction from SOC. The obtained phase structure helps qualitative understanding of magnetic orderings in various kagome-layered materials with Weyl or Dirac electrons.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Development of evaluation method for photocatalytic ability by ion chromatography combined with a flow-type reactor; Application to immobilized photocatalyst materials prepared by double-layer coating method

Sugita, Tsuyoshi; Kobayashi, Kentaro*; Yamazaki, Taiki*; Isaka, Mayu*; Itabashi, Hideyuki*; Mori, Masanobu*

Journal of Photochemistry and Photobiology A; Chemistry, 400, p.112662_1 - 112662_8, 2020/09

 Times Cited Count:1 Percentile:2.52(Chemistry, Physical)

In this study, we developed an in-line photocatalytic performance evaluation system in which a flow reactor was connected to the ion chromatography to accurately evaluate the performance of the photocatalyst. This system was used to evaluate the photocatalyst supported by the two-layer support method on the substrate, such as glass beads. The performance of the photocatalyst was evaluated using dimethyl sulfoxide (DMSO), and it was possible to monitor the decomposition of DMSO by UV and the formation of by-products, such as methane sulfonate (MSO) and sulfate (SA). This system can be expected to be useful not only for evaluating the decomposition performance of an object using a photocatalyst but also for evaluating the byproducts.

Journal Articles

Evaluation of photocatalytic abilities by variation of conductivity and dimethyl sulfoxide; Photocatalytically active TiO$$_{2}$$-coated wire mesh prepared via a double-layer coating method

Mori, Masanobu*; Sugita, Tsuyoshi; Fujii, Kengo*; Yamazaki, Taiki*; Isaka, Mayu*; Kobayashi, Kentaro*; Iwamoto, Shinji*; Itabashi, Hideyuki*

Analytical Sciences, 34(12), p.1449 - 1453, 2018/12

 Times Cited Count:2 Percentile:7.07(Chemistry, Analytical)

The photocatalyst coating stainless-steel wire mesh (TiO$$_{2}$$-WM) was prepared by double-layer coating method. The TiO$$_{2}$$-WM was evaluated using flow analytical system, which included the reactor and conductimetric detector (FAS-CD). The DMSO decomposition test through the FAS-CD reveal that photocatalytst was stable coating on the stainless-steel wire mesh.

Journal Articles

Enhanced aqueous adsorption and photodecomposition of anionic organic target by amino group-modified TiO$$_{2}$$ as anionic adsorptive photocatalyst

Sugita, Tsuyoshi; Kobayashi, Kenichi*; Kobayashi, Kentaro*; Yamazaki, Taiki*; Fujii, Kengo*; Itabashi, Hideyuki*; Mori, Masanobu*

Journal of Photochemistry and Photobiology A; Chemistry, 356, p.71 - 80, 2018/04

 Times Cited Count:5 Percentile:13.28(Chemistry, Physical)

Photocatalysts shows high redox property only by light irradiation. However, the reaction performance is lowered in aqueous phase due to the low contact efficiency between catalyst and targets. In this study, to enhance aqueous adsorption and photodecomposition of anionic organic target, we developed an amino functional-based spacer (3-[2-(2- aminoethylamino)ethylamino]propyl-trimethoxysilane, DETA), and used it to modify TiO$$_{2}$$. The modified catalyst with positively charged amino groups could enhance the adsorption and photodecomposition of anionic organic targets.

Journal Articles

Numerical evaluation of the light transport properties of alternative He-3 neutron detectors using ceramic scintillators

Ozu, Akira; Takase, Misao*; Haruyama, Mitsuo; Kurata, Noritaka*; Kobayashi, Nozomi*; Kureta, Masatoshi; Nakamura, Tatsuya; To, Kentaro; Sakasai, Kaoru; Suzuki, Hiroyuki; et al.

Nuclear Instruments and Methods in Physics Research A, 798, p.62 - 69, 2015/10

 Times Cited Count:2 Percentile:17.57(Instruments & Instrumentation)

The light transport properties of scintillator light inside alternative He-3 neutron detector modules using scintillator sheets have been investigated by a ray-tracing simulation code. The detector module consists of a light-reflecting tube, a thin rectangular ceramic scintillator sheet laminated on a glass plate, and two photo-multiplier tubes (PMTs) mounted at both ends of the detector tube. The light induced on the surface of the scintillator sheet via nuclear interaction between the scintillator and neutrons are detected by the two PMTs. The light output of various detector modules in which the scintillator sheets are installed with several different arrangements were examined and evaluated in comparison with experimental results. The results derived from the simulation reveal that the light transport property is strongly dependent on the arrangement of the scintillator sheet inside the tube and the shape of the tube.

