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Yokoyama, Hiroya; Maehara, Yushi; Fujita, Hiroki; Takada, Chie
KEK Proceedings 2023-2, p.126 - 131, 2023/11
no abstracts in English
Yasuoka, Yumi*; Fujita, Hiroki; Tsuji, Tomoya; Tsujiguchi, Takakiyo*; Sasaki, Michiya*; Miyazaki, Tomoyuki*; Hashima, Shun*; Yasuda, Hiroshi*; Shimada, Kazumasa; Hirota, Seiko*
Hoken Butsuri (Internet), 57(3), p.146 - 155, 2022/12
no abstracts in English
Hokama, Tomonori; Fujita, Hiroki; Nakano, Masanao; Iimoto, Takeshi*
Radiation Protection Dosimetry, 196(3-4), p.136 - 140, 2021/11
Times Cited Count：0 Percentile：0.01(Environmental Sciences)During the early phase of a nuclear accident, major radioactive materials are released into the environment, necessitating the prompt deployment of various protective actions to avoid or reduce radiation exposure. To implement these actions, the levels of radioactivity in the environment should be determined. However, the radioactivity concentrations of artificial alpha-particle-emitting radionuclides such as plutonium are difficult to measure in airborne samples, because they are interfered with natural radionuclides such as uranium decay products. Therefore, chemical separation is required to measure the concentrations. This study presents a new emergency monitoring system for airborne samples, which performs multiple-pulse time-interval analysis (MTA) without chemical separation. The system is used in conjunction with an alpha/beta-particle survey meter and adopted an analysis method focusing on the detected time interval of each particle. Its features are that a short time to output measurement result, easy handling and nondestructive. The estimated detection limit of the system was 9.5
10
Bq m
. The MTA-based monitoring system could be useful in situations requiring prompt measurement and screening of samples.
Kato, Takuma*; Nagaoka, Mika; Guo, H.*; Fujita, Hiroki; Aida, Taku*; Smith, R. L. Jr.*
Environmental Science and Pollution Research, 28(39), p.55725 - 55735, 2021/10
Times Cited Count：0 Percentile：0(Environmental Sciences)In this work, hydrothermal leaching was applied to simulated soils (clay minerals vermiculite, montmorillonite, kaolinite) and actual soils (Terunuma, Japan) to generate organic acids with the objective to develop an additive-free screening method for determination of Sr in soil. Stable strontium (SrCl
) was adsorbed onto soils for study and ten organic acids were evaluated for leaching Sr from simulated soils under hydrothermal conditions (120 to 200
C) at concentrations up to 0.3 M. For strontium-adsorbed vermiculite (Sr-V), 0.1 M citric acid was found to be effective for leaching Sr at 150C and 1 h treatment time. Based on these results, the formation of organic acids from organic matter in Terunuma soil was studied. Hydrothermal treatment of Terunuma soil produced a maximum amount of organic acids at 200C and 0.5 h reaction time. To confirm the possibility for leaching of Sr from Terunuma soil, strontium-adsorbed Terunuma soil (Sr-S) was studied. For Sr-S, hydrothermal treatment at 200C for 0.5 h reaction time allowed 40% of the Sr to be leached at room temperature, thus demonstrating an additive-free method for screening of Sr in soil. The additive-free hydrothermal leaching method avoids calcination of solids in the first step of chemical analysis and has application to both routine monitoring of metals in soils and to emergency situations.
Nagaoka, Mika; Fujita, Hiroki; Aida, Taku*; Guo, H.*; Smith, R. L. Jr.*
Applied Radiation and Isotopes, 168, p.109465_1 - 109465_6, 2021/02
Times Cited Count：0 Percentile：0.01(Chemistry, Inorganic & Nuclear)The radioactivities in the environmental samples are analyzed to monitor the nuclear power facilities. The pretreatment of radioactive nuclides of alpha and beta emitters in the environmental samples is performed with acid to decompose organic matter and extract object nuclide such as 
Sr, U and Pu. However, the pretreatment methods are time-consuming and used many concentrated acid solutions that are unsafe and hazardous. Therefore, we develop to the new pretreatment method using supercritical water instead of acid. Hydrothermal pretreatment of soils (Andosols) from Ibaraki prefecture (Japan) was used to improve methods for monitoring radioactive Sr and U. Calcined samples were pretreated with subcritical or supercritical water (SCW) followed by extraction with 0.5 M HNO
solutions. With SCW pretreatment, recoveries of Sr and U were 70% and 40%, respectively. Experimental recoveries obtained can be described by a linear relationship in water density. The proposed method is robust and can lower environmental burden of routine analytical protocols.
Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Nagaoka, Mika; Inoue, Kazumi; Koike, Yuko; Yamada, Ryohei; Yoshii, Hideki*; Hiyama, Yoshinori*; Otani, Kazunori*; et al.
JAEA-Review 2018-028, 120 Pages, 2019/02
JAEA-Review-2018-028.pdf:2.69MB
Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and by law of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2017. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Hokama, Tomonori; Nishimura, Tomohiro; Matsubara, Natsumi; et al.
JAEA-Review 2018-025, 171 Pages, 2019/02
JAEA-Review-2018-025.pdf:3.81MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2016 to March 2017. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Electric Power Company Holdings, Inc. in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and were exceeded the normal range of fluctuation in the monitoring, were evaluated.
Nakano, Masanao; Fujita, Hiroki; Nagaoka, Mika; Inoue, Kazumi; Koike, Yuko; Yoshii, Hideki*; Hiyama, Yoshinori*; Otani, Kazunori*; Kikuchi, Masaaki*; Sakauchi, Nobuyuki*; et al.
JAEA-Review 2017-037, 119 Pages, 2018/03
JAEA-Review-2017-037.pdf:2.58MB
Based on the regulations (the safety regulation of Tokai Reprocessing Plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and bylaw of Ibaraki Prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2016. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Nemoto, Masashi; Tobita, Keiji; Hosomi, Kenji; Nagaoka, Mika; Hokama, Tomonori; Nishimura, Tomohiro; Koike, Yuko; et al.
JAEA-Review 2017-028, 177 Pages, 2018/01
JAEA-Review-2017-028.pdf:3.61MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2016 to March 2017. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Electric Power Company Holdings, Inc. in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and were exceeded the normal range of fluctuation in the monitoring, were evaluated.
Fujita, Hiroki; Maehara, Yushi; Nagaoka, Mika; Koarashi, Jun
KEK Proceedings 2017-6, p.35 - 39, 2017/11
no abstracts in English
Cs concentrations in marine samples offshore Ibaraki PrefectureNagaoka, Mika; Matsubara, Natsumi; Fujita, Hiroki; Nakano, Masanao
KEK Proceedings 2017-6, p.212 - 217, 2017/11
no abstracts in English
Nakano, Masanao; Fujita, Hiroki; Kono, Takahiko; Nagaoka, Mika; Inoue, Kazumi; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; Kikuchi, Masaaki*; Sakauchi, Nobuyuki*; et al.
JAEA-Review 2017-001, 115 Pages, 2017/03
JAEA-Review-2017-001.pdf:3.57MB
Based on the regulations (the safety regulation of Tokai reprocessing plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and bylaw of Ibaraki prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2015. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Nakano, Masanao; Fujita, Hiroki; Mizutani, Tomoko; Hosomi, Kenji; Nagaoka, Mika; Hokama, Tomonori; Yokoyama, Hiroya; Nishimura, Tomohiro; Matsubara, Natsumi; Maehara, Yushi; et al.
JAEA-Review 2016-035, 179 Pages, 2017/03
JAEA-Review-2016-035.pdf:4.2MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2015 to March 2016. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Electric Power Company Holdings, Inc. in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and were exceeded the normal range of fluctuation in the monitoring, were evaluated.
Fujita, Hiroki; Nojima, Takehiro; Nagaoka, Mika; Osawa, Takahito; Yokoyama, Hiroya; Ono, Hironobu*
KEK Proceedings 2016-8, p.168 - 172, 2016/10
An automatic analysis system was developed to analyze Strontium-90 (Sr) radioactivity in environmental sample for 2013-2015. Various kinds of ashed environmental samples were used in performance tests of the automatic system. These tests were successful without any system trouble. However, Sr concentration had not been measured using the samples analyzed by the system. In this research, Sr concentration in seaweed sample was compared by between the system's analysis and worker's one. Moreover, the system was improved in each analysis process.
