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Journal Articles

Activity report of the Task Group on Parameters Used in Biospheric Dose Assessment Models for Radioactive Waste Disposal

Takahashi, Tomoyuki*; Fukaya, Yukiko*; Iimoto, Takeshi*; Uni, Yasuo*; Kato, Tomoko; Sun, S.*; Takeda, Seiji; Nakai, Kunihiro*; Nakabayashi, Ryo*; Uchida, Shigeo*; et al.

Hoken Butsuri (Internet), 56(4), p.288 - 305, 2021/12

We report the results of activities related to the Task Group of Parameters Used in Biospheric Dose Assessment Models for Radioactive Waste Disposal at the Japan Health Physics Society.

Journal Articles

Discussion; Making databases of parameter values of radionuclide transfer in environment and application for biospheric dose assessment

Takahashi, Tomoyuki*; Uchida, Shigeo*; Takeda, Seiji; Nakai, Kunihiro*

KURNS-EKR-11, p.97 - 102, 2021/03

This paper outlines the status of IAEA database compilation for migration parameters depending elements in a biosphere such as soil-to-plant transfer factor and bioconcentration factor of marine products, and the status of utilization of the database in dose evaluation of radioactive waste disposal in Japan. Additionally, in the case of applying a new database to the dose evaluation for future radioactive waste disposal in a specific area. We summarized the opinions of specialists and result of general discussion about future strategies to make a new database for their parameters, perspectives to be considered in it, issues, etc.

Journal Articles

Simple pretreatment method for tritium measurement in environmental water samples using a liquid scintillation counter

Nakasone, Shunya*; Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; et al.

Plasma and Fusion Research (Internet), 16, p.2405035_1 - 2405035_5, 2021/02

Removal of impurities such as organic and other types of dissolved matters from environmental water samples is required for precise analysis of tritium with a liquid scintillation counting method. In general, a distillation method is a conventional one for tritium analysis in environmental water samples, but is a time-consuming process that takes 24 hours for removal of impurities. We have proposed a rapid pretreatment method for tritium analysis, that uses ion exchange resins. In this study, we performed batch experiments, to evaluate the effectiveness of the ion exchange resins on the tritium measurement. The results obtained demonstrated that removal of impurities in the sample water by ion exchange resins can be achieved during a short period of time (i.e., in 5 min).

Journal Articles

Observation of morphological abnormalities in silkworm pupae after feeding $$^{137}$$CsCl-supplemented diet to evaluate the effects of low dose-rate exposure

Tanaka, Sota; Kinouchi, Tadatoshi*; Fujii, Tsuguru*; Imanaka, Tetsuji*; Takahashi, Tomoyuki*; Fukutani, Satoshi*; Maki, Daisuke*; Notomi, Akihiro*; Takahashi, Sentaro*

Scientific Reports (Internet), 10, p.16055_1 - 16055_7, 2020/09

 Times Cited Count:7 Percentile:49.75(Multidisciplinary Sciences)

Since the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident, morphological abnormalities of the lepidopteran insects have been reported. However, it is unclear whether the abnormalities were caused directly by radiation because they did not study on absorbed dose and dose-effect relationship. In this study, we conducted an internal exposure experiment on silkworm using $$^{137}$$CsCl-supplemented artificial diet and estimated the absorbed dose to evaluate the morphological abnormalities in silkworm. The ratio of wing to whole body of pupae was compared between the $$^{137}$$CsCl-exposured and control groups and no significant differences were observed between the groups. This result suggest that morphological abnormalities in lepidopterans are unlikely due to direct radiation effects from $$^{137}$$Cs contamination after the FDNPP accident.

Journal Articles

Preliminary investigation of pretreatment methods for liquid scintillation measurements of environmental water samples using ion exchange resins

Nakasone, Shunya*; Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; et al.

Plasma and Fusion Research (Internet), 15, p.2405027_1 - 2405027_3, 2020/05

A quick preprocessing system for tritium analysis of environmental samples is important to judge environmental influence of tritium releases due to accident or tritium-handling facilities. Analysis of tritium in water samples with liquid scintillation counting method requires removal of impurities such as organic matter and ion species from water samples. Generally, a distillation method is adopted as a pretreatment of analysis for tritium; however, the distillation method is a time-consuming process. The aim of this study is to evaluate a rapid pretreatment method for tritium analysis with ion exchange resin. From batch and column experiments that used inland water and ion exchange resin, we confirmed removals of impurities of the water sample and that the removal of impurities was possible for a short time (by 5 minutes).

