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Search Results: Records 1-7 displayed on this page of 7
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Journal Articles

Defect structure analysis of heterointerface between Pt and CeO$$_{rm x}$$ promoter on Pt electro-catalyst

Fugane, Keisuke*; Mori, Toshiyuki*; Yan, P.*; Masuda, Takuya*; Yamamoto, Shunya; Ye, F.*; Yoshikawa, Hideki*; Auchterlonie, G.*; Drennan, J.*

ACS Applied Materials & Interfaces, 7(4), p.2698 - 2707, 2015/02

https://doi.org/10.1021/am507754w
 Times Cited Count：30 Percentile：66.8(Nanoscience & Nanotechnology)

no abstracts in English

Journal Articles

Role of cerium oxide in the enhancement of activity for the oxygen reduction reaction at Pt-CeO$$_{x}$$ nanocomposite electrocatalyst; An in situ electrochemical X-ray absorption fine structure study

Masuda, Takuya*; Fukumitsu, Hitoshi*; Fugane, Keisuke*; Togasaki, Hirotaka*; Matsumura, Daiju; Tamura, Kazuhisa; Nishihata, Yasuo; Yoshikawa, Hideki*; Kobayashi, Keisuke*; Mori, Toshiyuki*; et al.

Journal of Physical Chemistry C, 116(18), p.10098 - 10102, 2012/05

https://doi.org/10.1021/jp301509t
 Times Cited Count：118 Percentile：93.69(Chemistry, Physical)

In situ electrochemical X-ray absorption fine structure (XAFS) measurements were performed at the Pt L$$_{3}$$ and Ce L$$_{3}$$ edges of the Pt-CeO$$_{x}$$/C catalyst, which was prepared by a combined process of precipitation and coimpregnation methods, as well as at the Pt L$$_{3}$$ edge of the conventional Pt/C catalyst in oxygen-saturated H$$_{2}$$SO$$_{4}$$ solution to clarify the role of CeO$$_{x}$$ in the reduction of the overpotential for the oxygen reduction reaction (ORR) at the Pt-CeO$$_{x}$$ nanocomposite compared with the conventional Pt/C catalyst. XAFS measurements clearly show that the enhancement of ORR activity is attributed to the inhibition of Pt oxide formation by the CeO$$_{x}$$ layer, of which Ce$$^{3+}$$ was oxidized to Ce$$^{4+}$$ instead of Pt at the Pt oxide formation potential.

Journal Articles

Measured and simulated transport of 1.9 MeV laser-accelerated proton bunches through an integrated test beam line at 1 Hz

Nishiuchi, Mamiko; Sakaki, Hironao; Hori, Toshihiko; Bolton, P.; Ogura, Koichi; Sagisaka, Akito; Yogo, Akifumi; Mori, Michiaki; Orimo, Satoshi; Pirozhkov, A. S.; et al.

Physical Review Special Topics; Accelerators and Beams, 13(7), p.071304_1 - 071304_7, 2010/07

https://doi.org/10.1103/PhysRevSTAB.13.071304
 Times Cited Count：25 Percentile：79.33(Physics, Nuclear)

A laser-driven repetition-rated 1.9 MeV proton beam line composed of permanent quadrupole magnets (PMQs), a radio frequency (rf) phase rotation cavity, and a tunable monochromator is developed to evaluate and to test the simulation of laser-accelerated proton beam transport through an integrated system for the first time. In addition, the proton spectral modulation and focusing behavior of the rf phase rotationcavity device is monitored with input from a PMQ triplet. In the 1.9 MeV region we observe very weakproton defocusing by the phase rotation cavity. The final transmitted bunch duration and transverse profile are well predicted by the PARMILA particle transport code. The transmitted proton beam duration of 6 ns corresponds to an energy spread near 5% for which the transport efficiency is simulated to be 10%. The predictive capability of PARMILA suggests that it can be useful in the design of future higher energy transport beam lines as part of an integrated laser-driven ion accelerator system.

JAEA Reports

None

Cho, Hisashi*; Noguchi, Yoshifumi*; Morita, Masaya*; Nakamura, Naoaki*; Iwasaki, Hiroshi*; Hotta, Masakuni*; Hokari, Toshiyuki*

PNC TJ1380 91-001, 470 Pages, 1991/05

PNC-TJ1380-91-001.pdf:26.46MB

None

Oral presentation

Investigation of oxygen reduction reaction (ORR)on Pt-CeO$$_{x}$$ model interface for polymer electrolyte fuel cells

Fugane, Keisuke*; Mori, Toshiyuki*; Masuda, Takuya*; Uosaki, Kohei*; Yamamoto, Shunya; Maekawa, Yasunari

no journal, , 

no abstracts in English

Oral presentation

Effect of electrochemical pre-treatment and interface structure between Pt and CeO$$_{x}$$ for improvement of oxygen reduction reaction activity on Pt-CeO$$_{x}$$ model electro catalysis

Fugane, Keisuke*; Mori, Toshiyuki*; Wu, Y. Y.*; Yamamoto, Shunya; Maekawa, Yasunari; Yoshikawa, Hideki*; Yamashita, Yoshiyuki*; Ueda, Shigenori*; Vladimir, M.*; Suzuki, Akira*; et al.

no journal, , 

no abstracts in English

Oral presentation

Precipitation of Pt nanoparticles on CeO$$_{2}$$ films using electron beams and $$gamma$$-rays

Yamamoto, Shunya; Sugimoto, Masaki; Miyashita, Atsumi; Hakoda, Teruyuki; Yamaki, Tetsuya; Mori, Toshiyuki*

no journal, , 

Platinum modified with cerium oxide (Pt-CeO$$_{x}$$) is considered as promising cathode materials for use in polymer membrane electrolyte fuel cells. A key process to make this active is formation of highly dispersed Pt nanoparticles on a CeO$$_{2}$$ surface. Therefore, there is a strong motivation for us to use this radiation technique for precipitation of the Pt nanoparticles on CeO$$_{2}$$ films, which would be expected to be a model electrocatalyst of Pt-CeO$$_{x}$$. We deposited the CeO$$_{2}$$ films on a SiO$$_{2}$$ substrate by magnetron sputtering. The CeO$$_{2}$$ films in an aqueous solution containing H$$_{2}$$PtCl$$_{6}$$ and C$$_{2}$$H$$_{5}$$OH were irradiated with 2 MeV electron beams and $$^{60}$$Co $$gamma$$-rays at 50 kGy at maximum. The detailed analysis revealed homogeneous precipitation of metallic Pt by the irradiation with both the radiations, suggesting high applicability of the radiation-induced precipitation method to the preparation of the model Pt-CeO$$_{x}$$ electrocatalysts.

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