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JAEA Reports

Acquisition of saltwater infiltration behavior data in unsaturated compacted bentonite

Sato, Hisashi*; Takayama, Yusuke; Suzuki, Hideaki*; Sato, Daisuke*

JAEA-Data/Code 2023-010, 47 Pages, 2023/09

JAEA-Data-Code-2023-010.pdf:1.45MB

When a high-level radioactive waste repository is constructed in a coastal area, it is necessary to fully evaluate the impact of seawater-based groundwater on engineered barriers, including buffer materials. In this report, one-dimensional saltwater infiltration tests were conducted to obtain data to understand the impact of seawater-based groundwater on the migration phenomena of water and solutes in the buffer material during the transient period. As a result, it was confirmed that the infiltration rate increased as the NaCl concentration in the infiltration solution increased. And it was confirmed that the water content ratio distribution changed as the NaCl concentration in the infiltration solution increased. As a result of analysis of the chloride ion concentration of the post-test specimens confirmed that chloride ion enrichment was occurred with infiltration. As a result of verifying the mechanism by which chloride ion enrichment occurs, it was confirmed that the phenomenon of chloride ion enrichment due to infiltration depends on the initial water content ratio.

Journal Articles

Multiple mechanisms in proton-induced nucleon removal at $$sim$$100 MeV/nucleon

Pohl, T.*; Sun, Y. L.*; Obertelli, A.*; Lee, J.*; G$'o$mez-Ramos, M.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Cai, B. S.*; Yuan, C. X.*; Brown, B. A.*; et al.

Physical Review Letters, 130(17), p.172501_1 - 172501_8, 2023/04

 Times Cited Count:5 Percentile:92.42(Physics, Multidisciplinary)

We report on the first proton-induced single proton- and neutron-removal reactions from the neutron deficient $$^{14}$$O nucleus with large Fermi-surface asymmetry at $$sim$$100 MeV/nucleon. Our results provide the first quantitative contributions of multiple reaction mechanisms including the quasifree knockout, inelastic scattering, and nucleon transfer processes. It is shown that the inelastic scattering and nucleon transfer, usually neglected at such energy regime, contribute about 50% and 30% to the loosely bound proton and deeply bound neutron removal, respectively.

JAEA Reports

Assessment of the infiltration behaviour of buffer material in seawater-type groundwater environments using a coupled THMC analysis model (Contract research)

Suzuki, Hideaki*; Takayama, Yusuke; Sato, Hisashi*; Watahiki, Takanori*; Sato, Daisuke*

JAEA-Research 2022-013, 41 Pages, 2023/03

JAEA-Research-2022-013.pdf:3.99MB

It is anticipated that the coupled thermal-hydraulic-mechanical and chemical (THMC) processes will occur, involving an interactive process with radioactive decay heat arising from the vitrified waste, infiltration of groundwater from the host rock into the buffer material, swelling pressure of buffer material due to its saturation and chemical reaction between bentonite and pore-water in the near-field of a geological disposal system for high-level radioactive waste repository. In order to evaluate these phenomena in the near-field, the THMC model has been developed. In this study, For the purpose of evaluating the near-field infiltration behavior in seawater-type groundwater environment, a hydraulic model was set in which the permeability of the buffer material change depending on the salt concentration in the pore-water. In order to evaluate the drying phenomenon of the buffer material due to waste heat, a temperature gradient water transfer model was set in consideration of the dependence of temperature and pore-water saturation. The THMC analysis of the in-situ experiment of engineered barrier system (EBS) experiment at the Horonobe Underground Research Laboratory was carried out. The validity of the model was then checked through comparison with measured data.

Journal Articles

Survival probabilities of charmonia as a clue to measure transient magnetic fields

Iwasaki, Sachio*; Jido, Daisuke*; Oka, Makoto; Suzuki, Kei

Physics Letters B, 820, p.136498_1 - 136498_6, 2021/09

 Times Cited Count:2 Percentile:18.91(Astronomy & Astrophysics)

We investigate time evolution of $$S$$-wave charmonium populations under a time-dependent homogeneous magnetic field and evaluate survival probabilities of the low-lying charmonia to the goal of estimating the magnetic field strength at heavy-ion collisions. Our approach implements mixing between different spin eigenstates and transitions to radially excited states. We show that the survival probabilities can change even by an extremely short magnetic field. Furthermore, we find that the survival probabilities depend on the initial spin states. We propose the sum of the survival probabilities over spin partners as an observable insensitive to the initial states. We also find that the sum can be approximately given as a function of $$sigma B_0^2$$ with a duration time $$sigma$$ and the maximum strength of the magnetic field $$B_0$$.

Journal Articles

High-spin states in $$^{35}$$S

Go, Shintaro*; Ideguchi, Eiji*; Yokoyama, Rin*; Aoi, Nori*; Azaiez, F.*; Furutaka, Kazuyoshi; Hatsukawa, Yuichi; Kimura, Atsushi; Kisamori, Keiichi*; Kobayashi, Motoki*; et al.

