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Journal Articles

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

 Times Cited Count:2 Percentile:14.88(Chemistry, Multidisciplinary)

The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 $$^circ$$C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$. From the obtained experimental results, thermochemical data for DbOCl$$_3$$ were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:43 Percentile:96.93(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:259 Percentile:99.73(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Progress of JT-60SA Project; EU-JA joint efforts for assembly and fabrication of superconducting tokamak facilities and its research planning

Shirai, Hiroshi; Barabaschi, P.*; Kamada, Yutaka; JT-60SA Team

Fusion Engineering and Design, 109-111(Part B), p.1701 - 1708, 2016/11

 Times Cited Count:21 Percentile:88.83(Nuclear Science & Technology)

The JT-60SA Project has shown steady progress toward the first plasma in 2019. JT-60SA is a superconducting tokamak designed to operate in the break-even conditions for a long pulse duration with a maximum plasma current of 5.5 MA. Design and fabrication of JT-60SA components shared by EU and Japan started in 2007. Assembly in the torus hall started in January 2013, and welding work of the vacuum vessel sectors is currently on going on the cryostat base. Other components such as TF coils, PF coils, power supplies, cryogenic system, cryostat vessel, thermal shields and so forth were or are being delivered to Naka site for installation, assembly and commissioning. This paper gives technical progress on fabrication, installation and assembly of tokamak components and ancillary systems, as well as progress of JT-60SA Research Plan being developed jointly by EU and Japanese fusion communities.

Journal Articles

Present status of manufacturing and R&Ds for the JT-60SA tokamak

Higashijima, Satoru; Kamada, Yutaka; Barabaschi, P.*; Shirai, Hiroshi; JT-60SA Team

Fusion Science and Technology, 68(2), p.259 - 266, 2015/09

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Deep-sea record of impact apparently unrelated to mass extinction in the Late Triassic

Onoue, Tetsuji*; Sato, Honami*; Nakamura, Tomoki*; Noguchi, Takaaki*; Hidaka, Yoshihiro*; Shirai, Naoki*; Ebihara, Mitsuru*; Osawa, Takahito; Hatsukawa, Yuichi; Toh, Yosuke; et al.

Proceedings of the National Academy of Sciences of the United States of America, 109(47), p.19134 - 19139, 2012/11

 Times Cited Count:40 Percentile:72.81(Multidisciplinary Sciences)

The 34 million year (My) interval of the Late Triassic is marked by the formation of several large impact structures on Earth. As with the Chicxulub impact event at the Cretaceous/Paleogene boudary, the Late Triassic impact events have been considered a factor in biotic extinction events in the Late Triassic (e.g., the Triassic/Jurassic boundary). However, the causal link between these impact events and a mass extinction event in the Late Triassic remains controversial because of a lack of stratigraphic records of their ejecta deposits. Here we report evidence for an impact event (platinum group elements anomaly, nickel-rich magnetite and microspherules) deposited within a Paleo-Pacific basin in the middle Norian (Upper Triassic) deep-sea sediment in Japan. This includes anomalously high abundances of iridium, up to 41.5 parts per billion (ppb), in the ejecta deposit, which suggests that the iridium anomaly may be found on a global scale. The middle Norian age of the ejecta deposit suggests that the impact event that produced the 100-km-wide Manicouagan crater in Canada8 is most likely related to its deposition. Our analysis of siliceous microfossils shows no evidence of a mass extinction event across the impact event horizon, and no contemporaneous faunal turnover is seen in other marine fossils. However, such an event has been reported among terrestrial tetrapods and floras in North America. We therefore hypothesize that the Manicouagan impact caused the catastrophic collapse of terrestrial ecosystems near the impact site, but not within the marine realm.

Journal Articles

Irradiation history of Itokawa regolith material deduced from noble gases in the Hayabusa samples

Nagao, Keisuke*; Okazaki, Ryuji*; Nakamura, Tomoki*; Miura, Yayoi*; Osawa, Takahito; Bajo, Kenichi*; Matsuda, Shintaro*; Ebihara, Mitsuru*; Ireland, T.*; Kitajima, Fumio*; et al.

