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Nagai, Takayuki; Okamoto, Yoshihiro; Yamagishi, Hirona*; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2023-004, 45 Pages, 2023/09
JAEA-Research-2023-004.pdf:6.07MB
The local structure of glass-forming elements and waste elements in borosilicate glasses varies with its chemical composition. In this study, simulated waste glass samples were prepared and the chemical state regarding boron (B), silicon (Si) and waste elements of iron (Fe), cesium (Cs) were estimated by using XAFS measurement in soft X-ray region. To understand the chemical stability of simulated waste glasses, XANES spectra of B K-edge, Fe L
, L
-edge, and Cs M
, M
-edge were measured on the glass surface exposed to the leachate. As a result, it was found that the glass surface exposed to the leachate was changed and it was difficult to obtain a clear XANES spectrum. From the B K-edge XANES spectra on glass surfaces exposed to the leachate, an increase in three-coordination of B-O (BO) and a decrease in four-coordination of B-O (BO) were observed compared to the glass surfaces before immersion. The XANES spectra of Fe L, L-edge, and Cs M, M-edge show that as the exposure time in the leachate increases, the Cs present on the glass surface dissolves into the leachate. The XANES spectra of Si K-edge were measured on simulated waste glass surfaces before immersion, and it was confirmed that the change in XANES spectra given by NaO concentration had a larger effect than the waste component concentration.
Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
JPS Conference Proceedings (Internet), 33, p.011050_1 - 011050_6, 2021/03
R&D of the beam window is crucial in the ADS, which serves as a partition between the accelerator and the target region. Although the displacement per atom (DPA) is used to evaluate the damage on the window, experimental data on the displacement cross section is scarce in the energy region above 20 MeV. We started to measure the displacement cross section for the protons in the energy region between 0.4 to 3 GeV. The displacement cross section can be derived by resistivity change divided by the proton flux and the resistivity change per Frankel pair on cryo-cooled sample to maintain damage. Experiments were conducted at the 3 GeV proton synchrotron at the J-PARC Center, and aluminum and copper was used as samples. As a result of comparison between the present experiment and the calculation of the NRT model, which is widely used for calculation of the displacement cross section, it was found that the calculation of the NRT model overestimated the experiment by about 3 times.
Matsuda, Hiroki; Meigo, Shinichiro; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
Journal of Nuclear Science and Technology, 57(10), p.1141 - 1151, 2020/10
Times Cited Count：11 Percentile：75.12(Nuclear Science & Technology)To estimate the structural damages of materials in accelerator facilities, displacement per atom (dpa) is widely employed as a damage index, calculated based on the displacement cross-section obtained using a calculation model. Although dpa is applied as standard, the experimental data of the displacement cross-section for a proton in the energy region above 20 MeV are scarce. Among the calculation models, difference of about factor 8 exist, so that the experimental data of the cross-section are crucial to validate the model. To obtain the displacement cross-section, we conducted experiments at J-PARC. The displacement cross-section of copper and iron was successfully obtained for a proton projectile with the kinetic energies, 0.4 - 3 GeV. The results were compared with those obtained using the widely utilized Norgertt-Robinson-Torrens (NRT) model and the athermal-recombination-corrected (arc) model based on molecular dynamics. It was found that the NRT model overestimates the present displacement cross-section by 3.5 times. The calculation results obtained using with the arc model based on the Nordlund parameter show remarkable agreement with the experimental data. It can be concluded that the arc model must be employed for the dpa calculation for the damage estimation of copper and iron.
Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
EPJ Web of Conferences, 239, p.06006_1 - 06006_4, 2020/09
Times Cited Count：0 Percentile：0.1(Nuclear Science & Technology)R&D of the beam window is crucial in the ADS, which serves as a partition between the accelerator and the target region. Although the displacement per atom (DPA) is used to evaluate the damage on the window, experimental data on the displacement cross section is scarce in the energy region above 20 MeV. We started to measure the displacement cross section for the protons in the energy region between 0.4 to 3 GeV. The displacement cross section can be derived by resistivity change divided by the proton flux and the resistivity change per Frankel pair on cryo-cooled sample to maintain damage. Experiments were conducted at the 3 GeV proton synchrotron at the J-PARC Center, and copper was used as samples. As a result of comparison between the present experiment and the calculation of the NRT model, which is widely used for calculation of the displacement cross section, it was found that the calculation of the NRT model overestimated the experiment by about 3 times.
Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Yoshida, Makoto*; Hasegawa, Shoichi; Maekawa, Fujio; Iwamoto, Hiroki; Nakamoto, Tatsushi*; Ishida, Taku*; Makimura, Shunsuke*
JPS Conference Proceedings (Internet), 28, p.061004_1 - 061004_6, 2020/02
no abstracts in English
Aso, Tomokazu; Teshigawara, Makoto; Hasegawa, Shoichi; Muto, Hideki; Aoyagi, Katsuhiro; Nomura, Kazutaka; Takada, Hiroshi
Journal of Physics; Conference Series, 1021(1), p.012085_1 - 012085_4, 2018/06
Times Cited Count：0 Percentile：0.11(Nuclear Science & Technology)Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Yosuke; Iwamoto, Hiroki; Hasegawa, Shoichi; Maekawa, Fujio; Yoshida, Makoto*; Ishida, Taku*; Makimura, Shunsuke*; Nakamoto, Tatsushi*
Proceedings of 9th International Particle Accelerator Conference (IPAC '18) (Internet), p.499 - 501, 2018/06
no abstracts in English
Aso, Tomokazu; Teshigawara, Makoto; Hasegawa, Shoichi; Aoyagi, Katsuhiro*; Muto, Hideki*; Nomura, Kazutaka*; Takada, Hiroshi; Ikeda, Yujiro
JAEA-Technology 2017-021, 75 Pages, 2017/08
JAEA-Technology-2017-021.pdf:33.03MB
Liquid hydrogen is employed as a cold neutron moderator material at the spallation neutron source of Materials and Life science experimental Facility of Japan Proton Accelerator Research Complex (J-PARC). From January 2015, it became observable that the differential pressure between heat exchangers and an 80 K adsorber (ADS) in a helium refrigerator system increased with operating time. In November 2015, the differential pressure rise became more significant, leading to degrade the refrigerating performance in cooling liquid hydrogen. In order to investigate the cause of the abnormal differential pressure rise between the heat exchangers and the ADS, we carried out visual inspection inside the heat exchangers and analyzed the impurities contained in the helium gas. Unfortunately, we could not identify the impurities causing the performance degradation, but observed a trace of oil in the inlet piping of the heat exchanger. Based on investigations of the abnormal events occurred in the refrigerators with similar refrigerating capacity at other facilities, we took measures that cleaning the heat exchangers with Freon and replacing the ADS with new one. As a result, the differential pressure rise phenomenon was removed to recover the performance. We have detected oil from the Freon used for cleaning the heat exchangers and at a felt supporting charcoal packed in the ADS. In particular, oil was accumulated in membranous form onto the felt at the entrance side in the ADS. The amount of oil contained in the helium gas was about 10 ppb or so, less than the design value, in the helium refrigerator. However, the oil accumulated onto the felt in the ADS through long operating period may cause abnormal differential pressure rise, leading to the performance degradation of the helium refrigerator. Further study is needed to specify the cause more clearly.
Li, Y.; Hasegawa, Kunio*; Udagawa, Makoto
Journal of Pressure Vessel Technology, 139(2), p.021202_1 - 021202_13, 2017/04
Times Cited Count：2 Percentile：12.73(Engineering, Mechanical)Ozeki, Hidemasa; Isono, Takaaki; Kawano, Katsumi; Saito, Toru; Kawasaki, Tsutomu; Nishino, Katsumi; Okuno, Kiyoshi; Kido, Shuichi*; Semba, Tomoyuki*; Suzuki, Yozo*; et al.
IEEE Transactions on Applied Superconductivity, 25(3), p.4200804_1 - 4200804_4, 2015/06
Times Cited Count：0 Percentile：0(Engineering, Electrical & Electronic)Suzuki, Sadaaki; Yagyu, Junichi; Masaki, Kei; Nishiyama, Tomokazu; Nakamura, Shigetoshi; Saeki, Hisashi; Hoshi, Ryo; Sawai, Hiroaki; Hasegawa, Koichi; Arai, Takashi; et al.
NIFS-MEMO-67, p.266 - 271, 2014/02
no abstracts in English
Kakei, Sadanori*; Kimura, Akihiro; Niizeki, Tomotake*; Ishida, Takuya; Nishikata, Kaori; Kurosawa, Makoto; Yoshinaga, Hideo*; Hasegawa, Yoshio*; Tsuchiya, Kunihiko
Proceedings of 6th International Symposium on Material Testing Reactors (ISMTR-6) (Internet), 7 Pages, 2013/10
The Japan Materials Testing Reactor (JMTR) is expected to contribute to the expansion of industrial utilization, such as the domestic production of 
Mo for the medical diagnosis medicine 
Tc. Production by the (n, 
) method is proposed as domestic Mo production in JMTR because of the low amount of radioactive wastes and the easy Mo/Tc production process. Molybdenum oxide (MoO) pellets, poly zirconium compounds (PZC) and poly titanium compounds (PTC) are used as the irradiation target and generator for the production of Mo/Tc by the (n, ) method. However, it is necessary to use the enriched 
MoO, which is very expensive, to increase the specific activity of Mo. Additionally, a large amount of used PZC and PTC is generated after the decay of Mo. Therefore, this recycling technology of used PZC/PTC has been developed to recover molybdenum (Mo) as an effective use of resources and a reduction of radioactive wastes. The total Mo recovery rate of this process was 95.8%. From the results of the hot experiments, we could demonstrate that the recovery of MoO and the recycling of PZC are possible. In the future, the equipment of recovering Mo will be installed in JMTR-Hot Cell, and this recycling process will be able to contribute to the reduction of production costs of Tc and the reduction of radioactive wastes.
