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Goto, Kenji*; Osakabe, Toyotaka; Kakurai, Kazuhisa; Uwatoko, Yoshiya*; Osawa, Akira*; Kawakami, Jun*; Tanaka, Hidekazu*
Journal of the Physical Society of Japan, 76(5), p.053704_1 - 053704_4, 2007/05
Times Cited Count:12 Percentile:57.82(Physics, Multidisciplinary)The neutron scattering investigation on magnetic excitations in KCuCl under applied pressure was performed. The softening of the excitation mode at a hydrostatic pressure of 4.7kbar was clearly observed. From the analysis of the dispersion relations, it was found that the intradimer interaction decreases under hydrostatic pressure, while most of the interdimer interactions increase.
Kakurai, Kazuhisa; Osakabe, Toyotaka; Goto, Kenji*; Osawa, Akira*; Fujisawa, Masashi*; Tanaka, Hidekazu*
Physica B; Condensed Matter, 385-386(Part 1), p.450 - 452, 2006/11
Times Cited Count:1 Percentile:6.63(Physics, Condensed Matter)KCuCl and TlCuCl are singlet ground state systems with excitation gap of 31K and 7.7K, respectively. The origin of the spin gap is the strong antiferromagnetic spin dimer of the chemical CuCl unit. These spin dimers are weakly coupled three dimensionally via non-frustrating inter dimer exchanges. The magnetization measurements under applied hydrostatic pressure show the existence of the magnetic order above certain critical pressure Pc=8.8 kbar and 0.42 kbar, respectively. We report on the elastic neutron scattering results of the pressure induced magnetic ordering in these quantum systems. The observed magnetic structures and the possible role of the spin-lattice coupling in the spin reorientation in TlCuCl3 under pressure will be discussed.
Goto, Kenji; Fujisawa, Masashi*; Tanaka, Hidekazu*; Uwatoko, Yoshiya*; Osawa, Akira*; Osakabe, Toyotaka; Kakurai, Kazuhisa
Journal of the Physical Society of Japan, 75(6), p.064703_1 - 064703_7, 2006/06
Times Cited Count:30 Percentile:76.29(Physics, Multidisciplinary)Magnetization and neutron elastic scattering experiments under hydrostatic pressure were performed on KCuCl, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that the intradimer interaction decreases with increasing hydrostatic pressure, while the sum of the interdimer interactions increases. This leads to the shrinkage of the spin gap. A quantum phase transition from a gapped state to an antiferromagnetic state occurs at Pc8.2 kbar. For PPc, magnetic reflections were observed at reciprocal lattice points equivalent to those for the lowest magnetic excitation at zero temperature. This confirms that the spin gap decreases and closes under applied pressure.
Ota, Kunio; Nakano, Katsushi; Metcalfe, R.; Ikeda, Koki; ; Amano, Kenji; Takeuchi, Shinji; Hama, Katsuhiro; Matsui, Hiroya
JNC TN7410 99-007, 44 Pages, 1999/08
*; Saido, Masahiro; Nakamura, Kazuyuki; Akiba, Masato; ; Goto, Yoshitaka*; *; *; Yamaki, Takahiro*; *; et al.
Journal of Nuclear Materials, 233-237(PT.A), p.781 - 786, 1996/00
Times Cited Count:13 Percentile:72.37(Materials Science, Multidisciplinary)no abstracts in English
Goto, Kenji*; Fujisawa, Masashi*; Osawa, Akira*; Kakurai, Kazuhisa; Osakabe, Toyotaka; Uwatoko, Yoshiya*; Tanaka, Hidekazu*
no journal, ,
no abstracts in English
Goto, Ichiro; Watanabe, So; Koizumi, Kenji; Hirano, Hiroyasu; Sano, Yuichi; Koma, Yoshikazu
no journal, ,
no abstracts in English