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Journal Articles

Measurement of double-differential neutron yields for iron, lead, and bismuth induced by 107-MeV protons for research and development of accelerator-driven systems

Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.

EPJ Web of Conferences, 284, p.01023_1 - 01023_4, 2023/05

 Times Cited Count:0 Percentile:0.21(Nuclear Science & Technology)

For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron, lead, and bismuth have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics. The measured TTNYs and DDXs were compared with calculations by the Monte Carlo transport code PHITS with its default physics model of INCL version 4.6 combined with GEM and those with the JENDL-4.0/HE nuclear data library.

Journal Articles

Measurement of 107-MeV proton-induced double-differential thick target neutron yields for Fe, Pb, and Bi using a fixed-field alternating gradient accelerator at Kyoto University

Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.

Journal of Nuclear Science and Technology, 60(4), p.435 - 449, 2023/04

 Times Cited Count:3 Percentile:68.71(Nuclear Science & Technology)

Double-differential thick target neutron yields (TTNYs) for Fe, Pb, and Bi targets induced by 107-MeV protons were measured using the fixed-field alternating gradient accelerator at Kyoto University for research and development of accelerator-driven systems (ADSs) and fundamental ADS reactor physics research at the Kyoto University Critical Assembly (KUCA). Note that TTNYs were obtained with the time-of-flight method using a neutron detector system comprising eight neutron detectors; each detector has a small NE213 liquid organic scintillator and photomultiplier tube. The TTNYs obtained were compared with calculation results using Monte Carlo-based spallation models (i.e., INCL4.6/GEM, Bertini/GEM, JQMD/GEM, and JQMD/SMM/GEM) and the evaluated high-energy nuclear data library, i.e., JENDL-4.0/HE, implemented in the particle and heavy iontransport code system (PHITS). All models, including JENDL-4.0/HE, failed to predict high-energy peaks at a detector angle of 5$$^{circ}$$. Comparing the energy- and angle-integrated spallation neutron yields at energies of $$le$$20 MeV estimated using the measured TTNYs and the PHITS indicated that INCL4.6/GEM would be suitable for the Monte Carlo transport simulation of ADS reactor physics experiments at the KUCA.

Journal Articles

Measurement of 107-MeV proton-induced double-differential neutron yields for iron for research and development of accelerator-driven systems

Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; Nishio, Katsuhisa; et al.

JAEA-Conf 2022-001, p.129 - 133, 2022/11

For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors composed of the NE213 liquid organic scintillators and photomultiplier tubes, which were connected to a multi-channel digitizer mounted with a field-programmable gate array (FPGA), for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination applying the gate integration method to the FPGA. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics.

Journal Articles

High density mapping systems for SRF cavities

Fuwa, Yasuhiro; Iwashita, Yoshihisa*; Kuriyama, Yasutoshi*; Tongu, Hiromu*; Hayano, Hitoshi*; Geng, R. L.*

Proceedings of 20th International Conference on RF Superconductivity (SRF 2021) (Internet), p.323 - 325, 2022/05

In order to evaluate the performance of a superconducting cavity, we are developing a mapping system to measure the distribution of cavity temperature, field emission X-rays, and trapped magnetic flux with high positional resolution. In order to construct a system with high positional resolution, a large number of sensors are required. However, as the number of sensors increases, so does the amount of wiring, which increases the complexity of the wiring in the cryogenic apparatus, and also increases the heat transfer through the wiring, which disturb efficient operation of cavity tests. We are developing an efficient mapping system with a multiplexer that scans the readout signal on the same circuit as the sensor in the cryogenic dewar where the cavity test is conducted. In this presentation, we report the outline and test results of the mapping system under development

Journal Articles

Improvement of inner surface inspection system for superconducting cavities applying image processing technique

Kuriyama, Yasutoshi*; Iwashita, Yoshihisa*; Hirota, Katsuya*; Hayano, Hitoshi*; Fuwa, Yasuhiro

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.32 - 35, 2019/10

Research and development of gradient enhancement of superconducting RF accelerating cavity is carried out by accelerator research institute in the world, but defects on the cavity surface limit accelerating electric field. Therefore, development of "Inside inspection system for superconducting accelerated cavity" that optically visualizes the state of the inner surface of the superconducting cavity has been carried out, and results have been achieved. In this research, we apply image processing technology that has developed remarkably in recent years to the internal inspection system, and advanced the defect recognition method. Extraction of depth information and image synthesis were performed from images obtained with different focal positions with the camera for internal surface inspection. Also, by performing pattern recognition processing on the images, automatic detection of defects has become possible. By integrating these techniques into the cavity inner surface inspection system, it becomes possible to shorten the scan time for defect search and acquire the defect shape.