][1]benzothiophene monolayer on bismuth-terminated Si(111) vicinal surfaces with wettability optimizationOtomo, Manabu; Tsuchida, Yuya*; Muraya, Naoki*; Yanase, Takashi*; Sakai, Seiji; Yonezawa, Tetsu*; Nagahama, Taro*; Hasegawa, Tetsuya*; Shimada, Toshihiro*
Journal of Physical Chemistry C, 117(22), p.11555 - 11561, 2013/06
Times Cited Count：2 Percentile：8.68(Chemistry, Physical)We report in-plane orientation control of newly developed high-mobility organic semiconductor: 2,7-diphenyl[1]benzothieno[3,2-][1]benzothiophene (DPh-BTBT). As previously reported on monolayer pentacene, it was revealed that bunched steps on vicinal Si(111) with bismuth termination break the surface symmetry and reduce three-fold symmetry of DPh-BTBT grains into quasi-single orientation. Interestingly, the critical step height necessary for the orientation control was different from that of pentacene. We examined several mechanisms of orientation control and concluded that the facet nano structure fabricated by step bunching is working as an anisotropic template. We will also show the wettability control of bismuth terminated silicon surface and show that the growth mode of DPh-BTBT is dependent on the surface nanostructure of Bi-Si.
Murakami, Haruyuki; Kizu, Kaname; Tsuchiya, Katsuhiko; Yoshida, Kiyoshi; Yamauchi, Kunihito; Shimada, Katsuhiro; Terakado, Tsunehisa; Matsukawa, Makoto; Hasegawa, Mitsuru*; Minato, Tsuneaki*; et al.
IEEE Transactions on Applied Superconductivity, 22(3), p.9501405_1 - 9501405_5, 2012/06
Times Cited Count：4 Percentile：29.13(Engineering, Electrical & Electronic)The withstand voltage of turn insulation is essential issues for the superconducting magnet. The actual turn voltage is larger than the turn voltage under the ideal condition because of the voltage fluctuations of the power supply and the resonance phenomenon in the magnet. In this paper, the voltage measurement of the JT-60U power supply and the resonance characteristics of the EF4 are described. The actual maximum turn voltage is almost same as the voltage under the ideal condition.
Sakai, Kenji; Sakamoto, Shinichi; Kinoshita, Hidetaka; Seki, Masakazu; Haga, Katsuhiro; Kogawa, Hiroyuki; Wakui, Takashi; Naoe, Takashi; Kasugai, Yoshimi; Tatsumoto, Hideki; et al.
JAEA-Technology 2011-039, 121 Pages, 2012/03
JAEA-Technology-2011-039.pdf:10.87MB
This report investigates the behavior, damage and restoration of a neutron source station of the MLF at the Great East Japan Earthquake and verified the safety design for emergency accidents in the neutron source station. In the MLF, after an occurrence of the Earthquake, strong quakes were detected at the instruments, the external power supply was lost, all of the circulators shut down automatically, and the hydrogen gas was released. The leakages of mercury, hydrogen and radio-activation gases did not occur. While, the quakes made gaps between the shield blocks and ruptured external pipe lines by subsidence around the building. But significant damages to the components were not found though the pressure drop of compressed air lines influenced on a target trolley lock system and so on. These results substantiated the validity of the safety design for emergency accidents in the source station, and suggested several points of improvement.
Sakai, Kenji; Futakawa, Masatoshi; Takada, Hiroshi; Sakamoto, Shinichi; Maekawa, Fujio; Kinoshita, Hidetaka; Seki, Masakazu; Haga, Katsuhiro; Kogawa, Hiroyuki; Wakui, Takashi; et al.