Journal Articles

Real-time observation of irradiated HeLa-cell modified by fluorescent ubiquitination-based cell-cycle indicator using synchrotron X-ray microbeam

Narita, Ayumi; Kaminaga, Kiichi; Yokoya, Akinari; Noguchi, Miho; Kobayashi, Katsumi*; Usami, Noriko*; Fujii, Kentaro

Radiation Protection Dosimetry, 166(1-4), p.192 - 196, 2015/09

 Times Cited Count:3 Percentile:25.85(Environmental Sciences)

For the knowledge about irradiation effects of mammalian cells depending on the cell cycle, most of them had been analyzed by statistical approches. Our purpose is to establish the method for real-time observation of irradiated cells under a microscope. Fluorescent ubiquitination-based cell cycle indicator (FUCCI) human cancer (HeLa) cells (red indicates G1; green, S/G2) were exposed to a synchrotron X-ray microbeam. Cells in either G1 or S/G2 were selectively irradiated according to cell color observed in the same microscopic field in a culture dish. Time-lapse micrographs of the irradiated cells were acquired for 24 h after irradiation. The cell cycle was strongly arrested by irradiation at S/G2 and never progressed to G1. In contrast, cells irradiated at G1 progress to S/G2 with a similar time course as non-irradiated control cells. These results show single FUCCI cell exposure and live cell imaging are powerful methods for studying radiation effects on the cell cycle.

Journal Articles

Evaluation of light transport property in alternative He-3 neutron detectors using ceramic scintillators by a ray-tracing simulation

Ozu, Akira; Takase, Misao*; Kurata, Noritaka*; Kobayashi, Nozomi*; Tobita, Hiroshi; Haruyama, Mitsuo; Kureta, Masatoshi; Nakamura, Tatsuya; Suzuki, Hiroyuki; To, Kentaro; et al.

Proceedings of 2014 IEEE Nuclear Science Symposium and Medical Imaging Conference; 21st International Symposium on Room-Temperature Semiconductor X-ray and $$gamma$$-ray detectors (NSS/MIC 2014), 5 Pages, 2014/00

In Japan Atomic Energy Agency, the helium-3 alternative neutron detector using ceramic scintillators for nuclear safeguards is under development with the support of the government. The alternative detector module consists of four components: an aluminum regular square tube, a light reflecting foil put on the inner surface of the square tube, a rectangular scintillator sheet sintered on a glass plate, and two PMTs provided at both ends of the tube. The scintillator sheet is fit on the diagonal inside the square tube. The light transport property of scintillator lights inside the tube influences on the fundamental performance of the alternative detector. Therefore, the properties of the lights emitted on the surface of the scintillator sheet and scintillation lights passing through the glass plate to the PMTs in several arrangements of the scintillator in the tubes were investigated with a ray-tracing simulation. The results are described in comparison with the experimental results.

Journal Articles

Development of an alternative plutonium canister assay system (APCA) using He-3 alternative neutron detector

Ozu, Akira; Kureta, Masatoshi; Haruyama, Mitsuo; Takase, Misao; Kurata, Noritaka; Kobayashi, Nozomi; Soyama, Kazuhiko; Nakamura, Tatsuya; Sakasai, Kaoru; To, Kentaro; et al.

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-34-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2013/10

no abstracts in English

Journal Articles

Detection and activity of iodine-131 in brown algae collected in the Japanese coastal areas

Morita, Takami*; Niwa, Kentaro*; Fujimoto, Ken*; Kasai, Hiromi*; Yamada, Haruya*; Nishiuchi, Ko*; Sakamoto, Tatsuya*; Godo, Waichiro*; Taino, Seiya*; Hayashi, Yoshihiro*; et al.

Science of the Total Environment, 408(16), p.3443 - 3447, 2010/06

 Times Cited Count:13 Percentile:33(Environmental Sciences)

Iodine-131 ($$^{131}$$I) was detected in brown algae collected off the Japanese coast. The maximum measured specific activity of $$^{131}$$I in brown algae was 0.37$$pm$$0.010 Bq/kg-wet. Cesium-137 ($$^{137}$$Cs) was also detected in all brown algal samples used in this study. There was no correlation between specific activities of $$^{131}$$I and $$^{137}$$Cs in these seaweeds. Low specific activity and minimal variability of $$^{137}$$Cs in brown algae indicated that past nuclear weapon tests were the source of $$^{137}$$Cs. Although nuclear power facilities are known to be pollution sources of $$^{131}$$I, there was no relationship between the sites where $$^{131}$$I was detected and the locations of nuclear power facilities. Most of the sites where $$^{131}$$I was detected were near big cities with large populations. On the basis of the results, we suggest that the likely pollution source of $$^{131}$$I, detected in brown seaweeds, is not nuclear power facilities, but nuclear medicine procedures.

