Experimental visualization of water/ice phase distribution at cold start for practical-sized polymer electrolyte fuel cells

Higuchi, Yuki*; Yoshimune, Wataru*; Kato, Satoru*; Hibi, Shogo*; Setoyama, Daigo*; Isegawa, Kazuhisa*; Matsumoto, Yoshihiro*; Hayashida, Hirotoshi*; Nozaki, Hiroshi*; Harada, Masashi*; et al.

Communications Engineering (Internet), 3, p.33_1 - 33_7, 2024/02

https://doi.org/10.1038/s44172-024-00176-6

Dirac Kondo effect under magnetic catalysis

Hattori, Koichi*; Suenaga, Daiki*; Suzuki, Kei; Yasui, Shigehiro*

Physical Review B, 108(24), p.245110_1 - 245110_11, 2023/12

https://doi.org/10.1103/PhysRevB.108.245110

We develop a mean-field theory of a novel Kondo effect emerging in systems without a Fermi surface, which instead emerges under strong magnetic fields. We determine the magnitude of the Kondo condensate, which is a particle pairing composed of conducting Dirac fermions and localized impurities. We focus on the competition between the Kondo effect and the energy gap formation that stems from the pairing among the Dirac fermions leading to the dynamical chiral symmetry breaking. We find that this competition induces a quantum critical point. We also investigate finite-temperature effects. This system at vanishing fermion density can be studied with Monte Carlo lattice simulations, which do not suffer from the sign problem.

Factors regulating the concentration of particulate iodine in coastal seawater

Sato, Yuhi*; Otosaka, Shigeyoshi*; Suzuki, Takashi; Nakanishi, Takahiro

Limnology and Oceanography, 68(7), p.1580 - 1594, 2023/07

https://doi.org/10.1002/lno.12369

To investigate the factors regulating the concentration of particulate iodine (PI) in seawater, it was measured in two Pacific coastal areas adjacent to Japan in two seasons along with parameters such as particulate organic carbon (POC) and nitrogen (PON), dissolved iodine (DI), and phytoplankton pigments. The dataset was divided in three groups namely, lower (Group A), average (Group B), and higher (Group C) atomic ratios of PI to POC (I/C). The three groups were characterized by phytoplanktonic physiological states as highly productive, steady, and senescent states, respectively. Based on the finding that PI production is associated with the phytoplankton physiological state, the seasonal and regional differences in PI concentration and I/C in the observation areas were consistently explained. Finally, we suggest that the phytoplanktonic physiological state is one of the vital factors regulating the PI concentration in seawater.

Phase diagram of the QCD Kondo effect and inactivation of the magnetic catalysis

Hattori, Koichi*; Suenaga, Daiki*; Suzuki, Kei; Yasui, Shigehiro*

EPJ Web of Conferences, 276, p.01015_1 - 01015_5, 2023/03

https://doi.org/10.1051/epjconf/202327601015

We investigate the QCD phase diagram in strong magnetic fields with heavy-quark impurities and determine the ground state within the mean-field analysis. The ground state is characterized by magnitudes of the pairing not only between the light quark and antiquark, i.e., chiral condensate, but also between the light quark and heavy-quark impurity, dubbed the Kondo condensate. We propose signatures of the interplay and/or competition between those two pairing phenomena reflected in the magnitude of the chiral condensate that is saturated with respect to the magnetic-field strength and anomalously increases with increasing temperature.

Nested antiferromagnetic spin fluctuations and non-Fermi-liquid behavior in electron-doped CeCoNiIn

Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Kotegawa, Hisashi*; To, Hideki*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.

Physical Review B, 106(23), p.235152_1 - 235152_8, 2022/12

https://doi.org/10.1103/PhysRevB.106.235152

We investigate the electronic state of Ni-substituted CeCoNiIn by nuclear quadrupole and magnetic resonance (NQR/NMR) techniques. The heavy fermion superconductivity below K for is suppressed by Ni substitutions, and reaches zero for . The In NQR spectra for and 0.25 can be explained by simulating the electrical field gradient that is calculated for a virtual supercell with density functional theory. The spin-lattice relaxation rate indicates that Ni substitution weakens antiferromagnetic correlations that are not localized near the substituent but instead are uniform in space. The temperature () dependence of for shows a maximum around K and decreases toward almost zero when temperature is further reduced as if a gap might be opening in the magnetic excitation spectrum; however, the magnetic specific heat and the static magnetic susceptibility evolve smoothly through with a dependence. The peculiar T dependence of and non-Fermi-liquid specific heat and susceptibility can be interpreted in a unified way by assuming nested antiferromagnetic spin fluctuations in a quasi-two-dimensional electronic system.

