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Porcheron, E.*; Journeau, C.*; Delacroix, J.*; Berlemont, R.*; Bouland, A.*; Lallot, Y.*; Tsubota, Yoichi; Ikeda, Atsushi; Mitsugi, Takeshi
Proceedings of International Conference on Environmental Remediation and Radioactive Waste Management (ICEM2023) (Internet), 5 Pages, 2023/10
Results of the URASOL project aimed at evaluating the generation and dispersion of radioactive aerosols during the cutting of fuel debris, a key issue in the decommissioning of the damaged reactors at the Fukushima Daiichi Nuclear Power Station (1F), are presented in this report. Characterization of aerosols generated during heating and mechanical cutting of simulated fuel debris in terms of mass concentration, real-time number density, mass-based particle size distribution, morphology, and chemical properties is reported. In the heating tests, an increase in particle size with increasing temperature was observed, and in terms of particle number density, the case using depleted uranium simulated fuel debris had a smaller number density than the test using Hf-containing simulated fuel debris. In mechanical cleavage, the aerodynamic median mass diameter of the aerosol was almost the same for the radioactive and non-radioactive samples (about 3.74.4 m).
Ikeda, Yoichi*; Umemoto, Yoshihiko*; Matsumura, Daiju; Tsuji, Takuya; Hashimoto, Yuki*; Kitazawa, Takafumi*; Fujita, Masaki*
Materials Transactions, 64(9), p.2254 - 2260, 2023/09
Times Cited Count:0Kitazawa, Takafumi; Ikeda, Yoichi*; Sakakibara, Toshiro*; Matsuo, Akira*; Shimizu, Yusei*; Tokunaga, Yo; Haga, Yoshinori; Kindo, Koichi*; Nambu, Yusuke*; Ikeuchi, Kazuhiko*; et al.
Physical Review B, 108(8), p.085105_1 - 085105_7, 2023/08
Porcheron, E.*; Leblois, Y.*; Journeau, C.*; Delacroix, J.*; Molina, D.*; Suteau, C.*; Berlemont, R.*; Bouland, A.*; Lallot, Y.*; Roulet, D.*; et al.
Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR2022) (Internet), 5 Pages, 2022/10
One of the important challenges for the decommissioning of the damaged reactors of the Fukushima Daiichi Nuclear Power Station (1F) is the fuel debris retrieval. The URASOL project, which is undertaken by a French consortium consisting of ONET Technologies, CEA, and IRSN for JAEA/CLADS, is dedicated to acquiring basic scientific data on the generation and characteristics of radioactive aerosols from the thermal or mechanical processing of fuel debris simulant. Heating process undertaken in the VITAE facility simulates some representative conditions of thermal cutting by LASER. For mechanical cutting, the core boring technique is implemented in the FUJISAN facility. Fuel debris simulants have been developed for inactive and active trials. The aerosols are characterized in terms of mass concentration, real time number concentration, mass size distribution, morphology, and chemical properties. The chemical characterization aims at identifying potential radioactive particles released and the associated size distribution, both of which are important information for assessing possible safety and radioprotection measures during the fuel debris retrieval operations at 1F.
Tsubota, Yoichi; Honda, Fumiya; Tokonami, Shinji*; Tamakuma, Yuki*; Nakagawa, Takahiro; Ikeda, Atsushi
Nuclear Instruments and Methods in Physics Research A, 1030, p.166475_1 - 166475_7, 2022/05
Times Cited Count:1 Percentile:33.4(Instruments & Instrumentation)In the long-lasting decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), the dismantling of nuclear fuel debris (NFD) remaining in the damaged reactors is an unavoidable but significant issue with many technical difficulties. The dismantling is presumed to involve mechanical cutting, generating significant concentrations of particulates containing -radionuclides (-aerosols) that pose significant health risk upon inhalation. In order to minimize the radiation exposure of workers with -aerosols during the dismantling/decommissioning process at 1F, it is essential to monitor the concentration of -aerosols at the point of initial generation, i.e. inside the primary containment vessels (PCV) of the damaged reactors. Toward this end, an monitoring system for -aerosols ( alpha air monitor: IAAM) was developed and its technical performance was investigated under the conditions expected for the actual environments at 1F. IAAM was confirmed to fulfill four technical requirements: (1) steady operation under high humidity, (2) operation without using filters, (3) capability of measuring a high counting rate of -radiation, and (4) selective measurement of -radiation even under high radiation background with /-rays. IAAM is capable of selectively measuring -aerosols with a concentration of 3.3 10 Bq/cm or higher without saturation under a high humid environment (100%-relative humidity) and under high background with /-radiation (up to 100 mSv/h of -radiation). These results demonstrate promising potential of IAAM to be utilized as a reliable monitoring system for -aerosols during the dismantling of NFD, as well as the whole long-lasting decommissioning of 1F.
