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Journal Articles

Fuel cycle scenarios and back-end technologies of HTGR in Japan

Fukaya, Yuji; Goto, Minoru; Shibata, Taiju

IAEA-TECDOC-2040, p.133 - 136, 2023/12

Japan has developed back-end technologies to establish a multi-recycling fuel cycle with fast breeder reactors (FBRs) to ensure energy resources. Even though the development of FBR has been retreated to one of fundamental research, the reprocessing technologies for uranium fuel and disposal technologies had been completed for Light Water Reactor (LWR) fuel cycle on the process. These technologies were inherited to utilities and are about to be practical. Now, Japan had been completed High Temperature Engineering Test Reactor (HTTR) a prototype and research reactor, a commercial High Temperature Gas-cooled Reactor (HTGR) design Gas Turbine High Temperature Reactor 300 (GTHTR300) with related reprocessing technologies, and is planning domestic demonstration reactor project. In this context, a representative fuel cycle policy is reprocessing in Japan. However, Japan has investigated various fuel cycle scenarios to expand the usage of the commercial HTGR. Then, we would like to introduce the scenarios and development status of related technologies in the present study.

JAEA Reports

Analysis of the radioactivity concentrations in radioactive waste generated from JRR-3, JRR-4 and JRTF facilities, 2

Tobita, Minoru*; Goto, Katsunori*; Omori, Takeshi*; Osone, Osamu*; Haraga, Tomoko; Aono, Ryuji; Konda, Miki; Tsuchida, Daiki; Mitsukai, Akina; Ishimori, Kenichiro

JAEA-Data/Code 2023-011, 32 Pages, 2023/11

JAEA-Data-Code-2023-011.pdf:0.93MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field as trench and pit. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to the study of radioactivity concentration evaluation methods for radioactive wastes generated from nuclear research facilities, we collected and analyzed concrete samples generated from JRR-3, JRR-4 and JAERI Reprocessing Test Facility. In this report, we summarized the radioactivity concentrations of 23 radionuclides ($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{137}$$Cs, $$^{133}$$Ba, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{235}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples in fiscal years 2021-2022.

Journal Articles

Molecular dynamics analysis of reactor graphite for preparing thermal neutron scattering law

Okita, Shoichiro; Goto, Minoru

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 10 Pages, 2023/10

JAEA Reports

Study on disposal of waste from reprocessing for commercial HTGR spent fuel

Fukaya, Yuji; Maruyama, Takahiro; Goto, Minoru; Ohashi, Hirofumi; Higuchi, Hideaki

JAEA-Research 2023-002, 19 Pages, 2023/06

JAEA-Research-2023-002.pdf:1.48MB

A study on disposal of waste derived from commercial High Temperature Gas-cooled Reactor ("HTGR") has been performed. Because of significant difference between the reprocessing of Light Water Reactor ("LWR") and that of HTGR due to difference in structures of the fuel, adoptability of the laws relating to reprocessing waste disposal, which is enacted for LWR, to HTGR waste should be confirmed. Then, we compared the technologies and waste of reprocessing and evaluated radioactivity concentration in graphite waste by activation and contamination based on whole core burn-up calculation. As a result, it was found that SiC residue waste should be disposed of into a geological repository as 2nd class designated radioactive waste in the Designated Radioactive Waste Final Disposal Act (Act No.117 of 2000), by way of amendment of the applicable order, same as hull and end-piece of LWR, and graphite waste should be shallowly disposed of than geological disposal as 2nd class waste for pit disposal in the Act on the Regulation of Nuclear Source Material, Nuclear Fuel Material and Reactors (Act No.166 of 1957) same as a channel box of LWR.

Journal Articles

Research on improvement of HTGR core power-density, 4; Feasibility study for a reactor core

Okita, Shoichiro; Mizuta, Naoki; Takamatsu, Kuniyoshi; Goto, Minoru; Yoshida, Katsumi*; Nishimura, Yosuke*; Okamoto, Koji*

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 10 Pages, 2023/05

Journal Articles

Feasibility study on reprocessing of HTGR spent fuel by existing PUREX plant and technology

