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Journal Articles

Hyperfine splitting and nuclear spin polarization in NdPd$$_5$$Al$$_2$$ and Nd$$_3$$Pd$$_{20}$$Ge$$_6$$

Metoki, Naoto; Shibata, Kaoru; Matsuura, Masato*; Kitazawa, Hideaki*; Suzuki, Hiroyuki*; Yamauchi, Hiroki; Hagihara, Masato; Frontzek, M. D.*; Matsuda, Masaaki*

Journal of the Physical Society of Japan, 91(5), p.054710_1 - 054710_6, 2022/05

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Hyperfine splitting of Nd nuclei in NdPd$$_5$$Al$$_2$$ has been studied by means of high-resolution neutron spectroscopy. We observed inelastic peaks at $$hbaromega =pm3;{mu}$$eV coming from the hyperfine splitting in the magnetically ordered phase due to the hyperfine interactions between Nd nuclei ($$I$$=7/2) and the 4$$f$$ electrons with $$Gamma_6$$ ground state composed of mainly $$|pm9/2rangle$$. At very low temperatures, nuclear spin of Nd is polarized with increasing occupation probability of low energy levels and contributes to the enhancement of the antiferromagnetic Bragg intensities: the elastic non-spin-flip channel is dominant. As an application of this phenomenon, we determined the Nd moment and hyperfine splitting from the temperature dependence of an antiferromagnetic Bragg intensities for Nd$$_3$$Pd$$_{20}$$Ge$$_6$$.

Journal Articles

Anomaly of structural relaxation in complex liquid metal of bismuth; Dynamic correlation function of coherent quasi-elastic neutron scattering

Kawakita, Yukinobu; Kikuchi, Tatsuya*; Inamura, Yasuhiro; Tahara, Shuta*; Maruyama, Kenji*; Hanashima, Takayasu*; Nakamura, Mitsutaka; Kiyanagi, Ryoji; Yamauchi, Yasuhiro*; Chiba, Kaori*; et al.

Physica B; Condensed Matter, 551, p.291 - 296, 2018/12

 Times Cited Count:9 Percentile:45.52(Physics, Condensed Matter)

There are elemental liquid metals with complex structures far from the hard sphere (HS) packing model. Liquid Bi has an asymmetric first peak in the structure factors S(Q). The pair distribution function g(r) exhibits strange distance ratio of 1:2 between the first and the second peaks. Since a HS model with two kinds of radius produces asymmetry of the main peak in S(Q), existence of short-lived covalent bonds was discussed. Contrarily, modulation of the atomic distribution by the Friedel oscillations of shielding electrons around metallic ions was discussed. To examine its bonding nature from viewpoints of dynamic correlation functions, we have measured neutron quasielastic scattering of liquid Bi by using cold disk chopper spectrometer installed at MLF of J-PARC. The van Hove function revealed that the shoulder structure located at a longer side of the first peak in g(r) exhibits a longer relaxation time than the main structures such as the first and second peaks.

Journal Articles

Neutron scattering study of yttrium iron garnet

Shamoto, Shinichi; Ito, Takashi; Onishi, Hiroaki; Yamauchi, Hiroki; Inamura, Yasuhiro; Matsuura, Masato*; Akatsu, Mitsuhiro*; Kodama, Katsuaki; Nakao, Akiko*; Moyoshi, Taketo*; et al.

Physical Review B, 97(5), p.054429_1 - 054429_9, 2018/02

 Times Cited Count:16 Percentile:66.02(Materials Science, Multidisciplinary)

Nuclear and magnetic structure and full magnon dispersions of yttrium iron garnet Y$$_3$$Fe$$_5$$O$$_{12}$$ have been studied by neutron scattering. The lowest-energy dispersion below 14 meV exhibits a quadratic dispersion as expected from ferromagnetic magnons. The imaginary part of $$q$$-integrated dynamical spin susceptibility $$chi$$"($$E$$) exhibits a square-root energy-dependence in the low energies. The magnon density of state is estimated from the $$chi$$"($$E$$) obtained on an absolute scale. The value is consistent with a single chirality mode for the magnon branch expected theoretically.