Sombillo, D. L. B.*; Ikeda, Yoichi*; Sato, Toru*; Hosaka, Atsushi
Physical Review D, 104(3), p.036001_1 - 036001_12, 2021/08
Times Cited Count:8 Percentile:61.27(Astronomy & Astrophysics)Horibe, Yoichi*; Mori, Shigeo*; Ikeda, Naoshi*; Yoshii, Kenji; Maeno, Hiroshi*; Murakami, Yasukazu*
Ferroelectrics, 584(1), p.20 - 30, 2021/00
Times Cited Count:1 Percentile:7.92(Materials Science, Multidisciplinary)Temperature dependence of charge-ordered crystal structures and domain structures in RFeO (R: Y and Lu) was investigated by energy-filtered transmission electron microscopy, combined with conventional transmission electron microscopy. The presence of three-dimensional to two-dimensional charge ordering transition were observed in both RFeO on heating. Furthermore, real-space images obtained with the energy-filtered transmission electron microscopy revealed that YRFeO has less anisotropic nanometer-scale charge-ordered domains than LuRFeO. These findings in RFeO indicate the importance of the interchange interactions between Fe-O bilayers in addition to those within bilayers in the structural phase transitions associated with charge ordering in this system.
Ikeda, Yoichi*; Ueta, Daichi*; Yoshizawa, Hideki*; Nakao, Akiko*; Munakata, Koji*; Ohara, Takashi
Journal of the Physical Society of Japan, 84(12), p.123701_1 - 123701_5, 2015/12
Times Cited Count:4 Percentile:34.89(Physics, Multidisciplinary)Single-crystal neutron diffraction study was performed for anomalous antiferromagnetic ordering in a heavy-electron superconductor CeNiGe. We observed incommensurate magnetic Bragg reflections characterized with the propagation vector of = (0; 0:41; 1=2) below the Nel temperature of 5 K, while there is no significant magnetic reflection at the commensurate propagation vector of = (1; 0; 0) at which another magnetic reflection was observed in the previous neutron diffraction study with a polycrystalline sample. From the single crystal study, we suggest that the magnetic phase of CeNiGe at ambient pressure is characterized only by the incommensurate propagation vector .
Ito, Shinichi*; Yokoo, Tetsuya*; Masuda, Takatsugu*; Yoshizawa, Hideki*; Soda, Minoru*; Ikeda, Yoichi*; Ibuka, Soshi*; Kawana, Daichi*; Sato, Taku*; Nambu, Yusuke*; et al.
JPS Conference Proceedings (Internet), 8, p.034001_1 - 034001_6, 2015/09
Araki, Shingo*; Hayashida, Minami*; Nishiumi, Naoto*; Manabe, Hiroki*; Ikeda, Yoichi*; Kobayashi, Tatsuo*; Murata, Keizo*; Inada, Yoshihiko*; Winiewski, P.*; Aoki, Dai*; et al.
Journal of the Physical Society of Japan, 84(2), p.024705_1 - 024705_8, 2015/02
Times Cited Count:9 Percentile:55.91(Physics, Multidisciplinary)Araki, Shingo*; Hayashida, Minami*; Nishiumi, Naoto*; Manabe, Hiroki*; Ikeda, Yoichi*; Kobayashi, Tatsuo*; Murata, Keizo*; Inada, Yoshihiko*; Winiewski, P.*; Aoki, Dai*; et al.
JPS Conference Proceedings (Internet), 3, p.011081_1 - 011081_6, 2014/06
Shimizu, Yusei*; Haga, Yoshinori; Ikeda, Yoichi*; Yanagisawa, Tatsuya*; Amitsuka, Hiroshi*
Physical Review Letters, 109(21), p.217001_1 - 217001_5, 2012/11
Times Cited Count:17 Percentile:67.41(Physics, Multidisciplinary)Yoshii, Kenji; Ikeda, Naoshi*; Nishihata, Yasuo; Maeda, Daisuke*; Fukuyama, Ryota*; Nagata, Tomoko*; Kano, Jun*; Kambe, Takashi*; Horibe, Yoichi*; Mori, Shigeo*
Journal of the Physical Society of Japan, 81(3), p.033704_1 - 033704_4, 2012/03
Times Cited Count:10 Percentile:55.37(Physics, Multidisciplinary)Exchange bias (EB) behavior has been observed for multiferroic FeO (=Y, Er, Tm, Yb, Lu and In). The materials with the small ions (=Tm, Yb, Lu and In) exhibit large EB fields ( 1 kOe) below 100-150 K. This property is rooted in a magnetically glassy state, arising from the competition between ferro- and antiferromagnetic domain interactions. In addition, the exchange bias field tends to be more enhanced for smaller ions. Hence, the EB is controlled by the substitution at the -site in this series.