Fukaya, Yuji; Goto, Minoru; Ohashi, Hirofumi

Annals of Nuclear Energy, 181, p.109534_1 - 109534_10, 2023/02

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Feasibility of reprocessing of High Temperature Gas-cooled Reactor (HTGR) spent fuel by existing Plutonium Uranium Redox EXtraction (PUREX) plant and technology has been investigated. The spent fuel dissolved solution includes approximately 3 times amount of uranium-235 and 1.5 times amount of protonium because of the 3 times higher burnup compared with that of Light Water Reactor (LWR). Then, the heavy metal of the spent fuel is planned to be diluted to 3.1 times by depleted uranium to satisfy the limitation of Rokkasho Reprocessing Plant (RRP) plant. In the present study, recoverability of uranium and plutonium with the dilution is confirmed by a simulation with a reprocessing process calculation code. Moreover, the case without the dilution from the economic perspective is investigated. As a result, the feasibility is confirmed without the dilution, and it is expected that the reprocessed amount is reduced to 1/3 compared with a diluted case even though the facility should be optimized from the perspective of mass flow and criticality.

Journal Articles

Study on evaluation method of kernel migration of TRISO fuel for High Temperature Gas-cooled Reactor

Fukaya, Yuji; Okita, Shoichiro; Sasaki, Koei; Ueta, Shohei; Goto, Minoru; Ohashi, Hirofumi; Yan, X.

Nuclear Engineering and Design, 399, p.112033_1 - 112033_9, 2022/12

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Kernel migration of TRi-structural ISOtropic (TRISO) fuel for High Temperature Gas-cooled Reactor (HTGR) has been analyzed to investigate the potential dominating effects. Kernel migration is a major fuel failure mode and dominant to determine the lifetime of the fuel for High Temperature engineering Test Reactor (HTTR). However, this study shows that the result and reliability depend on the evaluation method. The evaluation method used in this study takes into account of actual distribution of Coated Fuel Particles (CFPs) and the resulting heterogeneous fuel temperature calculation with such distribution. The result shows that the Kernel Migration Rate (KMR) is predicted to be about 10% less compared with the most conservative evaluation.

Journal Articles

Calculation of shutdown gamma distribution in the high temperature engineering test reactor

Ho, H. Q.; Ishii, Toshiaki; Nagasumi, Satoru; Ono, Masato; Shimazaki, Yosuke; Ishitsuka, Etsuo; Goto, Minoru; Simanullang, I. L.*; Fujimoto, Nozomu*; Iigaki, Kazuhiko

Nuclear Engineering and Design, 396, p.111913_1 - 111913_9, 2022/09

 Times Cited Count:1 Percentile:31.61(Nuclear Science & Technology)

Journal Articles

Re-evaluation of electricity generation cost of HTGR

Fukaya, Yuji; Ohashi, Hirofumi; Sato, Hiroyuki; Goto, Minoru; Kunitomi, Kazuhiko

Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 21(2), p.116 - 126, 2022/06

An improvement electricity generation cost evaluation method for High Temperature Gas-cooled Reactors (HTGRs) has been performed. Japan Atomic Energy Agency (JAEA) had completed the commercial HTGR concept named Gas Turbine High Temperature Reactor (GTHTR300) and the electricity generation cost evaluation method approximately a decade ago. The cost evaluation was developed based on the method of Federation of Electric Power Companies (FEPC). The FEPC method was drastically revised after the Fukushima Daiichi nuclear disaster. Moreover, the escalation of material and labor cost for the decade should be consider to evaluate the latest cost. Therefore, we revised the cost evaluation method for GTHTR300 and the cost was compared with that of Light Water Reactor (LWR). As a result, it was found that the electricity generation cost of HTGR of 7.9 yen/kWh is cheaper than that of LWR of 11.7 yen/kWh by approximately 30% at the capacity factor of 70%.

Journal Articles

Computed tomography neutron detector system to observe power distribution in a core with long neutron flight path

Fukaya, Yuji; Okita, Shoichiro; Nakagawa, Shigeaki; Goto, Minoru; Ohashi, Hirofumi

Annals of Nuclear Energy, 168, p.108911_1 - 108911_7, 2022/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A power distribution monitoring system by using a moving detector for a core with a long neutron flight path has been proposed. High Temperature Gas-cooled Reactor (HTGR) and Fast Reactor (FR) has a long neutron flight path and the neutrons reach to detector far from fuel assembly in the center of the core unlike Light Water Reactor (LWR). By using the feature, power distribution can be observed with a few detectors by moving the detector and computed tomography technology similar to X-ray Computed Tomography (CT). For a small-sized core, the power distribution can be evaluated only by an ex-core neutron detector. For a large-sized core with inner detectors, the power distribution can be observed with a small number of in-core detectors even if the deployment is limited due to material integrity conditions such as temperature environment. The feasibility is numerically confirmed by simulations of the HTGR core and its detector response. It is expected to observe the power distribution in the core of HTGR and FR, which is difficult continuously to deploy in-core detectors because of high temperature and/or high irradiation damage.