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

Journal Articles

Progress in R&D efforts on the energy recovery linac in Japan

Sakanaka, Shogo*; Ago, Tomonori*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; Harada, Kentaro*; Hiramatsu, Shigenori*; Honda, Toru*; et al.

Proceedings of 11th European Particle Accelerator Conference (EPAC '08) (CD-ROM), p.205 - 207, 2008/06

Future synchrotron light sources based on the energy-recovery linacs (ERLs) are expected to be capable of producing super-brilliant and/or ultra-short pulses of synchrotron radiation. Our Japanese collaboration team is making efforts for realizing an ERL-based hard X-ray source. We report recent progress in our R&D efforts.

Journal Articles

Cement based encapsulation trials for low-level radioactive effluent containing nitrate salts

Sugaya, Atsushi; Horiguchi, Kenichi; Tanaka, Kenji; Kobayashi, Kentaro

Materials Research Society Symposium Proceedings, Vol.1107, p.173 - 179, 2008/00

In Nuclear Fuel Reprocessing Plant, it is necessary to dispose of a large amount of low level radioactive effluent containing nitrate as a major ingredient, safely and economically. Therefore, engineering developments concerning a cement based encapsulation process have been carried out in JAEA. From the viewpoint of disposal cost decrease, a low level radioactive effluent is passed through the nuclide separation process before cementation to concentrate the radioactivity into the minimum volume for conditioning and disposal. Two kinds of effluents are generated as a result of the nuclide separation; Non-radioactive simulants were prepared for each of these waste streams, and used in encapsulation trials to investigate a special slag cement, on a beaker scale and at full scale (200-litres). The results have confirmed that the nitrate effluent, evaporated up to a predetermined density, can be successfully encapsulated at a salt filling rate of 50wt%, to produce a wasteform which satisfies the required conditions. In the slurry effluent, the strength of the product decreased when carbonate concentration was high. However, it was confirmed that the product made at salt filling rate 50wt% satisfied the required conditions, if the carbonate concentration in the effluent was decreased to 10 g/L or less.

Journal Articles

Design study of the compact ERL optics

Shiraga, Takashi*; Nakamura, Norio*; Harada, Kentaro*; Shimada, Miho*; Sakanaka, Shogo*; Kobayashi, Yukinori*; Hajima, Ryoichi

Proceedings of 5th Annual Meeting of Particle Accelerator Society of Japan and 33rd Linear Accelerator Meeting in Japan (CD-ROM), p.589 - 591, 2008/00

An energy recovery linac (ERL) is expected to be the next generation synchrotron radiation source that can provide synchrotron radiation of higher brilliance, shorter pulse and higher coherence than the existing third-generation synchrotron light sources. The compact ERL is planned to be constructed in order to solve some problems in achievement of such synchrotron radiation and to confirm advantages of ERLs. We studied and optimized the compact ERL optics to achieve subpico-second bunch generation and efficient energy recovery and to transport the beam to the beam dump without serious beam loss. The design study of the compact ERL optics was done by using the simulation code Elegant. As a result, we succeeded in obtaining a 40-fs bunch with a charge of 77 pC just after the first TBA cell. Furthermore we could suppress the maximum beam size to less than 8.5 mm even after deceleration.

Journal Articles

Development of new treatment process for low level liquid waste at Tokai reprocessing plant

Saito, Yasuo; Takano, Masato; Tanaka, Kenji; Kobayashi, Kentaro; Otani, Yoshikuni

Proceedings of International Symposium on Radiation Safety Management 2007 (ISRSM 2007), p.275 - 280, 2007/11

The Low-radioactive Waste Treatment Facility (LWTF), which aims to provide the safe, efficient and economic treatment and disposal of Low-level Liquid Waste (LLW) generated from LWR spent fuel reprocessing, was constructed at the Tokai Reprocessing Plant (TRP), and a cold test is now being carried out. New treatment processes such as a removal process for radio-nuclides and the ROBE (BORSAURE EINENGUNG ANLAGE) solidification process are being implemented in the LWTF. In order to treat the large amount of sodium nitrate contained in the concentrated LLW with higher safety and economy, R&D work on nitrate-ion decomposition technology using a catalytic reduction method and on the solidification process by cementation is being undertaken. The results of this R&D will be adopted in the LWTF in the near future. This report describes an outline of liquid waste treatment in the LWTF and new treatment technologies for LLW to achieve safe, efficient and economic treatment and disposal.

