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Journal Articles

Ion beam induced luminescence analysis of europium complexes in styrene-divinylbenzene copolymer-coated spherical silica by proton and argon ion beams irradiation

Nakahara, Masaumi; Watanabe, So; Takeuchi, Masayuki; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Kada, Wataru*; et al.

Nuclear Instruments and Methods in Physics Research B, 542, p.144 - 150, 2023/09

The structures of Eu complexes in the adsorbents prepared with various extractants were evaluated by ion beam induced luminescence analysis in an extraction chromatography for minor actinides recovery. The luminescence of Eu was measured with a proton beam obtained from the single-ended accelerator and an argon ion beam obtained from the azimuthally varying field cyclotron in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In this study, it was confirmed that the spectral shape of Eu complexes in the adsorbents varied depending on the kinds of extractants, and the correlation between the change in the spectra and the structures of Eu complexes was investigated.

Journal Articles

Ion beam induced luminescence spectra of europium complexes in silica-based adsorbent

Nakahara, Masaumi; Watanabe, So; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Kada, Wataru*; Hagura, Naoto*

QST-M-39; QST Takasaki Annual Report 2021, P. 62, 2023/02

In an extraction chromatography method for minor actinides recovery, analysis for the structure of complex in a silica-based adsorbent has been studied to separate minor actinides efficiently. In this study, Eu was used as simulated material of minor actinides, and silica-based adsorbents containing Eu complex were prepared. The ion beam induced luminescence spectra of Eu complexes in silica-based adsorbents were measured, and the basic data for the structures of Eu complexes were obtained.

Journal Articles

Initiatives to address the lifetime improvement of HBC stripper foil for 3GeV synchrotron of J-PARC

Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*

Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.850 - 854, 2021/10

no abstracts in English

Journal Articles

Analysis of J-HBC stripper foil for the J-PARC RCS

Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*

JPS Conference Proceedings (Internet), 33, p.011019_1 - 011019_7, 2021/03

BB2019-1209.pdf:0.86MB

The multi-turn charge-exchange H$$^{-}$$ beam injection scheme with stripper foils is one of the key techniques to achieve a MW-class high power proton beam. The J-PARC RCS adopts Hybrid type Boron-doped Carbon (HBC) stripper foil, which was developed in KEK to improve the lifetime. Indeed, the RCS user operation confirmed that HBC foil has the great advantage of a longer lifetime against high beam irradiation. To examine characteristics of the HBC foils, various beam studies were performed, such as the stripping efficiency measurement and long-term observation with an H$$^{-}$$ beam in the J-PARC RCS, foil analysis using RBS, EDR and PIXE methods, and SEM and TEM observation after the ion beam irradiation in Takasaki Ion Accelerators for Advanced Radiation Application (TIARA) on National Institutes for Quantum and Radiological Science and Technology (QST). Recently, the deposition apparatus for the HBC foils from the KEK Tsukuba-site was relocated to the JAEA Tokai-site, and we started fabrication of new HBC foil in 2017. (The new one fabricated in JAEA we call J-HBC foil.) And, we continue investigations in TIARA with the J-HBC foils. Furthermore, in-depth researches by changing the process parameters of the foil deposition are carried on. Recent results suggest that the amount of the boron doped in the foil is more important parameter than the ratio of the discharge amount of carbon from cathode and anode electrodes. In this presentation, we will report the details of recent analysis of the J-HBC foil.