Journal Articles

Design of a portable backup shutdown system for the high temperature gas cooled reactor

Hamamoto, Shimpei; Ho, H. Q.; Iigaki, Kazuhiko; Goto, Minoru; Shimazaki, Yosuke; Sawahata, Hiroaki; Ishitsuka, Etsuo

Nuclear Engineering and Design, 386, p.111564_1 - 111564_8, 2022/01

 Times Cited Count:1 Percentile:31.61(Nuclear Science & Technology)

The experience of Fukushima Daiichi Nuclear Power Plant accident caused by the great earthquake that occurred in eastern Japan in 2011 showed the importance of preparing for the loss of function of the engineered safety features. Increasing the strength of equipment to prevent loss of function in an accident is effective, but the possibility of loss of function remains. Therefore, it is important to have an alternative to lost functions in order to put the accident under control early. Thus, this study designed an alternative shutdown system, namely a portable backup shutdown system (PBSS), to make countermeasures in the event of a loss of shutdown function more robust without impairing economic efficiency of the High Temperature Gas-cooled Reactor (HTGR). The PBSS is portable and capable of being installed manually so that it can operate in a total loss of off-site electricity. Various neutron absorber materials for the PBSS were also considered from the viewpoints of technical and cost-effective properties. As results of optimization, the boron nitride (BN) was selected as it shows a good neutronic property as well as a reasonable cost in comparison with other materials.

Journal Articles

Reduction of the source term of an assumed criticality accident in a fuel fabrication facility with solution system

Fukaya, Yuji; Goto, Minoru

Annals of Nuclear Energy, 164, p.108617_1 - 108617_6, 2021/12

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A reasonable source term of a hypothetical criticality accident for fuel fabrication facility with solution system has been proposed. The public exposure must not exceed the limitation of 5 mSv during an accident. Then, we proposed the reasonable source term of the first burst peak due to the hydrogen gas generation by radiation decomposition of water. With the criticality control system composed of the Criticality Accident Alarm System (CAAS) and soluble neutron absorber, safety is ensured by the reduced fission number. We confirmed the effect by environmental impact assessment during a criticality accident by using site condition of a fuel fabrication facility in Tokai-mura, Japan. As a result, the public exposure is reduced at a site boundary from 68 mSv to 0.6 mSv under the current regulatory guideline.

Journal Articles

Study on chemical form of tritium in coolant helium of high temperature gas-cooled reactor with tritium production device

Hamamoto, Shimpei; Ishitsuka, Etsuo; Nakagawa, Shigeaki; Goto, Minoru; Matsuura, Hideaki*; Katayama, Kazunari*; Otsuka, Teppei*; Tobita, Kenji*

Proceedings of 2021 International Congress on Advances in Nuclear Power Plants (ICAPP 2021) (USB Flash Drive), 5 Pages, 2021/10

Impurity concentrations of hydrogen and hydride in the coolant were investigated in detail for the HTTR, a block type high-temperature gas reactor owned by Japan. As a result, it was found that CH$$_{4}$$ was 1/10 of H$$_{2}$$ concentration, which was under the conventional detection limit. If the ratio of H$$_{2}$$ to CH$$_{4}$$ in the coolant is the same as the ratio of HT to CH$$_{3}$$T, the CH$$_{3}$$T has a larger dose conversion factor, and this compositional ratio is an important finding for the optimal dose evaluation. Further investigation of the origin of CH$$_{4}$$ suggested that CH$$_{4}$$ was produced as a result of a thermal equilibrium reaction rather than being released as an impurity from the core.

