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Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.
Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12
Times Cited Count:6 Percentile:49.29(Geosciences, Multidisciplinary)The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.
Miao, P.*; Tan, Z.*; Lee, S. H.*; Ishikawa, Yoshihisa*; Torii, Shuki*; Yonemura, Masao*; Koda, Akihiro*; Komatsu, Kazuki*; Machida, Shinichi*; Sano, Asami; et al.
Physical Review B, 103(9), p.094302_1 - 094302_18, 2021/03
Times Cited Count:2 Percentile:17.05(Materials Science, Multidisciplinary)The layered perovskite PrBaCoO demonstrates a strong negative thermal expansion (NTE) which holds potential for being fabricated into composites with zero thermal expansion. The NTE was found to be intimately associated with the spontaneous magnetic ordering, known as magneto-volume effect (MVE). Here we report with compelling evidences that the continuous-like MVE in PrBaCoO is intrinsically of discontinuous character, originating from an magnetoelectric transition from an antiferromagnetic insulating large-volume (AFILV) phase to a ferromagnetic less-insulating small-volume (FLISV) phase. Furthermore, the magnetoelectric effect (ME) shows high sensitivity to multiple external stimuli such as temperature, carrier doping, hydrostatic pressure, magnetic field etc. In contrast to the well-known ME such as colossal magnetoresistance and multi-ferroic effect which involve symmetry breaking of crystal structure, the ME in the cobaltite is purely isostructural. Our discovery provides a new path way to realizing the ME as well as the NTE, which may find applications in new techniques.
Oguri, Hidetomo; Hasegawa, Kazuo; Ito, Takashi; Chishiro, Etsuji; Hirano, Koichiro; Morishita, Takatoshi; Shinozaki, Shinichi; Ao, Hiroyuki; Okoshi, Kiyonori; Kondo, Yasuhiro; et al.
Proceedings of 11th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.389 - 393, 2014/10
no abstracts in English
Toyoshima, Atsushi; Li, Z.*; Asai, Masato; Sato, Nozomi; Sato, Tetsuya; Kikuchi, Takahiro; Kaneya, Yusuke; Kitatsuji, Yoshihiro; Tsukada, Kazuaki; Nagame, Yuichiro; et al.
Inorganic Chemistry, 52(21), p.12311 - 12313, 2013/11
Times Cited Count:6 Percentile:23.49(Chemistry, Inorganic & Nuclear)The reduction behavior of mendelevium (Md) was studied using a flow electrolytic chromatography apparatus. By applying appropriate potentials on the chromatography column, the more stable Md is reduced to Md. The reduction potential of the Md + e Md couple was determined to be -0.160.05 V vs. a normal hydrogen electrode.
Nagai, Takayuki; Kikuchi, Kotaro*; Kano, Yoshiharu*
Nihon Genshiryoku Gakkai Wabun Rombunshi, 12(1), p.76 - 88, 2013/03
To understand the corrosion behavior of stainless steel and Ni-Cr alloys in sodium molybdate melts, the immersed corrosion tests of Fe, Cr, Ni, SUS316, 55Ni-45Cr, and Inconel 690 specimens were carried out in NaMoO and NaMoO melts at 750 C. The results of the immersed test, it was found that the corrosion rate decreased with an increase of chromium content in chemical composition of specimens. It was observed that CrO formed on the surface of Cr, 55Ni-45Cr, and Inconel 690 specimens by immersed in NaMoO melt, which corrosion rates were low in the melt, and we presumed that this CrO on the surface controlled the corrosion behavior of their material in the melt.
Li, Z.*; Toyoshima, Atsushi; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Sato, Nozomi; Kikuchi, Takahiro; Nagame, Yuichiro; Schdel, M.; Pershina, V.*; et al.
Radiochimica Acta, 100(3), p.157 - 164, 2012/03
Times Cited Count:14 Percentile:68.93(Chemistry, Inorganic & Nuclear)Hoshi, Harutaka; Kikuchi, Takahiro; Asakura, Toshihide; Morita, Yasuji; Kimura, Takaumi
JAEA-Research 2010-016, 70 Pages, 2010/07
We have studied selective separation of Cs and Sr, which are included in high level liquid waste (HLLW) generated from reprocessing of spent nuclear fuel and are major heat generators, by using extractant impregnated adsorbents. Cs adsorbent using calix arane derivatives showed excellent selectivity for Cs. It also showed significant stability against -irradiation. Sr adsorbent using crown ether derivatives also showed high selectivity for Sr from nitric acid solution, except for Ba and Tc. Dynamic capacity decreased ca. 30% after -irradiation. Hot test using genuine HLLW stored in NUCEF was performed for separation of Cs and Sr through columns, respectively. Each Cs and Sr was separated from other typical fission product elements as well as the results obtained in preliminary experiments. Finally, Cs and Sr were separated according to a supposed separation scheme. Although some complexing agents were added in simulate HLLW, no negative effect was found.
