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Journal Articles

Measurement of radiolytic yield of nitric acid in air

Kanda, Yukio*; Oki, Yuichi*; Yokoyama, Sumi; Sato, Kaoru; Noguchi, Hiroshi; Tanaka, Susumu*; Iida, Takao*

Radiation Physics and Chemistry, 74(5), p.338 - 340, 2005/12

 Times Cited Count:5 Percentile:35.8(Chemistry, Physical)

The operation of high-energy accelerators leads to the production of radiolytic noxious gases, such as ozone and nitrogen compounds in the air of the beam-line tunnels. Among nitrogen compounds, nitric acid is a principal radiolytic compound produced in large quantities. In the high-intensity proton accelerator, such as J-PARC, a very strong radiation environment leads to an abundant production of nitric acid. A quantitative assessment of the damage due to corrosion with nitric acid is essential for machine maintenance and information concerning the formation of nitric acid is a requisite for that. In this work, the G-value for nitric acid production was measured by irradiating atmospheric air with 48MeV-protons. The G-value was obtained to be 1.46$$pm$$0.12. The G-value for nitric acid production obtained in this experiment was larger than the estimated value, but very close to the value of 1.5 given by irradiating the air with Co-60-$$gamma$$rays.

Journal Articles

Characterization of radionuclides formed by high-energy neutron irradiation

Yokoyama, Sumi; Sato, Kaoru; Noguchi, Hiroshi; Tanaka, Susumu; Iida, Takao*; Furuichi, Shinya*; Kanda, Yukio*; Oki, Yuichi*; Kaneto, Taihei*

Radiation Protection Dosimetry, 116(1-4), p.401 - 405, 2005/12

 Times Cited Count:1 Percentile:10.45(Environmental Sciences)

The physicochemical property of radionuclides suspended in the air is an important parameter to evaluate internal doses due to the inhalation of the airborne radionuclides and to develop the air monitoring system in high-energy proton accelerator facilities. This study focuses on the property of radioactive airborne chlorine ($$^{38}$$Cl and $$^{39}$$Cl) and sulfur ($$^{38}$$S) formed from Ar gas by irradiation with high-energy neutrons. As a result of the irradiation to a mixture of Ar gas and dry air, $$^{38}$$Cl and $$^{39}$$Cl existed as non-acidic gas and $$^{38}$$S was present as acidic gas. Further, it was found that in the high-energy neutron irradiation to aerosol containing-Ar gas, the higher the amount of radioactive aerosols becomes, the lower that of radioactive acidic gas becomes.

Journal Articles

Study of particle size distribution and formation mechanism of radioactive aerosols generated in high-energy neutron fields

Endo, Akira; Sato, Kaoru; Noguchi, Hiroshi; Tanaka, Susumu; Iida, Takao*; Furuichi, Shinya*; Kanda, Yukio*; Oki, Yuichi*

Journal of Radioanalytical and Nuclear Chemistry, 256(2), p.231 - 237, 2003/05

 Times Cited Count:7 Percentile:45.83(Chemistry, Analytical)

Size distributions of $$^{38}$$Cl, $$^{39}$$Cl, $$^{82}$$Br and $$^{84}$$Br aerosols generated by irradiations of argon and krypton gases containing di-octyl phthalate (DOP) aerosols with 45MeV and 65MeV quasi-monoenergetic neutrons were measured to study the formation mechanism of radioactive particles in high energy radiation fields. Effects of the size distribution of the radioactive aerosols on the size of added DOP aerosols, the energy of irradiation neutrons and the kinds of nuclides were studied. The observed size distributions of the radioactive particles were explained by attachment of the radioactive atoms generated by the neutron-induced reactions to the DOP aerosols.

Journal Articles

Particle size analysis of radioactive aerosols formed by irradiation of argon using 65MeV quasi-monoenergetic neutrons

Endo, Akira; Noguchi, Hiroshi; Tanaka, Susumu; Kanda, Yukio*; Oki, Yuichi*; Iida, Takao*; Sato, Kaoru; Tsuda, Shuichi

Applied Radiation and Isotopes, 56(4), p.615 - 620, 2002/04

 Times Cited Count:3 Percentile:23.41(Chemistry, Inorganic & Nuclear)

Formation mechanism and size distribution of radioactive aerosol particles generated in a high-energy neutron field were studied in order to evaluate a particle size parameter for internal dose evaluation in high-energy accelerator facilities. Argon gas containing DOP aerosols was irradiated by a 65MeV quasi-monoenergetic neutron beam of TIARA. The number size distribution of the DOP aerosols and the activity-weighted size distribution of $$^{38}$$Cl and $$^{39}$$Cl aerosols, formed from the (n, 2np) and (n, np) reactions of $$^{40}$$Ar, were measured using an electrical low-pressure impactor. The activity-weighted size distribution of the radioactive aerosols was well explained by the simple attachment model of the radioactive atoms to the DOP aerosols.

Journal Articles

Airborne gaseous $$^{13}$$N species and noxious gases produced at the 12GeV proton synchrotron

Kanda, Yukio*; Oki, Yuichi*; Endo, Akira; Numajiri, Masaharu*; Kondo, Kenjiro*

Journal of Radioanalytical and Nuclear Chemistry, 247(1), p.25 - 31, 2001/01

 Times Cited Count:9 Percentile:56.08(Chemistry, Analytical)

no abstracts in English

Journal Articles

Evaluation of internal and external doses from $$^{11}$$C produced in the air in high energy proton accelerator tunnels

Endo, Akira; Oki, Yuichi*; Kanda, Yukio*; Oishi, Tetsuya; Kondo, Kenjiro*

Radiation Protection Dosimetry, 93(3), p.223 - 230, 2001/00

 Times Cited Count:6 Percentile:44.09(Environmental Sciences)

no abstracts in English

Journal Articles

Characterization of $$^{11}$$C, $$^{13}$$N and $$^{15}$$O produced in air through nuclear spallation reactions by high energy protons

Endo, Akira; Oki, Yuichi*; Kanda, Yukio*; Kondo, Kenjiro*

Proceedings of 10th International Congress of the International Radiation Protection Association (IRPA-10) (CD-ROM), 8 Pages, 2000/05

no abstracts in English

Journal Articles

Radiation protection in high-intensity and high-energy accelerator facilities; Mainly on activation and protection of internal exposure due to induced radionuclides

Endo, Akira; *; *; Kanda, Yukio*; *

Nihon Genshiryoku Gakkai-Shi, 39(3), p.210 - 218, 1997/00

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

no abstracts in English

Oral presentation

Physicochemical properties of airborne radioactive chlorine and non-radioactive aerosol formed in high-energy proton accelerator facilities

Yokoyama, Sumi; Sato, Kaoru; Manabe, Kentaro; Endo, Akira; Noguchi, Hiroshi; Kaneko, Hirohisa; Oki, Yuichi*; Osada, Naoyuki*; Kanda, Yukio*; Iida, Takao*; et al.

no journal, , 

no abstracts in English

Oral presentation

Formation and the properties of aerosol by proton irradiation to air

Osada, Naoyuki*; Oki, Yuichi*; Kanda, Yukio*; Yokoyama, Sumi; Sato, Kaoru; Manabe, Kentaro; Noguchi, Hiroshi; Endo, Akira; Tanaka, Susumu*; Kaneko, Hirohisa; et al.

no journal, , 

no abstracts in English

10 (Records 1-10 displayed on this page)
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