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Journal Articles

Secondary consolidation characteristic of bentonite by long-term consolidation tests of 2.7, 3.7 and 4 years

Takayama, Yusuke; Yamamoto, Yoichi*; Goto, Takahiro*

Jiban Kogaku Janaru (Internet), 18(3), p.317 - 330, 2023/09

It has been reported that the deformation greatly increased in the secondary consolidation process in the past long-term consolidation test of 1.8 years on Na-type bentonite/sand mixed soil. Therefore, we analyzed potential contributing factors in this behavior. A long-term consolidation test for about 10 years on bentonite and kaolinite was started using the test equipment with countermeasures against these factors. In this paper, the secondary consolidation behavior of bentonite was investigated based on the long-term consolidation test data for 2.7, 3.7 and 4 years. The results were generally consistent with the conventional findings on soil mechanics that the deformation due to secondary consolidation progresses linearly with respect to logarithm of time. This test will be continued for about 10 years and longer-term secondary consolidation behavior will be investigated.

Journal Articles

Methodology development and determination of solubility-limiting solid phases for a performance assessment of geological disposal of high-level radioactive and TRU wastes

Kitamura, Akira; Yoshida, Yasushi*; Goto, Takahiro*; Shibutani, Sanae*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 27(2), p.58 - 71, 2020/12

Evaluation and estimation of solubility values are required for a performance assessment of geological disposal of high-level radioactive and TRU wastes. Selection of solubility-limiting solid phases (SSPs) that control the solubility of radionuclides is necessary for the evaluation and estimation of solubility values. The authors have developed a methodology for selection of the SSP through a calculation of saturation indices (SIs) using thermodynamic database to show a transparent procedure for the selection. Literature survey should be performed to confirm decision of the SSP from candidate SSPs which generally have larger SIs from realistic point of view for precipitation and solubility control. The authors have selected the SSPs for the elements of interest for the latest Japanese performance assessment in bentonite and cement porewaters after grouping various water compositions.

Journal Articles

Development of performance assessment models for glass dissolution

Goto, Takahiro*; Mitsui, Seiichiro; Takase, Hiroyasu*; Kurosawa, Susumu*; Inagaki, Manabu*; Shibata, Masahiro; Ishiguro, Katsuhiko*

MRS Advances (Internet), 1(63-64), p.4239 - 4245, 2016/00

NUMO and JAEA have conducted a joint research since FY2011, which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage for deep geological disposal of radioactive waste. As a part of this joint research, we have been developing glass dissolution models which consider various processes in EBS, such as precipitation of Fe-silicates associated with iron overpack corrosion, and Si transport through corrosion products in the cracked overpack. The objectives of the modeling work are to evaluate relative importance of relevant processes and to identify further R&D issues towards development of a convincing safety case. Sensitivity analyses suggested that predicted glass dissolution time ranges from 1$$times$$10$$^3$$ to 1$$times$$10$$^7$$ years or more due to uncertainties in the current understanding of the key processes, namely precipitation of Fe-silicates and transport characteristics of the altered glass layer.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 3; Progress report on NUMO-JAEA collaborative research in FY2013 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Kitamura, Akira; Yoshikawa, Hideki; Oda, Chie; Ishidera, Takamitsu; et al.

JAEA-Research 2014-030, 457 Pages, 2015/03

JAEA-Research-2014-030.pdf:199.23MB

JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and post-closure performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, based on some examples of developing method of hydro-geological structure model, acquired knowledge are arranged using the tree diagram, and model uncertainty and its influence on the evaluation items were discussed. With regard to (2) study on scenario development, the developed approach for "defining conditions" has been reevaluated and improved from practical viewpoints. In addition, the uncertainty evaluation for the effect of use of cementitious material, as well as glass dissolution model, was conducted with analytical evaluation. With regard to (3) study on setting radionuclide migration parameters, based on survey of precedent procedures, multiple-approach for distribution coefficient of rocks was established, and the adequacy of the approach was confirmed though its application to sedimentary rock and granitic rock. Besides, an approach for solubility setting was developed including the procedure of selection of solubility limiting solid phase. The adequacy of the approach was confirmed though its application to key radionuclides.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 2; Progress report on NUMO-JAEA collaborative research in FY2012 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Hayano, Akira; Makino, Hitoshi; Wakasugi, Keiichiro; Mitsui, Seiichiro; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.

