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Journal Articles

Neutron reflectivity study on the nanostructure of PMMA chains near substrate interfaces based on contrast variation accompanied with small molecule sorption

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Nakanishi, Yohei*; Shibata, Motoki*; Takenaka, Mikihito*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; Miyazaki, Tsukasa*

Soft Matter, 19(11), p.2082 - 2089, 2023/03

 Times Cited Count:0 Percentile:0(Chemistry, Physical)

Journal Articles

Interfacial distribution of Nafion ionomer thin films on nitrogen-modified carbon surfaces

Yoshimune, Wataru*; Kikkawa, Nobuaki*; Yoneyama, Hiroaki*; Takahashi, Naoko*; Minami, Saori*; Akimoto, Yusuke*; Mitsuoka, Takuya*; Kawaura, Hiroyuki*; Harada, Masashi*; Yamada, Norifumi*; et al.

ACS Applied Materials & Interfaces, 14(48), p.53744 - 53754, 2022/11

 Times Cited Count:6 Percentile:59.75(Nanoscience & Nanotechnology)

Journal Articles

Neutron reflectivity study on the suppression of interfacial water accumulation between a polypropylene thin film and Si substrate using a silane-coupling agent

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Nakanishi, Yohei*; Takenaka, Mikihito*; Shibata, Motoki*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; et al.

Langmuir, 38(41), p.12457 - 12465, 2022/10

 Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)

Journal Articles

New design of a sample cell for neutron reflectometry in liquid-liquid systems and its application for studying structures at air-liquid and liquid-liquid interfaces

Akutsu-Suyama, Kazuhiro*; Yamada, Norifumi*; Ueda, Yuki; Motokawa, Ryuhei; Narita, Hirokazu*

Applied Sciences (Internet), 12(3), p.1215_1 - 1215_10, 2022/02

 Times Cited Count:1 Percentile:28.33(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

Neutron reflectometry-based ${it in situ}$ structural analysis of an aligning agent additive for the alignment of nematic liquid crystals on solid substrates

Nemoto, Fumiya*; Yamada, Norifumi*; Hino, Masahiro*; Aoki, Hiroyuki; Seto, Hideki*

Soft Matter, 18(3), p.545 - 553, 2022/01

 Times Cited Count:0 Percentile:0(Chemistry, Physical)

Journal Articles

Multilayered lamellar materials and thin films by instant self-assembly of amphiphilic random copolymers

Ikami, Takaya*; Watanabe, Yuki*; Ogawa, Hiroki*; Takenaka, Mikihito*; Yamada, Norifumi*; Ouchi, Makoto*; Aoki, Hiroyuki; Terashima, Takaya*

ACS Macro Lett (Internet), 10(12), p.1524 - 1528, 2021/12

 Times Cited Count:7 Percentile:48.3(Polymer Science)

Journal Articles

Neutron reflectivity on the mobile surface and immobile interfacial layers in the poly(vinyl acetate) adsorption layer on a Si substrate with deuterated toluene vapor-induced swelling

Miyazaki, Tsukasa*; Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Aoki, Hiroyuki; Yamada, Norifumi*; Miyata, Noboru*

Langmuir, 36(49), p.15181 - 15188, 2020/12

 Times Cited Count:6 Percentile:31.74(Chemistry, Multidisciplinary)

Journal Articles

Water distribution in Nafion thin films on hydrophilic and hydrophobic carbon substrates

Ito, Kanae; Harada, Masashi*; Yamada, Norifumi*; Kudo, Kenji*; Aoki, Hiroyuki; Kanaya, Toshiji*

Langmuir, 36(43), p.12830 - 12837, 2020/11

 Times Cited Count:13 Percentile:58.64(Chemistry, Multidisciplinary)

JAEA Reports

Presentation Materials Related to Neutron Instruments in the Technical Study Meetings for Future MLF

Nakajima, Kenji; Harjo, S.; Yamada, Norifumi*; Oikawa, Kenichi; Kajimoto, Ryoichi

JAEA-Review 2018-032, 43 Pages, 2019/02

JAEA-Review-2018-032.pdf:9.78MB

A series of meetings to discuss future neutron/muon sources and instruments at Materials and Life Science Experimental Facility (MLF) in Japan Proton Accelerator Research Complex (J-PARC) has been held since 2017. Each of the neutron instrument groups in MLF proposed required features for future instruments, while addressing issues of the current instruments and facilities. This report compiles the presentation materials presented by the neutron instrument groups in the meetings to help future discussion for the coming MLF.

Journal Articles

Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex, 2; Neutron scattering instruments

Nakajima, Kenji; Kawakita, Yukinobu; Ito, Shinichi*; Abe, Jun*; Aizawa, Kazuya; Aoki, Hiroyuki; Endo, Hitoshi*; Fujita, Masaki*; Funakoshi, Kenichi*; Gong, W.*; et al.