Journal Articles

Stabilization of a high-order harmonic generation seeded extreme ultraviolet free electron laser by time-synchronization control with electro-optic sampling

Tomizawa, Hiromitsu*; Sato, Takahiro*; Ogawa, Kanade*; Togawa, Kazuaki*; Tanaka, Takatsugu*; Hara, Toru*; Yabashi, Makina*; Tanaka, Hitoshi*; Ishikawa, Tetsuya*; Togashi, Tadashi*; et al.

High Power Laser Science and Engineering, 3, p.e14_1 - e14_10, 2015/04

 Times Cited Count:6 Percentile:34.58(Optics)

no abstracts in English

Journal Articles

Electron and ion coincidence momentum imaging of multichannel dissociative ionization of ethanol in intense laser fields

Itakura, Ryuji; Hosaka, Koichi*; Yokoyama, Atsushi; Ikuta, Tomoya*; Kannari, Fumihiko*; Yamanouchi, Kaoru*

Progress in Ultrafast Intense Laser Science XI; Springer Series in Chemical Physics, Vol.109, p.23 - 42, 2015/00

We investigate the multichannel dissociative ionization of ethanol in intense laser fields by the photoelectron-photoion coincidence momentum imaging and identify separately the ionization and subsequent electronic excitation in ethanol. From the energy correlation between a photoelectron and a fragment ion, we reveal the amount of the internal energy gained by ethanol cations from the laser field varies depending on the respective ionization and electronic excitation pathways.

Journal Articles

Compact XFEL and AMO sciences; SACLA and SCSS

Yabashi, Makina*; Tanaka, Hitoshi*; Tanaka, Takashi*; Tomizawa, Hiromitsu*; Togashi, Tadashi*; Nagasono, Mitsuru*; Ishikawa, Tetsuya*; Harries, J.; Hikosaka, Yasumasa*; Hishikawa, Akiyoshi*; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 46(16), p.164001_1 - 164001_19, 2013/08

 Times Cited Count:71 Percentile:95.24(Optics)

Journal Articles

Full-coherent free electron laser seeded by 13th- and 15th-order harmonics of near-infrared femtosecond laser pulses

Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Togashi, Tadashi*; Fukami, Kenji*; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 46(16), p.164006_1 - 164006_6, 2013/08

 Times Cited Count:3 Percentile:19.12(Optics)

By introducing 13th- (61.7 nm) and 15th-order harmonics (53.4 nm) of femtosecond laser pulses at 800 nm into an undulator of SCSS (SPring-8 Compact SASE Source) test accelerator at RIKEN, these harmonic pulses were amplified by a factor of more than 10$$^{2}$$ with a high contrast ratio through the interaction between accelerated electron bunches and the harmonic pulses. From numerical simulations of the amplification processes of high-order harmonic pulses in the undulator, optimum conditions of the electron bunch duration interacting with the high-order harmonic pulses were investigated for generating full-coherent and intense pulses in the extreme ultraviolet wavelength region.

Journal Articles

Full-coherent HHG-seeded EUV-FEL locked by EOS timing feedback

Ogawa, Kanade*; Sato, Takahiro*; Matsubara, Shinichi*; Okayasu, Yuichi*; Togashi, Tadashi*; Watanabe, Takahiro*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; et al.

Proceedings of 10th Conference on Lasers and Electro-Optics Pacific Rim and 18th OptoElectronics and Communications Conference and Photonics in Switching 2013 (CLEO-PR & OECC/PS 2013) (USB Flash Drive), 2 Pages, 2013/06

no abstracts in English

Journal Articles

Correlation between a photoelectron and a fragment ion in dissociative ionization of ethanol in intense near-infrared laser fields

Hosaka, Koichi*; Yokoyama, Atsushi; Yamanouchi, Kaoru*; Itakura, Ryuji

Journal of Chemical Physics, 138(20), p.204301_1 - 204301_9, 2013/05

 Times Cited Count:15 Percentile:50.42(Chemistry, Physical)

