Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Yoshida, Hisao*; Yamamoto, Akira*; Hosokawa, Saburo*; Yamazoe, Seiji*; Kikkawa, Soichi*; Hara, Kenji*; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Tanaka, Tsunehiro*
Topics in Catalysis, 64(9-12), p.660 - 671, 2021/08
Times Cited Count:2 Percentile:10.95(Chemistry, Applied)Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count:44 Percentile:97.1(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
Yamazoe, Seiji*; Yamamoto, Akira*; Hosokawa, Saburo*; Fukuda, Ryoichi*; Hara, Kenji*; Nakamura, Mitsutaka; Kamazawa, Kazuya*; Tsukuda, Tatsuya*; Yoshida, Hisao*; Tanaka, Tsunehiro*
Catalysis Science & Technology, 11(1), p.116 - 123, 2021/01
Times Cited Count:6 Percentile:33.04(Chemistry, Physical)Haba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.
Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08
Times Cited Count:6 Percentile:58.52(Physics, Nuclear)Ikeda, Shugo*; Kaneko, Koji; Tanaka, Yuki*; Kawasaki, Takuro; Hanashima, Takayasu*; Munakata, Koji*; Nakao, Akiko*; Kiyanagi, Ryoji; Ohara, Takashi; Mochizuki, Kensei*; et al.
Journal of the Physical Society of Japan, 89(1), p.014707_1 - 014707_7, 2020/01
Times Cited Count:1 Percentile:11.81(Physics, Multidisciplinary)Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.
Science, 364(6437), p.272 - 275, 2019/04
Times Cited Count:262 Percentile:99.73(Multidisciplinary Sciences)The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.
Seki, Kotaro; Sasaki, Takayuki*; Akimoto, Yuji*; Tokunaga, Takahito; Tanaka, Kiwamu; Haraga, Tomoko; Ueno, Takashi; Ishimori, Kenichiro; Hoshi, Akiko; Kameo, Yutaka
JAEA-Technology 2016-013, 37 Pages, 2016/07
In this study, based on the simple and rapid analytical method established from the wastes from research facilities, we created analytical schemes which is applicable to rubble and plants collected at Fukushima Daiichi, then transported to Nuclear Science Research Institute of JAEA. We examined the applicability, and confirmed quantifiability of radioactivity concentration with high recovery rate without being affected by fission products such as Sr and Cs.
Kaji, Daiya*; Morimoto, Koji*; Wakabayashi, Yasuo*; Takeyama, Mirei*; Yamaki, Sayaka*; Tanaka, Kengo*; Haba, Hiromitsu*; Huang, M.*; Murakami, Masashi*; Kanaya, Jumpei*; et al.
JPS Conference Proceedings (Internet), 6, p.030107_1 - 030107_4, 2015/06
Performance of the new gas-filled recoil ion separator GARIS-II was investigated using asymmetric Ne-induced fusion reactions. The use of He-H mixture gas for the gas-filled magnet significantly reduced background scattered particles detected at the focal-plane Si detector, and increased a transmission of the asymmetric reaction products. A target-identification system was newly installed for efficient measurements of excitation functions without changing beam energy nor target.
Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05
Times Cited Count:3 Percentile:25.64(Chemistry, Analytical)A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived Nb and Ta were produced with nuclear reactions using a F beam whose energy was the same as that to produce Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the Nb and Ta to a chemistry device for Db without changing other experimental conditions.
Arisaka, Makoto; Watanabe, Masayuki; Ishizaki, Manabu*; Kurihara, Masato*; Chen, R.*; Tanaka, Hisashi*
Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1543 - 1547, 2015/02
Times Cited Count:13 Percentile:72.94(Chemistry, Analytical)The influence of irradiation with -rays to metal hexacyanoferrate (MHCF: M = Fe, Cu or Ni), which is known as an adsorbent for selective adsorption of cesium (Cs) ion in solution, on Cs adsorption ability and stability was investigated in HNO solutions. Under the adsorbed dose conditions (50-300 kGy), it was found that the MHCF is fully stable although the radiolytic decomposition of MHCF was slightly observed with an increase of the total adsorbed dose, which was confirmed by an increment of Fe, Cu or Ni concentration in HNO solution after the irradiation. The weight percent of the metal in the solution to initial weight of MHCF was less than unity. Moreover, no change in composition of carbon, hydrogen and nitrogen in MHCF was observed. On the other hand, the distribution coefficients of Cs to the irradiated MHCF were independent of the total adsorbed dose. This indicates that the Cs adsorption ability was maintained under -ray irradiation.
