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Otosaka, Shigeyoshi*; Kambayashi, Shota*; Fukuda, Miho*; Tsuruta, Tadahiko; Misono, Toshiharu; Suzuki, Takashi; Aono, Tatsuo*
Environmental Science & Technology, 54(21), p.13778 - 13785, 2020/11
Times Cited Count：12 Percentile：54.1(Engineering, Environmental)Concentrations of 
Cs in seawater, seabed sediment, and pore water collected from the area around Fukushima were investigated from 2015 to 2018, and the potential of coastal sediments to supply radiocesium to the bottom environment was evaluated. The Cs concentration in the pore water ranged from 33 to 1934 mBq L
and was 10-40 times higher than that in the overlying water (seawater overlying within 30 cm on the seabed). At most stations, the Cs concentrations in the overlying water and the pore water were approximately proportional to those in the sediment. The conditional partition coefficient between pore water and sediment was 0.9-14
10
L kg, independent of the year of sampling. These results indicated that an equilibrium of Cs between pore water and sediment has established in a relatively short period, and Cs in the pore water is gradually exported to seawater near the seabed. A simple box model estimation based on these results showed that the Cs in the sediment was decreased by about 6% per year by desorption/diffusion of Cs from the seabed.
Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11
Times Cited Count：2 Percentile：21.58(Chemistry, Analytical)We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the Cs results were within 
2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.
Pu, 
Pu and 
Pu) in radioactive particles derived from Fukushima Daiichi Nuclear Power Plant accidentIgarashi, Junya*; Zheng, J.*; Zhang, Z.*; Ninomiya, Kazuhiko*; Satou, Yukihiko; Fukuda, Miho*; Ni, Y.*; Aono, Tatsuo*; Shinohara, Atsushi*
Scientific Reports (Internet), 9(1), p.11807_1 - 11807_10, 2019/08
Times Cited Count：20 Percentile：65.32(Multidisciplinary Sciences)Radioactive particles were released into the environment during the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. Many studies have been conducted to elucidate the chemical composition of released radioactive particles in order to understand their formation process. However, whether radioactive particles contain nuclear fuel radionuclides remains to be investigated. Here, we report the first determination of Pu isotopes in radioactive particles. To determine the Pu isotopes (Pu, Pu and Pu) in radioactive particles derived from the FDNPP accident which were free from the influence of global fallout, radiochemical analysis and inductively coupled plasma-mass spectrometry measurements were conducted. Radioactive particles derived from unit 1 and unit 2 or 3 were analyzed. For the radioactive particles derived from unit 1, activities of 
Pu and Pu were (1.70-7.06)10
Bq and (4.10-8.10)10
Bq, respectively and atom ratios of Pu/Pu and Pu/Pu were 0.330-0.415 and 0.162-0.178, respectively. These ratios were consistent with the simulation results from ORIGEN code and measurements from various environmental samples. In contrast, Pu was not detected in the radioactive particles derived from unit 2 or 3. The difference in Pu contents is clear evidence towards different formation processes of radioactive particles, and detailed formation processes can be investigated from Pu analysis.
Cs activity concentrations in sediment collected off the coast of Fukushima Prefecture in 2013-2015Fukuda, Miho*; Aono, Tatsuo*; Yamazaki, Shinnosuke*; Ishimaru, Takashi*; Kanda, Jota*; Nishikawa, Jun*; Otosaka, Shigeyoshi
Geochemical Journal, 52(2), p.201 - 209, 2018/00
Times Cited Count：3 Percentile：16.65(Geochemistry & Geophysics)To elucidate recent activity levels and the behavior of radiocesium in the coast off Fukushima Prefecture, lateral and vertical distributions of Cs in sediment were observed in 2013-2015 at 12 monitoring stations. At stations around the water depth of 100 m, relatively higher Cs activities were observed from surface sedimentary layer (0-3 cm). In these stations, sediments had high content of silt to clay particles and organic matter. The high Cs activities in the surface sediments were attributed to accumulation of highly mobile sediment particles. In October 2014, at some coastal stations, sharp peaks of Cs activities were observed in the subsurface (5-16 cm) sediments, whereas such broad peaks were not found in October 2015. These results suggest that the Cs activities in sediment had largely changed by lateral transport and re-sedimentation on the surface, as well as sediment mixing in the middle-layers.