Proceedings of 20th Meeting of the International Collaboration on Advanced Neutron Sources (ICANS-20) (USB Flash Drive), 6 Pages, 2012/03
This report investigates behaviors and damages of each component in a neutron target station of the MLF at the J-PARC at the time of the Great East Japan Earthquake (GEJE). At the date of the GEJE, in the MLF, strong quakes were detected at several instruments, an external power supply were lost, all of the circulation systems were shut down automatically, and a hydrogen gas was released as planned. Leakage of activation liquids and gases did not occur. While, the quakes made gaps between shield blocks and ruptured external pipe lines for air and water by subsidence. But significant damages on the components of the target station were not found though a loss of compressed air supply affected lock systems with air cylinders and pneumatic operation values. These results substantiated a validity of safety design on the target station for emergency accidents.
Fang, Z.*; Michizono, Shinichiro*; Anami, Shozo*; Yamaguchi, Seiya*; Naito, Fujio*; Fukui, Yuji*; Kawamura, Masato*; Kubota, Chikashi*; Nammo, Kesao*; Kobayashi, Tetsuya; et al.
Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.1434 - 1436, 2010/05
The output energy of the J-PARC proton linac will be upgraded from 181 to 400 MeV in the next two years by adding high-b acceleration sections. The upgrade of the FPGA-based digital LLRF controller for the 400 MeV linac will be presented in this paper. This new LLRF controller works for both the 324-MHz low-b and 972-MHz high-b sections. Many functions have been added into the LLRF controller, such as (1) working for different RF systems, (2) gradually increasing the feedback gains in the feedback loop instead of fixed ones, (3) automatic chopped beam compensation, (4) automatically switching the beam loading compensation in accordance with different beam operation mode, (5) input RF-frequency tuning to match the RF cavities during RF start-up, and (6) auto-tuning of the RF cavity tuner by detecting the phase curve of the RF cavity during the field decay instead of the phase difference between the cavity input and output signals.
Hasegawa, Kazuo; Morishita, Takatoshi; Kondo, Yasuhiro; Oguri, Hidetomo; Kobayashi, Tetsuya; Naito, Fujio*; Yoshioka, Masakazu*; Matsumoto, Hiroshi*; Kawamata, Hiroshi*; Hori, Yoichiro*; et al.
Proceedings of 6th Annual Meeting of Particle Accelerator Society of Japan (CD-ROM), p.693 - 695, 2010/03
The J-PARC RFQ (length 3.1m, 4-vane type, 324 MHz) accelerates a beam from the ion source to the DTL. The beam test of the linac was started in November 2006 and 181 MeV beam was successfully accelerated in January 2007. Since then, the linac has been delivered beams for commissioning of the linac itself, downstream accelerators and facilities. Trip rates of the RFQ, however, suddenly increased in Autumn 2008, and we are suffering from this issue for user run operation. We tried to recover by tender conditioning, modification of RF control, improvement of vacuum and so on. We manage to have beam operation. In this report, we describe the status of the RFQ.
Maekawa, Fujio; Oikawa, Kenichi; Harada, Masahide; Kai, Tetsuya; Meigo, Shinichiro; Kasugai, Yoshimi; Oi, Motoki; Sakai, Kenji; Teshigawara, Makoto; Hasegawa, Shoichi; et al.
Nuclear Instruments and Methods in Physics Research A, 600(1), p.335 - 337, 2009/02
Times Cited Count：42 Percentile：92.82(Instruments & Instrumentation)A neutron beam line (BL10) of JSNS, NOBORU, has been constructed in the Materials and Life Science Experimental Facility (MLF) at J-PARC. A primal mission of NOBORU is to study neutronic performance of JSNS. We will measure the memorable first neutron pulse of JSNS at the Day-one by using NOBORU, and then measure neutron pulse shape, spectrum, intensity distribution, etc. for facility diagnostics. Since NOBORU also has an aspect as a test port, it welcomes trial uses to develop innovative instruments. Trial experiments to demonstrate several innovative instruments at NOBORU are under planning.
Hasegawa, Kazuo; Asano, Hiroyuki; Chishiro, Etsuji; Hori, Toshihiko; Ito, Takashi; Kobayashi, Tetsuya; Kondo, Yasuhiro; Namekawa, Yuya; Oguri, Hidetomo; Okoshi, Kiyonori; et al.
Proceedings of 24th International Linear Accelerator Conference (LINAC 2008) (CD-ROM), p.55 - 57, 2009/00
The beam commissioning of the J-PARC linac started in November 2006 and 181 MeV acceleration was successfully achieved in January 2007. The linac has delivered beams to the 3 GeV Rapid Cycling Synchrotron for its commissioning, and then, the subsequent Main Ring Synchrotron and the neutron target commissioning. The linac uses a Cs-free LaB
-driven ion source and 20 units of 324 MHz klystrons. As of June 2008, the operation times are about 3,000 and 6,000 hours for the ion source and the RF source, respectively. The operating experience of the linac is described.