Physical Review C, 103(3), p.034327_1 - 034327_8, 2021/03

 Times Cited Count:4 Percentile:57.13(Physics, Nuclear)

Journal Articles

Shell structure of the neutron-rich isotopes $$^{69,71,73}$$Co

Lokotko, T.*; Leblond, S.*; Lee, J.*; Doornenbal, P.*; Obertelli, A.*; Poves, A.*; Nowacki, F.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Authelet, G.*; et al.

Physical Review C, 101(3), p.034314_1 - 034314_7, 2020/03

 Times Cited Count:10 Percentile:69.78(Physics, Nuclear)

The structures of the neutron-rich $$^{69,71,73}$$Co isotopes were investigated via ($$p,2p$$) knockout reactions at the Radioactive Isotope Beam Factory, RIKEN. Level schemes were reconstructed using the $$gamma-gamma$$ coincidence technique, with tentative spin-parity assignments based on the measured inclusive and exclusive cross sections. Comparison with shell-model calculations suggests coexistence of spherical and deformed shapes at low excitation energies in the $$^{69,71,73}$$Co isotopes.

Journal Articles

An Experimental setup for creating and imaging $$^{4}$$He$$_{2}$$$$^{ast}$$ excimer cluster tracers in superfluid helium-4 via neutron-$$^{3}$$He absorption reaction

Sonnenschein, V.*; Tsuji, Yoshiyuki*; Kokuryu, Shoma*; Kubo, Wataru*; Suzuki, So*; Tomita, Hideki*; Kiyanagi, Yoshiaki*; Iguchi, Tetsuo*; Matsushita, Taku*; Wada, Nobuo*; et al.

Review of Scientific Instruments, 91(3), p.033318_1 - 033318_12, 2020/03

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

Journal Articles

Interfacial ferromagnetism and atomic structures in high-temperature grown Fe$$_3$$O$$_4$$/Pt/Fe$$_3$$O$$_4$$ epitaxial trilayers

Kikkawa, Takashi*; Suzuki, Motohiro*; Ramos, R.*; Aguirre, M. H.*; Okabayashi, Jun*; Uchida, Kenichi*; Lucas, I.*; Anad$'o$n, A.*; Kikuchi, Daisuke*; Algarabel, P. A.*; et al.

Journal of Applied Physics, 126(14), p.143903_1 - 143903_11, 2019/10

 Times Cited Count:10 Percentile:49.82(Physics, Applied)

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:56.2(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Generation of $$^{4}$$He$$_2^{*}$$ clusters via neutron-$$^{3}$$He absorption reaction toward visualization of full velocity field in quantum turbulence

Matsushita, Taku*; Sonnenschein, V.*; Guo, W.*; Hayashida, Hirotoshi*; Hiroi, Kosuke; Hirota, Katsuya*; Iguchi, Tetsuo*; Ito, Daisuke*; Kitaguchi, Masaaki*; Kiyanagi, Yoshiaki*; et al.

Journal of Low Temperature Physics, 196(1-2), p.275 - 282, 2019/07

 Times Cited Count:1 Percentile:4.76(Physics, Applied)

Journal Articles

Nuclear structure of $$^{76}$$Ni from the ($$p$$,$$2p$$) reaction

Elekes, Z.*; Kripk$'o$, $'A$*; Sohler, D.*; Sieja, K.*; Ogata, Kazuyuki*; Yoshida, Kazuki; Doornenbal, P.*; Obertelli, A.*; Authelet, G.*; Baba, Hidetada*; et al.

Physical Review C, 99(1), p.014312_1 - 014312_7, 2019/01

 Times Cited Count:10 Percentile:64.15(Physics, Nuclear)

The nuclear structure of the $$^{76}$$Ni nucleus was investigated by ($$p$$,$$2p$$) reaction using a NaI(Tl) array to detect the deexciting prompt $$gamma$$ rays. A new transition with an energy of 2227 keV was identified by $$gamma gamma$$ and $$gamma gamma gamma$$ coincidences. Our shell-model calculations using the Lenzi, Nowacki, Poves, and Sieja interaction produced good candidates for the experimental proton hole states in the observed energy region, and the theoretical cross sections showed good agreement with the experimental values. Although we could not assign all the experimental states to the theoretical ones unambiguously, the results are consistent with a reasonably large Z = 28 shell gap for nickel isotopes in accordance with previous studies.

Journal Articles

Shell evolution beyond $$Z$$=28 and $$N$$=50; Spectroscopy of $$^{81,82,83,84}$$Zn

Shand, C. M.*; Podoly$'a$k, Zs.*; G$'o$rska, M.*; Doornenbal, P.*; Obertelli, A.*; Nowacki, F.*; Otsuka, T.*; Sieja, K.*; Tostevin, J. A.*; Tsunoda, T.*; et al.