Fukuda, Miho*; Aono, Tatsuo*; Yamazaki, Shinnosuke*; Nishikawa, Jun*; Otosaka, Shigeyoshi; Ishimaru, Takashi*; Kanda, Jota*
Journal of Radioanalytical and Nuclear Chemistry, 311(2), p.1479 - 1484, 2017/02
Times Cited Count：6 Percentile：51.46(Chemistry, Analytical)In order to investigate processes affecting distribution of radiocaesium in seawater in the adjacent region of Fukushima Daiichi Nuclear Power Plant (FDNPP), relationships between Cs activity in seawater and physical properties of seawater (salinity, temperature, and potential density) were observed in seven stations within 10 km radius from the FDNPP. As a whole, Cs concentrations in seawater were higher in the vicinity of the FDNPP, and were negatively correlated with potential density. From these results, it can be considered that river water discharge or export of seawater from the FDNPP's harbor has affected the higher activity levels of Cs in seawater. It was also observed that the Cs-elevated seawater can be advected to the 20
50 m depths.
Saito, Kenji; Homma, Fumitaka; Omata, Toru; Aono, Tetsuya; Kawaji, Satoshi; Kawasaki, Kozo; Iyoku, Tatsuo
Proceedings of International Topical Meeting on Nuclear Plant Instrumentation, Controls, and Human-Machine Interface Technologies (NPIC&HMIT 2000) (CD-ROM), 8 Pages, 2000/00
no abstracts in English
Suzuki, Kiichi; Murakami, Tatsutoshi; Aono, Shigenori; Hatanaka, Nobuhiro; Takano, Tatsuo
no journal, ,
no abstracts in English
Otosaka, Shigeyoshi; Fukuda, Miho*; Aono, Tatsuo*
no journal, ,
Behavior of dissolved radiocesium near the seafloor is discussed from the distributions of Cs in overlying water (seawater collected from 30 cm above the seabed) at 14 stations and in pore water at 3 stations off Fukushima (170 km from Fukushima Daiichi Nuclear Power Plant). The Cs concentrations in overlying water, collected during 2015 and 2016, ranged between 5 and 283 mBq/L. The Cs concentrations in overlying water were 23 times higher than those in seawater collected from intermediate (5 m above the bottom) layers. The Cs concentrations in pore water were 1030 times higher than those in overlying water. We can consider that radiocesium is dissolved in the overlying water and has been diffused from the seabed through the porewater. Nevertheless, it was estimated that the amount of Cs transferred from porewater to benthic organisms does not lead to Cs activities exceeding the regulation limits at most stations.
-ray emitters including Cs, 1; Collaborative experiment by the committee on preparation of reference materials for radioactivity analysis of JSACYonezawa, Chushiro*; Kakita, Kazutoshi*; Takahashi, Takanori*; Aono, Tatsuo*; Maeda, Satoshi; Abe, Takaaki*; Arakawa, Fumihiro*; Kiho, Nobuharu*; Akiyama, Masakazu*; Muramatsu, Isamu*; et al.
no journal, ,
no abstracts in English
Otosaka, Shigeyoshi; Fukuda, Miho*; Aono, Tatsuo*
no journal, ,
Behavior of dissolved radiocesium near the seafloor is discussed from the distributions of Cs in seawater, seabed sediment and pore water collected from the area around Fukushima. The Cs concentrations in the pore water, collected from 2015 to 2017, ranged between 33 and 1186 mBq/L, and were 1040 times higher than those in seawater on the sediment surface. The Cs concentration in the overlying water did not show clear differences regardless of the pore size of the filter used for filtration. From these results, it was confirmed that radiocesium in the seabed sediment was dissolved in pore water and diffused to the benthic layer. The apparent distribution coefficient between pore water and sediment was [0.94.2]10 L/kg, with no difference depending on the year of sampling. These results indicated that an equilibrium of Cs between pore water and sediment has established during the observation period.
