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Journal Articles

Estimation of external dose for wild Japanese macaques captured in Fukushima prefecture; Decomposition of electron spin resonance spectrum

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.

Radiation Protection Dosimetry, 199(14), p.1620 - 1625, 2023/09

 Times Cited Count:0 Percentile:0.01(Environmental Sciences)

We have been conducting dose assessments for Japanese macaques captured in Fukushima to reveal radiobiological effects on the low-dose expose animals. To accurately determine the external exposure dose, it is desirable to examine the analysis of the CO$$_{2}^{-}$$ radical intensity. We examined ESR spectra of teeth of 10 macaques captured in Fukushima by two spectrum-decomposition algorithms.

Journal Articles

A Study on accuracy of analysis of the radiation-induced component in the ESR spectra of teeth

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; et al.

KEK Proceedings 2022-2, p.120 - 125, 2022/11

We investigate the effect of sample's anisotropy and measurement condition to obtain the higher reproducibility for the shape of the ESR spectrum and the intensity of CO$$_{2}^{-}$$ radical.

Journal Articles

Development of dose estimation method using wild animal teeth for low dose exposure

Mitsuyasu, Yusuke*; Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Kino, Yasushi*; Okutsu, Kenichi*; Sekine, Tsutomu*; Yamashita, Takuma*; Shimizu, Yoshinaka*; Chiba, Mirei*; et al.

KEK Proceedings 2021-2, p.91 - 96, 2021/12

We examined whether the ESR dose estimation method could be applied to wild Japanese macaque. In this work, we investigated the enamel preparation protocol and the analytical method of the ESR spectra.

Journal Articles

External exposure dose estimation by electron spin resonance technique for wild Japanese macaque captured in Fukushima Prefecture

Oka, Toshitaka; Takahashi, Atsushi*; Koarai, Kazuma; Mitsuyasu, Yusuke*; Kino, Yasushi*; Sekine, Tsutomu*; Shimizu, Yoshinaka*; Chiba, Mirei*; Suzuki, Toshihiko*; Osaka, Ken*; et al.

Radiation Measurements, 134, p.106315_1 - 106315_4, 2020/06

 Times Cited Count:5 Percentile:53.85(Nuclear Science & Technology)

The relationship between the CO$$_{2}$$ radical intensity and the absorbed dose (dose response curve) of tooth enamel of Japanese macaque was observed by electron spin resonance and the detection limit of our system was estimated to be 33.5 mGy, which is comparable to the detection limit for human molar teeth. Using the dose response curve, external exposure dose for seven wild Japanese macaques captured in Fukushima prefecture were examined. The results suggest that the external exposure dose for the wild Japanese macaques were ranged between 45 mGy to 300 mGy.

Journal Articles

Effects of diluents on the separation of minor actinides from lanthanides with tetradodecyl-1,10-phenanthroline-2,9-diamide from nitric acid medium

Tsutsui, Nao; Ban, Yasutoshi; Suzuki, Hideya*; Nakase, Masahiko*; Ito, Sayumi*; Inaba, Yusuke*; Matsumura, Tatsuro; Takeshita, Kenji*

Analytical Sciences, 36(2), p.241 - 246, 2020/02

 Times Cited Count:21 Percentile:79.8(Chemistry, Analytical)

To investigate the effective separation of actinides (Ans) from lanthanides (Lns), single-stage batch extraction experiments were performed with a novel extractant, tetradodecyl-1,10-phenanthroline-2,9-diamide (TDdPTDA) with various diluents such as 3-nitrobenzotrifluoride (F-3), nitrobenzene, and ${it n}$-dodecane for Am, Cm, and Lns. The extraction kinetics with TDdPTDA was rapid enough to perform the actual extraction flow sheet. The slopes of the distribution ratio versus TDdPTDA concentration and the distribution ratio versus nitric acid concentration were similar for F-3 and nitrobenzene systems but different from ${it n}$-dodecane system. These differences were attributed to the characteristics of the diluents. This study reveals high distribution ratios of Am (${it D}$ $$_{Am}$$) and Cm (${it D}$ $$_{Cm}$$) for TDdPTDA, with the high separation factors (${it SF}$s) of Am from Lns enough for their separation.