Ishizaki, Manabu*; Akiba, Sae*; Otani, Asako*; Hoshi, Yuji*; Ono, Kenta*; Matsuba, Mayu*; Togashi, Takanari*; Kanaizuka, Katsuhiko*; Sakamoto, Masatomi*; Takahashi, Akira*; et al.
Dalton Transactions, 42(45), p.16049 - 16055, 2013/12
Times Cited Count:179 Percentile:99.58(Chemistry, Inorganic & Nuclear)We have revealed the fundamental mechanism of specific Cs adsorption into Prussian blue (PB) in order to develop high-performance PB-based Cs adsorbents in the wake of the Fukushima nuclear accident. We compared two types of PB nanoparticles with formulae of Fe[Fe(CN)]3xHO (x = 10-15) (PB-1) and (NH)0.70Fe1.10[Fe(CN)]1.7HO (PB-2) with respect to the Cs adsorption ability. The synthesised PB-1, by a common stoichiometric aqueous reaction between 4Fe and 3[Fe(CN)], showed much more efficient Cs adsorption ability than did the commercially available PB-2.
Chen, R.*; Tanaka, Hisashi*; Kawamoto, Toru*; Asai, Miyuki*; Fukushima, Chikako*; Na, H.*; Kurihara, Masato*; Watanabe, Masayuki; Arisaka, Makoto; Nankawa, Takuya
Electrochimica Acta, 87, p.119 - 125, 2013/01
Times Cited Count:108 Percentile:94.84(Electrochemistry)A novel electrochemical adsorption system using a nanoparticle film of copper (II) hexacyanoferrate (III) was proposed for selectively removing cesium from wastewater. This system can be used for cesium separation without extra chemical reagents or any filtration treatment. Cesium uptake and elution can be simply controlled by switching the applied potentials between anodes and cathodes. Data from batch kinetic studies well fitted the intraparticle diffusion equation, reflecting a two-step process: a steepest ascent portion followed by a plateau extending to the equilibrium. The effective cesium removal with a high distribution coefficient ( 510 mL/g) can be adopted in a large pH range from 0.3 to 9.2, and in the presence of several diverse coexisting alkaline cations, suggesting it can be taken as a promising technology for actual nuclear wastewater treatment.
Toyoshima, Yoshiyuki*; Takahashi, Akemi*; Tanaka, Hisaki*; Watanabe, Jun*; Mogi, Yoshinobu*; Yamazaki, Tatsuo*; Hamada, Ryoko*; Iwashita, Kazuhiro*; Sato, Katsuya; Narumi, Issei
Mutation Research; Fundamental and Molecular Mechanisms of Mutagenesis, 740(1-2), p.43 - 49, 2012/12
Times Cited Count:18 Percentile:49.08(Biotechnology & Applied Microbiology)Chen, R.*; Tanaka, Hisashi*; Kawamoto, Toru*; Asai, Miyuki*; Fukushima, Chikako*; Kurihara, Masato*; Watanabe, Masayuki; Arisaka, Makoto; Nankawa, Takuya
Electrochemistry Communications, 25, p.23 - 25, 2012/11
Times Cited Count:50 Percentile:79.65(Electrochemistry)We first synthesized water-dispersed nanoparticle copper hexacyanoferrate (CuHCF) ink and then coated its nanoparticles on electrodes to electrochemically remove cesium from wastewater. Cesium uptake and elution can be controlled by switching the potentials between anodes and cathodes. Effective cesium removal can be adopted in a large pH range from 0.2 to 8.9, and in the presence of several diverse coexisting alkaline cations, suggesting that it can be taken as a promising technology for actual radioactive wastewater treatment. The prepared CuHCF nanoparticles can be simply and uniformly coated on electrodes by wet process like conventional printing methods, so any sizes or patterns are feasible at low cost, which indicated the potential as a promising sorption electrode of large size in the columns for sequential removal and recycle of Cs from wastewater.
Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sumita, Takayuki*; Wakabayashi, Yasuo*; Yoneda, Akira*; Tanaka, Kengo*; et al.