JAEA-Research 2013-037, 455 Pages, 2013/12

JAEA-Research-2013-037.pdf:42.0MB

Following FY2011, JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation stage. With regard to (1) study on rock suitability in terms of hydrology, the tree diagram of methodology of groundwater travel time has been extended for crystalline rock, in addition, tree diagram for sedimentary rock newly has been organized. With regard to (2) study on scenario development, the existing approach has been improved in terms of a practical task, and applied and tested for near field focusing on the buffer. In addition, the uncertainty of some important processes and its impact on safety functions are discussed though analysis. With regard to (3) study on setting radionuclide migration parameters, the approaches for parameter setting have been developed for sorption for rocks and solubility, and applied and tested through parameter setting exercises for key radionuclides.

JAEA Reports

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage; Progress report on NUMO-JAEA collaborative research in FY2011 (Joint research)

Shibata, Masahiro; Sawada, Atsushi; Tachi, Yukio; Makino, Hitoshi; Hayano, Akira; Mitsui, Seiichiro; Taniguchi, Naoki; Oda, Chie; Kitamura, Akira; Osawa, Hideaki; et al.

JAEA-Research 2012-032, 298 Pages, 2012/09

JAEA-Research-2012-032.pdf:33.68MB

JAEA and NUMO have conducted a collaborative research work which is designed to enhance the methodology of repository design and performance assessment in preliminary investigation phase. The topics and the conducted research are follows; (1) Study on selection of host rock: in terms of hydraulic properties, items for assessing rock property, and assessment methodology of groundwater travel time has been organized with interaction from site investigation. (2) Study on development of scenario: the existing approach has been embodied, in addition, the phenomenological understanding regarding dissolution of and nuclide release from vitrified waste, corrosion of the overpack, long-term performance of the buffer are summarized. (3) Study on setting nuclide migration parameters: the approach for parameter setting has been improved for sorption and diffusion coefficient of buffer/rock, and applied and tested for parameter setting of key radionuclides. (4) Study on ensuring quality of knowledge: framework for ensuring quality of knowledge has been studied and examined aimed at the likely disposal facility condition.

Oral presentation

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 3; Study on scenario development methodology

Shibata, Masahiro; Makino, Hitoshi; Wakasugi, Keiichiro; Ebashi, Takeshi; Kurosawa, Susumu*; Goto, Takahiro*; Inagaki, Manabu*

no journal, , 

no abstracts in English

Oral presentation

Enhancement of the methodology of repository design and post-closure performance assessment for preliminary investigation stage, 4; Parameter setting for radionuclide migration

Tachi, Yukio; Suyama, Tadahiro; Kitamura, Akira; Shibata, Masahiro; Shibutani, Sanae*; Goto, Takahiro*; Inagaki, Manabu*

no journal, , 

As part of the NUMO-JAEA collaborative research program, the methodology of parameter setting for performance assessment in preliminary investigation stage was developed and tested through the parameter setting exercises for key radionuclides sorption on rocks.

Oral presentation

Preparation of an information basis for development of practical performance assessment models on waste glass corrosion in geological disposal

Mitsui, Seiichiro; Oe, Toshiaki*; Inagaki, Yaohiro*; Okubo, Takahiro*; Kurosawa, Susumu*; Goto, Takahiro*; Inagaki, Manabu*; Ishiguro, Katsuhiko*; Takase, Hiroyasu*; Takahashi, Hirokazu*

no journal, , 

In order to develop robust performance assessment models, we have been preparing an information basis regarding glass properties and glass dissolution/alteration processes under disposal conditions as a part of NUMO-JAEA joint project. Our iterative working process for the preparation of the information basis comprises five steps: (1) integration of current knowledge; (2) development of glass dissolution scenarios based on current knowledge; (3) development of conceptual model; (4) sensitivity analyses to evaluate relative importance of relevant processes and associated uncertainties; and (5) identification of future R&D issues towards further improvement of the information basis. The current status will be presented in this talk.