Science, 333(6046), p.1128 - 1131, 2011/08

 Times Cited Count:130 Percentile:95.22(Multidisciplinary Sciences)

A steroid surface materials record regolith processes and a history of cosmic-ray irradiation. Noble gas isotopes in three rocky grains from Itokawa have been determined. High concentrations of solar He, Ne, and Ar, as high as those in lunar soils, are released at variable temperatures from each sample. The isotopic compositions are essentially identical to those of solar wind but distinguishable in He relative abundance. These noble gas characteristics can be explained by repeated implantation and preferential loss of solar He by removal of weathered He-rich rim on the grain surface through friction among regolith grains on Itokawa. Residence time of regolith materials on Itokawa is alculated to be shorter than 10 Myr, suggesting that regolith materials of small asteroids would escape easily to space.

Journal Articles

Measured and simulated transport of 1.9 MeV laser-accelerated proton bunches through an integrated test beam line at 1 Hz

Nishiuchi, Mamiko; Sakaki, Hironao; Hori, Toshihiko; Bolton, P.; Ogura, Koichi; Sagisaka, Akito; Yogo, Akifumi; Mori, Michiaki; Orimo, Satoshi; Pirozhkov, A. S.; et al.

Physical Review Special Topics; Accelerators and Beams, 13(7), p.071304_1 - 071304_7, 2010/07

 Times Cited Count:25 Percentile:79.43(Physics, Nuclear)

A laser-driven repetition-rated 1.9 MeV proton beam line composed of permanent quadrupole magnets (PMQs), a radio frequency (rf) phase rotation cavity, and a tunable monochromator is developed to evaluate and to test the simulation of laser-accelerated proton beam transport through an integrated system for the first time. In addition, the proton spectral modulation and focusing behavior of the rf phase rotationcavity device is monitored with input from a PMQ triplet. In the 1.9 MeV region we observe very weakproton defocusing by the phase rotation cavity. The final transmitted bunch duration and transverse profile are well predicted by the PARMILA particle transport code. The transmitted proton beam duration of 6 ns corresponds to an energy spread near 5% for which the transport efficiency is simulated to be 10%. The predictive capability of PARMILA suggests that it can be useful in the design of future higher energy transport beam lines as part of an integrated laser-driven ion accelerator system.

Journal Articles

C-axis critical current of a PrFeAsO$$_{0.7}$$ single crystal

Kashiwaya, Hiromi*; Shirai, Kazumi*; Matsumoto, Tetsuro*; Shibata, Hajime*; Kambara, Hiroshi*; Ishikado, Motoyuki; Eisaki, Hiroshi*; Iyo, Akira*; Shamoto, Shinichi; Kurosawa, Itaru*; et al.

Applied Physics Letters, 96(20), p.202504_1 - 202504_3, 2010/05

 Times Cited Count:28 Percentile:71.47(Physics, Applied)

The ${it c}$-axis transport properties of a high-pressure synthesized PrFeAsO$$_{0.7}$$ single crystal are studied using s-shaped junctions. Resistivity anisotropy of about 120 detected at 50 K shows the presence of strong anisotropy in the electronic states. The obtained critical current density for the ${it c}$-axis of 2.9 $$times$$ 10$$^{5}$$ A/cm$$^{2}$$ is two orders of magnitude larger than that in Bi$$_{2}$$Sr$$_{1.6}$$La$$_{0.4}$$CuO$$_{6+delta}$$. The appearance of a hysteresis in the current-voltage curve below ${it T}$ $$_{c}$$ is the manifestation of the intrinsic Josephson effect similar to that in cuprate superconductors. The suppression of the critical current-normal resistance (${it I}$ $$_{c}$$ ${it R}$ $$_{n}$$) product is explained by an inspecular transport in ${it s}$ $$_{pm}$$ -wave pair potential.

