Recent status of the cryogenic sample environment at the MLF, J-PARC

Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.

JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05

https://doi.org/10.7566/JPSCP.41.011010

Mode distribution analysis for superionic melt of CuI by coherent quasielastic neutron scattering

Kawakita, Yukinobu; Kikuchi, Tatsuya*; Tahara, Shuta*; Nakamura, Mitsutaka; Inamura, Yasuhiro; Maruyama, Kenji*; Yamauchi, Yasuhiro*; Kawamura, Seiko; Nakajima, Kenji

JPS Conference Proceedings (Internet), 33, p.011071_1 - 011071_6, 2021/03

BB2019-1144.pdf:0.7MB

https://doi.org/10.7566/JPSCP.33.011071

CuI is a well-known superionic conductor in a high temperature solid phase where the mobile cations migrate between interstitial sites in the f.c.c. sublattice formed by iodine ions. Even in the molten state, it shows several features suggesting collective or cooperative ionic motion. MD results show that Cu diffuses much faster than I. The Cu-Cu partial structure factor have a FSDP which indicates a medium-range ordering of Cu ions. Moreover the Cu-Cu partial pair distribution deeply penetrates into the nearest neighboring Cu-I shell. To reveal origin such anomalous behaviors of molten CuI, we performed quaiselastic neutron scattering (QENS) by the disk-chopper spectrometer AMATERAS at MLF, J-PARC. To interpret the total dynamic structure factor obtained from coherent QENS, the mode distribution analysis was applied. It is found that the motion of iodine is a kind of fluctuating within an almost local area while Cu ions diffuse much faster than iodine ions.

Anomaly of structural relaxation in complex liquid metal of bismuth; Dynamic correlation function of coherent quasi-elastic neutron scattering

Kawakita, Yukinobu; Kikuchi, Tatsuya*; Inamura, Yasuhiro; Tahara, Shuta*; Maruyama, Kenji*; Hanashima, Takayasu*; Nakamura, Mitsutaka; Kiyanagi, Ryoji; Yamauchi, Yasuhiro*; Chiba, Kaori*; et al.

Physica B; Condensed Matter, 551, p.291 - 296, 2018/12

https://doi.org/10.1016/j.physb.2017.12.037

There are elemental liquid metals with complex structures far from the hard sphere (HS) packing model. Liquid Bi has an asymmetric first peak in the structure factors S(Q). The pair distribution function g(r) exhibits strange distance ratio of 1:2 between the first and the second peaks. Since a HS model with two kinds of radius produces asymmetry of the main peak in S(Q), existence of short-lived covalent bonds was discussed. Contrarily, modulation of the atomic distribution by the Friedel oscillations of shielding electrons around metallic ions was discussed. To examine its bonding nature from viewpoints of dynamic correlation functions, we have measured neutron quasielastic scattering of liquid Bi by using cold disk chopper spectrometer installed at MLF of J-PARC. The van Hove function revealed that the shoulder structure located at a longer side of the first peak in g(r) exhibits a longer relaxation time than the main structures such as the first and second peaks.

Recent progress in the chopper spectrometer 4SEASONS at J-PARC

Kajimoto, Ryoichi; Nakamura, Mitsutaka; Inamura, Yasuhiro; Kamazawa, Kazuya*; Ikeuchi, Kazuhiko*; Iida, Kazuki*; Ishikado, Motoyuki*; Nakajima, Kenji; Kawamura, Seiko; Nakatani, Takeshi; et al.

JAEA-Conf 2015-002, p.319 - 329, 2016/02

https://doi.org/10.11484/jaea-conf-2015-002

Real-time monitoring of oxidation on the Ti(0001) surface by synchrotron radiation photoelectron spectroscopy and RHEED-AES

Takakuwa, Yuji*; Ishizuka, Shinji*; Yoshigoe, Akitaka; Teraoka, Yuden; Yamauchi, Yasuhiro*; Mizuno, Yoshiyuki*; Tonda, Hideki*; Homma, Teiichi*