Dissociative ionization of ethanol (C$$_{2}$$H$$_{5}$$OH) induced by an intense near-infrared laser pulse are investigated using photoelectron-photoion coincidence method. It is shown that both the electronic ground state and the first electronically excited state of C$$_{2}$$H$$_{5}$$OH$$^{+}$$ are produced at the moment of photoelectron emission. From the observed correlation between the electronic states of C$$_{2}$$H$$_{5}$$OH$$^{+}$$ prepared at the moment of photoelectron emission and the kinetic energy release of the fragment ions, it is revealed that C$$_{2}$$H$$_{5}$$OH$$^{+}$$ prepared in the electronic ground state at the photoelectron emission gains larger internal energy in the end than that prepared in the electronically excited state. The averaged internal energy of C$$_{2}$$H$$_{5}$$OH$$^{+}$$ just before the dissociation is found to increase when the laser field intensity increases from 9 to 23 TW/cm$$^{2}$$. And when the laser pulse duration increases from 35 to 800 fs.

Journal Articles

High intense full-coherent radiation of free electron laser seeded by high-order harmonics in extreme-ultraviolet region

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of Ultrafast Optics IX (CD-ROM), 2 Pages, 2013/03

We have demonstrated free-electron laser radiation seeded by high-order harmonics in the extreme-ultraviolet region. Strong enhancement of the radiation intensity by a factor of 104 was observed with timing control of an electro-optical sampling technique.

Journal Articles

Photoionization of atoms and molecules by intense EUV-FEL pulses and FEL seeded by high-order harmonic of ultrashort laser pulses

Iwasaki, Atsushi*; Sato, Takahiro*; Owada, Shigeki*; Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Kannari, Fumihiko*; Yagishita, Akira*; et al.

Reza Kenkyu, 40(9), p.687 - 690, 2012/09

no abstracts in English

Journal Articles

Synchronization of FEL and high-order harmonics of ultrashort-pulsed laser for generating intense full-coherent EUV light pulses

Iwasaki, Atsushi*; Sato, Takahiro*; Owada, Shigeki*; Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Matsubara, Shinichi*; Okayasu, Yuichi*; et al.

Proceedings of International Conference on Ultrafast Phenomena 2012 (UP 2012) (Internet), 3 Pages, 2012/07

 Times Cited Count:0 Percentile:0.03

no abstracts in English

Journal Articles

Extreme ultraviolet free electron laser seeded by high-order harmonic

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of 11th International School and Symposium on Synchrotron Radiation in Natural Science (ISSRNS 2012), p.1 - 21, 2012/05

The 13th harmonic of a Ti:sapphire laser has been significantly amplified with the SCSS test accelerator. The temporal and spatial overlap of the electron beam and the high harmonic radiation were precisely tuned for achieving the seeded free electron laser operation. With numerical simulation the present HH-seeded FEL scheme could readily be applied to the wavelength region down to 10 nm.

Journal Articles

Separation of ionization and subsequent electronic excitation for formation of electronically excited ethanol cation in intense laser fields

Ikuta, Tomoya*; Hosaka, Koichi*; Akagi, Hiroshi; Yokoyama, Atsushi; Yamanouchi, Kaoru*; Kannari, Fumihiko*; Itakura, Ryuji

Journal of Physics B; Atomic, Molecular and Optical Physics, 44(19), p.191002_1 - 191002_5, 2011/10

 Times Cited Count:10 Percentile:47.26(Optics)

Ionization and subsequent electronic excitation occurring within the same laser pulse (400 nm, 96 fs, 1.3$$sim$$18 TW/cm$$^{-2}$$) are separately investigated by measuring in coincidence an electron and a product ion produced from C$$_{2}$$H$$_{5}$$OH. We reveal that the nascent population in the electronically excited C$$_{2}$$H$$_{5}$$OH$$^{+}$$ prepared by the ionization decreases as the laser intensity increases, while the subsequent electronic excitation is enhanced through the resonant electronic transitions. Ionization and electronic excitation mechanisms are described based on the electronic state distributions of C$$_{2}$$H$$_{5}$$OH$$^{+}$$.

Journal Articles

XUV-FEL spectroscopy; He two-photon ionization cross-sections

Sato, Takahiro*; Iwasaki, Atsushi*; Ishibashi, Kazuki*; Okino, Tomoya*; Yamanouchi, Kaoru*; Adachi, Junichi*; Yagishita, Akira*; Yazawa, Hiroki*; Kannari, Fumihiko*; Aoyama, Makoto; et al.