Nagaoka, Mika; Matsubara, Natsumi; Fujita, Hiroki; Nakano, Masanao
KEK Proceedings 2016-8, p.134 - 138, 2016/10
no abstracts in English
C from the Tokai reprocessing plant; Comprehensive chronology and environmental impact assessmentKoarashi, Jun; Fujita, Hiroki; Nagaoka, Mika
Journal of Nuclear Science and Technology, 53(4), p.546 - 553, 2016/04
Times Cited Count：6 Percentile：49.29(Nuclear Science & Technology)Quantitative evaluation of the atmospheric discharge of radiocarbon (C) is of primary importance for accurately assessing the radioecological impact of the operation of the Tokai reprocessing plant (TRP). However, monitoring the atmospheric C discharge was not conducted at the TRP prior to October 1991. The main purpose of this study was to establish the chronology of atmospheric C discharges for the entire operation period (1977-2014). We found strong correlation between the C discharge and spent fuel reprocessing data obtained after October 1991; we used this correlation to estimate the monthly C discharges in the 1977-1991 period. The total amount of atmospheric C discharge was estimated at 7741 
217 GBq for the entire period. Tree-ring C analysis and model calculations using the established discharges were conducted to assess the excess C concentrations around the TRP in the past. The results indicated no significant radioecological impact of atmospheric C discharges from the TRP.
Watanabe, Hitoshi; Nakano, Masanao; Fujita, Hiroki; Takeyasu, Masanori; Mizutani, Tomoko; Isozaki, Tokuju*; Nagaoka, Mika; Hokama, Tomonori; Yokoyama, Hiroya; Nishimura, Tomohiro; et al.
JAEA-Review 2015-034, 175 Pages, 2016/03
JAEA-Review-2015-034.pdf:8.13MB
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2014 to March 2015. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co. in March 2011.
Watanabe, Hitoshi; Nakano, Masanao; Fujita, Hiroki; Kono, Takahiko; Inoue, Kazumi; Yoshii, Hideki*; Otani, Kazunori*; Hiyama, Yoshinori*; Kikuchi, Masaaki*; Sakauchi, Nobuyuki*; et al.
JAEA-Review 2015-030, 115 Pages, 2015/12
JAEA-Review-2015-030.pdf:25.28MB
Based on the regulations (the safety regulation of Tokai reprocessing plant, the safety regulation of nuclear fuel material usage facilities, the radiation safety rule, the regulation about prevention from radiation hazards due to radioisotopes, which are related with the nuclear regulatory acts, the local agreement concerning with safety and environment conservation around nuclear facilities, the water pollution control law, and bylaw of Ibaraki prefecture), the effluent control of liquid waste discharged from the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency has been performed. This report describes the effluent control results of the liquid waste in the fiscal year 2014. In this period, the concentrations and the quantities of the radioactivity in liquid waste discharged from the reprocessing plant, the plutonium fuel fabrication facilities, and the other nuclear fuel material usage facilities were much lower than the limits authorized by the above regulations.
Fujita, Hiroki
Isotope News, (740), p.52 - 58, 2015/12
In this paper, analytical procedures of radioactive strontium and cesium written in Radioactivity Measurement Method Series compiled by MEXT are introduced with test method compiled by MHLW and recent procedures. Moreover, collection and pretreatment procedure of environmental sample are also described.
Nojima, Takehiro; Fujita, Hiroki; Nagaoka, Mika; Osawa, Takahito; Yokoyama, Hiroya; Ono, Hironobu*
KEK Proceedings 2015-4, p.111 - 115, 2015/11
Automatic strontium-90 analysis system was developed for environmental sample in this research. The system was successful to do wet ashing, chemical separation and ion exchange processes using robot, automatic heating system and so on. Hand-made control program can operate the system by itself.
