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SGo, Shintaro*; Ideguchi, Eiji*; Yokoyama, Rin*; Aoi, Nori*; Azaiez, F.*; Furutaka, Kazuyoshi; Hatsukawa, Yuichi; Kimura, Atsushi; Kisamori, Keiichi*; Kobayashi, Motoki*; et al.
Physical Review C, 103(3), p.034327_1 - 034327_8, 2021/03
Times Cited Count：4 Percentile：57.13(Physics, Nuclear)
F from 
O
?Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.
Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05
Times Cited Count：14 Percentile：74.18(Physics, Multidisciplinary)The structure of a neutron-rich F nucleus is investigated by a quasifree (
) knockout reaction. The sum of spectroscopic factors of 
orbital is found to be 1.0 
0.3. The result shows that the O core of F nucleus significantly differs from a free O nucleus, and the core consists of 
35% O
, and 65% excited O. The result shows that the O core of F nucleus significantly differs from a free O nucleus. The result may infer that the addition of the 
proton considerably changes the neutron structure in F from that in O, which could be a possible mechanism responsible for the oxygen dripline anomaly.
Yokoyama, Tatsunori; Misawa, Keiji*; Okano, Osamu*; Minowa, Haruka*; Fukuoka, Takaaki*
Journal of Radioanalytical and Nuclear Chemistry, 310(1), p.81 - 89, 2016/10
Times Cited Count：1 Percentile：10.71(Chemistry, Analytical)The identification of alkali-rich components in extraterrestrial materials along with their separation from other constituents is indispensable for subsequent cosmochemical and isotopic studies. This paper presents a simple pre-screening method for such materials by autoradiography using imaging plates (IPs), which is applicable to identification of mm-sized samples containing ca. 30 
g of potassium in the Yamayo-74442 chondrite. The detection limit of IPs was 1 mBq of 
K under 49 days exposure. The method provides an opportunity to screen meteorite materials non-destructively and to inexpensively check potassium-rich areas and suitable for the K-Ca and K-Ar (
Ar-Ar) age determinations.
SGo, Shintaro*; Ideguchi, Eiji*; Yokoyama, Rin*; Kobayashi, Motoki*; Kisamori, Keiichi*; Takaki, Motonobu*; Miya, Hiroyuki*; Ota, Shinsuke*; Michimasa, Shinichiro*; Shimoura, Susumu*; et al.
JPS Conference Proceedings (Internet), 6, p.030005_1 - 030005_4, 2015/06
Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*; Yokoyama, Kaoru; Takahashi, Nobuo; Hata, Haruhi; Sugitsue, Noritake
JAEA-Research 2011-035, 53 Pages, 2012/01
JAEA-Research-2011-035.pdf:3.13MB
System decontamination has been generally carried out with the aim of reducing the amount of radioactive waste generated and minimizing exposure to radiation released from nuclear fuel facilities. At the Ningyo-Toge Environmental Engineering Center, metal surfaces that are contaminated by uranium are dry decontaminated by using iodine heptafluoride (IF
) as a system decontaminator. Only a few studies have been carried out on the decontamination efficiency, mechanism, level, etc. of dry decontamination techniques that use a decontamination gas. Therefore, the generalization of dry decontamination techniques is required. In the present study, the efficiency of a dry decontamination technique was assessed by a numerical method using decontamination data obtained at the Ningyo-Toge Environmental Engineering Center. A concrete analytical content is a depositing of uranium hexafluoride.
Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*; Yokoyama, Kaoru; Takahashi, Nobuo; Hata, Haruhi; Sugitsue, Noritake
JAEA-Research 2010-032, 32 Pages, 2010/10
JAEA-Research-2010-032.pdf:1.72MB
System decontamination has been generally carried out with the aim of reducing the amount of radioactive waste generated and minimizing human exposure to radiation released from nuclear fuel facilities. At the Ningyo-Toge Environmental Engineering Center, metal surfaces that are contaminated by uranium are dry decontaminated by using iodine heptafluoride (IF) as a system decontaminator. In this dry decontamination technique, a chemical reaction occurs between the uranium compound attached to the metal surface and IF. Only a few studies have been carried out on the decontamination efficiency, mechanism, level, etc. of dry decontamination techniques that use a decontamination gas. Therefore, the generalization of dry decontamination technique was assessed by a numerical method using decontamination data obtained at the Ningyo-Toge Environmental Engineering Center. A concrete analytical content is a depositing of Uranium Hexafluoride.
Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*; Yokoyama, Kaoru; Takahashi, Nobuo; Tsunashima, Yasumichi; Ema, Akira; Sugitsue, Noritake
JAEA-Research 2009-047, 92 Pages, 2010/01
JAEA-Research-2009-047.pdf:5.13MB
System decontamination has been generally carried out with the aim of reducing the amount of radioactive waste generated and minimizing human exposure to radiation released from nuclear fuel facilities. At the Ningyo-Toge Environmental Engineering Center, metal surfaces that are contaminated by uranium are dry decontaminated by using iodine heptafluoride (IF) as a system decontaminator. In this dry decontamination technique, a chemical reaction occurs between the uranium compound attached to the metal surface and IF. Only a few studies have been carried out on the decontamination efficiency, mechanism, level, etc. of dry decontamination techniques that use a decontamination gas. Therefore, the generalization of dry decontamination techniques is required. In the present study, the efficiency of a dry decontamination technique was assessed by a numerical method using decontamination data obtained at the Ningyo-Toge Environmental Engineering Center.
Tsukada, Takashi; Miwa, Yukio; ; Tsuji, Hirokazu; Nakajima, Hajime
Proc. of 2nd Japan-Central Europe Joint Workshop on Modelling of Materials and Combustion, 0, p.80 - 83, 1996/00
no abstracts in English
Yokoyama, Kaoru; Hata, Haruhi; Sugitsue, Noritake; Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*
no journal, ,
The decontamination technique using the iodine heptafluoride is known as a system decontamination technique of facilities like the uranium enrichment plant where the uranium hexafluoride was handled. In this report, the mechanism of the system decontamination using the iodine heptafluoride is clarified at a molecular level. The generation process of the uranium tetrafluoride is estimated using the plant operation data. In addition, the generation speed of the uranium tetrafluoride and the activation energy are of the uranium tetrafluoride and iodine heptafluoride reaction are estimated.
Hata, Haruhi; Yokoyama, Kaoru; Sugitsue, Noritake; Hyakutake, Toru*; Muto, Akinori*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*
no journal, ,
As a first step to elucidate the molecular mechanism of decontamination systems for iodine heptafluoride, uranium hexafluoride and the metal (iron), the possibility of physical adsorption and chemical reactions with uranium hexafluoride and uranium tetrafluoride (solid), we investigate the possibility of physical adsorption and chemical reactions of this. Therefore, the intermolecular of uranium hexafluorides, iron and uranium hexafluoride, uranium tetrafluoride and uranium hexafluoride (solid) and evaluated by molecular orbital method to the intermolecular potential between, based on this data, MD law adhesion mechanism was estimated by uranium hexafluoride.
Yokoyama, Kaoru; Hata, Haruhi; Takahashi, Nobuo; Sugitsue, Noritake; Hyakutake, Toru*; Sasakura, Mariko*; Minowa, Hirotsugu*
no journal, ,
Fundamental study in the molecular level about the system decontamination using iodine heptafluoride was performed. When UF
entered to the surface to which UF
stuck, activation energy for UF to perform a chemical reaction on the surface of a wall was analyzed. The molecular dynamics method was used for calculation.
Hata, Haruhi; Yokoyama, Kaoru; Takahashi, Nobuo; Sugitsue, Noritake; Hyakutake, Toru*; Sasakura, Mariko*; Minowa, Hirotsugu*; Suzuki, Kazuhiko*
no journal, ,
The IF treatment technique belongs to the systematic decontamination technology. It has the high performance decontamination technique for the plant that accumulates the uranium intermediate fluoride, such as UF, UF
, U
F
, and UF
, which exist in the uranium enrichment plant. This report will show the chemical reactions and the physical adsorption between the metal and the uranium fluoride on the molecular scale, which was calculated by the molecular dynamics method.
