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Journal Articles

New insights into the Cs adsorption on montmorillonite clay from $$^{133}$$Cs solid-state NMR and density functional theory calculations

Okubo, Takahiro*; Okamoto, Takuya*; Kawamura, Katsuyuki*; Gu$'e$gan, R.*; Deguchi, Kenzo*; Oki, Shinobu*; Shimizu, Tadashi*; Tachi, Yukio; Iwadate, Yasuhiko*

Journal of Physical Chemistry A, 122(48), p.9326 - 9337, 2018/12

 Times Cited Count:14 Percentile:61.08(Chemistry, Physical)

The structures of Cs adsorption on montmorillonite were investigated by the nuclear magnetic resonance (NMR) spectroscopy. The NMR spectra of Cs adsorbed on montmorillonite samples were measured under different Cs contents and relative humidity levels. NMR parameters were evaluated by the first principle calculations in order to identify the relationship between adsorbed Cs structures and NMR parameters. The comparisons between experimental and theoretical NMR spectra revealed that Cs is preferentially adsorbed at sites near Al for low Cs substituted montmorillonites, and that non-hydrated Cs present in partially Cs substituted samples, even after being hydrated under high relative humidity.

Journal Articles

Measurements of electron-induced neutrons as a tool for determination of electron temperature of fast electrons in the task of optimization laser-produced plasma ions acceleration

Sakaki, Hironao; Nishiuchi, Mamiko; Maeda, Shota; Sagisaka, Akito; Pirozhkov, A. S.; Pikuz, T.; Faenov, A.*; Ogura, Koichi; Fukami, Tomoyo; Matsukawa, Kenya*; et al.

Review of Scientific Instruments, 85(2), p.02A705_1 - 02A705_4, 2014/02

 Times Cited Count:2 Percentile:11.31(Instruments & Instrumentation)

High intensity laser-plasma interaction has attracted considerable interest for a number of years. The laser-plasma interaction is accompanied by generation of various charged particle beams. Results of simultaneous novel measurements of electron-induced photonuclear neutrons (photoneutron), which are a diagnostic of the laser-plasma interaction, are proposed to use for optimization of the laser-plasma ion generation. The proposed method is demonstrated by the laser irradiation with the intensity os 1$$times$$10$$^{21}$$ W/cm$$^{2}$$ on the metal foil target. The photoneutrons are measured by using NE213 liquid scintillation detectors. Heavy-ion signal is registered with the CR39 track detector simultaneously. The measured signals of the electron-induced photoneutrons are well reproduced by using the Particle and Heavy Ion Transport code System (PHITS). The results obtained provide useful approach for analyzing the various laser based ion beams.

Oral presentation

Off-axis XUV harmonics from relativistic laser - gas jet interaction

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

Off-axis high-order harmonics from relativistic laser - gas jet interaction

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

High-order harmonic comb from relativistic electron spikes

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

On-axis and off-axis high order harmonics generation by relativistic laser in gas jet target

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

Laser driven ion acceleration experiment by high contrast high intensity laser J-KAREN system

Nishiuchi, Mamiko; Sakaki, Hironao; Sagisaka, Akito; Maeda, Shota; Pirozhkov, A. S.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Fukuda, Yuji; Matsukawa, Kenya*; et al.

no journal, , 

no abstracts in English

Oral presentation

Measurement of electron spectrum generated by irradiating thin-Foil target with Ultra-intense Ultra-short pulse laser

Maeda, Shota; Nishiuchi, Mamiko; Sakaki, Hironao; Sagisaka, Akito; Pirozhkov, A. S.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Fukuda, Yuji; Matsukawa, Kenya*; et al.

no journal, , 

In JAEA, the high energy ions generated by the interaction between Ultra-intense Ultra-Short pulse laser and thin-foil target is being studied. Irradiating condition must be optimized to generate higher energy ions while suppress the becoming gigantic of laser. It is necessary to know the physical phenomenon in plasma to determine the parameter to optimize from the information on the electron and neutron, X-rays, which are generated simultaneously with ion. In this study, in order to measure electron temperature accurately, an electron spectrometer was developed which have broad range (1-200 MeV). The detector is comprised of permanent magnets and a fluorescent plate, CCD camera. In the presentation, the result of the calibration experiment carried out using 4, 9, 12, 15 MeV quasi-monoenergetic electron beam in HIBMC will be reported. Moreover, response analysis method was inspected using PHITS which is particle transporting Monte Carlo simulation code, and will also report the result.

Oral presentation

High-order harmonics from relativistic electron spikes

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

Source structure of high-order harmonics from relativistic electron spikes

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

High-resolution XUV imaging of catastrophes in relativistic plasma

Pirozhkov, A. S.; Kando, Masaki; Esirkepov, T. Z.; Pikuz, T.; Faenov, A. Ya.*; Ogura, Koichi; Hayashi, Yukio; Kotaki, Hideyuki; Ragozin, E. N.*; Neely, D.*; et al.

no journal, , 

Oral presentation

Structural analysis of Cs adsorption on Cs-montmorillonite using ab initio calculation and $$^{133}$$Cs solid state NMR, 2; $$^{133}$$Cs MAS and 3Q MAS NMR

Okamoto, Takuya*; Okubo, Takahiro*; Iwadate, Yasuhiko*; Deguchi, Kenzo*; Shimizu, Tadashi*; Oki, Shinobu*; Tachi, Yukio

no journal, , 

The structures of Cs adsorption on montmorillonite were investigated by the nuclear magnetic resonance (NMR) spectroscopy. The NMR spectra of Cs adsorbed montmorillonite samples with different Cs contents were collected by $$^{133}$$Cs Magic Angle Spinning (MAS) NMR and $$^{133}$$Cs Triple Quantum (3Q) MAS NMR. The adsorbed Cs structures were evaluated based on the correlations between the structural characteristics and the values of the NMR parameters predicted by the first principal calculations.

Oral presentation

Structure of hydrated Cs on montmorillonite

Okamoto, Takuya*; Okubo, Takahiro*; Iwadate, Yasuhiko*; Deguchi, Kenzo*; Shimizu, Tadashi*; Oki, Shinobu*; Tachi, Yukio

no journal, , 

The structures of Cs adsorbed on montmorillonite were investigated by $$^{133}$$Cs Magic Angle Spinning (MAS) NMR spectroscopy. The NMR spectra of Cs adsorbed on montmorillonite samples were measured under different relative humidity levels and were analyzed to evaluate the change in the structure of hydrated Cs sorbed on montmorillonite.

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