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Journal Articles

Occupation sites and valence states of Co dopants in (La, Co)-codoped M-type Sr ferrite; $$^{57}$$Fe and $$^{59}$$Co nuclear magnetic resonance studies

Sakai, Hironori; Hattori, Taisuke; Tokunaga, Yo; Kambe, Shinsaku; Ueda, Hiroaki*; Tanioku, Yasuaki*; Michioka, Chishiro*; Yoshimura, Kazuyoshi*; Takao, Kenta*; Shimoda, Aiko*; et al.

Physical Review B, 98(6), p.064403_1 - 064403_10, 2018/08

 Times Cited Count:10 Percentile:45.99(Materials Science, Multidisciplinary)

To specify preferential occupation sites of Co substituents and to clarify charge and spin states of Co ions in (La, Co)-cosubstituted hexagonal magnetoplumbite-type (M-type) Sr ferrite, $$^{57}$$Fe and $$^{59}$$Co nuclear magnetic resonance (NMR) spectra are measured under zero and external magnetic fields using powdered and single crystalline specimens. To a considerable degree, the charge compensation between La$$^{3+}$$ and Co$$^{2+}$$ works in the equal (La, Co)-codoped case, where more than half of the Co ions are considered to be present in the minority spin $$4f_1$$ sites at the center of the oxygen tetrahedra, with the $$S$$ = 3/2 state carrying a small orbital moment owing to spin-orbit interaction. The remaining small number of high-spin Co$$^{2+}$$ ($$S$$ = 3/2, $$L$$ = 1) ions with unquenched orbital moments would be distributed to the other octahedral $$12k$$, $$2a$$, and $$4f_2$$ sites.

Journal Articles

NMR investigation of spin fluctuations in the itinerant-electron magnetic compound $${rm Sr}_{1-x}{rm Ca}_x{rm Co}_2{rm P}_2$$

Imai, Masaki; Michioka, Chishiro*; Ueda, Hiroaki*; Yoshimura, Kazuyoshi*

Physical Review B, 95(5), p.054417_1 - 054414_7, 2017/02

 Times Cited Count:2 Percentile:11.52(Materials Science, Multidisciplinary)

We took $$^{31}$$P NMR measurements of mainly paramagnetic phase $${rm Sr}_{1-x}{rm Ca}_x{rm Co}_2{rm P}_2$$ to reveal the itinerant-electron metamagnetic transition, and of its magnetically ordered phase, and characterized their spin fluctuations by estimating the spin fluctuation parameter $$T_{0}$$ corresponding to the width of the spin fluctuation in the spectrum in frequency space. As $$x$$ increases from 0 to 0.5, the in-plane component of $$T_{0}$$ decreases proportionally with the metamagnetic transition field. In the antiferromagnetic cT phase, $$T_{0}$$ is constant and spin fluctuations show an isotropic character in contrast to their behavior in the paramagnetic ucT phase. These results indicate that the in-plane spin fluctuations due to the quasi-two-dimensional crystal structure play a significant role in the metamagnetic transition of this system.

Journal Articles

Spin-orbit fluctuations in frustrated heavy-fermion metal LiV$$_{2}$$O$$_{4}$$

Tomiyasu, Keisuke*; Iwasa, Kazuaki*; Ueda, Hiroaki*; Niitaka, Seiji*; Takagi, Hidenori*; Kawamura, Seiko; Kikuchi, Tatsuya; Inamura, Yasuhiro; Nakajima, Kenji; Yamada, Kazuyoshi*

Physical Review Letters, 113(23), p.236402_1 - 236402_5, 2014/12

 Times Cited Count:16 Percentile:68.53(Physics, Multidisciplinary)

Spin fluctuations were studied over a wide momentum ($$hbar$$$$Q$$) and energy ($$E$$) space in the frustrated ${it d}$-electron heavy-fermion metal LiV$$_{2}$$O$$_{4}$$ by time-of-flight inelastic neutron scattering. We observed the overall ${it Q-E}$ evolutions near the characteristic ${it Q}$ = 0.6 $AA $^{-1}$$ peak and found another weak broad magnetic peak around 2.4 $AA $^{-1}$$. The data are described by a simple response function, a partially delocalized magnetic form factor, and antiferromagnetic short-range spatial correlations, indicating that heavy-fermion formation is attributable to spin-orbit fluctuations with orbital hybridization.

Journal Articles

Universal magnetic structure of the half-magnetization phase in Cr-based spinels

Matsuda, Masaaki; Oyama, Kenji*; Yoshii, Shunsuke*; Nojiri, Hiroyuki*; Frings, P.*; Duc, F.*; Vignolle, B.*; Rikken, G. L. J. A.*; Regnault, L.-P.*; Lee, S.-H.*; et al.

