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Kaneda-Nakashima, Kazuko*; Shirakami, Yoshifumi*; Kadonaga, Yuichiro*; Watabe, Tadashi*; Oe, Kazuhiro*; Yin, X.*; Haba, Hiromitsu*; Shirasaki, Kenji*; Kikunaga, Hidetoshi*; Tsukada, Kazuaki; et al.
International Journal of Molecular Sciences (Internet), 25(2), p.933_1 - 933_14, 2024/01
Times Cited Count：1 Percentile：0.01(Biochemistry & Molecular Biology)Yakushev, A.*; Lens, L.*; D
llmann, Ch. E.*; Khuyagbaatar, J.*; J
ger, E.*; Krier, J.*; Runke, J.*; Albers, H. M.*; Asai, Masato; Block, M.*; et al.
Frontiers in Chemistry (Internet), 10, p.976635_1 - 976635_11, 2022/08
Times Cited Count：9 Percentile：79.28(Chemistry, Multidisciplinary)Flerovium (Fl, element 114) is the heaviest element chemically studied so far. The first chemical experiment on Fl suggested that Fl is a noble-gas-like element, while the second studies suggested that Fl has a volatile-metal-like character. To obtain more reliable conclusion, we performed further experimental studies on Fl adsorption behavior on Si oxide and gold surfaces. The present results suggest that Fl is highly volatile and less reactive than the volatile metal, Hg, but has higher reactivity than the noble gas, Rn.
At]NaAt and [
I]NaI in an NIS-expressing thyroid cancer mouse modelWatabe, Tadashi*; Liu, Y.*; Kaneda, Kazuko*; Sato, Tatsuhiko; Shirakami, Yoshifumi*; Oe, Kazuhiro*; Toyoshima, Atsushi*; Shimosegawa, Eku*; Wang, Y.*; Haba, Hiromitsu*; et al.
International Journal of Molecular Sciences (Internet), 23(16), p.9434_1 - 9434_11, 2022/08
Times Cited Count：7 Percentile：78.48(Biochemistry & Molecular Biology)In this study, we compare the therapeutic effect between [At]NaAt and [I]NaI. In vitro analysis of double-stranded DNA break (DSB) and colony formation assay were performed using K1-NIS cells. [At]NaAt induced higher numbers of DSBs and had a reduced colony formation than [I]NaI. In K1-NIS mice, dose-dependent therapeutic effects were observed in both [At]NaAt and [I]NaI. The superior therapeutic effect of [At]NaAt suggests the promising clinical applicability of targeted alpha therapy using [At]NaAt in patients with differentiated thyroid cancer refractory to standard [I]NaI treatment.
Bh in the 
Cm(
Na,5
)Bh reaction and its decay propertiesHaba, Hiromitsu*; Fan, F.*; Kaji, Daiya*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Komori, Yukiko*; Kondo, Narumi*; Kudo, Hisaaki*; Morimoto, Koji*; Morita, Kosuke*; et al.
Physical Review C, 102(2), p.024625_1 - 024625_12, 2020/08
Times Cited Count：6 Percentile：59.56(Physics, Nuclear)Tanaka, Taiki*; Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Boll, R. A.*; Brewer, N. T.*; Van Cleve, S.*; Dean, D. J.*; Ishizawa, Satoshi*; et al.
Physical Review Letters, 124(5), p.052502_1 - 052502_6, 2020/02
Times Cited Count：19 Percentile：81.08(Physics, Multidisciplinary)
Th nuclear clock isomer determined by absolute 
-ray energy differenceYamaguchi, Atsushi*; Muramatsu, Haruka*; Hayashi, Tasuku*; Yuasa, Naoki*; Nakamura, Keisuke; Takimoto, Misaki; Haba, Hiromitsu*; Konashi, Kenji*; Watanabe, Makoto*; Kikunaga, Hidetoshi*; et al.