Journal Articles

Development of cesium trap material for coated fuel particles in high temperature gas-cooled reactors

Sasaki, Koei; Miura, Shuichiro*; Fukumoto, Kenichi*; Goto, Minoru; Ohashi, Hirofumi

Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 6 Pages, 2021/08

Cs-Bi and Cs-Sb absorbed graphite samples (Cs-Bi/graphite and Cs-Sb/graphite) were synthesized and their high temperature chemical stabilities were tested up to 1500$$^{circ}$$C by TG and analyzed by TEM-EDS for the development of Cs trap material in high temperature gas-cooled reactor (HTGR) fuel particles. It was observed that Cs was stabilized by Sb but not by Bi in the specimens after the TG test. A rapid weight loss from 800 to 1000$$^{circ}$$C may be caused by evaporation of Cs (boiling point: 671$$^{circ}$$C) was seen in the TG result of both specimens. Precipitated Cs-Sb substance in the graphite matrix were not resolved even after the 1500$$^{circ}$$C heating. The chemical composition of the Cs-Sb was specified as Cs$$_{3}$$Sb. The experimental results suggest that Sb have potential to be a Cs getter material in graphite matrix. Long term heating test should be performed to confirm adaptability of Sb for Cs trap material in HTGR fuel particles.

Journal Articles

Manufacturability estimation on burnable poison mixed fuel for improving criticality safety of HTGR fuel fabrication

Hasegawa, Toshinari; Fukaya, Yuji; Ueta, Shohei; Goto, Minoru

Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 5 Pages, 2021/08

Burnable poison (BP) credit concept has been proposed as a criticality safety measure for commercial high temperature gas-cooled reactor (HTGR) fuel fabrication, so we estimated manufacturability of the BP-mixed UO$$_2$$ kernel for the practical use of the concept. As a BP, boron, gadolinium, erbium, and hafnium are investigated. Boron mixed fuel kernels are fabricated by mixing boric acid powder with U$$_3$$O$$_8$$ powder. In the case of the other BPs, BP nitrate powder is mixed with U$$_3$$O$$_8$$ powder. In order to confirm that BP remain in the kernels after the heat treatment processes, thermodynamic equilibrium analysis was performed. Above 450$$^circ$$C, boron would melt and vaporize during the heat treatment processes, so it was found that the boron mixed fuel kernel fabrication is difficult. On the other hand, it was found that gadolinium, erbium, and hafnium would change to solid oxides that do not melt and vaporize even at 2000$$^circ$$C, and there was no problem with manufacturability of the BP-mixed fuel kernel.

Journal Articles

Preparation for restarting the high temperature engineering test reactor; Development of utility tool for auto seeking critical control rod position

Ho, H. Q.; Fujimoto, Nozomu*; Hamamoto, Shimpei; Nagasumi, Satoru; Goto, Minoru; Ishitsuka, Etsuo

Nuclear Engineering and Design, 377, p.111161_1 - 111161_9, 2021/06

 Times Cited Count:3 Percentile:45.99(Nuclear Science & Technology)

Journal Articles

Feasibility study on burnable poison credit concept to HTGR fuel fabrication from core specification perspective

Fukaya, Yuji; Ueta, Shohei; Goto, Minoru; Ohashi, Hirofumi

Annals of Nuclear Energy, 151, p.107937_1 - 107937_9, 2021/02

 Times Cited Count:2 Percentile:31.78(Nuclear Science & Technology)

Feasibility study on Burnable Poison (BP) credit concept to High Temperature Gas-cooled Reactor (HTGR) fuel fabrication has been performed. By mixing BP into fuel material in the first place of fuel fabrication, criticality safety is ensured in the all fuel fabrication process even with high enrichment fuel such as 14 wt% used in commercial HTGR. However, the poison effect also prevents the criticality even in the HTGR core, and it may shorten cycle length and achievable burn-up of the core. Therefore, the effect is evaluated by whole core burn-up calculation. As a BP, boron, gadolinium, erbium, and hafnium are investigated. As a result, it is found that boron and gadolinium suit this concept and the 14 wt% fuel can be fabricated in the plant fabricating 9.9 wt% High Temperature engineering Test Reactor (HTTR) fuel. With the boron and gadolinium, the commercial HTGR fuel can be fabricated with the safety measure as same as Light Water Reactor (LWR) fuel facility to treat the fuel with the enrichment up to 5 wt%. Especially, gadolinium is significantly suitable to this concept due to the dependency to spectrum, and more enhanced safety measure is feasible as well.