Journal Articles

Micro-PIXE analysis study of ferrite products synthesized from simulated radioactive liquid waste containing chemical hazardous elements

Abe, Tomohisa; Shimazaki, Takejiro; Osugi, Takeshi; Nakazawa, Osamu; Yamada, Naoto*; Yuri, Yosuke*; Sato, Takahiro*

QST-M-16; QST Takasaki Annual Report 2017, P. 140, 2019/03

no abstracts in English

Journal Articles

Application of ferrite process to radioactive waste; Study of ferrite product stability by micro-PIXE analysis

Abe, Tomohisa; Shimazaki, Takejiro; Osugi, Takeshi; Yamada, Naoto*; Yuri, Yosuke*; Sato, Takahiro*

QST-M-8; QST Takasaki Annual Report 2016, P. 61, 2018/03

no abstracts in English

Journal Articles

Fabrication of neutron optical devices using PBW technique

Sakai, Takuro; Iikura, Hiroshi; Yamada, Naoto*; Sato, Takahiro*; Ishii, Yasuyuki*; Uchida, Masaya*

QST-M-8; QST Takasaki Annual Report 2016, P. 140, 2018/03

Journal Articles

Element distribution measurement in incineration ash using micro-PIXE analysis

Abe, Tomohisa; Shimazaki, Takejiro; Nakayama, Takuya; Osone, Osamu; Osugi, Takeshi; Nakazawa, Osamu; Yuri, Yosuke*; Yamada, Naoto*; Sato, Takahiro*

QST-M-2; QST Takasaki Annual Report 2015, P. 83, 2017/03

no abstracts in English

Journal Articles

Valence-band electronic structure evolution of graphene oxide upon thermal annealing for optoelectronics

Yamaguchi, Hisato*; Ogawa, Shuichi*; Watanabe, Daiki*; Hozumi, Hideaki*; Gao, Y.*; Eda, Goki*; Mattevi, C.*; Fujita, Takeshi*; Yoshigoe, Akitaka; Ishizuka, Shinji*; et al.

Physica Status Solidi (A), 213(9), p.2380 - 2386, 2016/09

 Times Cited Count:13 Percentile:52.76(Materials Science, Multidisciplinary)

We report valence-band electronic structure evolution of graphene oxide (GO) upon its thermal reduction. The degree of oxygen functionalization was controlled by annealing temperature, and an electronic structure evolution was monitored using real-time ultraviolet photoelectron spectroscopy. We observed a drastic increase in the density of states around the Fermi level upon thermal annealing at $$sim$$ 600$$^{circ}$$C. The result indicates that while there is an apparent bandgap for GO prior to a thermal reduction, the gap closes after an annealing around that temperature. This trend of bandgap closure was correlated with the electrical, chemical, and structural properties to determine a set of GO material properties that is optimal for optoelectronics. The results revealed that annealing at a temperature of 500$$^{circ}$$C leads to the desired properties, demonstrated by a uniform and an order of magnitude enhanced photocurrent map of an individual GO sheet compared to an as-synthesized counterpart.

JAEA Reports

Light ion microbeam analysis / processing system and its improvement

Koka, Masashi; Ishii, Yasuyuki; Yamada, Naoto; Okubo, Takeru; Kada, Wataru*; Kitamura, Akane; Iwata, Yoshihiro*; Kamiya, Tomihiro; Sato, Takahiro

JAEA-Technology 2016-006, 41 Pages, 2016/03

JAEA-Technology-2016-006.pdf:14.03MB

A MeV-class light ion microbeam system has been developed for micro-analysis and micro-fabrication with high spatial resolution at 3-MV single-ended accelerator in Takasaki Ion Accelerators for Advanced Radiation Application of Takasaki Advanced Radiation Research Institute, Sector of Nuclear Science Research, Japan Atomic Energy Agency. This report describes the technical improvements for the main apparatus (the accelerator, beam-transport lines, and microbeam system), and auxiliary equipments/ parts for ion beam applications such as Particle Induced X-ray/Gamma-ray Emission (PIXE/PIGE) analysis, 3-D element distribution analysis using PIXE-Computed Tomography(CT), Ion Beam-Induced Luminescence (IBIL) analysis, and Proton Beam Writing with the microbeam scanning, with functional outline of these apparatus and equipments/parts.