Physical Review Letters, 123(22), p.222501_1 - 222501_6, 2019/11
Times Cited Count：36 Percentile：89.11(Physics, Multidisciplinary)
acidic solutionsYokoyama, Akihiko*; Kitayama, Yuta*; Fukuda, Yoshiki*; Kikunaga, Hidetoshi*; Murakami, Masashi*; Komori, Yukiko*; Yano, Shinya*; Haba, Hiromitsu*; Tsukada, Kazuaki; Toyoshima, Atsushi*
Radiochimica Acta, 107(1), p.27 - 32, 2019/01
Times Cited Count：1 Percentile：11.15(Chemistry, Inorganic & Nuclear)
and Au surfaces in preparation for chemical investigations on Cn, Nh, and Fl at TASCALens, L.*; Yakushev, A.*; Dllmann, Ch. E.*; Asai, Masato; Ballof, J.*; Block, M.*; David, H. M.*; Despotopulos, J.*; Di Nitto, A.*; Eberhardt, K.*; et al.
Radiochimica Acta, 106(12), p.949 - 962, 2018/12
Times Cited Count：8 Percentile：62.99(Chemistry, Inorganic & Nuclear)Online gas-solid adsorption studies with single atom quantities of Hg, Tl, and Pb on SiO and Au surfaces were carried out using short-lived radioisotopes with half-lives in the range of 4-49 s. This is a model study to measure adsorption enthalpies of superheavy elements Cn, Nh, and Fl. The short-lived isotopes were produced and separated by the gas-filled recoil separator TASCA at GSI. The products were stopped in He gas, and flushed into gas chromatography columns made of Si detectors whose surfaces were covered by SiO or Au. The short-lived Tl and Pb were successfully measured by the Si detectors with the SiO surface at room temperature. On the other hand, the Hg did not adsorb on the SiO surface, but adsorbed on the Au surface. The results demonstrated that the adsorption properties of short-lived Hg, Tl, and Pb could be studied with this setup, and that this method is applicable to the experiment for Cn, Nh, and Fl.
SO
and HF/HCl solutions into toluene with Aliquat336; Sulfate and fluoride complex formation of Mo and W towards chemical studies of seaborgium (Sg)Toyoshima, Atsushi; Mitsukai, Akina; Tsukada, Kazuaki; Oe, Kazuhiro*; Haba, Hiromitsu*; Komori, Yukiko*; Murakami, Masashi; Kaneya, Yusuke*; Sato, Daisuke*; Asai, Masato; et al.
Journal of Radioanalytical and Nuclear Chemistry, 317(1), p.421 - 430, 2018/07
Times Cited Count：2 Percentile：20.93(Chemistry, Analytical)We have studied extraction behavior of group-6 elements Mo and W to search for suitable conditions for an on-line extraction experiment of their heavier homolog, seaborgium (Sg). Batch-wise extraction of carrier-free radiotracers 
Mo and 
W were carried out from 0.10 - 8.6 M HSO and 1.0
10
- 5.0 M HF/1.0 M HCl into toluene with a quaternary ammonium compound, Aliquat336. Anionic sulfate complexes of Mo and W with charge - 2 were extracted with Aliquat336 from HSO solutions with concentrations of [HSO] 
2 M. In HF/1.0 M HCl, oxyfluoro complexes of Mo and W with charge - 1 were interpreted to be formed and extracted with Aliquat336. From these results, favorable conditions for the extraction of Sg are discussed.
= 100 with a multireflection time-of-flight mass spectrographIto, Yuta*; Schury, P.*; Wada, Michiharu*; Arai, Fumiya*; Haba, Hiromitsu*; Hirayama, Yoshikazu*; Ishizawa, Satoshi*; Kaji, Daiya*; Kimura, Sota*; Koura, Hiroyuki; et al.