Journal Articles

Practical measurement of residual stresses using contour method

Ikushima, Kazuki*; Shibahara, Masakazu*; Kawajiri, Yoshitaka*; Okimi, Yui*; Uchida, Tomoki*; Akita, Koichi*; Suzuki, Hiroshi; Morooka, Satoshi

Nihon Senpaku Kaiyo Kogakkai Rombunshu, (30), p.123 - 130, 2019/12

In this research, the contour method was applied to measure the residual stress distribution of a bead-on-plate specimen. The measured residual stress distribution was compared with those measured by neutron diffraction method and calculated by thermal elastic plastic finite element analysis. As a result, it was found that the residual stress distribution obtained by these three methods are in good agreement. In addition, the equilibrium of reaction force on cut plane was considered in the contour method to measure residual stresses in asymmetric cutting which is assumed in the measurement of real structures. The proposed method was applied to the measurement of the residual stress in the multi-pass welded joint. The measured results indicated that the proposed method can measure the residual stress distribution in multi-pass welded joint in asymmetric test specimen.

Journal Articles

Zr separation from high-level liquid waste with a novel hydroxyacetoamide type extractant

Morita, Keisuke; Suzuki, Hideya; Matsumura, Tatsuro; Takahashi, Yuya*; Omori, Takashi*; Kaneko, Masaaki*; Asano, Kazuhito*

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.464 - 468, 2019/09

High level liquid waste (HLLW) contains several radionuclides with half-lives longer than 10$$^{6}$$ year. For reduce environmental burden of waste disposal, minor actinoids and long-lived fission products will to be partitioned and transmuted. JAEA and Toshiba developed process for recovering Se, Zr, Pd and Cs from HLLW. Solvent extraction for Zr with novel extractant, ${it N,N}$-didodecyl-2-hydroxyacetoamide (HAA) was detailed. The HAA system showed high selectivity for Zr, as indicated by the extraction order of Zr $$>$$ Mo $$>$$ Pd $$>$$ Ag $$approx$$ Sb $$>$$ Sn $$>$$ Lns $$>$$ Fe. The extracted species was determined as Zr(HAA)$$_{3}$$(NO$$_{3}$$)$$_{4}$$(HNO$$_{3}$$)$$_{x}$$. A continuous countercurrent extraction with HAA was applied to a simulated, concentrated HLLW after Pd, Se, and Cs removal, where the quantitative extraction of Zr and Mo was effectively demonstrated.

Journal Articles

Remote radiation imaging system using a compact $$gamma$$-ray imager mounted on a multicopter drone

Sato, Yuki; Ozawa, Shingo*; Terasaka, Yuta; Kaburagi, Masaaki; Tanifuji, Yuta; Kawabata, Kuniaki; Miyamura, Hiroko; Izumi, Ryo*; Suzuki, Toshikazu*; Torii, Tatsuo

Journal of Nuclear Science and Technology, 55(1), p.90 - 96, 2018/01

 Times Cited Count:43 Percentile:98.03(Nuclear Science & Technology)

Journal Articles

Reduction and resource recycling of high-level radioactive wastes through nuclear transmutation; Isolation techniques of Pd, Zr, Se and Cs in simulated high level radioactive waste using solvent extraction

Sasaki, Yuji; Morita, Keisuke; Ito, Keisuke; Suzuki, Shinichi; Shiwaku, Hideaki; Takahashi, Yuya*; Kaneko, Masaaki*; Omori, Takashi*; Asano, Kazuhito*

Proceedings of International Nuclear Fuel Cycle Conference (GLOBAL 2017) (USB Flash Drive), 4 Pages, 2017/09

no abstracts in English

Journal Articles

Radiation imaging system using a compact $$gamma$$-ray imager mounted on a remotely operated machine

Sato, Yuki; Kawabata, Kuniaki; Ozawa, Shingo*; Izumi, Ryo*; Kaburagi, Masaaki; Tanifuji, Yuta; Terasaka, Yuta; Miyamura, Hiroko; Kawamura, Takuma; Suzuki, Toshikazu*; et al.

IFAC-PapersOnLine, 50(1), p.1062 - 1066, 2017/07

 Times Cited Count:3 Percentile:66.37(Automation & Control Systems)

Journal Articles

Extraction and separation of Se, Zr, Pd, and Cs including long-lived radionuclides

Sasaki, Yuji; Morita, Keisuke; Suzuki, Shinichi; Shiwaku, Hideaki; Ito, Keisuke; Takahashi, Yuya*; Kaneko, Masaaki*

Solvent Extraction Research and Development, Japan, 24(2), p.113 - 122, 2017/06

The solvent extraction of Se, Zr, Pd, and Cs from nitric acid into 1-octanol (OC) and dodecane has been performed. These elements include long-lived radionuclides in spent nuclear fuels, so a simple separation method is indispensable for the development of the treatment of high-level liquid radioactive waste. It was found that Se can be extracted using phenylenediamine, Zr can be extracted using tetraoctyl diglycolamide and di-2-ethylhexyl phosphoric acid, and Pd can be extracted using (methylimino)bis(dioctylacetamide) and hexaoctylnitrilotriacetamide. These elements can be recovered in over 90% yield by these extractants from nitric acid into OC. A distribution ratio of Cs of greater than 1 can be obtained using di-t-butyldibenzo-18-crown-6. It is clear that 90% recovery of Cs can be achieved using an extraction solvent with ten times the volume of the aqueous phase.