Journal Articles

First nuclear transmutation of $$^{237}$$Np and $$^{241}$$Am by accelerator-driven system at Kyoto University Critical Assembly

Pyeon, C. H.*; Yamanaka, Masao*; Oizumi, Akito; Fukushima, Masahiro; Chiba, Go*; Watanabe, Kenichi*; Endo, Tomohiro*; Van Rooijen, W. G.*; Hashimoto, Kengo*; Sakon, Atsushi*; et al.

Journal of Nuclear Science and Technology, 56(8), p.684 - 689, 2019/08

 Times Cited Count:12 Percentile:80.27(Nuclear Science & Technology)

This study demonstrates, for the first time, the principle of nuclear transmutation of minor actinide (MA) by the accelerator-driven system (ADS) through the injection of high-energy neutrons into the subcritical core at the Kyoto University Critical Assembly. The main objective of the experiments is to confirm fission reactions of neptunium-237 ($$^{237}$$Np) and americium-241 ($$^{241}$$Am), and capture reactions of $$^{237}$$Np. Subcritical irradiation of $$^{237}$$Np and $$^{241}$$Am foils is conducted in a hard spectrum core with the use of the back-to-back fission chamber that obtains simultaneously two signals from specially installed test ($$^{237}$$Np or $$^{241}$$Am) and reference (uranium-235) foils. The first nuclear transmutation of $$^{237}$$Np and $$^{241}$$Am by ADS soundly implemented by combining the subcritical core and the 100 MeV proton accelerator, and the use of a lead-bismuth target, is conclusively demonstrated through the experimental results of fission and capture reaction events.

Journal Articles

Radiation damage calculation in PHITS and benchmarking experiment for cryogenic-sample high-energy proton irradiation

Iwamoto, Yosuke; Matsuda, Hiroki; Meigo, Shinichiro; Satoh, Daiki; Nakamoto, Tatsushi*; Yoshida, Makoto*; Ishi, Yoshihiro*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Yashima, Hiroshi*; et al.

Proceedings of 61st ICFA Advanced Beam Dynamics Workshop on High-Intensity and High-Brightness Hadron Beams (HB 2018) (Internet), p.116 - 121, 2018/07

The radiation damage model in the radiation transport code PHITS has been developed to calculate the basic data of the radiation damage including the energy of the target Primary Knock on Atom (PKA). For the high-energy proton incident reactions, a target PKA created by the secondary particles was more dominant than a target PKA created by the projectile. To validate the radiation damage model in metals irradiated by $$>$$100 MeV protons, we developed a proton irradiation device with a Gifford-McMahon cryocooler to cryogenically cool wire samples. By using this device, the defect-induced electrical resistivity changes related to the DPA cross section of copper and aluminum were measured under irradiation with 125 and 200 MeV protons at cryogenic temperature. A comparison of the experimental data with the calculated results indicates that the DPA cross section with defect production efficiencies provide better quantitative descriptions.

Journal Articles

Measurement of the displacement cross-section of copper irradiated with 125 MeV protons at 12 K

Iwamoto, Yosuke; Yoshiie, Toshimasa*; Yoshida, Makoto*; Nakamoto, Tatsushi*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Xu, Q.*; Yashima, Hiroshi*; et al.

