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Mukai, Yasunobu; Nakamura, Hironobu; Nakamichi, Hideo; Kurita, Tsutomu; Noguchi, Yoshihiko*; Tamura, Takayuki*; Ikegame, Ko*; Shimizu, Junji*
Proceedings of INMM 56th Annual Meeting (Internet), 9 Pages, 2015/07
The PIMS used at Rokkasho Reprocessing Plant can quantify plutonium amount in each process vessel located inside glovebox by means of neutron measurement. Since the PIMS is not used for the neutron coincidence counting, it is very important to maintain that those constants meet the actual process condition. PIMS was calibrated in 2006, and then JNFL has been started to measure the Pu amount directly in each glovebox for the purpose of facility NMA. However, it was found that PIMS counting was unexpectedly and continuously increased during long time of inter-campaign. In order to find out the main cause, JAEA and JNFL jointly conducted several investigations. In the investigations, correctness of system parameters and relevant constants, behavior of the neutron generation when MOX powder is stored in actual glovebox for a long time (to see O/M and moisture change) and the behavior focused on the relation between MOX powder and light element using inside glovebox (fluorine is included in the PTFE which is used in many gloveboxes as packing of instruments) were experimentally confirmed using MOX powder in PCDF. As a result, since the same behavior happened in the actual PIMS was confirmed in the testing environment in which MOX powder coexists with fluorine, it is concluded that the main potential cause of PIMS is the increasing of the probability of (
, 
) reactions by a contact between PTFE and MOX powder.
Kobayashi, Hidekazu; Amamoto, Ippei; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
Proceedings of 15th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM 2013) (CD-ROM), 6 Pages, 2013/09
no abstracts in English
as the dominant sludge constituent generated from the treatment of water used for cooling the stricken power reactorsAmamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
Proceedings of 15th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM 2013) (CD-ROM), 8 Pages, 2013/09
The great amount of water used for cooling the stricken power reactors at Fukushima Dai-ichi has resulted in accumulation of "remaining water". As the remaining water is subsequently contaminated by FPs, etc., it is necessary to decontaminate it in order to reduce the volume of liquid radioactive waste and to reuse it again for cooling the reactors. Various techniques are being applied to remove FP, etc. and to make stable waste forms. One of the methods using the iron phosphate glass as a medium is being developed to stabilize the strontium-bearing sludge whose main component is BaSO. From the results hitherto, the iron phosphate glass is regarded as a potential medium for the target sludge.
Mukai, Yasunobu; Nakamura, Hironobu; Yoshimoto, Katsunobu; Tamura, Takayuki*; Iwamoto, Tomonori*
Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-32-Kai Nenji Taikai Rombunshu (Internet), 9 Pages, 2011/11
JNFL and JAEA are collaboratively developing an advanced solution monitoring and measurement system (ASMS) that is direct Pu measurement NDA system in the solution tank containing plutonium nitrate solution for the improvement of current safeguards subjects to be solved, and for next generation safeguards instrument. The target measurement uncertainty of ASMS is set less than 6% that is equivalent to detection level of partial defect at interim inventory verification by NDA. The ASMS detector was designed based on MCNPX calculation, and then manufactured. As an actual test, the detector was set in a process tank at Plutonium Conversion Development Facility, the calibration tests (known-alpha) for quantitative measurement was conducted. As a result, the total measurement uncertainty for Pu mass is about 3.4% except for the low liquid height region that is satisfied the target value. In addition, the monitoring capability of ASMS was confirmed.