Physical Review Letters, 120(15), p.152501_1 - 152501_6, 2018/04
Times Cited Count：60 Percentile：93.36(Physics, Multidisciplinary)Masses of 
Es, 
Fm and the transfermium nuclei 
Md, and 
No, produced by hot- and cold-fusion reactions, in the vicinity of the deformed 
neutron shell closure, have been directly measured using a multi-reflection time-of-flight mass spectrograph. The masses of Es and 
Md were measured for the first time. Using the masses of 
Md as anchor points for 
decay chains, the masses of heavier nuclei, up to 
Bh and Mt, were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter 
derived from three isotopic masses was updated with the new masses and corroborate the existence of the deformed neutron shell closure for Md and Lr.
Sakurai, Hiroshi*; Shinohara, Atsushi*; Koura, Hiroyuki; Kamigaito, Osamu*; Morimoto, Koji*; Haba, Hiromitsu*; Enyo, Hideto*
Isotope News, (特別号2), p.2 - 14, 2018/01
no abstracts in English
Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.
Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01
Times Cited Count：18 Percentile：74.47(Physics, Multidisciplinary)Excitation functions of quasielastic scattering cross sections for the 
Ca + 
Pb, 
Ti + Pb, and Ca + Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the Ca + Pb and Ti + Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the Ca + Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.
-delayed fission of 
AmWilson, G. L.*; Takeyama, Mirei*; Andreyev, A. N.; Andel, B.*; Antalic, S.*; Catford, W. N.*; Ghys, L.*; Haba, Hiromitsu*; He
berger, F. P.*; Huang, M.*; et al.
Physical Review C, 96(4), p.044315_1 - 044315_7, 2017/10
Times Cited Count：6 Percentile：47.01(Physics, Nuclear)Schury, P.*; Wada, Michiharu*; Ito, Yuta*; Kaji, Daiya*; Haba, Hiromitsu*; Hirayama, Yoshikazu*; Kimura, Sota*; Koura, Hiroyuki; MacCormick, M.*; Miyatake, Hiroari*; et al.
Nuclear Instruments and Methods in Physics Research B, 407, p.160 - 165, 2017/06
Times Cited Count：14 Percentile：78.05(Instruments & Instrumentation)Various isotopes of Ac, Ra, Fr, and Rn were produced by fusion-evaporation reactions using a Ca beam. The energetic ions were stopped in and extracted from a helium gas cell. The extracted ions were identified using a multi-reflection time-of-fight mass spectrograph. In all cases, it was observed that the predominant charge state for the extracted ions, including the alkali Fr, was 2+.
Ca + Cm 
Lv
at RIKEN-GARISKaji, Daiya*; Morita, Kosuke*; Morimoto, Koji*; Haba, Hiromitsu*; Asai, Masato; Fujita, Kunihiro*; Gan, Z.*; Geissel, H.*; Hasebe, Hiroo*; Hofmann, S.*; et al.
Journal of the Physical Society of Japan, 86(3), p.034201_1 - 034201_7, 2017/03
Times Cited Count：28 Percentile：81.43(Physics, Multidisciplinary)The fusion reaction of Ca + Cm Lv was studied using the gas-filled recoil-ion separator GARIS at RIKEN. A total of seven and spontaneous-fission decay chains were observed, which would originate from the reaction products of the element 116, 
Lv and 
Lv. Decay properties observed in the chains are in good agreement with the previously published ones. However, one of the chains showed a discrepancy, indicating the new spontaneous-fission branch in 
Cn or the production of the new isotope 
Lv.
Schury, P.*; Wada, Michiharu*; Ito, Yuta*; Kaji, Daiya*; Arai, Fumiya*; MacCormick, M.*; Murray, I.*; Haba, Hiromitsu*; Jeong, S.*; Kimura, Sota*; et al.
Physical Review C, 95(1), p.011305_1 - 011305_6, 2017/01
Times Cited Count：48 Percentile：96.07(Physics, Nuclear)Using a multireflection time-of-flight mass spectrograph located after a gas cell coupled with the gas-filled recoil ion separator GARIS-II, the masses of several -decaying heavy nuclei were directly and precisely measured. The nuclei were produced via fusion-evaporation reactions and separated from projectilelike and targetlike particles using GARIS-II before being stopped in a helium-filled gas cell. Time-of-flight spectra for three isobar chains, 
Fr-Rn-At-Po, 
Fr- Rn-At-Po-Bi, and 
Fr-Rn-At, were observed. Precision atomic mass values were determined for 
Fr, 
Rn, and At. Identifications of Bi, Po, Rn, and At were made with N
10 detected ions, representing the next step toward use of mass spectrometry to identify exceedingly low-yield species such as superheavy element ions.