Oral presentation

Effect of interaction between carbon steel and simulated glass on glass dissolution behavior

Goto, Takahiro*; Matsubara, Ryuta*; Hamamoto, Takafumi*; Fujisaki, Kiyoshi*; Mitsui, Seiichiro; Taniguchi, Naoki

no journal, , 

For the purpose of improvement of long-term glass corrosion model, we conducted immersion tests with specimens of carbon steel and simulated waste glass at 50$$^{circ}$$C and 80$$^{circ}$$C under nitrogen gas atmosphere. We also conducted control immersion tests with a specimen of carbon steel or simulated waste glass under the same conditions. After the immersion tests, we determined glass corrosion rates and secondary phases on the surface of carbon steel specimen. Glass corrosion rates for the immersion tests with specimens of carbon steel and simulated waste glass were three times larger than those for the control immersion tests with simulated waste glass specimen. With X-ray diffraction, several peaks associated with an iron silicate mineral were identified. This observation is consistent with the results of geochemical calculation based on solution data and published study using carbon steel and simulated waste glass.

Oral presentation

Study on long term consolidation behavior of buffer materials, 1; Factor of secondary consolidation acceleration behavior

Yamamoto, Yoichi*; Goto, Takahiro*; Takayama, Yusuke; Kikuchi, Hirohito*; Miyakawa, Ryoma*

no journal, , 

no abstracts in English

Oral presentation

Study on long term consolidation behavior of buffer materials, 2; Preliminary long term consolidation test and numerical study on the dissipation delay of the excess pore water pressure

Takayama, Yusuke; Kikuchi, Hirohito*; Miyakawa, Ryoma*; Yamamoto, Yoichi*; Goto, Takahiro*

no journal, , 

In this research, in order to confirm the acceleration behavior of the secondary consolidation, a comparatively long consolidation test (about 1 year) was carried out. And in order to investigate the dissipation delay of the excess pore water pressure in consolidation test, a reproduction analysis was carried out in consideration of the density dependency of the coefficient of permeability.

Oral presentation

Corrosion behavior of simulated high-level waste glass in the presence of carbon steel

Goto, Takahiro*; Matsubara, Ryuta*; Hamamoto, Takafumi*; Fujisaki, Kiyoshi*; Mitsui, Seiichiro; Taniguchi, Naoki

no journal, , 

To improve long-term glass corrosion model, immersion tests with specimens of carbon steel and simulated waste glass were conducted at 50$$^{circ}$$C and 80$$^{circ}$$C under nitrogen gas atmosphere for 131 days. Control tests with a specimen of carbon steel or glass under the same conditions were also conducted. After the tests, the element concentration in the solution was analyzed to determine glass corrosion rates. We also analyzed the surface of specimens with XRD and TEM/ED (electron diffraction)/EDX to identify secondary phases. Glass corrosion rates for the tests with specimens of carbon steel and glass were two times larger than those for the control tests with glass specimen. With XRD and TEM/ED/EDX, we determined iron silicates on the surface of both carbon steel and glass. These observations are consistent with the results of geochemical calculation and published studies. The results indicate that glass corrosion could be enhanced by the precipitation of iron silicates.

Oral presentation

Study on long term consolidation behavior of buffer materials, 3; Comparison of basic properties of Kunigel V1 and Kaolinite

Takayama, Yusuke; Kikuchi, Hirohito*; Yamamoto, Yoichi*; Goto, Takahiro*

no journal, , 

In this report, permeability, swelling characteristics, and consolidation characteristics of kaolinite were examined and these characteristics of kaolinite were are compared with kunigel V1.

Oral presentation

Study on the long-term consolidation behavior of bentonite

Goto, Takahiro*; Yamamoto, Yoichi*; Takayama, Yusuke

no journal, , 

no abstracts in English

Oral presentation

Fe-silicate and -carbonate formations at C-steel- compacted bentonite interface hinders buffer degradation in high-level radioactive waste disposal

Kikuchi, Ryosuke*; Fujimura, Tatsuya*; Sato, Tsutomu*; Otake, Tsubasa*; Otomo, Yoko*; Goto, Takahiro*; Suzuki, Satoru*; Taniguchi, Naoki; Suzuki, Hiroyuki*

no journal, , 

16 (Records 1-16 displayed on this page)
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