Kikuchi, Takahiro; Hoshi, Harutaka; Asakura, Toshihide; Morita, Yasuji; Kimura, Takaumi; Dodbiba, G.*; Fujita, Toyohisa*
JAEA-Research 2010-010, 45 Pages, 2010/07
We have investigate that separation of Mo from simulated HLLW using various metal oxides adsorbent. Fe-Pb oxides and manganese oxide showed very high solubility in nitric acid solution. The distribution coefficient of Mo was decreased with increasing nitric acid concentration among tested adsorbents. Adsorption ability of Mo on alumina and cobalt oxide was low in 3M nitric acid. Hematite type iron oxide (Fe adsorbent) and amorphous zirconium oxide had high Mo adsorption ability, in 3M nitric acid. TRU, U and major fission products were not adsorbed on the adsorbent. So, separation of Mo can be achieved by using Fe adsorbent. A part of Mo was adsorbed irreversibly on Fe adsorbent, but reversibly-adsorbed Mo was recovered by oxalic acid, and the adsorbent was able to use repeatedly. Behavior of break-through of Mo is estimated from adsorption isotherm and overall mass transfer coefficient. We found that amount of throughput of Mo increased with decreasing grain size of the adsorbent.
Hoshi, Harutaka; Kikuchi, Takahiro; Morita, Yasuji; Kimura, Takaumi
JAEA-Review 2009-041, JAEA Takasaki Annual Report 2008, P. 24, 2009/12
Minimization of radioactive waste from reprocessing process of spent nuclear fuel is strongly desired. We develop an advanced technology for separation of heat generating elements (Cs and Sr) from high level waste to optimize radioactive waste by its characteristics. Some novel solvent impregnated resins (SIRs) were prepared and these SIRs indicated promising ability to separate Cs and Sr from other typical fission products dissolved in nitric acid solution. These adsorbents contacting with nitric acid solution were exposed to ray in a vial. After the irradiation, adsorbents were filtrated through a membrane filter. The adsorption capacity was examined by using irradiated adsorbents after drying. It is concluded that both SIRs maintained their high selectivity for Cs and Sr, respectively, after irradiation. Decreasing ratio of adsorption capacity by irradiation can be estimated from these results. It contributes significantly for conceptual design of separation plant.
Kasamatsu, Yoshitaka*; Toyoshima, Atsushi; Asai, Masato; Tsukada, Kazuaki; Li, Z.; Ishii, Yasuo; Tome, Hayato*; Sato, Tetsuya; Kikuchi, Takahiro; Nishinaka, Ichiro; et al.
Chemistry Letters, 38(11), p.1084 - 1085, 2009/10
Times Cited Count:16 Percentile:48.84(Chemistry, Multidisciplinary)We report on the characteristic anion-exchange behavior of the superheavy element dubnium (Db) with atomic number Z = 105 in HF/HNO solution at the fluoride ion concentration [F] = 0.003 M. The result clearly demonstrates that the fluoro complex formation of Db is significantly different from that of the group-5 homologue Ta in the 6th period of the periodic table while the behavior of Db is similar to that of the lighter homologue Nb in the 5th period.
Nagai, Takayuki; Kikuchi, Kotaro*; Kano, Yoshiharu*; Fukushima, Mineo
Nihon Genshiryoku Gakkai Wabun Rombunshi, 7(4), p.370 - 379, 2008/12
Study of a new pyrochemical processing using alkaline molybdate melt has been carrying out as a candidate reprocessing process for spent oxide fuels. In our previous study, we had confirmed that melting of UO pellet into a molten NaMoO-MoO and electrolytic recovering of UO from the melt included uranyl ions. In this report, the corrosion behavior of the SUS316 cladding tube in molten NaMoO-MoO was evaluated, and we confirmed the dissolution of SUS316 elements into the melt when the amount of additional MoO was excess. And, it is necessary to understand an appropriate amount of additional MoO since the result of this study.
Sakanaka, Shogo*; Ago, Tomonori*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; Harada, Kentaro*; Hiramatsu, Shigenori*; Honda, Toru*; et al.
