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Sekine, Yurina; Nankawa, Takuya; Hiroi, Kosuke; Oba, Yojiro*; Nagakawa, Yoshiyasu*; Sugita, Tsuyoshi; Shibayama, Yuki; Ikeda-Fukazawa, Tomoko*
Carbohydrate Polymers, 327, p.121538_1 - 121538_11, 2024/03
We describe non-toxic, tough nanocellulose (NC) hydrogels formed from chemically unmodified NC by cellulose crystalline transformation and subsequent freeze cross-linking reaction. Using low-concentration NaOH and freezing together induced the crystalline transformation of NC from cellulose I to II via freeze concentration. After the crystalline transformation, cross-linking between the NC and CA in the freeze concentration layer (FCL) provided a strong NC network structure, forming NC hydrogels with high mechanical strength. The freeze-cross-linked NC hydrogel easily retained powder adsorbents in its inner space by mixing the NC-NaOH sol and the powder, and the hydrogel showed high removal efficiency for heavy metals. The results highlight the versatility of chemically unmodified celluloses in developing functional materials, suggest possible practical applications.
Fujiwara, Hidenori*; Nakatani, Yasuhiro*; Aratani, Hidekazu*; Kanai-Nakata, Yuina*; Yamagami, Kohei*; Hamamoto, Satoru*; Kiss, Takayuki*; Sekiyama, Akira*; Tanaka, Arata*; Ebihara, Takao*; et al.
New Physics; Sae Mulli, 73(12), p.1062 - 1066, 2023/12
Fujiwara, Hidenori*; Nakatani, Yasuhiro*; Aratani, Hidekazu*; Kanai, Yuina*; Yamagami, Kohei*; Hamamoto, Satoru*; Kiss, Takayuki*; Yamasaki, Atsushi*; Higashiya, Atsushi*; Imada, Shin*; et al.
Physical Review B, 108(16), p.165121_1 - 165121_10, 2023/10
Kumada, Takayuki; Nakagawa, Hiroshi; Miura, Daisuke; Sekine, Yurina; Motokawa, Ryuhei; Hiroi, Kosuke; Inamura, Yasuhiro; Oku, Takayuki; Oishi, Kazuki*; Morikawa, Toshiaki*; et al.
Journal of Physical Chemistry Letters (Internet), 14(34), p.7638 - 7643, 2023/08
The structure of nano-ice crystals in rapidly frozen glucose solution was elucidated by using spin-contrast-variation small-angle neutron scattering, which distinguishes the nano-ice crystal signal from the frozen amorphous solution signal by the polarization-dependent neutron scattering. The analysis revealed that the nano-ice crystals form a planar structure with a diameter exceeding tens of nanometers and a thickness of 1 nm, which is close to the critical nucleation size. This result suggests that the glucose molecules are preferentially bound to a specific face of nano-ice crystals, and then block the crystal growth perpendicular to that face.
Ohshima, Hiroyuki; Asayama, Tai; Furukawa, Tomohiro; Tanaka, Masaaki; Uchibori, Akihiro; Takata, Takashi; Seki, Akiyuki; Enuma, Yasuhiro
Journal of Nuclear Engineering and Radiation Science, 9(2), p.025001_1 - 025001_12, 2023/04
This paper describes the outline and development plan for ARKADIA to transform advanced nuclear reactor design to meet expectations of a safe, economic, and sustainable carbon-free energy source. ARKADIA will realize Artificial Intelligence (AI)-aided integrated numerical analysis to offer the best possible solutions for the design and operation of a nuclear plant, including optimization of safety equipment. State-of-the-art numerical simulation technologies and a knowledge base that stores data and insights from past nuclear reactor development projects and R&D are integrated with AI. In the first phase of development, ARKADIA-Design and ARKADIA-Safety will be constructed individually, with the first target of sodium-cooled reactor. In a subsequent phase, everything will be integrated into a single entity applicable not only to advanced rectors with a variety of concepts, coolants, configurations, and output levels but also to existing light-water reactors.