Eichler, R.*; Asai, Masato; Brand, H.*; Chiera, N. M.*; Di Nitto, A.*; Dressler, R.*; Dllmann, Ch. E.*; Even, J.*; Fangli, F.*; Goetz, M.*; et al.
EPJ Web of Conferences, 131, p.07005_1 - 07005_7, 2016/12
Times Cited Count：3 Percentile：72.98(Chemistry, Inorganic & Nuclear)In recent years gas-phase chemical studies assisted by physical pre-separation allowed for the productions and investigations of fragile single molecular species of superheavy elements. The latest highlight is the formation of very volatile hexacarbonyl compound of element 106, Sg(CO)
. Following this success, second-generation experiments were performed to measure the first bond dissociation energy between the central metal atom and the surrounding ligand. The method using a tubular decomposition reactor was developed and successfully applied to short-lived Mo(CO), W(CO), and Sg(CO).
and W(CO)Usoltsev, I.*; Eichler, R.*; Wang, Y.*; Even, J.*; Yakushev, A.*; Haba, Hiromitsu*; Asai, Masato; Brand, H.*; Di Nitto, A.*; Dllmann, Ch. E.*; et al.
Radiochimica Acta, 104(3), p.141 - 151, 2016/03
Times Cited Count：31 Percentile：95.03(Chemistry, Inorganic & Nuclear)Conditions of the production and decomposition of hexacarbonyl complexes of short-lived Mo and W isotopes were investigated to study thermal stability of the heaviest group 6 hexacarbonyl complex Sg(CO). A tubular flow reactor was tested to decompose the hexacarbonyl complexes and to extract the first bond dissociation energies. A silver was found to be the most appropriate reaction surface to study the decomposition of the group 6 hexacarbonyl. It was found that the surface temperature at which the decomposition occurred was correlated to the first bond dissociation energy of Mo(CO) and W(CO), indicating that the first bond dissociation energy of Sg(CO) could be determined with this technique.
Bk and Am, and even-even nuclides Cm and PuKaji, Daiya*; Morimoto, Koji*; Haba, Hiromitsu*; Ideguchi, Eiji*; Koura, Hiroyuki; Morita, Kosuke*
Journal of the Physical Society of Japan, 85(1), p.015002_1 - 015002_2, 2016/01
Times Cited Count：9 Percentile：55.48(Physics, Multidisciplinary)A neutron deficient berkelium isotope of Bk produced via the 
Au(
Ar, 3n) reaction and the daughter product of Am were newly identified. Alpha-decay energies of eleven Bk were found in 7.62 - 7.96 MeV, and six fission events correlated with -decay of Bk were observed. The half-lives of Bk and Am were determined to be 19
s and 32
s, respectively. The Cm followed by -decay of Bk was also identified.
Kaji, Daiya*; Morimoto, Koji*; Wakabayashi, Yasuo*; Takeyama, Mirei*; Yamaki, Sayaka*; Tanaka, Kengo*; Haba, Hiromitsu*; Huang, M.*; Murakami, Masashi*; Kanaya, Jumpei*; et al.
JPS Conference Proceedings (Internet), 6, p.030107_1 - 030107_4, 2015/06
Performance of the new gas-filled recoil ion separator GARIS-II was investigated using asymmetric 
Ne-induced fusion reactions. The use of He-H mixture gas for the gas-filled magnet significantly reduced background scattered particles detected at the focal-plane Si detector, and increased a transmission of the asymmetric reaction products. A target-identification system was newly installed for efficient measurements of excitation functions without changing beam energy nor target.