Nakamura, Hironobu; Mukai, Yasunobu; Yoshimoto, Katsunobu; Tamura, Takayuki*; Iwamoto, Tomonori*
Proceedings of INMM 52nd Annual Meeting (CD-ROM), 9 Pages, 2011/07
JNFL and JAEA are collaboratively developing an Advanced Solution Measurement and monitoring System (ASMS) that is direct Pu measurement NDA system in the large scale solution tank containing purified plutonium nitrate for the improvement of current safeguards subjects to be solved, and for next generation safeguards instrument (NGSI). In this report, we summarize the first step results of ASMS development regarding quantitative measurement methodology. In order to establish quantitative measurement, accurate MCNPX modeling and calculations are very important and necessary. After calibration exercise implementation, we successfully obtained calibration constants (slope), and the total measurement uncertainty was about 3% for 
Pu effective mass for 2 hours measurement except for the low level region. In addition, the image of safeguards by design and collaboration of SMMS are also presented.
Mukai, Yasunobu; Nakamura, Hironobu; Hosoma, Takashi; Yoshimoto, Katsunobu; Tamura, Takayuki*; Iwamoto, Tomonori*
Proceedings of INMM 51st Annual Meeting (CD-ROM), 9 Pages, 2010/07
JNFL and JAEA are collaboratively developing an advanced solution monitoring and measurement system (ASMS) for Rokkasho Reprocessing Plant (RRP). In this study, as a second trial, we designed and fabricated a new demonstration-type detector for ASMS, then installed it to another process tank in PCDF. Using two detectors, tests for process monitoring capability were performed for several operational conditions such as sampling, bubbling, circulation, solution transfer between two tanks, followed by studies in sensitivity of monitoring and studies in stability for the duration of storage. As a result, excellent performances and advantages of ASMS compared with conventional SMMS were confirmed. It is concluded that ASMS can provide very useful information of operation status and Pu amount shared between operator and inspector. It is sure that the combination of current SMMS and the ASMS is very powerful tool to improve transparency in the future safeguards design.
Nakamura, Hironobu; Takaya, Akikazu; Mukai, Yasunobu; Hosoma, Takashi; Yoshimoto, Katsunobu; Tamura, Takayuki*; Iwamoto, Tomonori*
Kaku Busshitsu Kanri Gakkai (INMM) Nihon Shibu Dai-30-Kai Nenji Taikai Rombunshu (CD-ROM), 9 Pages, 2009/11
JNFL and JAEA have collaboratively started to develop an ASMS for RRP since 2007. The purpose of the development is to establish direct plutonium mass measurement technique by NDA of high concentrated pure plutonium nitrate solution in a strategic process tank. If it is established, ASMS provides direct Pu mass measurement and monitoring capability, substitutes for sampling and destructive analysis at IIV, and extends process monitoring to safety purposes. The target of the measurement uncertainty is set less than 6% which is equivalent to the detection level of partial defect at IIV by NDA. The principle is similar to the one of NDA for MOX powder, but extended such as introducing variable alpha depends on solution properties. As a first trial, a simple prototype system was constructed and calibrated at PCDF (Plutonium Conversion Development Facility) using plutonium nitrate solution. Consequently, good consistency between MCNP (Monte Carlo Neutron and Photon Transport Code) calculation and measured singles/doubles count rate were obtained. As a feasibility study, it was necessary to find out subjects to be solved. We would like to present benefits of ASMS, review installation and detector setup and summarize preliminary calibration results.
Nakamura, Hironobu; Takaya, Akikazu; Mukai, Yasunobu; Hosoma, Takashi; Yoshimoto, Katsunobu; Tamura, Takayuki*; Iwamoto, Tomonori*
Proceedings of INMM 50th Annual Meeting (CD-ROM), 9 Pages, 2009/00
JNFL and JAEA have collaboratively started to develop an ASMS for RRP since 2007 as a trial base. The purpose of the development is to establish quantitative plutonium mass measurement technique directly by NDA of high concentrated pure plutonium nitrate solution in a process tank. If it is established, ASMS provides direct Pu mass measurement and monitoring capability, substitutes for sampling and analysis at IIV, and extends process monitoring to safety purposes. The target of the measurement uncertainty is set less than 6% (1 
) which is equivalent to the detection level of partial defect at IIV by NDA. The principle is similar to the one of NDA for MOX powder, but extended such as introducing variable alpha depends on solution properties. As a first trial, a simple prototype system was constructed and tested at Plutonium Conversion Development Facility of JAEA. Prior to the installation, MCNP calculations for entire cell and tank were performed. Two detectors with a gap were installed just center of the annular tank, then we carried out calibration using plutonium nitrate solution in the range up to 52 kgPu. Consequently, good consistency between calculation and measured singles/doubles count rate were obtained. As a feasibility study, it was necessary to find out subjects to be solved. We would like to present benefits of ASMS, review installation and detector setup and summarize preliminary calibration results.
