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Journal Articles

Measurement of the displacement cross-section of copper irradiated with 125 MeV protons at 12 K

Iwamoto, Yosuke; Yoshiie, Toshimasa*; Yoshida, Makoto*; Nakamoto, Tatsushi*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Xu, Q.*; Yashima, Hiroshi*; et al.

Journal of Nuclear Materials, 458, p.369 - 375, 2015/03

 Times Cited Count:13 Percentile:73.22(Materials Science, Multidisciplinary)

To validate Monte Carlo codes for the prediction of radiation damage in metals irradiated by $$>$$100 MeV protons, defect-induced electrical resistivity changes of copper related to the displacement cross-section were measured with 125 MeV proton irradiation at 12 K. The cryogenic irradiation system was developed with a Gifford-McMahon cryocooler to cool the sample via an oxygen-free high-conductivity copper plate by conduction cooling. The sample was a copper wire with a 250$$mu$$m diameter and 99.999% purity sandwiched between two aluminum nitride ceramic sheets. The resistivity increase did not change during annealing after irradiation below 15 K. The experimental displacement cross-section for 125 MeV irradiation shows similar results to the experimental data for 1.1 and 1.94 GeV. Comparison with the calculated results indicated that the defect production efficiency in Monte Carlo codes gives a good quantitative description of the displacement cross-section in the energy region $$>$$ 100 MeV.

Oral presentation

Study of measurement of displacement cross section for copper irradiated with 125 MeV proton

Iwamoto, Yosuke; Yoshida, Makoto*; Nakamoto, Tatsushi*; Ogitsu, Toru*; Yoshiie, Toshimasa*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Mori, Yoshiharu*

no journal, , 

We measured the electrical resistivity under irradiation of 125 MeV proton in copper sample (0.2 um thickness) at cryogenic temperature at the FFAG accelerator facility in Kyoto university. Resistivity was measured by the four-terminal method. As a result, we measured the resistivity of copper at 7.3 K within 20 micro-ohm and temperature of sample. We measured the electrical resistivity under irradiation of 125 MeV proton in copper sample (0.2 um thickness) at cryogenic temperature at the FFAG accelerator facility in Kyoto university. Resistivity was measured by the four-terminal method. As a result, we measured the resistivity of copper at 7.3 K within 20 micro-ohm and temperature of sample.

Oral presentation

Development of the device for electrical resistivity measurements for proton irradiation under cryogenic condition

Iwamoto, Yosuke; Yoshiie, Toshimasa*; Yoshida, Makoto*; Nakamoto, Tatsushi*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Xu, Q.*; Yashima, Hiroshi*; et al.

no journal, , 

To validate the radiation damage calculation in the PHITS code for proton irradiation over 100 MeV, we have developed the device for electrical resistance measurement under cryogenic condition. A copper wire with 99.999% purity in a diameter of 250-$$mu$$m was set with a serpentine-shaped line on the AlN sheet which has high thermal conductivity and electric insulation. The sample was annealed for 1 h at 1,000$$^{circ}$$C before irradiation. After annealing, the sample was cooled with an oxygen-free high-conductivity copper plate by conduction cooling. The electrical resistivity changes in the sample were measured using the four-probe technique. As a result, the residual resistivity ratio of the sample was about 1,800 between room temperature and 11 K. After 125 MeV proton irradiation with 1.45$$times$$10$$^{14}$$(proton/cm$$^{2}$$) at 11 K, the total resistance increase was 1.53$$mu$$ $$Omega$$, while the resistivity of copper before irradiation was 29.41$$mu$$ $$Omega$$.

Oral presentation

Measurement of the damage rate of copper irradiated with 125 MeV protons at 12 K and comparison with calculated result with the PHITS code

Iwamoto, Yosuke; Yoshiie, Toshimasa*; Yoshida, Makoto*; Nakamoto, Tatsushi*; Sakamoto, Masaaki*; Kuriyama, Yasutoshi*; Uesugi, Tomonori*; Ishi, Yoshihiro*; Xu, Q.*; Yashima, Hiroshi*; et al.

no journal, , 

To validate Monte Carlo code PHITS for the prediction of radiation damage in metals, the damage rate (defect-induced electrical resistivity changes / particle fluence) related to the displacement cross-section of copper were measured with 125 MeV proton irradiation under 12 K at the FFAG facility in the Kyoto University Research Reactor Institute. The sample was a copper wire with a 250-$$mu$$m diameter and 99.999% purity and was cooled by conduction cooling. After 125 MeV proton irradiation with 1.45$$times$$10$$^{18}$$ protons/m$$^{2}$$ at 12 K, the total resistivity increase was 4.94$$times$$10$$^{-13}$$$$Omega$$m (resistance increase: 1.53$$mu$$$$Omega$$), while the resistivity of copper before irradiation was 9.49 $$times$$10$$^{-12}$$$$Omega$$m (resistance: 29.41$$mu$$$$Omega$$). Comparison with other experimental results indicated that the damage rate by 125 MeV protons is almost same with those by 1.1 GeV protons and is higher than the damage rate by 14 MeV neutrons by a factor of 1.4. For the comparison with the PHITS results, the experimental data is smaller than the calculated result without the defect production efficiency by a factor of about 2.5 and that with the defect production efficiency by a factor of about 1.4, respectively. It indicates that the defect production efficiency in PHITS gives a good quantitative description of the displacement cross-section.

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