Journal Articles

Radioactive cesium contamination of arthropods and earthworms after the Fukushima Daiichi Nuclear Power Plant Accident

Tanaka, Sota; Adachi, Taro*; Takahashi, Tomoyuki*; Takahashi, Sentaro*

Low-Dose Radiation Effects on Animals and Ecosystems; Long-Term Study on the Fukushima Nuclear Accident, p.43 - 52, 2020/00

 Times Cited Count:1 Percentile:12.16(Ecology)

To understand the behavior of radiocesium in terrestrial invertebrates, chronological changes in the concentration of radiocesium in arthropods and earthworms from different trophic levels were investigated after the Fukushima Daiichi Nuclear Power Plant accident. The median radiocesium concentrations in the rice grasshopper, Oxya yezoensis, and the Emma field cricket, Teleogryllus emma, were 0.46 and 0.15 Bq/g fw in 2012, respectively, which dropped continuously to 0.05 and 0.01 Bq/g fw in 2016. In contrast, no significant reduction in radiocesium concentration was observed in the Joro Spider, Nephila clavata, in which the concentration was 0.31 Bq/g fw in 2012 and remained at 0.14 Bq/g fw in 2016. The comparison of radiocesium concentrations at each trophic level showed that the amount in detritivorous earthworms was 85 times higher than in herbivorous grasshoppers. This suggests that detritus food web could be a primary pathway of radiocesium through food webs.

Journal Articles

Radiocesium concentration in flying insects collected from a radioactive contaminated area after the Fukushima Dai-ichi Nuclear Power Plant accident

Tanaka, Sota; Kakinuma, Hotaru*; Adachi, Taro*; Takahashi, Tomoyuki*; Takahashi, Sentaro*

KEK Proceedings 2019-2, p.179 - 182, 2019/11

The concentration of $$^{137}$$Cs in flying insects was investigated after the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. The insects were collected at about 11 km north west of the FDNPP at two different sites in the forest and riverside. The median concentration of $$^{137}$$Cs in flying insects in the forest was significantly higher than riverside. However, high concentration of $$^{137}$$Cs in detritus fly (Diptera: Calliphoridae) was observed at both sites. The concentration of fly at the forest and riverside were 16$$times$$10$$^{2}$$ Bq/kg fw and 18$$times$$10$$^{2}$$ Bq/kg fw, respectively. The result shows that the concentration of radiocesium in detritus fly were still high 8 years after the accident. This suggests that detritus food chain is a dominant transfer pathway of radiocesium to higher trophic level species such as spiders.

Journal Articles

Development of field estimation technique and improvement of environmental tritium behavior model

Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; Atarashi-Andoh, Mariko; et al.

Plasma and Fusion Research (Internet), 14(Sp.2), p.3405099_1 - 3405099_4, 2019/06

The Large Helical Device of the National Institute for Fusion Science started D-D experiments in 2017. To ensure the safety of the facility, it is important to develop evaluation methods for environmental tritium transfer. Tritiated water (HTO) in atmosphere and soil is transferred to plants, and organically bound tritium (OBT) is formed by photosynthesis. Prediction of OBT formation is important, because OBT accumulates in plants and causes dose through ingestion. The objective of this study is to estimate environmental tritium transfer using a simple compartment model and practical parameters. We proposed a simple compartment model consisting of air-soil-plant components, and tried to validate the model by comparison with a sophisticated model, SOLVEG. In this study, we plan to add wet deposition to the model and obtain parameters from measurements of soil permeability and tritium concentrations in air, soil and plants. We also establish rapid pretreatment methods for OBT analysis.

Journal Articles

Estimation of the release time of radio-tellurium during the Fukushima Daiichi Nuclear Power Plant accident and its relationship to individual plant events

Takahashi, Sentaro*; Kawashima, Shigeto*; Hidaka, Akihide; Tanaka, Sota*; Takahashi, Tomoyuki*

Nuclear Technology, 205(5), p.646 - 654, 2019/05

AA2017-0503.pdf:1.22MB

 Times Cited Count:4 Percentile:41.24(Nuclear Science & Technology)

Journal Articles

Long-term predictions of ambient dose equivalent rates after the Fukushima Daiichi Nuclear Power Plant accident

Kinase, Sakae; Takahashi, Tomoyuki*; Saito, Kimiaki

Journal of Nuclear Science and Technology, 54(12), p.1345 - 1354, 2017/12

 Times Cited Count:26 Percentile:92.78(Nuclear Science & Technology)

Journal Articles

Uncertainty in predictions of the ambient dose equivalent rates for 30 years following the Fukushima Daiichi Nuclear Power Plant accident

Kinase, Sakae; Takahashi, Tomoyuki*; Sato, Satoshi; Yamamoto, Hideaki; Saito, Kimiaki

Proceedings of 17th NSFS Conference (Internet), p.27 - 33, 2016/02

Journal Articles

Prediction of ambient dose equivalent rates for the next 30 years after the accident