Physics Letters B, 773, p.492 - 497, 2017/10

 Times Cited Count:25 Percentile:87.36(Astronomy & Astrophysics)

Journal Articles

Two-phase flow measurements in a simulated debris bed

Ito, Daisuke*; Rivera, M. N.*; Saito, Yasushi*; Aoyagi, Mitsuhiro; Kamiyama, Kenji; Suzuki, Toru*

Proceedings of 17th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-17) (USB Flash Drive), 10 Pages, 2017/09

Journal Articles

Measurements of two-phase pressure drop in a simulated debris bed

Nava, M.*; Ito, Daisuke*; Saito, Yasushi*; Aoyagi, Mitsuhiro; Kamiyama, Kenji; Suzuki, Toru*

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 5 Pages, 2017/07

Journal Articles

Detection of induced paramagnetic moments in Pt on Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$ via X-ray magnetic circular dichroism

Kikkawa, Takashi*; Suzuki, Motohiro*; Okabayashi, Jun*; Uchida, Kenichi*; Kikuchi, Daisuke*; Qiu, Z.*; Saito, Eiji

Physical Review B, 95(21), p.214416_1 - 214416_7, 2017/06

 Times Cited Count:16 Percentile:60.44(Materials Science, Multidisciplinary)

Journal Articles

Characteristics of pressure drop and void fraction in a simulated debris bed

Ito, Daisuke*; Nava, M.*; Saito, Yasushi*; Aoyagi, Mitsuhiro; Kamiyama, Kenji; Suzuki, Toru*

Proceedings of 2017 Japan-US Seminar on Two-Phase Flow Dynamics (JUS 2017), 4 Pages, 2017/06

Journal Articles

Deep microbial life in high-quality granitic groundwater from geochemically and geographically distinct underground boreholes

Ino, Kohei*; Konno, Yuta*; Kozuka, Mariko*; Hirota, Akinari*; Togo, Yoko*; Fukuda, Akari*; Komatsu, Daisuke*; Tsunogai, Urumu*; Tanabe, Akifumi*; Yamamoto, Satoshi*; et al.

Environmental Microbiology Reports (Internet), 8(2), p.285 - 294, 2016/04

 Times Cited Count:26 Percentile:68.59(Environmental Sciences)

To understand the subsurface biosphere, borehole investigation was conducted for 300-m deep granitic rocks at the Mizunami underground research laboratory, Japan. The initial biomass was the highest with the flourish of aerobic H$$_{2}$$-oxidizing Hydrogenophaga spp., whereas an uncultivated lineage of the phylum Nitrospirae became predominant after three years with decreasing biomass. The common occurrence of many species of Nitrospirae and Chlorobi phyla at the geographically distinct sites and the exclusive detection of their phylogenetically related environmental sequences from deep groundwaters and terrestrial hot springs, suggest that these bacteria are indigenous and potentially adapted to the deep terrestrial subsurface.

Journal Articles

Superdeformation in $$^{35}$$S

Go, Shintaro*; Ideguchi, Eiji*; Yokoyama, Rin*; Kobayashi, Motoki*; Kisamori, Keiichi*; Takaki, Motonobu*; Miya, Hiroyuki*; Ota, Shinsuke*; Michimasa, Shinichiro*; Shimoura, Susumu*; et al.

JPS Conference Proceedings (Internet), 6, p.030005_1 - 030005_4, 2015/06

Journal Articles

$$^{12}$$C + p resonant elastic scattering in the Maya active target

Sambi, S.*; Raabe, R.*; Borge, M. J. G.*; Caamano, M.*; Damoy, S.*; Fern$'a$ndez-Dom$'i$nguez, B.*; Flavigny, F.*; Fynbo, H.*; Gibelin, J.*; Grinyer, G. F.*; et al.

European Physical Journal A, 51(3), p.25_1 - 25_7, 2015/03

 Times Cited Count:6 Percentile:42.02(Physics, Nuclear)

Journal Articles

Biogeochemical signals from deep microbial life in terrestrial crust

Suzuki, Yohei*; Konno, Yuta*; Fukuda, Akari*; Komatsu, Daisuke*; Hirota, Akinari*; Watanabe, Katsuaki*; Togo, Yoko*; Morikawa, Noritoshi*; Hagiwara, Hiroki; Aosai, Daisuke*; et al.

PLOS ONE (Internet), 9(12), p.e113063_1 - e113063_20, 2014/12

 Times Cited Count:12 Percentile:34.33(Multidisciplinary Sciences)

We present multi-isotopic evidence of microbially mediated sulfate reduction in a granitic aquifer, a representative of the terrestrial crust habitat. Deep groundwater of meteoric origin was collected from underground boreholes drilled into the Cretaceous Toki granite, central Japan. A large sulfur isotopic fractionation of 20-60 permil diagnostic to microbial sulfate reduction is associated with the investigated groundwater containing sulfate below 0.2 mM. In contrast, a small carbon isotopic fractionation ($$<$$ 30 permil) is not indicative of methanogenesis. Our results demonstrate that the deep biosphere in the terrestrial crust is metabolically active and playing a crucial role in the formation of reducing groundwater even under low energy fluxes.

43 (Records 1-20 displayed on this page)