Journal Articles

Examination of determination to Pu amount in LASW from TRP

Makino, Risa; Tomikawa, Hirofumi; Hina, Tetsuro; Ozone, Takashi; Kurosu, Kazutoshi; Fukuhara, Junichi; Kobayashi, Kentaro; Kabuki, Toshihide*

Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-27-Kai Nenji Taikai Rombunshu (CD-ROM), 7 Pages, 2006/00

Tokai Reprocessing Center has developed method of determination of Pu contained in low activity solid wastes (LASWs), to make better accountancy control. Our final goal is to estimate of Pu amounts in wastes generated in TRP. Some of small size wastes (carton-boxes) and drums from TRP was measured by some kind of non-destructive assay system. It was found that high dose wastes have slight amounts of Pu. However, because some of wastes from TRP have Cm, the wastes could not be measured exactly. Near future, JAEA will try upgrading or development of NDA system, and determination of Pu amount of wastes from TRP.

JAEA Reports

Operating Document on Management Division Waste Management Section in Tokai Works in the 2003 Fiscal Year

Kobayashi, Kentaro; Akutsu, Shigeru; Sasayama, Yasuo; Nakanishi, Masahiro; Ozone, Takashi; Tomomi, Terunuma,; Mogaki, Isao*

JNC TN8440 2005-007, 138 Pages, 2005/07

JNC-TN8440-2005-007.pdf:7.47MB

This document is announced about the task of Waste Management Section of Waste Management Division in 2003. Mainly, our tasks are fractionating, incinerating and storing low active solid waste and storing high active solid waste. In addition, we are performing required correspondence about management program of low level waste. We had treated and stored waste safely according to our plan. As a result, we have achieved following outcomes. 1. We incinerated the combustible low active solid waste that is generated by the operation of Tokai Reprocessing Plant and the recovery operation of incident at Low Active Liquid Waste Asphalt Solidification Facility. Waste of this recovery operation is stored in the 2nd Low Active Liquid Waste Asphalt Solidification Storage Facility. We incinerated 58 ton of wastes. 2. We stored low active solid waste 854 drums that accommodate 200L. According to the time of Low-Level Waste Treatment Facility completion, we will be able to avoid full of storage. 3. We stored high active solid waste of 148 drums that accommodate 200L. For the time being, there is no problem as regards the administration of storage facility. 4. We carried out the management program of low level solid waste according to plan.

JAEA Reports

Operating Document on Management Division Waste Management Section in Tokai Works in the 2002 Fiscal Year

Kobayashi, Kentaro; Isozaki, Koei; Akutsu, Shigeru; Nakanishi, Masahiro; Ozone, Takashi; Mogaki, Isao*; Aizawa, Shuichi*

JNC TN8440 2004-001, 151 Pages, 2004/05

JNC-TN8440-2004-001.pdf:88.84MB

This document is announced about task of Waste Management Section in the 2003 fiscal year.

JAEA Reports

Operating document on management division waste management section in Tokai works in 2002 fiscal year

Kobayashi, Kentaro; Isozaki, Koei

JNC TN8440 2003-003, 139 Pages, 2003/04

JNC-TN8440-2003-003.pdf:19.77MB

This document is announced about task of Waste Management Division Waste Management Section in the 2002 fiscal year. Mainly, our task is that treated Low level solid waste, stored Low level solid waste and stored High level solid waste. Those wastes are generated from Tokai reprocessing plant in Tokai Works. We carried out task safety as planned. The results are as follows. (1)We incinerated that combustible Low level solid waste of 70.5 ton in Incinerate facility. Such wastes were generated from operation of Tokai reprocessing plant and cleaned up operation of Tokai bituminization facility (The fire and explosion incident of Tokai bituminization facility). (2)We stored Low level solid waste that generated the waste of 1,071 drums. It is found that Storage facilities will not fill on this condition Low level radioactive waste treatment facility is started operation. (3)We stored High level solid waste that generated the waste of 117 drums from Tokai reprocessing plant. And, it is found that there facilities will not fill on this condition generated wastes of about 100 drams by a year. (4)We started printing of the data from the 2002 fiscal year to intranet which amount of stored Low level solid waste and High level solid waste in order to educate the amount reduction of waste generating (at those facilities).

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