Shimizu, Yusei*; Ikeda, Yoichi*; Wakabayashi, Takumi*; Haga, Yoshinori; Tenya, Kenichi*; Hidaka, Hiroyuki*; Yanagisawa, Tatsuya*; Amitsuka, Hiroshi*
Journal of the Physical Society of Japan, 80(9), p.093701_1 - 093701_4, 2011/09
Times Cited Count:8 Percentile:50.77(Physics, Multidisciplinary)Shimizu, Yusei*; Ikeda, Yoichi*; Wakabayashi, Takumi*; Tenya, Kenichi*; Haga, Yoshinori; Hidaka, Hiroyuki*; Yanagisawa, Tatsuya*; Amitsuka, Hiroshi*
Journal of the Physical Society of Japan, 80(Suppl.A), p.SA100_1 - SA100_3, 2011/07
Times Cited Count:1 Percentile:11.35(Physics, Multidisciplinary)Shimizu, Yusei*; Ikeda, Yoichi*; Wakabayashi, Takumi*; Tenya, Kenichi*; Haga, Yoshinori; Hidaka, Hiroyuki*; Yanagisawa, Tatsuya*; Amitsuka, Hiroshi*
Journal of Physics; Conference Series, 273, p.012084_1 - 012084_4, 2011/02
Times Cited Count:3 Percentile:62.76(Physics, Condensed Matter)Horibe, Yoichi*; Ikeda, Naoshi*; Yoshii, Kenji; Mori, Shigeo*
Physical Review B, 82(18), p.184119_1 - 184119_5, 2010/11
Times Cited Count:9 Percentile:40.66(Materials Science, Multidisciplinary)The low-temperature superstructure of YFeO was carefully investigated by transmission electron microscopy. We found that the unique superstructure at about 100 K is characterized by /14 2/7 1/14-type superlattice reflection spots, suggesting the presence of charge reordering process. The low-temperature high-resolution images clearly show superlattice modulations in Y-O layers as well as Fe-O layers. The modification of intra-bilayer charge interactions due to lattice distortions in Y-O layers is discussed to play a crucial role in the stabilization of long-periodic superstructures at low temperatures.
Horibe, Yoichi*; Yoshii, Kenji; Ikeda, Naoshi*; Mori, Shigeo*
Physical Review B, 80(9), p.092104_1 - 092104_4, 2009/09
Times Cited Count:17 Percentile:57.91(Materials Science, Multidisciplinary)The effects of oxygen deficiency on charge ordering were investigated by transmission electron microscopy at various deficiencies and temperatures of YFeO. We found that the detailed nature of the charge ordering structures is associated with changes in the superlattice reflections and diffuse scattering. They go from (1/3 1/3 1/2)-type superlattice reflection to (1/3 1/3 )-type straight-type diffuse scattering, then to zigzag-type diffuse scattering. With the oxygen deficiencies increased, the interchange correlation of Fe-O bilayers obviously decreases, yet the triple super periodicity along [110] remains unchanged. These findings on frustrated ferritesindicate the stability of in-plane threefold charge ordering and the importance of the interchange interaction between bilayers in the structural phase transitions.
Matsuo, Yoji*; Hirata, Akihiko*; Horibe, Yoichi*; Yoshii, Kenji; Ikeda, Naoshi*; Mori, Shigeo*
Ferroelectrics, 380(1), p.56 - 62, 2009/06
Times Cited Count:6 Percentile:29.51(Materials Science, Multidisciplinary)Diluted effect on the charge ordered (CO) structure in dielectric materials LuFeO (=Cu, Co) were investigated by an energy-filtered transmission electron microscope (TEM), in combination with a conventional TEM. It is revealed that partial substitution of Cu and Co for Fe in LuFeO destabilized the CO structure. In LuFeCuO, there exist characteristic zigzag-shaped diffuse streaks and diffuse spots at the h/3- h/3- 0-type positions (h: integer, =0.06) in reciprocal space, which originate from static cationic ordering of Fe and Cu ions in the triangular lattice. Moreover, real-space images by the energy-filtered TEM revealed that nanometer-sized domain structures with the 510 nm size are formed. In contrast, honeycomb-shaped diffuse streaks were found in LuFeCoO, in which no domain structures are observed in real-space images.
Yoshii, Kenji; Ikeda, Naoshi*; Michiuchi, Takamasa*; Yokota, Yusuke*; Okajima, Yuka; Yoneda, Yasuhiro; Matsuo, Yoji*; Horibe, Yoichi*; Mori, Shigeo*
Journal of Solid State Chemistry, 182(7), p.1611 - 1618, 2009/06
Times Cited Count:15 Percentile:51.45(Chemistry, Inorganic & Nuclear)We have investigated the magnetic and dielectric properties of YbFeMnO (0x1), which is an Fe-site-substituted system of new multiferroic oxides RFeO (R=Y, Ho-Lu). X-ray diffraction measurements show that a solid solution is formed between YbFeO (x=0) and YbFeMnO (x=1) for 0x1. The valence of the Mn ion is determined to be 2+, consistently with the suppression of low-temperature magnetization by the Mn substitution. The magnetic transition temperature and the dielectric constant decrease monotonically with increasing x. This result plausibly confirms that the magnetic and dielectric properties in oxides isostructural with RFeO are governed by the electron transfer between Fe-site ions, unlike ordinary ferroelectrics and dielectrics, in which the ionic displacement plays a key role. The possibility for application is briefly discussed.