Journal Articles

Laser-driven proton accelerator for medical application

Nishiuchi, Mamiko; Sakaki, Hironao; Hori, Toshihiko; Bolton, P.; Ogura, Koichi; Sagisaka, Akito; Yogo, Akifumi; Mori, Michiaki; Orimo, Satoshi; Pirozhkov, A. S.; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.88 - 90, 2010/05

The concept of a compact ion particle accelerator has become attractive in view of recent progress in laser-driven ion acceleration. We report here the recent progress in the laser-driven proton beam transport at the Photo Medical Research Center (PMRC) at JAEA, which is established to address the challenge of laser-driven ion accelerator development for ion beam cancer therapy.

Journal Articles

Ion acceleration using temporally-controlled high-intensity laser pulses

Yogo, Akifumi; Daido, Hiroyuki; Mori, Michiaki; Kiriyama, Hiromitsu; Bulanov, S. V.; Bolton, P. R.; Esirkepov, T. Z.; Ogura, Koichi; Sagisaka, Akito; Orimo, Satoshi; et al.

Reza Kenkyu, 37(6), p.449 - 454, 2009/06

The acceleration of protons driven by a high-intensity laser is comprehensively investigated via control of the target density by using ASE just before the time of the main-laser interaction. Two cases were investigated for which the ASE intensity differed by three orders of magnitude: In the low contrast case the beam centre for higher energy protons is shifted closer to the laser-propagation direction of 45$$^{circ}$$, while the center of lower-energy beam remains near the target normal direction. Particle-in-cell simulations reveal that the characteristic proton acceleration is due to the quasistatic magnetic field on the target rear side with the magnetic pressure sustaining a charge separation electrostatic field.

Journal Articles

Interlaboratory comparison of positron annihilation lifetime measurements

Ito, Kenji*; Oka, Toshitaka*; Kobayashi, Yoshinori*; Shirai, Yasuharu*; Wada, Kenichiro*; Matsumoto, Masataka*; Fujinami, Masanori*; Hirade, Tetsuya; Honda, Yoshihide*; Hosomi, Hiroyuki*; et al.

Materials Science Forum, 607, p.248 - 250, 2009/00

So far no standard procedure for the positron annihilation lifetime (PAL) technique has been established. A lack of the standards has led to difficulty in ensuring the equivalency and reliability of data from different laboratories. As a first, we conducted an interlaboratory comparison of PAL measurements for metal, polymer and silica glass with agreed procedures for data recording and analysis. The PAL data recorded at different laboratories were analyzed with a single lifetime component for the metal sample and with three components for the others, respectively. Based on the results of the reported positron and ortho-positronium lifetimes, the possible sources of the uncertainties in the PAL measurements are discussed. To reduce the effect of scattered $$gamma$$ rays, a lead shield was placed between the detectors. The uncertainty was significantly decreased, signifying that placing lead shields between the detectors effectively reduced the false signals due to the scattered $$gamma$$ rays.

Journal Articles

New method to measure the rise time of a fast pulse slicer for laser ion acceleration research

Mori, Michiaki; Yogo, Akifumi; Kiriyama, Hiromitsu; Nishiuchi, Mamiko; Ogura, Koichi; Orimo, Satoshi; Ma, J.*; Sagisaka, Akito; Kanazawa, Shuhei; Kondo, Shuji; et al.

IEEE Transactions on Plasma Science, 36(4), p.1872 - 1877, 2008/08

 Times Cited Count:7 Percentile:28.47(Physics, Fluids & Plasmas)

A dependence of cut-off proton kinetic energy on laser prepulse duration has been observed. ASE pedestal duration is controlled by a fast electro-optic pulse slicer where the risetime is estimated to be 130 ps. We demonstrate a new correlated spectral technique for determining this risetime using a stretched, frequency chirped pulse.