Physical Review Letters, 104(4), p.047201_1 - 047201_4, 2010/01

 Times Cited Count:28 Percentile:77.3(Physics, Multidisciplinary)

Journal Articles

Spin-lattice instability to a fractional magnetization state in the spinel HgCr$$_{2}$$O$$_{4}$$

Matsuda, Masaaki; Ueda, Hiroaki*; Kikkawa, Akiko*; Tanaka, Yoshikazu*; Katsumata, Koichi*; Narumi, Yasuo*; Inami, Toshiya; Ueda, Yutaka*; Lee, S.-H.*

Nature Physics, 3(6), p.397 - 400, 2007/06

 Times Cited Count:104 Percentile:93.31(Physics, Multidisciplinary)

Cr-CrCr-based spinel compounds ACr$$_{2}$$O$$_{4}$$ (A=Mg, Zn, Cd, and Hg) are so far the best model systems for a network of corner-sharing tetrahedrons with isotropic nearest-neighbor antiferromagnetic interactions. The systems exhibit novel spin-Peierls phase transitions from cubic spin liquid to non-cubic N$'e$el states at low temperatures. Recent bulk magnetization studies on CdCr$$_{2}$$O$$_{4}$$ and HgCr$$_{2}$$O$$_{4}$$ revealed the magnetic field-induced half magnetization plateau states that are stable over a wide range of field. Recent bulk magnetization studies on CdCr$$_{2}$$O$$_{4}$$ and HgCr$$_{2}$$O$$_{4}$$ revealed the magnetic field-induced half magnetization plateau states that are stable over a wide range of field.

Journal Articles

Spiral spin structure in the Heisenberg pyrochlore magnet CdCr$$_2$$O$$_4$$

Matsuda, Masaaki; Takeda, Masayasu; Nakamura, Mitsutaka; Kakurai, Kazuhisa; Osawa, Akira*; Leli$`e$vre-Berna, E.*; Chung, J.-H.*; Ueda, Hiroaki*; Takagi, Hidenori*; Lee, S.-H.*

Physical Review B, 75(10), p.104415_1 - 104415_6, 2007/03

 Times Cited Count:43 Percentile:81.73(Materials Science, Multidisciplinary)

A frustrated spinel CdCr$$_2$$O$$_4$$ undergoes a three-dimensional spin-Peierls transition at $$T_N$$ = 7.8 K from a cubic paramagnetic to a tetragonal N$'e$el state. The N$'e$el state has a spiral magnetic structure with a characteristic wave vector of $$(0,delta,1)$$ when the $$c$$ axis elongated. Here we report our spherical neutron polarimetry experiments to investigate the spiral spin structure in detail. Our results indicate that the spins lie in the $$ac$$ plane perpendicular to the direction of the spiral modulation. We also found that the spiral structure in the $$ac$$ plane is elliptical with the $$c$$-component larger by $$sim$$24% than the $$a$$-component, suggesting a strong coupling between the magnetic structure and structural distortion. Unpolarized neutron diffraction under an external magnetic field has also been performed. The magnetic field dependence suggests existence of magnetic anisotropy in the N$'e$el state, which is consistent with our previous inelastic studies.

Journal Articles

Quest for the high-filed phase of CdCr$$_2$$O$$_4$$ using an X-ray diffraction technique

Inami, Toshiya; Owada, Kenji; Tsubota, Masami; Murata, Yuto*; Matsuda, Yasuhiro*; Nojiri, Hiroyuki*; Ueda, Hiroaki*; Murakami, Yoichi*

Journal of Physics; Conference Series, 51, p.502 - 505, 2006/00

 Times Cited Count:16 Percentile:97.58(Physics, Condensed Matter)

no abstracts in English

Journal Articles

Statics and dynamics of incommensurate spin order in a geometrically frustrated antiferromagnet CdCr$$_2$$O$$_4$$

Chung, J.-H.*; Matsuda, Masaaki; Lee, S.-H.*; Kakurai, Kazuhisa; Ueda, Hiroaki*; Sato, Taku*; Takagi, Hidenori*; Hong, K.-P.*; Park, S.*

Physical Review Letters, 95(24), p.247204_1 - 247204_4, 2005/12

 Times Cited Count:140 Percentile:95.25(Physics, Multidisciplinary)

no abstracts in English

Oral presentation

Detailed magnetic structure of a frustrated spinel CdCr$$_2$$O$$_4$$ studied by polarized neutron techniques