Journal of Nuclear Materials, 458, p.369 - 375, 2015/03

 Times Cited Count:13 Percentile:73.22(Materials Science, Multidisciplinary)

To validate Monte Carlo codes for the prediction of radiation damage in metals irradiated by $$>$$100 MeV protons, defect-induced electrical resistivity changes of copper related to the displacement cross-section were measured with 125 MeV proton irradiation at 12 K. The cryogenic irradiation system was developed with a Gifford-McMahon cryocooler to cool the sample via an oxygen-free high-conductivity copper plate by conduction cooling. The sample was a copper wire with a 250$$mu$$m diameter and 99.999% purity sandwiched between two aluminum nitride ceramic sheets. The resistivity increase did not change during annealing after irradiation below 15 K. The experimental displacement cross-section for 125 MeV irradiation shows similar results to the experimental data for 1.1 and 1.94 GeV. Comparison with the calculated results indicated that the defect production efficiency in Monte Carlo codes gives a good quantitative description of the displacement cross-section in the energy region $$>$$ 100 MeV.

Oral presentation

Study of measurement of displacement cross section for copper irradiated with 125 MeV proton

Iwamoto, Yosuke; Yoshida, Makoto*; Nakamoto, Tatsushi*; Ogitsu, Toru*; Yoshiie, Toshimasa*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Mori, Yoshiharu*

no journal, , 

We measured the electrical resistivity under irradiation of 125 MeV proton in copper sample (0.2 um thickness) at cryogenic temperature at the FFAG accelerator facility in Kyoto university. Resistivity was measured by the four-terminal method. As a result, we measured the resistivity of copper at 7.3 K within 20 micro-ohm and temperature of sample. We measured the electrical resistivity under irradiation of 125 MeV proton in copper sample (0.2 um thickness) at cryogenic temperature at the FFAG accelerator facility in Kyoto university. Resistivity was measured by the four-terminal method. As a result, we measured the resistivity of copper at 7.3 K within 20 micro-ohm and temperature of sample.

Oral presentation

Development of the device for electrical resistivity measurements for proton irradiation under cryogenic condition

Iwamoto, Yosuke; Yoshiie, Toshimasa*; Yoshida, Makoto*; Nakamoto, Tatsushi*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Xu, Q.*; Yashima, Hiroshi*; et al.

no journal, , 

To validate the radiation damage calculation in the PHITS code for proton irradiation over 100 MeV, we have developed the device for electrical resistance measurement under cryogenic condition. A copper wire with 99.999% purity in a diameter of 250-$$mu$$m was set with a serpentine-shaped line on the AlN sheet which has high thermal conductivity and electric insulation. The sample was annealed for 1 h at 1,000$$^{circ}$$C before irradiation. After annealing, the sample was cooled with an oxygen-free high-conductivity copper plate by conduction cooling. The electrical resistivity changes in the sample were measured using the four-probe technique. As a result, the residual resistivity ratio of the sample was about 1,800 between room temperature and 11 K. After 125 MeV proton irradiation with 1.45$$times$$10$$^{14}$$(proton/cm$$^{2}$$) at 11 K, the total resistance increase was 1.53$$mu$$ $$Omega$$, while the resistivity of copper before irradiation was 29.41$$mu$$ $$Omega$$.

Oral presentation

Measurement of the damage rate of copper irradiated with 125 MeV protons at 12 K and comparison with calculated result with the PHITS code

Iwamoto, Yosuke; Yoshiie, Toshimasa*; Yoshida, Makoto*; Nakamoto, Tatsushi*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Xu, Q.*; Yashima, Hiroshi*; et al.

no journal, , 

To validate Monte Carlo code PHITS for the prediction of radiation damage in metals, the damage rate (defect-induced electrical resistivity changes / particle fluence) related to the displacement cross-section of copper were measured with 125 MeV proton irradiation under 12 K at the FFAG facility in the Kyoto University Research Reactor Institute. The sample was a copper wire with a 250-$$mu$$m diameter and 99.999% purity and was cooled by conduction cooling. After 125 MeV proton irradiation with 1.45$$times$$10$$^{18}$$ protons/m$$^{2}$$ at 12 K, the total resistivity increase was 4.94$$times$$10$$^{-13}$$$$Omega$$m (resistance increase: 1.53$$mu$$$$Omega$$), while the resistivity of copper before irradiation was 9.49 $$times$$10$$^{-12}$$$$Omega$$m (resistance: 29.41$$mu$$$$Omega$$). Comparison with other experimental results indicated that the damage rate by 125 MeV protons is almost same with those by 1.1 GeV protons and is higher than the damage rate by 14 MeV neutrons by a factor of 1.4. For the comparison with the PHITS results, the experimental data is smaller than the calculated result without the defect production efficiency by a factor of about 2.5 and that with the defect production efficiency by a factor of about 1.4, respectively. It indicates that the defect production efficiency in PHITS gives a good quantitative description of the displacement cross-section.