Quantum Beam Science (Internet), 1(3), p.9_1 - 9_59, 2017/12

The neutron instruments suite, installed at the spallation neutron source of the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), is reviewed. MLF has 23 neutron beam ports and 21 instruments are in operation for user programs or are under commissioning. A unique and challenging instrumental suite in MLF has been realized via combination of a high-performance neutron source, optimized for neutron scattering, and unique instruments using cutting-edge technologies. All instruments are/will serve in world-leading investigations in a broad range of fields, from fundamental physics to industrial applications. In this review, overviews, characteristic features, and typical applications of the individual instruments are mentioned.

Journal Articles

Dynamical behavior of human $$alpha$$-synuclein studied by quasielastic neutron scattering

Fujiwara, Satoru; Araki, Katsuya*; Matsuo, Tatsuhito; Yagi, Hisashi*; Yamada, Takeshi*; Shibata, Kaoru; Mochizuki, Hideki*

PLOS ONE (Internet), 11(4), p.e0151447_1 - e0151447_17, 2016/04

 Times Cited Count:24 Percentile:64.99(Multidisciplinary Sciences)

Journal Articles

Neutron reflectometers in J-PARC

Yamada, Norifumi*; Takeda, Masayasu; Yamazaki, Dai

Hamon, 24(4), p.288 - 295, 2014/11

no abstracts in English

Journal Articles

Treatment of radioactive wastes

Kozawa, Kazushige; Yamada, Satoshi

Hoshasen Gyomu Jujisha Sai Kyoiku Kunren Tekisuto, p.133 - 150, 2011/00

no abstracts in English

Journal Articles

Producing new gene resources in Fig by using ion-beam irradiation

Asami, Itsuo*; Fukuta, Shiro*; Kuroyanagi, Satoru*; Yamada, Masato*; Hase, Yoshihiro; Yoshihara, Ryohei; Narumi, Issei

JAEA-Review 2009-041, JAEA Takasaki Annual Report 2008, P. 78, 2009/12

no abstracts in English

Journal Articles

Crystal structure of frustrated antiferromagnet UNi$$_4$$B

Haga, Yoshinori; Oyamada, Akira*; Matsuda, Tatsuma; Ikeda, Shugo; Onuki, Yoshichika

Physica B; Condensed Matter, 403(5-9), p.900 - 902, 2008/04

 Times Cited Count:9 Percentile:40.55(Physics, Condensed Matter)

Crystal structure of a frustrated antiferomagnet UNi$$_4$$B was investigated precisely by the X-ray diffraction on a Czhochralski-grown high-quality single crystal. The unit cell was unambiguously determined as orthorhombic (space group Cmcm) with the lattice parameters $$a$$ = 6.97, $$b$$ = 17.14, and $$c$$ = 14.89 ${AA}$. These orthorhombic lattice parameters are approximately related to the reported hexagonal unit cell parameters $$a$$$$_{rm hex}$$ and $$c_{rm hex}$$ as $$a$$ = 2$$c_{rm hex}$$, $$b$$ = 2$$sqrt{3}$$$$a$$$$_{rm hex}$$ and $$c$$=3$$a$$$$_{rm hex}$$. They are also consistent with the previously reported weak superlattice reflections measured by the neutron scattering assuming the hexagonal lattice. We have found that four different uranium sites with the different local environment exist. Therefore UNi$$_4$$B can no more be regarded as a pure frustrated system as previously assumed and its magnetic properties should be reanalized based on the correct structure.

Journal Articles

Extended steady-state and high-beta regimes of net-current free heliotron plasmas in the Large Helical Device

Motojima, Osamu*; Yamada, Hiroshi*; Komori, Akio*; Oyabu, Nobuyoshi*; Muto, Takashi*; Kaneko, Osamu*; Kawahata, Kazuo*; Mito, Toshiyuki*; Ida, Katsumi*; Imagawa, Shinsaku*; et al.

Nuclear Fusion, 47(10), p.S668 - S676, 2007/10

 Times Cited Count:34 Percentile:73.71(Physics, Fluids & Plasmas)

The performance of net-current free heliotron plasmas has been developed by findings of innovative operational scenarios in conjunction with an upgrade of the heating power and the pumping/fuelling capability in the Large Helical Device (LHD). Consequently, the operational regime has been extended, in particular, with regard to high density, long pulse length and high beta. Diversified studies in LHD have elucidated the advantages of net-current free heliotron plasmas. In particular, an internal diffusion barrier (IDB) by a combination of efficient pumping of the local island divertor function and core fuelling by pellet injection has realized a super dense core as high as 5$$times$$10$$^{20}$$ m$$^{-3}$$, which stimulates an attractive super dense core reactor. Achievements of a volume averaged beta of 4.5% and a discharge duration of 54 min with a total input energy of 1.6 GJ (490 kW on average) are also highlighted. The progress of LHD experiments in these two years is overviewed by highlighting IDB, high-beta and long pulse.