Journal Articles

Investigation of phosphor materials for the real-time measurement of the transverse intensity distribution of large-area ion beams at the JAEA AVF cyclotron facility

Yuri, Yosuke; Yuyama, Takahiro; Ishizaka, Tomohisa; Koka, Masashi; Yamada, Naoto

Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.420 - 423, 2015/09

no abstracts in English

Journal Articles

Current status of electrostatic accelerators at TIARA

Usui, Aya; Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; et al.

Dai-27-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.118 - 121, 2015/03

no abstracts in English

Journal Articles

Operation of electrostatic accelerators

Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Usui, Aya; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Nara, Takayuki; et al.

JAEA-Review 2013-059, JAEA Takasaki Annual Report 2012, P. 179, 2014/03

Three electrostatic accelerators at TIARA were operated on schedule in fiscal year 2012 except changing its schedule by cancellations of users. The yearly operation time of the 3 MV tandem accelerator, the 400 kV ion implanter and the 3MV single-ended accelerator were in the same levels as the ordinary one, whose operation time totaled to 2,073, 1,847 and 2,389 hours, respectively. The tandem accelerator had no trouble, whereas the ion implanter and the single-ended accelerator stopped by any troubles for one day and four days, respectively. The molecular ion beam of helium hydride was generated by the ion implanter, because the users required irradiation of several cluster ions in order to study the effect of irradiation. As a result, its intensity of beam was 50 nA at 200 kV. The ion beam of tungsten (W) at 15 MeV was accelerated by the tandem accelerator, whose intensity was 20 nA at charge state of 4+, because of the request from a researcher in the field of nuclear fusion.

Journal Articles

Current status of electrostatic accelerators at TIARA

Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Usui, Aya; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; et al.

Dai-26-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.79 - 81, 2013/07

Three electrostatic accelerators at TIARA were operated on schedule in fiscal year 2012 except changing its schedule by cancellations of users. The yearly operation time of the 3MV tandem accelerator, the 400 kV ion implanter and the 3 MV single-ended accelerator were in the same levels as the ordinary one, whose operation time totaled to 2,073, 1,847 and 2,389 hours, respectively. The tandem accelerator had no trouble, whereas the ion implanter and the single-ended accelerator stopped by any troubles for one day and four days, respectively. The ion implanter generated molecular ion beam of helium hydride by using the Freeman type ion source, because of the request from the user. As a result, its intensity of beam was 50 nA at 200 kV.

Journal Articles

Operation of electrostatic accelerators

Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Nara, Takayuki; Kitano, Toshihiko*; et al.

JAEA-Review 2012-046, JAEA Takasaki Annual Report 2011, P. 173, 2013/01

The three electrostatic accelerators at the TIARA had no mechanical damage when the Tohoku earthquake happened on March 11, 2011. But, they could not be operated during April, due to the influence of planned power outage by TEPCO. These accelerators additionally operated on Saturday for ten days in order to compensate for the lost experiment time. As a result, the yearly operation time had kept the same level as the ordinary one. The ion beam of erbium (Er) with 11.7MeV was accelerated newly by the tandem accelerator, whose intensity was 20nA at charge state of 3+. The sequential generation/irradiation of two different kinds of fullerene ions was achieved at the ion implanter by a mixed powder method without exchange of the Freeman type ion source by the user's request.

Journal Articles

Operation of electrostatic accelerators at TIARA

Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Nara, Takayuki; Kitano, Toshihiko*; et al.

Dai-7-Kai Takasaki Oyo Kenkyu Shimpojiumu Yoshishu, P. 119, 2012/10

The three electrostatic accelerators at TIARA had no damage when the Tohoku earthquake happened on March 11, 2011. But, they could not be operated until end of April, due to the influence of planned power outage and keep out into the controlled area for radiation. These accelerators additionally operated on Saturday for twelve days in order to compensate for the lost experiment time. Therefore, the yearly operation time had kept the same level as the ordinary one. The tandem accelerator has stopped leakage of the SF$$_{6}$$ gas from the base flange on the tank by the Viton gasket of rectangular cross section at the new type.