Proceedings of 11th European Particle Accelerator Conference (EPAC '08) (CD-ROM), p.205 - 207, 2008/06
Future synchrotron light sources based on the energy-recovery linacs (ERLs) are expected to be capable of producing super-brilliant and/or ultra-short pulses of synchrotron radiation. Our Japanese collaboration team is making efforts for realizing an ERL-based hard X-ray source. We report recent progress in our R&D efforts.
Ito, Tanio*; Tsumura, Noriko*; Takeuchi, Akira*; Ishimaru, Tsuneari; Takami, Akira*; Ikawa, Hidemasa*; Komada, Nozomi*; Yamamoto, Shuji*; Kikuchi, Shinsuke*; Miyauchi, Takahiro*; et al.
Geodynamics of Atotsugawa Fault System, p.17 - 24, 2007/00
no abstracts in English
Suzuki, Motofumi*; Takahashi, Michiko*; Tsukamoto, Takashi*; Watanabe, Satoshi; Matsuhashi, Shimpei; Yazaki, Junshi*; Kishimoto, Naoki*; Kikuchi, Shoshi*; Nakanishi, Hiromi*; Mori, Satoshi*; et al.
Plant Journal, 48(1), p.85 - 97, 2006/10
Times Cited Count:172 Percentile:95.74(Plant Sciences)Sakasai, Akira; Ishida, Shinichi; Matsukawa, Makoto; Akino, Noboru; Ando, Toshinari*; Arai, Takashi; Ezato, Koichiro; Hamada, Kazuya; Ichige, Hisashi; Isono, Takaaki; et al.
Nuclear Fusion, 44(2), p.329 - 334, 2004/02
no abstracts in English
Sakasai, Akira; Ishida, Shinichi; Matsukawa, Makoto; Akino, Noboru; Ando, Toshinari*; Arai, Takashi; Ezato, Koichiro; Hamada, Kazuya; Ichige, Hisashi; Isono, Takaaki; et al.
Nuclear Fusion, 44(2), p.329 - 334, 2004/02
Times Cited Count:7 Percentile:22.88(Physics, Fluids & Plasmas)no abstracts in English
Ando, Toshinari*; Ishida, Shinichi; Kato, Takashi; Kikuchi, Mitsuru; Kizu, Kaname; Matsukawa, Makoto; Miura, Yushi; Nakajima, Hideo; Sakasai, Akira; Sugimoto, Makoto; et al.
IEEE Transactions on Applied Superconductivity, 12(1), p.500 - 503, 2002/03
Times Cited Count:11 Percentile:52.56(Engineering, Electrical & Electronic)no abstracts in English
Sakasai, Akira; Ishida, Shinichi; Matsukawa, Makoto; Kurita, Genichi; Akino, Noboru; Ando, Toshinari*; Arai, Takashi; Ichige, Hisashi; Kaminaga, Atsushi; Kato, Takashi; et al.
Proceedings of 19th IEEE/NPSS Symposium on Fusion Engineering (SOFE), p.221 - 225, 2002/00
no abstracts in English
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PNC TN9410 94-052, 251 Pages, 1994/01
The structure of the pressure tube rolled joint portion for the ATR Demonstration Reactor is somewhat changed from that for Fugen, in order reduce the residual stress around the portion. Therefore, Constant Temperature Endurance Test and Thermal Cycle Endurance Test have been conducted under the reactor operating conditions except irradiation to examine the rolled joint integrity. (1)Constant Temperature Endurance Test. In fiscal 1988, Constant Temperature Endurance Test have been performed in the Component Test Loop for 2,033 hours under the reactor operating conditions (pressure 75kg/cm, temperature 280C) for the JP-3 specimen (total testing period 4,033 hours) and the JP-4, JP-5 specimens (total testing period 9,533 hours). After the endurance test it was found by the helium leak test that the rolled joint tightness was maintained enough. Therefore, it was confirmed that the reduction of the residual atress at the rolled joint portion which occurred at the initial stage of the operation did not affect the rolled joint tightness. (2)Thermal Cycle Endurance Test. The helium leak test and the ultrasonic flaw detection test were performed before and after Thermal Cycle Endurance Test (the unmber of thermal cycle increaced from 60 times to 140 times in fisical 1988), of which results showed the integrity of the rolled joint tightness and no crack propagation near the rolled joint portion. Therefore, it was confirmed that 140 times thermal cycle which was the design value for the reactor life of 30 years did not affect the rolled joint tightness and the initiation and propagation of a crack even for the specimen with 200 ppm hydrogen.