Kinase, Sakae; Takahashi, Tomoyuki*; Sato, Satoshi*; Yamamoto, Hideaki; Saito, Kimiaki

Proceedings of International Symposium on Radiological Issues for Fukushima's Revitalized Future, p.40 - 43, 2015/00

To support recovery and rehabilitation in Fukushima, prediction models have been developed for ambient dose equivalent rate distribution within the 80 km-radius around the Fukushima Daiichi Nuclear Power Plant. The prediction models that are based on bi-exponential functions characterized by ecological half-lives of radioactive caesium for land-use, enable Fukushima residents to obtain distribution maps of ambient dose equivalent rates for the next 30 years after the accident. Model parameters were evaluated using ambient dose equivalent rates through car-borne surveys. The model parameters in deciduous and evergreen forest areas were found to be different from those in other areas. In addition, it was found that distribution maps of ambient dose equivalent rates for the next 30 years after the accident, created by the prediction models would be useful for follow-up of the radiological situation.

Journal Articles

Development of prediction models for radioactive caesium distribution within the 80-km radius of the Fukushima Daiichi Nuclear Power Plant

Kinase, Sakae; Takahashi, Tomoyuki*; Sato, Satoshi; Sakamoto, Ryuichi*; Saito, Kimiaki

Radiation Protection Dosimetry, 160(4), p.318 - 321, 2014/00

 Times Cited Count:32 Percentile:92.29(Environmental Sciences)

Journal Articles

Behavior of environmental tritium at NIFS Toki Site of Japan

Sugihara, Shinji*; Tanaka, Masahiro*; Tamari, Toshiya*; Shimada, Jun*; Takahashi, Tomoyuki*; Momoshima, Noriyuki*; Fukutani, Satoshi*; Atarashi-Andoh, Mariko; Sakuma, Yoichi*; Yokoyama, Sumi*; et al.

Fusion Science and Technology, 60(4), p.1300 - 1303, 2011/11

 Times Cited Count:2 Percentile:18.29(Nuclear Science & Technology)

The purpose of this study is to develop the technique to evaluate the environmental tritium behavior of the nuclear facility origin. Tritium concentrations of river water, precipitation and ground water around the NIFS site were determined by low background liquid scintillation measurement system combined with the electrolysis using solid polymer electrolyte. The electric conductivity and flow rate of the river and isotopic ratio of oxygen and hydrogen of water samples were also measured. The tritium concentrations in precipitation showed the seasonal variation and the range were 0.09-0.78 Bq/L. The tritium concentrations of river water and ground water were almost constant, 0.34 and 0.24 Bq/L respectively. The simple dynamic model for the site around the NIFS facilities was developed using measured data, and the behavior of tritium was simulated.

Journal Articles

Development of a code MOGRA for predicting the migration of ground additions and its application to various land utilization areas

Amano, Hikaru; Takahashi, Tomoyuki*; Uchida, Shigeo*; Matsuoka, Shungo*; Ikeda, Hiroshi*; Hayashi, Hiroko*; Kurosawa, Naohiro*

Journal of Nuclear Science and Technology, 40(11), p.975 - 979, 2003/11

 Times Cited Count:2 Percentile:19(Nuclear Science & Technology)

MOGRA is a migration prediction code for toxic ground additions including radioactive materials in a terrestrial environment. MOGRA consists of computational codes that are applicable to various evaluation target systems, and can be used on personal computers. The computational code has the dynamic compartment analysis block, GUI for computation parameter settings and results displays, data bases. The compartments are obtained by classifying various natural environments into groups that exhibit similar properties. A hypothetical combination of land usage was supposed to check the function of MOGRA. The land usage was consisted from cultivated lands, forests, uncultivated lands, urban area, river, and lake. Each land usage has its own inside model which is basic module. Also supposed was homogeneous contamination of the surface land from atmospheric deposition of $$^{137}$$Cs (1.0 Bq/m$$^{2}$$). The system analyzed the dynamic changes of $$^{137}$$Cs concentrations in each compartment, fluxes from one compartment to another compartment.

Journal Articles

MOGRA-DB; Database system for migration prediction code MOGRA

Amano, Hikaru; Ikeda, Hiroshi*; Sasaki, Toshihisa*; Matsuoka, Shungo*; Kurosawa, Naohiro*; Takahashi, Tomoyuki*; Uchida, Shigeo*

KEK Proceedings 2003-11, p.239 - 244, 2003/11

A Code MOGRA (Migration Of GRound Additions) is a migration prediction code for toxic ground additions including radioactive materials in a terrestrial environment, which consists of computational codes that are applicable to various evaluation target systems, and can be used on personal computers. The computational code has the dynamic compartment analysis block at its core, the graphical user interface (GUI) for model formation, computation parameter settings, and results displays. The code MOGRA has varieties of databases, which is called MOGRA-DB. Another additional code MOGRA-MAP can take in graphic map and calculate the square measure about the target land.