Sato, Tatsuhiko; Iwamoto, Yosuke; Hashimoto, Shintaro; Ogawa, Tatsuhiko; Furuta, Takuya; Abe, Shinichiro; Kai, Takeshi; Matsuya, Yusuke; Matsuda, Norihiro; Hirata, Yuho; et al.
Journal of Nuclear Science and Technology, 9 Pages, 2023/00
The Particle and Heavy Ion Transport code System (PHITS) is a general-purpose Monte Carlo radiation transport code that can simulate the behavior of most particle species with energies up to 1 TeV (per nucleon for ions). Its new version, PHITS3.31, was recently developed and released to the public. In the new version, the compatibility with high-energy nuclear data libraries and the algorithm of the track-structure modes have been improved. In this paper, we summarize the upgraded features of PHITS3.31 with respect to the physics models, utility functions, and application software introduced since the release of PHITS3.02 in 2017.
Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.
JAEA-Research 2020-007, 249 Pages, 2020/10
The accident of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, Japan Atomic Energy Agency (JAEA) has been conducting "Long-term Assessment of Transport of Radioactive Contaminants in the Environment of Fukushima" concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.
Seki, Akiyuki; Mayumi, Akie; Wainwright-Murakami, Haruko*; Saito, Kimiaki; Takemiya, Hiroshi; Idomura, Yasuhiro
Proceedings of Joint International Conference on Supercomputing in Nuclear Applications + Monte Carlo 2020 (SNA + MC 2020), p.158 - 164, 2020/10
We developed a method to estimate the temporal change of the air dose rate at the location with sparse (in time) measurements by using the continuous measurement data from the nearby monitoring post. This method determines an observation model from the correlation between sparse data at the target location and dense data at the monitoring post based on a hierarchical Bayesian model. The developed method was validated against the air dose rate measured at the monitoring posts in Fukushima prefecture from 2012 to 2017. The results showed that the developed method can predict the air dose rate at almost all target locations with an error rate of less than 10%.
Sekihara, Takayasu; Oset, E.*; Ramos, A.*
JPS Conference Proceedings (Internet), 26, p.023009_1 - 023009_4, 2019/11
Nagao, Fumiya; Niizato, Tadafumi; Sasaki, Yoshito; Ito, Satomi; Watanabe, Takayoshi; Dohi, Terumi; Nakanishi, Takahiro; Sakuma, Kazuyuki; Hagiwara, Hiroki; Funaki, Hironori; et al.
JAEA-Research 2019-002, 235 Pages, 2019/08
The accident of the Fukushima Daiichi Nuclear Power Station (hereinafter referred to 1F), Tokyo Electric Power Company Holdings, Inc. occurred due to the Great East Japan Earthquake, Sanriku offshore earthquake, of 9.0 magnitude and the accompanying tsunami. As a result, large amount of radioactive materials was released into the environment. Under these circumstances, JAEA has been conducting Long-term Environmental Dynamics Research concerning radioactive materials released in environment, especially migration behavior of radioactive cesium since November 2012. This report is a summary of the research results that have been obtained in environmental dynamics research conducted by JAEA in Fukushima Prefecture.
Yamagata-Sekihara, Junko*; Sekihara, Takayasu
Physical Review C, 100(1), p.015203_1 - 015203_12, 2019/07
Times Cited Count:2 Percentile:23.44(Physics, Nuclear)Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.
Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09
Times Cited Count:4 Percentile:26.15(Materials Science, Multidisciplinary)Kitayama, Kyo*; Morino, Yu*; Takigawa, Masayuki*; Nakajima, Teruyuki*; Hayami, Hiroshi*; Nagai, Haruyasu; Terada, Hiroaki; Saito, Kazuo*; Shimbori, Toshiki*; Kajino, Mizuo*; et al.
Journal of Geophysical Research; Atmospheres, 123(14), p.7754 - 7770, 2018/07
Times Cited Count:24 Percentile:70.42(Meteorology & Atmospheric Sciences)We compared seven atmospheric transport model results for Cs released during the Fukushima Daiichi Nuclear Power Plant accident. All the results had been submitted for a model intercomparison project of the Science Council of Japan in 2014. We assessed model performance by comparing model results with observed hourly atmospheric concentrations of Cs, focusing on nine plumes over the Tohoku and Kanto regions. The results showed that model performance for Cs concentrations was highly variable among models and plumes. We also assessed model performance for accumulated Cs deposition. Simulated areas of high deposition were consistent with the plume pathways, though the models that best simulated Cs concentrations were different from those that best simulated deposition. The ensemble mean of all models consistently reproduced Cs concentrations and deposition well, suggesting that use of a multimodel ensemble results in more effective and consistent model performance.