Journal Articles

Reactor physics experiment in a graphite-moderation system for HTGR

Fukaya, Yuji; Goto, Minoru; Nakagawa, Shigeaki; Nakajima, Kunihiro*; Takahashi, Kazuki*; Sakon, Atsushi*; Sano, Tadafumi*; Hashimoto, Kengo*

EPJ Web of Conferences, 247, p.09017_1 - 09017_8, 2021/02

The Japan Atomic Energy Agency (JAEA) started the Research and Development (R&D) to improve nuclear prediction techniques for High Temperature Gas-cooled Reactors (HTGRs). The objectives are to introduce a generalized bias factor method to avoid full mock-up experiment for the first commercial HTGR and to introduce reactor noise analysis to High Temperature Engineering Test Reactor (HTTR) experiment to observe subcriticality. To achieve the objectives, the reactor core of graphite-moderation system named B7/4"G2/8"p8EUNU+3/8"p38EU(1) was newly composed in the B-rack of Kyoto University Critical Assembly (KUCA). The core is composed of the fuel assembly, driver fuel assembly, graphite reflector, and polyethylene reflector. The fuel assembly is composed of enriched uranium plate, natural uranium plate and graphite plates to realize the average fuel enrichment of HTTR and it's spectrum. However, driver fuel assembly is necessary to achieve the criticality with the small-sized core. The core plays a role of the reference core of the bias factor method, and the reactor noise was measured to develop the noise analysis scheme. In this study, the overview of the criticality experiments is reported. The reactor configuration with graphite moderation system is rare case in the KUCA experiments, and this experiment is expected to contribute not only for an HTGR development but also for other types of a reactor in the graphite moderation system such as a molten salt reactor development.

Journal Articles

High temperature gas-cooled reactors

Takeda, Tetsuaki*; Inagaki, Yoshiyuki; Aihara, Jun; Aoki, Takeshi; Fujiwara, Yusuke; Fukaya, Yuji; Goto, Minoru; Ho, H. Q.; Iigaki, Kazuhiko; Imai, Yoshiyuki; et al.

High Temperature Gas-Cooled Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.5, 464 Pages, 2021/02

As a general overview of the research and development of a High Temperature Gas-cooled Reactor (HTGR) in JAEA, this book describes the achievements by the High Temperature Engineering Test Reactor (HTTR) on the designs, key component technologies such as fuel, reactor internals, high temperature components, etc., and operational experience such as rise-to-power tests, high temperature operation at 950$$^{circ}$$C, safety demonstration tests, etc. In addition, based on the knowledge of the HTTR, the development of designs and component technologies such as high performance fuel, helium gas turbine and hydrogen production by IS process for commercial HTGRs are described. These results are very useful for the future development of HTGRs. This book is published as one of a series of technical books on fossil fuel and nuclear energy systems by the Power Energy Systems Division of the Japan Society of Mechanical Engineers.

Journal Articles

Influences of the ZrC coating process and heat treatment on ZrC-coated kernels used as fuel in Pu-burner high temperature gas-cooled reactor in Japan

Aihara, Jun; Ueta, Shohei; Honda, Masaki*; Mizuta, Naoki; Goto, Minoru; Tachibana, Yukio; Okamoto, Koji*

Journal of Nuclear Science and Technology, 58(1), p.107 - 116, 2021/01

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The concept of a Pu-burner high temperature gas-cooled reactor (HTGR) has been proposed for purpose of more safely reducing amount of recovered Pu. This concept employs coated fuel particles (CFPs) with ZrC coated PuO$$_{2}$$-YSZ kernel and with tristructural (TRISO) coating for very high Pu burn-up and high nuclear proliferation resistance. In this report, we investigate the microstructure of the region that includes the surface of an as-fabricated CeO$$_{2}$$-YSZ kernel simulating PuO$$_{2}$$-YSZ kernel. We found both Zr-rich grains and Ce-rich grains to be densely distributed in that region including surface of CeO$$_{2}$$-YSZ kernel. On the other hand, it has been reported that there was a porous region near surface of the CeO$$_{2}$$-YSZ kernel of Batch I. This finding confirms that Ce-rich grains near surface of CeO$$_{2}$$-YSZ kernels coated with ZrC layers have been corroded during the deposition of the ZrC layer, whereas the Zr-rich grains were hardly affected.

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