Oral presentation

Reduction and resource recycling of high-level radioactive wastes through nuclear transmutation; Status of the proof-of-principle experiment on MERIT scheme

Okabe, Kota; Yoshimoto, Masahiro; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Kinsho, Michikazu; Taniguchi, Akihiro*; Sato, Akira*; Miyake, Yasuhiro*; Mori, Yoshiharu*

no journal, , 

no abstracts in English

Oral presentation

Experimental study on nuclear data for accelerator-driven systems using FFAG accelerator; Research outline and measurement of neutron energy spectrum for iron target

Iwamoto, Hiroki; Meigo, Shinichiro; Nishio, Katsuhisa; Ishi, Yoshihiro*; Hirose, Kentaro; Iwamoto, Yosuke; Kuriyama, Yasutoshi*; Maekawa, Fujio; Makii, Hiroyuki; Nakano, Keita; et al.

no journal, , 

no abstracts in English

Oral presentation

Measurement of neutron energy spectra from Fe target using FFAG proton accelerator

Nakano, Keita; Iwamoto, Hiroki; Meigo, Shinichiro; Nishio, Katsuhisa; Ishi, Yoshihiro*; Hirose, Kentaro; Iwamoto, Yosuke; Kuriyama, Yasutoshi*; Maekawa, Fujio; Makii, Hiroyuki; et al.

no journal, , 

For accurate prediction of neutronic characteristics for accelerator-driven system (ADS), an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University has been launched. As a part of this program, energy spectra of spallation neutron from 100-MeV proton-induced reactions on Fe, Pb, and Bi are plan to be measured. In this report, the results of the measurement on Fe target will be presented.

Oral presentation

Measurement of neutron energy spectra from Pb and Bi targets using FFAG proton accelerator

Nakano, Keita; Iwamoto, Hiroki; Meigo, Shinichiro; Nishio, Katsuhisa; Ishi, Yoshihiro*; Hirose, Kentaro; Iwamoto, Yosuke; Kuriyama, Yasutoshi*; Maekawa, Fujio; Makii, Hiroyuki; et al.

no journal, , 

Toward the realization of Accelerator-Driven System (ADS), we have been measuring the nuclear data for ADS using Kyoto University FFAG accelerator. In this presentation, we report the outline and the results of the energy spectrum measurement of neutrons produced by 107 MeV proton-induced reactions on lead and bismuth, which are the most important nuclides in ADS.

Oral presentation

Measurement and analysis of 107-MeV proton-induced neutron yields for iron, lead and bismuth

Iwamoto, Hiroki; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta; Nakano, Keita; Nishio, Katsuhisa; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; et al.

no journal, , 

For the purpose of research and development of accelerator-driven nuclear transmutation systems, neutron yields of 107-MeV proton incident on iron, lead and bismuth targets were measured by the flight time method using the FFAG accelerator at Kyoto University. The energy spectra of the neutron yield obtained by the measurements were compared with results of particle transport analysis with the nuclear reaction models (INCL4.6/GEM, Bertini/GEM, JQMD/GEM and JQMD/SMM/GEM) incorporated in the Monte Carlo particle transport calculation code PHITS and the nuclear data library JENDL-4.0/HE. As a result, it was found that the INCL4.6/GEM, which was the reference model of PHITS, best reproduced the experimental values.