Journal Articles

Current status of electrostatic accelerators at TIARA

Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; Yamada, Naoto*; et al.

Dai-25-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.64 - 66, 2012/07

The three electrostatic accelerators at the TIARA had no damage when the Tohoku earthquake happened on March 11, 2011. But, they could not be operated until end of April, due to the influence of planned power outage and keep out into the controlled area for radiation. These accelerators additionally operated on Saturday for twelve days in order to compensate for the lost experiment time. Therefore, the yearly operation time had kept the same level as the ordinary one. The tandem accelerator has stopped leakage of the SF$$_{6}$$ gas from the base flange on the tank by the Viton gasket of rectangular cross section at the new type. The ion implanter could generate two kinds of fullerene ions by a mixed material of ions and a controlled temperature of the oven without exchange of ion source.

Journal Articles

Operation of the electrostatic accelerators

Agematsu, Takashi; Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Yokota, Wataru; et al.

JAEA-Review 2011-043, JAEA Takasaki Annual Report 2010, P. 173, 2012/01

Three electrostatic accelerators of TIARA were operated smoothly in FY 2010, and all the planned experiments were carried out except those canceled by users or the impact of Great East Japan Earthquake on March 11, 2011. On the other hand, Saturday operation for experiments was carried out after October on the Global Nuclear-Human Resource Development Initiative. The yearly operation time of the tandem accelerator, the single-ended accelerator and the ion implanter amounted to 2116, 2367 and 1800 hours, respectively, which were similar to those of usual years. Regarding the single-ended accelerator, the generator in the high-voltage terminal failed and was replaced with new one. A switching magnet was installed for a new branch beam line of the ion implanter. As to the tandem accelerator, In ion was generated and accelerated at intensity of 500 nA.

Journal Articles

Current status of electrostatic accelerators at TIARA

Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Agematsu, Takashi; Kitano, Toshihiko*; Takayama, Terumitsu*; Orimo, Takao*; Kanai, Shinji*; Aoki, Yuki*; et al.

Dai-24-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.125 - 128, 2011/07

The yearly operation time of three electrostatic accelerators at TIARA of Japan Atomic Energy Agency is keeping the same level since 2000, the tandem accelerator, the ion implanter and the single-ended accelerator amounted to about 2000, 1900 and 2500 hours, respectively. Three electrostatic accelerators did not have damage when the Tohoku Earthquake occurred on March 11, 2011. However, these accelerators were not able to operate during the planned power outage by Tokyo Electric Power Company (TEPCO). The tandem accelerator accelerated ion beam of In, which gave intensity of 500nA with stability. Additionally, the ion implanter generated maximum 400nA at ion beam of Gd, which was used in experiments for the users.

Journal Articles

Operation of the electrostatic accelerators

Agematsu, Takashi; Uno, Sadanori; Chiba, Atsuya; Yamada, Keisuke; Yokoyama, Akihito; Saito, Yuichi; Ishii, Yasuyuki; Sato, Takahiro; Okubo, Takeru; Yokota, Wataru; et al.

JAEA-Review 2010-065, JAEA Takasaki Annual Report 2009, P. 181, 2011/01

Three electrostatic accelerators of TIARA were operated smoothly in FY 2009, and all the planned experiments were carried out except those canceled by users. The yearly operation time of the tandem accelerator, the single-ended accelerator and the ion implanter amounted to 2100, 2416 and 1866 hours, respectively. Regarding the single-ended accelerator, the radio frequency oscillator of the ion source mounted in high-voltage terminal and the sequencer for control of the SB beam line failed, and they were replaced. The oven controller of Freeman ion source of the ion implanter was renewed. As to the tandem accelerator, Mn ion was successfully generated and accelerated with intensity of 150 nA.

52 (Records 1-20 displayed on this page)