Journal Articles

Fundamental experiments of jet impingement and fragmentation simulating the fuel relocation in the core disruptive accident of sodium-cooled fast reactors

Imaizumi, Yuya; Kamiyama, Kenji; Matsuba, Kenichi; Isozaki, Mikio; Suzuki, Toru; Emura, Yuki

Proceedings of 2017 International Congress on Advances in Nuclear Power Plants (ICAPP 2017) (CD-ROM), 5 Pages, 2017/04

In order to simulate the typical accident conditions of the fuel relocation phase in SFRs, the molten alloy of low melting point was discharged into a shallow water pool. The distance between the nozzle exit and the bottom plate was set to a value which was indicated to be insufficient to fragment. As the experimental result, the melt jet reached the bottom plate, and dispersed in all directions along the plate, together with the progress of fragmentation. In addition, the melt temperature on the bottom plate decreased rapidly along the radius direction. These results suggest that the fragmentation which would accompany this rapid cooling would be enhanced by the plate. This enhancement would be caused by the extension of the melt-water interface when the melt was dispersed forcibly by the plate. The solidified debris remained after the discharge showed remarkable fragmentation which was assumed to be caused by the formations of small vapor bubbles in the interface.

JAEA Reports

Study of HTGR contribution to Japan's CO$$_{2}$$ emission reduction goal in 2050

Kamiji, Yu; Suzuki, Koichi*; Yan, X.

JAEA-Technology 2016-010, 24 Pages, 2016/07

JAEA-Technology-2016-010.pdf:1.05MB

Japanese government has set the goal of reducing CO$$_{2}$$ emission by 26% in 2030 below the 2013 level, in longer term, by 80% below the 1990 level. To achieve the goals, various measures should be taken. The GTHTR300, a commercial High Temperature Gas-cooled Reactor (HTGR) design being developed by JAEA offers spectrum of heat applications by using its high temperature heat up to 950$$^{circ}$$C. The potential contribution of CO$$_{2}$$ emission reduction by HTGR is estimated considering domestic and overseas deployment of the GTHTR300. The best estimate for domestic CO$$_{2}$$ reduction is 2.07$$times$$10$$^{8}$$ ton- CO$$_{2}$$/yr and that from oversea is 2.25$$times$$10$$^{8}$$ ton- CO$$_{2}$$/yr. The sum of these is about 47% of 9.13$$times$$10$$^{8}$$ ton- CO$$_{2}$$/yr which is CO$$_{2}$$ reduction target in 2050, for which deployment of 52 plants in Japan and 113 plants abroad, with each plant containing four 600 MWt reactor units, is required.

JAEA Reports

Development of non-destructive inspection method for on-site observation; Preliminary examination for internal visualization of HTTR

Takegami, Hiroaki; Terada, Atsuhiko; Noguchi, Hiroki; Kamiji, Yu; Ono, Masato; Takamatsu, Kuniyoshi; Ito, Chikara; Hino, Ryutaro; Suzuki, Keiichi*; Onuma, Hiroshi*; et al.

JAEA-Research 2013-032, 25 Pages, 2013/12

JAEA-Research-2013-032.pdf:3.56MB

We focused on a non-destructive inspection method using cosmic-ray muons as a candidate method for observation of internal the reactor from the outside of a reactor building. In this study, the applicability of this method for the reactor investigation was confirmed by a preliminary examination with High Temperature Engineering Test Reactor (HTTR). From the results of this examination, it appears that high density structures, such as the core and concrete walls, were able to observe by using muon telescope with coincidence method from the outside of the pressure vessel. Furthermore, we proposed some improvements of this muon inspection system for on-site investigation at the Fukushima Daiichi NPS.

Journal Articles

Performance of a remotely located muon radiography system to identify the inner structure of a nuclear plant

Fujii, Hirofumi*; Hara, Kazuhiko*; Hashimoto, Shugo*; Ito, Fumiaki*; Kakuno, Hidekazu*; Kim, S.*; Kochiyama, Mami; Nagamine, Kanetada*; Suzuki, Atsuto*; Takada, Yoshihisa*; et al.