Oral presentation

Analysis of neutron-production double-differential cross sections in nuclear data measurements using the Kyoto University FFAG accelerator and measurement of a spallation neutron field using a $$^{237}$$Np fission chamber

Iwamoto, Hiroki; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Sugihara, Kenta*; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; Nishio, Katsuhisa; et al.

no journal, , 

no abstracts in English

Oral presentation

An Experimental program of nuclear data for development of accelerator-driven systems

Iwamoto, Hiroki; Meigo, Shinichiro; Nishio, Katsuhisa; Ishi, Yoshihiro*; Hirose, Kentaro; Iwamoto, Yosuke; Kuriyama, Yasutoshi*; Makii, Hiroyuki; Maekawa, Fujio; Mori, Yoshiharu*; et al.

no journal, , 

An experimental program for the research and development of Accelerator-Driven System (ADS) was carried out from FY2019 to FY2022. In this program, nuclear data on 100 MeV proton-induced spallation reactions on ADS target materials were experimentally obtained using the FFAG accelerator at Institute for Integrated Radiation and Nuclear Science, Kyoto University. Specifically, the proton-induced double-differential thick target neutron yield (TTNY) for $$^{rm nat}$$Fe, $$^{rm nat}$$Pb, and $$^{rm 209}$$Bi, neutron-production double-differential cross sections (DDX) for $$^{rm nat}$$Pb and $$^{209}$$Bi, fission rate of $$^{237}$$Np by spallation neutrons, $$^{208}$$Pb(p,f) reaction and $$^{209}$$Bi(p,f) reactions, the mass number distribution of fission fragments produced in the $$^{208}$$Pb(p,f) and $$^{209}$$Bi(p,f) reactions, and the fission neutrons. As a result of comparing the measured data with the analytical values obtained by various nuclear reaction models, issues to be addressed toward the advancement of nuclear reaction models for proton-induced spallation reactions in the 100 MeV region were clarified.

Oral presentation

Neutron mirror with magnetic repulsive wall

Fuwa, Yasuhiro; Kuriyama, Yasutoshi*; Iwashita, Yoshihisa*; Hirota, Katsuya*; Yamada, Masako*; Kitaguchi, Masaaki*; Shimizu, Hirohiko*

no journal, , 

A neutron mirror with a magnetic repulsive wall is under development. Since neutrons have a magnetic dipole moment, they are subject to forces in a magnetic field gradient. Using this phenomenon, a potential wall for neutrons can be formed by arranging permanent magnets in a planar configuration of a Halbach array. This potential wall acts as a mirror for a polarized neutron beam. A prototype mirror 20 mm high and 30 mm wide was fabricated, and preliminary neutron reflection experiments were conducted at the MINE2 port of JRR-3. As the next step, we plan to fabricate a mirror with a larger size and conduct experiments at the J-PARC MLF. In this presentation, the principle of the mirror, the results of preliminary experiments at JRR-3, and the status of the mirror fabrication for the experiment at J-PARC will be reported.

Oral presentation

Neutron beam manipulation utilizing spin magnetic dipole moment

Fuwa, Yasuhiro; Iwashita, Yoshihisa*; Kuriyama, Yasutoshi*; Yamada, Masako*; Hirota, Katsuya*; Kitaguchi, Masaaki*; Shimizu, Hirohiko*

no journal, , 

Since neutrons have a spin magnetic moment, they are subject to a force due to their interaction with the magnetic field gradient. The direction of this force coincides with the direction of the magnetic field gradient vector, and the force acts in the opposite direction depending on the direction of the spin. By utilizing this force, the neutron beam can be manipulated. If the magnetic field gradient is transverse to the beam axis, the beam is deflected. Therefore, if a sextupole magnet is used to generate a magnetic field, the magnetic field gradient changes in proportion to the distance from the center of the beam axis, which causes the same effect as a lens, and the neutron beam can be focused. In addition, by arranging permanent magnets in a Halbach array on a plane and generating a uniform magnetic field gradient in the direction normal to the plane, a neutron beam reflecting wall can be formed, which can be combined in a duct-like configuration to form a guide tube. The magnetic field gradient in the longitudinal direction relative to the beam axis can change the energy of the neutrons. The integral value of this energy change is zero if the neutrons just pass through, but if the spins are flipped in the magnetic field gradient, the neutron beam can be accelerated or decelerated with the energy corresponding to the magnetic flux density at the flipped location. By applying this technique, spatial focusing and energy modulation of neutron beams are possible. In this presentation, the principle and configuration of the instruments we are developing for neutron beam manipulation and the planned experiments are described, and their potential applications are discussed.

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