Journal Articles

Highly polarized cold neutron beam obtained by using a quadrupole magnet

Oku, Takayuki; Yamada, Satoru; Shinohara, Takenao; Suzuki, Junichi; Mishima, Kenji*; Hirota, Katsuya*; Sato, Hiromi*; Shimizu, Hirohiko

Physica B; Condensed Matter, 397(1-2), p.188 - 191, 2007/07

 Times Cited Count:5 Percentile:27.18(Physics, Condensed Matter)

We have studied a neutron polarization method by means of a quadrupole magnet. By passing through the aperture of the quadrupole magnet (QM), positive and negative polarity neutrons are accelerated in opposite directions and spatially separated due to the magnetic field gradient. Then, by extracting one spin component, we can obtain a highly polarized neutron beam. Since polarized neutrons do not interact with any substances in this method, we can obtain the polarized neutron beam free from neutron attenuation. As a result of a cold neutron beam polarization experiment by using the QM, we obtained extremely high neutron polarization degree P0.999. In this paper, we show some experimental results of the neutron polarization experiment and discuss the application of the QM-based polarizing device to neutron scattering experiments.

Journal Articles

A Focusing-geometry small-angle neutron scattering instrument with a magnetic neutron lens

Oku, Takayuki; Iwase, Hiroki; Shinohara, Takenao; Yamada, Satoru; Hirota, Katsuya*; Koizumi, Satoshi; Suzuki, Junichi; Hashimoto, Takeji; Shimizu, Hirohiko

Journal of Applied Crystallography, 40(s1), p.s408 - s413, 2007/04

 Times Cited Count:28 Percentile:89.68(Chemistry, Multidisciplinary)

Measuring efficiency and/or angular resolution of small-angle neutron scattering experiments can be improved by focusing neutrons on a detector plane. Thus, a magnetic focusing lens (MNL) have been installed into the SANS instrument, SANS-J-II, of JRR-3 in AEA for the focusing-geometry SANS (FSANS) experiments. The MNL is an extended Halbach-type permanent sextupole magnet. The inner diameter and length of the MNL are 35 mm and 1200 mm, respectively. As the MNL functions as the focusing lens only for the polarized neutron with positive polarity, the incident neutron polarization is set positive by using the supermirror polarizer and the two-coil spin flipper. The intensity distribution of the neutrons focused by the MNL at the detector position was measured by using a high-resolution photomultiplier-based scintillation detector. In this paper, the neutron focusing property of the focusing setup is investigated, and the performance of the FSANS instrument is discussed.

Journal Articles

Extended steady-state and high-beta regimes of net-current free heliotron plasmas in the large helical device

Motojima, Osamu*; Yamada, Hiroshi*; Komori, Akio*; Oyabu, Nobuyoshi*; Kaneko, Osamu*; Kawahata, Kazuo*; Mito, Toshiyuki*; Muto, Takashi*; Ida, Katsumi*; Imagawa, Shinsaku*; et al.

Proceedings of 21st IAEA Fusion Energy Conference (FEC 2006) (CD-ROM), 12 Pages, 2007/03

The performance of net-current free Heliotron plasmas has been developed by findings of innovative operational scenarios in conjunction with an upgrade of the heating power and the pumping/fueling capability in the Large Helical Device (LHD). Consequently, the operational regime has been extended, in particular, with regard to high density, long pulse length and high beta. Diversified studies in LHD have elucidated the advantages of net-current free heliotron plasmas. In particular, an Internal Diffusion Barrier (IDB) by combination of efficient pumping of the local island divertor function and core fueling by pellet injection has realized a super dense core as high as 5$$times$$10$$^{20}$$m$$^{-3}$$, which stimulates an attractive super dense core reactor. Achievements of a volume averaged beta of 4.5 % and a discharge duration of 54-min. with a total input energy of 1.6 GJ (490 kW in average) are also highlighted. The progress of LHD experiments in these two years is overviewed with highlighting IDB, high $$beta$$ and long pulse.

Journal Articles

A Magnetic neutron lens based on an extended Halbach-type permanent sextupole magnet

Oku, Takayuki; Yamada, Satoru; Sasao, Hajime*; Suzuki, Junichi; Shinohara, Takenao*; Hirota, Katsuya*; Ikeda, Kazuaki*; Tsuzaki, Tsuyoshi*; Kiyanagi, Yoshiaki*; Furusaka, Michihiro*; et al.

Physica B; Condensed Matter, 385-386(2), p.1225 - 1228, 2006/11

 Times Cited Count:10 Percentile:44.47(Physics, Condensed Matter)

We have developed a magnetic neutron lens based on an extended Halbach-type permanent sextupole magnet with magnet pieces of NEOMAX-44H, -35EH and high saturation magnetization material, permendule. The aperture size of the magnet is 35 mm in diameter and the magnet length is 2,400 mm. The magnet generates a sextupole magnetic field $$B_s=(C/2)r^2$$ with a gradient coefficient $$C$$=10,600 T/m$$^2$$ inside the aperture, where $$r$$ is a distance from the magnet center axis. To prevent neutrons from hitting and reflecting at the inner surface of the magnet, the surface is covered with cadmium (Cd) sheets and also Cd pinhole slits with size of 30 mm in diameter are positioned in series inside the magnet aperture, resulting in the effective diameter of 30 mm. The neutron focusing property of the magnet is investigated by using pulsed polarized neutrons. The obtained results are discussed with the precise simulation results. Its application to the focusing-geometry small-angle neutron scattering experiments is also discussed.

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