Applied Surface Science, 216(1-4), p.395 - 401, 2003/06

https://doi.org/10.1016/S0169-4332(03)00453-7

Real-time in-situ observation using photoelectron spectroscopy for elementary processes of Ti(0001) oxidation by O molecules has been performed at the surface reaction analysis apparatus installed at the BL23SU in the SPring-8. And the real-time observation has been also performed by RHEED-AES methods at Tohoku University. The partial pressure region of oxygen was from 2x10 Torr to 8x10 Torr. The surface temperature was 473 K and 673 K. The variation from clean Ti surface toward TiO was comfirmed by observation of Ti-2p and O-1s photoelectron spectra. Reflected electron intensity and O-KLL Auger electron intensity oscillated in the RHEED-AES measurements. These facts revealed that the surface morphological change of the oxidized Ti(0001) surface was associated not only with a disappearance of the surface metallic layer but also with a change of the oxidation state.

Hydrogen-methanol production system using nuclear process heat

; Omoto, Akira*; *; *; *; *; *; *; *; *; et al.

Enerugi, Shigen Gakkai Dai-11-Kai Kenkyu Happyokai Koen Rombunshu, p.33 - 38, 1992/00

no abstracts in English

Current status of sample environment in MLF, J-PARC

Kawamura, Seiko; Yokoo, Tetsuya*; Kambara, Wataru; Inamura, Yasuhiro; Nakatani, Takeshi; Torii, Shuki*; Kajimoto, Ryoichi; Nakajima, Kenji; Kaneko, Koji; Kawakita, Yukinobu; et al.

no journal, , 

Materials and Life Science Experimental Facility at J-PARC started the user program in December 2008. Various neutron experiments are currently performed there in wide range of scientific researches and industrial applications. Standardization of sample environment (SE) equipments is one of the most important things at the beginning stage. Especially in our country, it often happens that each instrument carries and operates SE devices independently. This situation results in an excess of the cost and incompatibility among the instruments unless we have any guidelines. Thus the SE team has discussed the SE-protocol, in which flange size, thermometers, controllers etc. are standardized. This should bring about saving the cost and manpower and increasing compatibility. The SE team is now discussing user support system in SE, preparation of the SE area, and so on. The technical staff members started working on practical things such as cooling test of cryostats.

Current status and future plan of sample environment in MLF, J-PARC

Kawamura, Seiko; Yokoo, Tetsuya*; Kambara, Wataru; Munakata, Koji*; Kajimoto, Ryoichi*; Nakatani, Takeshi; Kaneko, Koji; Kawakita, Yukinobu; Takata, Shinichi; Nakajima, Kenji; et al.

no journal, , 

In large user facilities such as neutron experimental facilities, sample environment (SE) is one of the most important factors to yield high-quality output. In the Materials and Life Science Experimental Facility (MLF) in J-PARC, various neutron experiments have been performed in wide range of scientific researches and industrial applications, and the number and variety of proposals will further increase after resuming operation of J-PARC. At the beginning stage, the SE team in MLF has discussed SE standardization, to save the cost and manpower, to make compatibility among instruments, and to increase the experimental efficiency by sharing the SE devices and techniques for operation. Recently we started preparation of "SE area" in the experimental hall, where we can do maintenance of equipments, pre-cooling of cryostats and so on. The SE team is now discussing future plan including user support system.

The Construction report of the Si crystal analyzer near backscattering spectrometer, 6

Shibata, Kaoru*; Takahashi, Nobuaki; Kawakita, Yukinobu; Kamazawa, Kazuya*; Yamada, Takeshi*; Ueno, Hiroki; Shimakura, Hironori; Nakajima, Kenji; Kambara, Wataru; Inamura, Yasuhiro; et al.

no journal, , 

no abstracts in English

Specifications and reports of on-beam commissioning of the BL02; Si Backscattering spectrometer DNA

Shibata, Kaoru*; Takahashi, Nobuaki; Yamada, Takeshi*; Kamazawa, Kazuya*; Kawakita, Yukinobu; Nakajima, Kenji; Kambara, Wataru; Inamura, Yasuhiro; Nakatani, Takeshi; Aizawa, Kazuya; et al.

no journal, , 

no abstracts in English