Europhysics News, 42(5), P. 10, 2011/09

The resonant and non-resonant two-photon single ionization processes of He were investigated using intense free electron laser light in the extreme ultraviolet (XUV) region (53.4-61.4 nm) covering the 1s-2p and 1s-3p resonant transitions of He. On the basis of the dependences of the yield of He$$^{+}$$ on the XUV light-field intensity at 53.4, 58.4, 56.0 and 61.4 nm, the absolute values of the two-photon ionization cross sections of He at the four different wavelengths and their dependence on the light-field intensity were determined for the first time.

Journal Articles

Determination of the absolute two-photon ionization cross section of He by an XUV free electron laser

Sato, Takahiro*; Iwasaki, Atsushi*; Ishibashi, Kazuki*; Okino, Tomoya*; Yamanouchi, Kaoru*; Adachi, Junichi*; Yagishita, Akira*; Yazawa, Hiroki*; Kannari, Fumihiko*; Aoyama, Makoto; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 44(16), p.161001_1 - 161001_5, 2011/08

 Times Cited Count:35 Percentile:82.86(Optics)

The resonant and non-resonant two-photon single ionization processes of He were investigated using intense free electron laser light in the extreme ultraviolet (XUV) region (53.4-61.4 nm) covering the 1s-2p and 1s-3p resonant transitions of He. On the basis of the dependences of the yield of He$$^{+}$$ on the XUV light-field intensity at 53.4, 58.4, 56.0 and 61.4 nm, the absolute values of the two-photon ionization cross sections of He at the four different wavelengths and their dependence on the light-field intensity were determined for the first time.

Journal Articles

Extreme ultraviolet free electron laser seeded by high-order harmonic

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Okino, Tomoya*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of 2011 Conference on Lasers and Electro-Optics (CLEO 2011) (CD-ROM), p.1527 - 1528, 2011/05

We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.

Journal Articles

Seeding of extreme ultraviolet free electron laser with high-order harmonic

Takahashi, Eiji*; Togashi, Tadashi*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; et al.

Proceedings of European Conference on Lasers and Electro-Optics and the 12th European Quantum Electronics Conference (CLEO/Europe-EQEC 2011) (CD-ROM), 1 Pages, 2011/05

We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.

Journal Articles

EUV-FEL seeded by high-order harmonic

Takahashi, Eiji*; Togashi, Tadashi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Hara, Toru*; Matsubara, Shinichi*; et al.

Proceedings of International Quantum Electronics Conference and the Pacific Rim Conference on Lasers and Electro-Optics (IQEC/CLEO Pacific Rim 2011) (CD-ROM), p.199 - 200, 2011/05

We succeeded in generating the seeded free electron laser (FEL) with wavelengths of 61 nm at the SCSS test accelerator. The 13th (61 nm) harmonics generated by focusing the high peak power Ti:Sapphire laser to the Xe gas cell was directed to the undulator. This is first realization of the seeded FEL in extreme ultraviolet region.

Journal Articles

Extreme ultraviolet free electron laser seeded with high-order harmonic of Ti:sapphore laser

Togashi, Tadashi*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Okino, Tomoya*; Yamanouchi, Kaoru*; et al.

Optics Express (Internet), 19(1), p.317 - 324, 2011/01

 Times Cited Count:93 Percentile:96.48(Optics)

The 13th harmonic of a Ti:sapphire (Ti:S) laser in the plateau region was injected as a seeding source to a 250-MeV free-electron-laser (FEL) amplifier. When the amplification conditions were fulfilled, strong enhancement of the radiation intensity by a factor of 650 was observed. The random and uncontrollable spikes, which appeared in the spectra of the Self-Amplified Spontaneous Emission (SASE) based FEL radiation without the seeding source, were found to be suppressed drastically to form to a narrow-band, single peak profile at 61.2 nm. The properties of the seeded FEL radiation were well reproduced by numerical simulations. We discuss the future precept of the seeded FEL scheme to the shorter wavelength region.

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