Journal of the Physical Society of Japan, 81(10), p.103201_1 - 103201_4, 2012/10
Times Cited Count:167 Percentile:97.31(Physics, Multidisciplinary)An isotope of the 113th element, 113, was produced in a nuclear reaction with a Zn beam on a Bi target. We observed six consecutive decays following the implantation of a heavy particle in nearly the same position in the semiconductor detector, in extremely low background condition. The fifth and sixth decays are fully consistent with the sequential decays of Db and Lr both in decay energies and decay times. This indicates that the present decay chain consisted of 113, Rg (Z = 111), Mt (Z = 109), Bh (Z = 107), Db (Z = 105), and Lr (Z = 103) with firm connections. This result, together with previously reported results from 2004 and 2007, conclusively leads the unambiguous production and identification of the isotope 113, of the 113th element.
Ueda, Yoshio*; Oya, Kaoru*; Ashikawa, Naoko*; Ito, Atsushi*; Ono, Tadayoshi*; Kato, Daiji*; Kawashima, Hisato; Kawamura, Gakushi*; Kenmotsu, Takahiro*; Saito, Seiki*; et al.
Purazuma, Kaku Yugo Gakkai-Shi, 88(9), p.484 - 502, 2012/09
no abstracts in English
Toyoshima, Yoshiyuki*; Tanaka, Hisaki*; Watanabe, Jun*; Yamazaki, Tatsuo*; Iwashita, Kazuhiro*; Mikami, Shigeaki*; Sato, Katsuya; Narumi, Issei
JAEA-Review 2009-041, JAEA Takasaki Annual Report 2008, P. 82, 2009/12
no abstracts in English
Oya, Kaoru*; Inai, Kensuke*; Shimizu, Katsuhiro; Takizuka, Tomonori; Kawashima, Hisato; Hoshino, Kazuo; Hatayama, Akiyoshi*; Toma, Mitsunori*; Tomita, Yukihiro*; Kawamura, Gakushi*; et al.
Purazuma, Kaku Yugo Gakkai-Shi, 85(10), p.695 - 703, 2009/10
no abstracts in English
Asakura, Nobuyuki; Ono, Noriyasu*; Tanaka, Hirohiko*; Kawashima, Hisato; Nakano, Tomohide
Journal of Nuclear Materials, 390-391, p.364 - 367, 2009/06
Times Cited Count:4 Percentile:30.43(Materials Science, Multidisciplinary)Characteristics of the fluctuations at three locations (Low-Field-Side midplane, X-point, and High-Field-Side SOLs) of the JT-60U SOL were investigated in L-mode and ELMy H-mode plasmas. Influence of their poloidal asymmetry at the LFS and HFS on the parallel plasma flow was investigated. For the L-mode, poloidal asymmetry in djs/js was enhanced at the LFS midplane (40-60%), while it was small (10-20%) at the HFS SOL and LFS X-point. On the other hand, djs/js was similar (20-30) for the ELMy H-mode. Statistical properties (Skewness) and their poloidal asymmetry were different in the ELMy H-mode and L-mode plasmas. In the ELMy H-mode, positive S (= 0.3-0.5) was seen near the separatrix. However, in the L-mode, larger S (=0.5-0.9) was observed at the LFS midplane, and it extended to the far SOL (r 10 cm). In-out asymmetry in the intermittent transport will contribute to produce the SOL flow pattern.
Tanaka, Hirohiko*; Ono, Noriyasu*; Asakura, Nobuyuki; Tsuji, Yoshiyuki*; Kawashima, Hisato; Takamura, Shuichi*; Uesugi, Yoshihiko*; JT-60U Team
Nuclear Fusion, 49(6), p.065017_1 - 065017_7, 2009/06
Times Cited Count:38 Percentile:79.52(Physics, Fluids & Plasmas)Comparison between fluctuation characteristics at high-field-side (HFS) and low-field-side (LFS) scrape off layers (SOLs) has been made, for the first time, in the L mode plasma of the JT-60U tokamak using reciprocating Langumuir probes. Statistical analysis based on probability distribution function (PDF) was employed to describe intermittent (non-diffusion) transport in SOL plasma fluctuations. The positive bursty events appeared most frequently at LFS midplane associated with blobby plasma transport, then the PDF is strongly skewed positively, while the PDF in HFS SOL is close to Gaussian distribution. Conditional averaging analysis of the positive bursty events at LFS midplane indicates the intermittent feature with a rapid increase and a slow decay is similar to that of plasma blobs theoretically predicted. Statistical self-similarity was also investigated with Fourier power spectrum and statistics of waiting-time and duration-time of the fluctuation.