Journal Articles

Interlaboratory comparison of positron annihilation lifetime measurements for synthetic fused silica and polycarbonate

Ito, Kenji*; Oka, Toshitaka*; Kobayashi, Yoshinori*; Shirai, Yasuharu*; Wada, Kenichiro*; Matsumoto, Masataka*; Fujinami, Masanori*; Hirade, Tetsuya; Honda, Yoshihide*; Hosomi, Hiroyuki*; et al.

Journal of Applied Physics, 104(2), p.026102_1 - 026102_3, 2008/07

 Times Cited Count:48 Percentile:83.5(Physics, Applied)

Interlaboratory comparison of positron annihilation lifetime measurements using synthetic fused silica and polycarbonate was conducted with the participation of 12 laboratories. By regulating procedures for the measurement and data analysis the uncertainties of the positron lifetimes obtained at different laboratories were significantly reduced in comparison with those reported in the past.

Journal Articles

Simultaneous proton and X-ray imaging with femtosecond intense laser driven plasma source

Orimo, Satoshi; Nishiuchi, Mamiko; Daido, Hiroyuki; Yogo, Akifumi; Ogura, Koichi; Sagisaka, Akito; Li, Z.*; Pirozhkov, A. S.; Mori, Michiaki; Kiriyama, Hiromitsu; et al.

Japanese Journal of Applied Physics, Part 1, 46(9A), p.5853 - 5858, 2007/09

 Times Cited Count:17 Percentile:54.99(Physics, Applied)

A laser-driven proton beam with a maximum energy of a few MeV is stably obtained using an ultra-short and high-intensity Titanium Sapphire laser. At the same time, keV X-ray is also generated at almost the same place where protons are emitted. Here, we show the successful demonstration of simultaneous proton and X-ray projection images of a test sample placed close to the source with a resolution of $$sim$$10$$mu$$m, which is determined from the source sizes. Although the experimental configuration is very simple, the simultaneity is better than a few hundreds of ps. A CR-39 track detector and imaging plate, which are placed as close as possible to the CR-39, are used as detectors of protons and X-ray. The technique is applicable to the precise observation of microstructures.

Journal Articles

Characterization of an intense laser-produced preformed plasma for proton generation

Sagisaka, Akito; Daido, Hiroyuki; Ogura, Koichi; Orimo, Satoshi; Hayashi, Yukio; Mori, Michiaki; Nishiuchi, Mamiko; Yogo, Akifumi; Kado, Masataka; Fukumi, Atsushi*; et al.

Journal of the Korean Physical Society, 51(1), p.442 - 446, 2007/07

 Times Cited Count:1 Percentile:10.86(Physics, Multidisciplinary)

The recent progress of the laser driven accelerators which include high power laser driven electrons and ions are reviewed. The studies at JAEA Kansai are mainly described. Based on the recent progres, the various aspects of the applications are also reviewed.

Journal Articles

Electrochemical evaluation of the distribution of a metal ion at the aqueous$$|$$organic solution interface in chelate extraction

Uehara, Akihiro*; Kasuno, Megumi*; Okugaki, Tomohiko*; Kitatsuji, Yoshihiro; Shirai, Osamu*; Yoshida, Zenko; Kihara, Sorin*

Journal of Electroanalytical Chemistry, 604(2), p.115 - 124, 2007/06

The distribution ratio of a metal ion between an aqueous solution and an organic solution in solvent extraction with a chelating agent was evaluated by using physicochemical constants determined electrochemically such as standard Gibbs energies for transfers of the ions, the overall complex formation constants and the acid dissociation constants of the chelating agent. The distribution ratio thus evaluated agreed well with those determined by the distribution experiment.

Journal Articles

Laser prepulse dependency of proton-energy distributions in ultraintense laser-foil interactions with an online time-of-flight technique

Yogo, Akifumi; Daido, Hiroyuki; Fukumi, Atsushi*; Li, Z.*; Ogura, Koichi; Sagisaka, Akito; Pirozhkov, A. S.; Nakamura, Shu*; Iwashita, Yoshihisa*; Shirai, Toshiyuki*; et al.