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

https://doi.org/10.1080/00223131.2022.2038301

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Hyperfine splitting and nuclear spin polarization in NdPdAl and NdPdGe

Metoki, Naoto; Shibata, Kaoru; Matsuura, Masato*; Kitazawa, Hideaki*; Suzuki, Hiroyuki*; Yamauchi, Hiroki; Hagihara, Masato; Frontzek, M. D.*; Matsuda, Masaaki*

Journal of the Physical Society of Japan, 91(5), p.054710_1 - 054710_6, 2022/05

https://doi.org/10.7566/JPSJ.91.054710

Hyperfine splitting of Nd nuclei in NdPdAl has been studied by means of high-resolution neutron spectroscopy. We observed inelastic peaks at eV coming from the hyperfine splitting in the magnetically ordered phase due to the hyperfine interactions between Nd nuclei (=7/2) and the 4 electrons with ground state composed of mainly . At very low temperatures, nuclear spin of Nd is polarized with increasing occupation probability of low energy levels and contributes to the enhancement of the antiferromagnetic Bragg intensities: the elastic non-spin-flip channel is dominant. As an application of this phenomenon, we determined the Nd moment and hyperfine splitting from the temperature dependence of an antiferromagnetic Bragg intensities for NdPdGe.

Characterization of deformation by cold rolling in ferritic steel containing Cu particles using neutron transmission analysis

Oba, Yojiro; Morooka, Satoshi; Oishi, Kazuki*; Suzuki, Junichi*; Tsuchiyama, Toshihiro*

ISIJ International, 62(1), p.173 - 178, 2022/01

https://doi.org/10.2355/isijinternational.ISIJINT-2021-144

Nanoscale heterogeneity induced by nonmagnetic Zn dopants in the quantum critical metal CeCoIn; In NQR/NMR and Co NMR study

Sakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Ramakrishna, S. K.*; Reyes, A. P.*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.

Physical Review B, 104(8), p.085106_1 - 085106_12, 2021/08

https://doi.org/10.1103/PhysRevB.104.085106

Antiferromagnetism in a prototypical quantum critical metal CeCoIn is known to be induced by slight substitutions of non-magnetic Zn atoms for In. In nominally 7% Zn substituted CeCoIn, an antiferromagnetic (AFM) state coexists with heavy fermion superconductivity. Heterogeneity of the electronic states is investigated in Zn doped CeCoIn by means of nuclear quadrupole and magnetic resonances (NQR and NMR). Site-dependent NQR relaxation rates indicate that the AFM state is locally nucleated around Zn substituents in the matrix of a heavy fermion state, and percolates through the bulk at the AFM transition temperature . At lower temperatures, an anisotropic superconducting (SC) gap below the SC transition temperature , and the SC state permeates through the AFM regions via a SC proximity effect. Applying an external magnetic field induces a spin-flop transition near 5 T, reducing the volume of the AFM regions. Consequently, a short ranged inhomogeneous AFM state survives and coexists with a paramagnetic Fermi liquid state at high fields.

Spin-orbital magnetic response of relativistic fermions with band hybridization

Araki, Yasufumi; Suenaga, Daiki*; Suzuki, Kei; Yasui, Shigehiro*

Physical Review Research (Internet), 3(2), p.023098_1 - 023098_17, 2021/05

https://doi.org/10.1103/PhysRevResearch.3.023098

Spins of relativistic fermions are related to their orbital degrees of freedom. In order to quantify the effect of hybridization between relativistic and nonrelativistic degrees of freedom on spin-orbit coupling, we focus on the spin-orbital (SO) crossed susceptibility arising from spin-orbit coupling. The SO crossed susceptibility is defined as the response function of their spin polarization to the "orbital" magnetic field, namely the effect of magnetic field on the orbital motion of particles as the vector potential. Once relativistic and nonrelativistic fermions are hybridized, their SO crossed susceptibility gets modified at the Fermi energy around the band hybridization point, leading to spin polarization of nonrelativistic fermions as well. These effects are enhanced under a dynamical magnetic field that violates thermal equilibrium, arising from the interband process permitted by the band hybridization. Its experimental realization is discussed for Dirac electrons in solids with slight breaking of crystalline symmetry or doping, and also for quark matter including dilute heavy quarks strongly hybridized with light quarks, arising in a relativistic heavy-ion collision process.