Progress of Theoretical and Experimental Physics (Internet), 2013(7), p.073C01_1 - 073C01_20, 2013/07

 Times Cited Count:26 Percentile:76.73(Physics, Multidisciplinary)

Journal Articles

R&D on nuclear forensics technology at JAEA

Sakurai, Satoshi; Watahiki, Masaru; Suzuki, Mitsutoshi; Kuno, Yusuke

Proceedings of INMM 52nd Annual Meeting (CD-ROM), 6 Pages, 2011/07

The national statement made by the Japan Government at 2010 Nuclear Security Summit at Washington D.C., U.S.A. was to develop its nuclear forensics detection and analysis technologies in a three-year period and to share them with the international community to contribute to strengthening the nuclear security regime. The Japan Atomic Energy Agency, JAEA, is the organization that possesses analytical capabilities with the potential to fulfill this nuclear forensics mission, since JAEA has been developing a wide range of analytical techniques for nuclear material samples from large size ones to trace level ones of environmental sampling. For this reason, JAEA starts R&D on nuclear forensics technology from JFY 2011. In the presentation reported will be JAEA's outline of R&D to establish nuclear forensics analytical capabilities including international cooperation. The summary of International Workshop on Nuclear Forensics on 5-6 October 2010 at Tokai, Japan will be also reported.

Journal Articles

Analysis of cell-survival fractions for heavy-ion irradiations based on microdosimetric kinetic model implemented in the particle and heavy ion transport code system

Sato, Tatsuhiko; Watanabe, Ritsuko; Kase, Yuki*; Tsuruoka, Chizuru*; Suzuki, Masao*; Furusawa, Yoshiya*; Niita, Koji*

Radiation Protection Dosimetry, 143(2-4), p.491 - 496, 2011/02

 Times Cited Count:33 Percentile:91.42(Environmental Sciences)

We reanalyzed the survival fraction data, using the microdosimetric-kinetic (MK) model implemented in the PHITS code. It is found from the analysis that the MK model successfully accounts for the cell survival-fractions under a variety of irradiation conditions, using only y* parameter.

Journal Articles

Transmission imaging and strain mapping in the vicinity of internal crack tip using synchrotron white X-ray

Shibano, Junichi*; Kajiwara, Kentaro*; Kiriyama, Koji*; Shobu, Takahisa; Suzuki, Kenji*; Nishimura, Suguru*; Miura, Setsuo*; Kobayashi, Michiaki*

Materials Science Forum, 638-642, p.2476 - 2481, 2010/01

Journal Articles

Initial oxidation of Si(110) surface evaluated by photoemission spectroscopy and substrate-curvature measurements

Yamamoto, Yoshihisa*; Suzuki, Yasushi*; Miyamoto, Yu*; Bantaculo, R.*; Suemitsu, Maki*; Enta, Yoshiharu*; Teraoka, Yuden; Yoshigoe, Akitaka; Asaoka, Hidehito; Yamazaki, Tatsuya

Hakumaku, Hyomen Butsuri Bunkakai, Shirikon Tekunoroji Bunkakai Kyosai Tokubetsu Kenkyukai Kenkyu Hokoku, p.207 - 210, 2009/01

The bending of Si substrate has been measured optically in the oxidation of Si(110) surface and variation of curvature for (001) and (-110) directions have been evaluated. Furthermore, time evolutions of oxygen adsorption content and its chemical bonding states have been measured by photoemission spectroscopy to discuss inisotropy of the Si(110) oxidation in comjunction with substrate curvature measurements. Oxygen adsorption content was evaluated from O1s photoemission and chemical bonding states were evaluated from Si2p photoemission. O$$_{2}$$ gas pressure was ranging from 5.0$$times$$10$$^{-6}$$ Pa to 6.7$$times$$10$$^{-6}$$ and substrate temperature was 873 K. Compressive stress was detected in the (-110) direction. In turn, stretching stress was detected. The photoemission spectroscopy indicated that a layer-by-layer oxidation was not took place. The stretching stress in the (001) direction implies that oxidation of B-bonds which have components along the (001) direction takes place.

Journal Articles

Status of JT-60SA tokamak under the EU-JA broader approach agreement

Matsukawa, Makoto; Kikuchi, Mitsuru; Fujii, Tsuneyuki; Fujita, Takaaki; Hayashi, Takao; Higashijima, Satoru; Hosogane, Nobuyuki; Ikeda, Yoshitaka; Ide, Shunsuke; Ishida, Shinichi; et al.

Fusion Engineering and Design, 83(7-9), p.795 - 803, 2008/12

 Times Cited Count:17 Percentile:72.86(Nuclear Science & Technology)

no abstracts in English

113 (Records 1-20 displayed on this page)