Journal Articles

Status of development of a code for predicting the migration of ground additions: MOGRA

Amano, Hikaru; Takahashi, Tomoyuki*; Uchida, Shigeo*; Matsuoka, Shungo*; Ikeda, Hiroshi*; Hayashi, Hiroko*; Kurosawa, Naohiro*

JAERI-Conf 2003-010, p.32 - 36, 2003/09

MOGRA (Migration Of GRound Additions) is a migration prediction code for toxic ground additions including radioactive materials in a terrestrial environment. MOGRA consists of computational codes that are applicable to various evaluation target systems, and can be used on personal computers. The computational code has the dynamic compartment analysis block at its core, the graphical user interface (GUI) for computation parameter settings and results displays, data files and so on. The compartments are obtained by classifying various natural environments into groups that exhibit similar properties. MOGRA has varieties of databases, which consist of radionuclides decay chart, distribution coefficients between solid and liquid, transfer factors from soil to plant, transfer coefficients from feed to beef and milk, concentration factors, and age dependent dose conversion factors for many radionuclides. Here the status of development of MOGRA is presented.

Journal Articles

Application of MOGRA for migration of contaminants through different land utilization areas

Amano, Hikaru; Takahashi, Tomoyuki*; Uchida, Shigeo*; Matsuoka, Shungo*; Ikeda, Hiroshi*; Hayashi, Hiroko*; Kurosawa, Naohiro*

JAERI-Conf 2003-010, p.112 - 121, 2003/09

The functionality of MOGRA is being verified by applying it in the analyses of the migration rates of radioactive substances from the atmosphere to soils and plants and flow rates into the rivers. This has been achieved by also taking their mode classifications into consideration. In this report, a hypothetical combination of land usage was supposed to check the function of MOGRA. The land usage was consisted from cultivated lands, forests, uncultivated lands, urban area, river, and lake. Each land usage has its own inside model which is basic module. Also supposed was homogeneous contamination of the surface land from atmospheric deposition of Cs-137 (1.0 Bq/m$$^{2}$$). The system can analyze the dynamic changes of Cs-137 concentrations in each compartment, fluxes from one compartment to another compartment.

Journal Articles

Construction of river transfer models for MOGRA

Hayashi, Hiroko*; Matsuoka, Shungo*; Takahashi, Tomoyuki*; Amano, Hikaru

JAERI-Conf 2003-010, p.122 - 130, 2003/09

Two dynamic compartment models were constructed as basic river models for MOGRA (Migration Of GRound Additions), an environmental-load effect predicting code. One is 1 component river model, in which radionuclides in particulate form and dissolved form are considered to be in equilibrium in the river water. Another one is 2 component river model, in which particulate form and dissolved form are considered to be different component and are separately compartmentalized. In each model the river sediment is set in a compartment, and the sedimentation of particulate form and resuspension of radionuclides in the river sediment are taken into account.To verify the analysis function of the constructed models, calculation conditions were set using data of Cs-137 concentration in the river water derived from Kuji river, Japan, and analysis was carried out. Comparing two models, almost no difference is seen when sedimentation velocity is low, while there is apparent difference when sedimentation velocity is high.

Journal Articles

Overview of the 3rd phase crossover research on migration of radionuclides in biosphere

Uchida, Shigeo*; Amano, Hikaru; Takahashi, Tomoyuki*; Chiba, Masaru*; Hisamatsu, Shunichi*; Enomoto, Shuichi*; Matsumoto, Shiro*

JAERI-Conf 2003-010, p.25 - 31, 2003/09

In the 3rd Stage Crossover Research (1998 to 2003), a project on Development of a dynamic transfer model of radionuclides in the soil ecosphere,is currently being promoted. The following five researches are carried out in this project. 1) Research into the forms of existence of nuclides and their change in the soil (NIRS and JAERI), 2) Research into the transition behavior of radionuclides in plants (IES, RIKEN and NIRS), 3) Research into the relation to the microorganism and on environmental remediation (RIKEN, JAERI and NIRS), 4) Research on the migration of radionuclides from atmosphere to soil and plant (MRI and JAERI), and 5) Database construction on transfer parameters (JAERI, NIRS and MRI). JAERI, MRI and NIRS are working on the development of a dynamic transfer model such as MOGRA for radionuclides on the basis of a gained knowledge about the environmental behavior through cooperation with universities, etc. This model is also capable of the predicting the behavior of materials that are harmful to the environment such as hazardous heavy metals discharged in the soil ecosphere. In this presentation, we will overview the ourcome of the 3rd stage research.

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