Matsuda, Masaaki; Osawa, Akira*; Takeda, Masayasu; Kakurai, Kazuhisa; Chung, J.-H.*; Lee, S.-H.*; Ueda, Hiroaki*; Takagi, Hidenori*

no journal, , 

CdCr$$_2$$O$$_4$$ has the spinel structure, in which geometrical frustration exists between the Cr$$^{3+}$$ moments located at the corners of the tetrahedron. It shows an incommensurate antiferromagnetic ordering below $$Trm_N$$=7.8K with a characteristic wave vector of $$Q=(0, delta, 1)$$ ($$deltasim0.09$$). We first performed a 1D polarized neutron analysis and determined that the Cr$$^{3+}$$ moments has a planer anisotropy in the $$ac$$ plane, indicating that the magnetic structure is spiral. Finally, the 3D polarized neutron analysis using a CRYOPAD on TAS-1 at JRR-3 determined that the magnetic structure is elliptical spiral in the $$ac$$ plane with ellipsoid slightly elongated along the $$c$$ axis. The origin of the structure will be discussed.

Oral presentation

Spiral structure of a frustrated spinel CdCr$$_2$$O$$_4$$ studied by polarized neutron techniques

Matsuda, Masaaki; Osawa, Akira*; Takeda, Masayasu; Nakamura, Mitsutaka; Leli$`e$vre-Berna, E.*; Kakurai, Kazuhisa; Chung, J.-H.*; Lee, S.-H.*; Ueda, Hiroaki*; Takagi, Hidenori*

no journal, , 

no abstracts in English

Oral presentation

Magnetic Structure of a Frustrated Spinel CdCr$$_{2}$$O$$_{4}$$

Matsuda, Masaaki; Osawa, Akira*; Takeda, Masayasu; Nakamura, Mitsutaka; Kakurai, Kazuhisa; Leli$`e$vre-Berna, E.*; Chung, J.-H.*; Lee, S.-H.*; Ueda, Hiroaki*; Takagi, Hidenori*

no journal, , 

no abstracts in English

Oral presentation

Neutron and X-ray diffraction studies of a frustrated spinel antiferromagnet HgCr$$_2$$O$$_4$$ in high magnetic field

Matsuda, Masaaki; Ueda, Hiroaki*; Kikkawa, Akiko*; Tanaka, Yoshikazu*; Katsumata, Koichi*; Narumi, Yasuo*; Inami, Toshiya; Ueda, Yutaka*; Lee, S.-H.*

no journal, , 

no abstracts in English

Oral presentation

An X-ray diffraction experiment of the magnetization plateau phase of CdCr$$_2$$O$$_4$$

Inami, Toshiya; Owada, Kenji; Tsubota, Masami; Matsuda, Yasuhiro*; Nojiri, Hiroyuki*; Ueda, Hiroaki*

no journal, , 

no abstracts in English

Oral presentation

Spin correlations in a frustrated spinel antiferromagnet LiCrMnO$$_4$$

Matsuda, Masaaki; Honda, Zentaro*; Katori, Hiroko*; Takagi, Hidenori*; Ueda, Hiroaki*; Ueda, Yutaka*; Mitamura, Hiroyuki*; Kindo, Koichi*

no journal, , 

Oral presentation

Neutron diffraction study of spinel CdCr$$_2$$O$$_4$$ in pulsed high magnetic field

Matsuda, Masaaki; Oyama, Kenji*; Yoshii, Shunsuke*; Nojiri, Hiroyuki*; Ueda, Hiroaki*; Ueda, Yutaka*; Regnault, L.-P.*; Vignole, B.*; Duc, F.*; Frings, P.*; et al.

no journal, , 

no abstracts in English

Oral presentation

Neutron diffraction study of spinel CdCr$$_2$$O$$_4$$ in pulsed high magnetic field

Matsuda, Masaaki; Oyama, Kenji*; Yoshii, Shunsuke*; Nojiri, Hiroyuki*; Ueda, Hiroaki*; Ueda, Yutaka*; Regnault, L.-P.*; Vignole, B.*; Duc, F.*; Frings, P.*; et al.

no journal, , 

no abstracts in English

Oral presentation

Universal magnetic structure of the half-magnetization phase in Cr-based spinels

Matsuda, Masaaki; Oyama, Kenji*; Yoshii, Shunsuke*; Nojiri, Hiroyuki*; Frings, P.*; Duc, F.*; Vignole, B.*; Rikken, G. L. J. A.*; Regnault, L.-P.*; Lee, S.-H.*; et al.

no journal, , 

17 (Records 1-17 displayed on this page)
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