Physics of Plasmas, 14(4), p.043104_1 - 043104_6, 2007/04

 Times Cited Count:63 Percentile:88.17(Physics, Fluids & Plasmas)

Fast protons are observed by a newly-developed $textit{online}$ time-of-flight spectrometer, which provides $textit{shot-to-shot}$ proton-energy distributions immediately after the irradiation of a laser pulse having an intensity of $$sim 10^{18}$$ W/cm$$^2$$ onto a 5-$$mu$$m-thick copper foil. The maximum proton energy is found to increase when the intensity of a fs-prepulse arriving 9 ns before the main pulse increases from 10$$^{14}$$ to 10$$^{15}$$ W/cm$$^2$$. Interferometric measurement indicates that the preformed-plasma expansion at the front surface is smaller than 15 $$mu$$m, which corresponds to the spatial resolution of the diagnostics. This sharp gradient of the plasma makes a beneficial effect on increasing the absorption efficiency of the main-pulse energy, resulting in the increase in the proton energy. This is supported by the result that the X-ray intensity from the laser plasma clearly increases with the prepulse intensity.

Journal Articles

ITB-events and their triggers in T-10 and JT-60U

Neudatchin, S. V.*; Takizuka, Tomonori; Sakamoto, Yoshiteru; Hayashi, Nobuhiko; Isayama, Akihiko; Kislov, A. Ya.*; Krylov, S. V.*; Pavlov, Yu. D.*; Shirai, Hiroshi; Borshegovskii, A. A.*

Proceedings of 21st IAEA Fusion Energy Conference (FEC 2006) (CD-ROM), 8 Pages, 2007/03

Non-local transport bifurcations inside and around ITB were found in various JT-60U reverse shear (RS) and normal shear (NrS) plasmas and called ITB-events. The abrupt reduction of transport in the central part of the plasma column often interrupts a slow diffusive inward cold pulse propagation (CPP) in T-10. CPP is created by a cut-off of the off-axis ECRH. This phenomenon may referred to ITB-events as well. In many cases these events occur, when the central safety factor q decreases below unity. In JT-60U low-power heated RS plasmas, ITB-events are observed at the crossing of minimum of q equal to 3.5, 3, 2.5 values. Internal MHD n=1 activity has been reported earlier as ITB-events trigger in JT-60U. The present paper shows that an ITB-event is triggered by a series of small internal disruptions probably associated with q=2.5 surface in RS plasmas. In a high-poloidal-beta NrS shot, an ITB-event occurs in correlation with the start of ELMs series. The total heat flux reduces abruptly in the zone 0.3$$<$$r/a$$<$$0.7. This new finding of this ITB event suggests the possibility to control the ITB formation by inducing the ELM-like MHD activity.

Journal Articles

High quality laser-produced proton beam generation by phase rotation

Noda, Akira*; Nakamura, Shu*; Iwashita, Yoshihisa*; Shirai, Toshiyuki*; Tongu, Hiromu*; Soda, Hikaru*; Daido, Hiroyuki; Mori, Michiaki; Kado, Masataka; Sagisaka, Akito; et al.

International Journal of Modern Physics B, 21(3&4), p.319 - 330, 2007/02

Laser ion production has been studied for downsizing of the accelerator dedicated for cancer therapy. For optimization of various parameters such as pre-pulse condition, target position, laser spot size on target, laser pulse width and so on, time of flight (TOF) measurement utilizing the detected signal by a plastic scintillation counter played an essential role for real time measurement. Protons up to 900 keV and 600 keV are produced from the thin foil targets of Ti 3 micron and 5 micron in thickness, respectively. Modification of the energy distribution of the laser-produced ions with Maxwell distribution by utilizing an RF electric field synchronized to the pulse laser, which is the rotation of the ion beam in the longitudinal phase space (phase rotation), has been demonstrated for the first time.

205 (Records 1-20 displayed on this page)