Rodriguez, D.; Tanigawa, Masafumi; Nishimura, Kazuaki; Mukai, Yasunobu; Nakamura, Hironobu; Kurita, Tsutomu; Takamine, Jun; Suzuki, Satoshi*; Sekine, Megumi; Rossi, F.; et al.
Journal of Nuclear Science and Technology, 55(7), p.792 - 804, 2018/07
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)Nuclear material in reprocessing facilities is safeguarded by random sample verification with additional continuous monitoring applied to solution masses and volume in important tanks to maintain continuity-of-knowledge of process operation. Measuring the unique rays of each solution as the material flows through pipes connecting all tanks and process apparatuses could potentially improve process monitoring by verifying the compositions in real time. We tested this ray pipe-monitoring method using plutonium-nitrate solution transferred between tanks at the PCDF-TRP. The rays were measured using a lanthanum-bromide detector with a list-mode data acquisition system to obtain both time and energy of -ray. The analysis and results of this measurement demonstrate an ability to determine isotopic composition, process timing, flow rate, and volume of solution flowing through pipes, introducing a viable capability for process monitoring safeguards verification.
Sekihara, Takayasu; Kamiya, Yuki*; Hyodo, Tetsuo*
Physical Review C, 98(1), p.015205_1 - 015205_20, 2018/07
Times Cited Count:20 Percentile:85.79(Physics, Nuclear)Sekihara, Takayasu; Fujioka, Hiroyuki*; Ishikawa, Takatsugu*
Physical Review C, 97(4), p.045202_1 - 045202_9, 2018/04
Times Cited Count:4 Percentile:36.63(Physics, Nuclear)Nakatani, Yasuhiro*; Aratani, Hidekazu*; Fujiwara, Hidenori*; Mori, Takeo*; Tsuruta, Atsushi*; Tachibana, Shoichi*; Yamaguchi, Takashi*; Kiss, Takayuki*; Yamasaki, Atsushi*; Yasui, Akira*; et al.
Physical Review B, 97(11), p.115160_1 - 115160_7, 2018/03
Times Cited Count:3 Percentile:20.97(Materials Science, Multidisciplinary)Sekihara, Takayasu; Oset, E.*; Ramos, A.*
Proceedings of Science (Internet), 310, p.199_1 - 199_5, 2018/03
Nagai, Kodai*; Fujiwara, Hidenori*; Aratani, Hidekazu*; Fujioka, Shuhei*; Yomosa, Hiroshi*; Nakatani, Yasuhiro*; Kiss, Takayuki*; Sekiyama, Akira*; Kuroda, Fumiaki*; Fujii, Hitoshi*; et al.
Physical Review B, 97(3), p.035143_1 - 035143_8, 2018/01
Times Cited Count:21 Percentile:70.56(Materials Science, Multidisciplinary)We have studied the electronic structure of ferrimagnetic MnVAl single crystals by means of soft X-ray absorption spectroscopy (XAS), X-ray absorption magnetic circular dichroism (XMCD), and resonant soft X-ray inelastic scattering (RIXS). We have successfully observed the XMCD signals for all the constituent elements. The Mn L XAS and XMCD spectra are reproduced by spectral simulations based on density-functional theory, indicating the itinerant character of the Mn 3 states. On the other hand, the V 3 electrons are rather localized since the ionic model can qualitatively explain the V L XAS and XMCD spectra. This picture is consistent with local excitations revealed by the V L RIXS.
Sekihara, Takayasu; Oset, E.*; Ramos, A.*
Acta Physica Polonica B, 48(10), p.1869 - 1874, 2017/10
Times Cited Count:1 Percentile:12.14(Physics, Multidisciplinary)