Nakamura, Hironobu; Takaya, Akikazu; Mukai, Yasunobu; Hosoma, Takashi; Yoshimoto, Katsunobu; Tamura, Takayuki*; Iwamoto, Tomonori*
no journal, ,
JNFL and JAEA have collaboratively started to develop an ASMS for RRP since 2007. The purpose of the development is to establish direct plutonium mass measurement technique by NDA of high concentrated pure plutonium nitrate solution in a strategic process tank. If it is established, ASMS provides direct Pu mass measurement and monitoring capability, substitutes for sampling and destructive analysis at IIV, and extends process monitoring to safety purposes. The target of the measurement uncertainty is set less than 6%(1) which is equivalent to the detection level of partial defect at IIV by NDA. The principle is similar to the one of NDA for MOX powder, but extended such as introducing variable alpha depends on solution properties. As a first trial, a simple prototype system was constructed and tested at PCDF. Two detectors with a gap were installed just center of the annular tank, then we carried out calibration using plutonium nitrate solution (-52kgPu). Consequently, good consistency between MCNP calculation and measured singles/doubles count rate were obtained. As a feasibility study, it was necessary to find out subjects to be solved. We would like to present benefits of ASMS, review installation and detector setup and summarize preliminary calibration results.
Amamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Suzuki, Yoshikazu*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
no journal, ,
The great amount of water used for cooling the stricken reactors at Fukushima Dai-ichi Nuclear Power Plant following the earthquake and tsunami of 11 March 2011 had resulted in accumulation of "remaining water" in some buildings. From public announcements, it seems likely the decontamination process of La Hague reprocessing plant would be employed as one of the treatment processes for the remaining water contaminated by FPs such as Cs, Sr, etc.. Based on literature study, Cs would precipitate with ferrocyanide compound as well as Sr with BaSO by applying the above-mentioned process. In this study, BaSO as the simulated sludge was loaded into the iron phosphate glass (IPG) medium under different melting temperature. Based on the results, the performance of IPG containing BaO (decomposed from BaSO) improved with increase loading of BaO up to 48 mol% at lower melting temperature.
Amamoto, Ippei; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Nakamura, Hirotaka*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*; Kobayashi, Hidekazu
no journal, ,
no abstracts in English
Amamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Suzuki, Yoshikazu*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
no journal, ,
no abstracts in English
Kobayashi, Hidekazu; Amamoto, Ippei; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
no journal, ,
no abstracts in English
by the IPG mediumAmamoto, Ippei; Kobayashi, Hidekazu; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
no journal, ,
no abstracts in English
Kobayashi, Hidekazu; Amamoto, Ippei; Yokozawa, Takuma; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
no journal, ,
no abstracts in English
Amamoto, Ippei; Kobayashi, Hidekazu; Yamashita, Teruo; Nagai, Takayuki; Kitamura, Naoto*; Takebe, Hiromichi*; Mitamura, Naoki*; Tsuzuki, Tatsuya*; Fukayama, Daigen*; Nagano, Yuichi*; et al.
no journal, ,
no abstracts in English
Kobayashi, Hidekazu; Nagai, Takayuki; Okamoto, Yoshihiro; Sasage, Kenichi; Amamoto, Ippei; Takebe, Hiromichi*; Nakamura, Hiroki*; Mitamura, Naoki*; Tsuzuki, Tatsuya*
no journal, ,
no abstracts in English