Igarashi, Junya*; Zheng, J.*; Zhang, Z.*; Ninomiya, Kazuhiko*; Satou, Yukihiko; Fukuda, Miho*; Ni, Y.*; Aono, Tatsuo*; Shinohara, Atsushi*
no journal, ,
Plutonium is one of the most notable radionuclides in the nuclear accident. The amounts of Pu released by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident were investigated so far. However, the existence of Pu isotopes from the global fallout makes it difficult to accurately assessment of Pu contamination by the FDNPP accident. To avoid this problem, identification of Pu contamination source from the Pu isotopic ratios is important. However, various ratios have been reported by the researches due to the contamination from global fallout. In this work, we focused on the insoluble radioactive Cs particles made of mainly SiO
(insoluble particles) released from the FDNPP to determine accurate Pu isotopic ratios. Due to its insolubility, the particles retained the original property at the time of emission from the reactor. Therefore, the insoluble particles are considered to be free from the contamination of global fallout. In addition, the amounts of Pu in the insoluble particles provide the information about their formation process in the reactor. In this study, we identified Pu isotopes in insoluble particles by radioactive analysis and ICP-MS measurement. The isotopic ratios of Pu/Pu and Pu/Pu were determined as 0.330-0.415 and 0.162-0.178, respectively and activity ratio of Pu/Cs was about 10
in each particle.
Taniguchi, Keisuke*; Takeuchi, Yukio*; Fujita, Kazuki*; Dohi, Terumi; Hayashi, Seiji*; Kuramoto, Takayuki*; Nomura, Naoki*; Aono, Tatsuo*
no journal, ,
In Fukushima Prefecture, although decontamination has been completed except for difficult-to-return areas, most of the forest has not been decontaminated yet. From the forest, radiocaesium may enter rivers and affect downstream areas. A survey was conducted in three forested watersheds of the Nanokazawa, Saruta, Nuno rivers located in Fukushima Prefecture to understand the amount and characteristics of radiocaesium flowing out. In each watershed, suspended solids (SS) were collected by a suspended sand sampler, water was collected every few months, and the water level and flow rate were measured. After freeze-drying the SS sample, the concentration of suspended Cs-137 was measured by a germanium semiconductor detector. The water sample was filtered through a membrane filter with a pore size of 0.45 
m, then the dissolved Cs-137 was collected by the solid-phase extraction disk method or AMP coprecipitation method, and the dissolved Cs-137 concentration was measured by a germanium semiconductor detector. The ranges of dissolved Cs-137 concentration in FY2019 were 69-190 mBq/L in the Saruta River, 9.7-16 mBq/L in the Nanokazawa river, and ND-3.2 mBq/L in the Nuno River. In the poster, we will also present the results of SS measurements and flow observations.
Aono, Tatsuo*; Nakanishi, Takahiro
no journal, ,
In order to elucidate the distribution, behavior and runoff process of radiocaesium in stream water collected from forest catchments, the activity concentrations of dissolved and particulate radiocaesium were monitored in this area. Although there is a very strong correlation between annual mean activity concentration of dissolved Cs-137 and mean air does rate in catchment area, no features were found with activity concentrations of particulate Cs-137 and mean air does rate in the area. The river water increased due to heavy rains caused by two typhoons in October 2019, and then the topography changed drastically with the inflow of sediment. The radioactivity concentrations of dissolved Cs-137 were decreased by about 50% compared to before the heavy rain. However, the change of radioactivity concentrations of particulate Cs-137 have not been observed. It is considered that the condition of the forest basin has changed as one of reasons.
Takeuchi, Yukio*; Taniguchi, Keisuke*; Arai, Hirotsugu*; Yoshita, Hirofumi*; Fujita, Kazuki*; Takahashi, Yusuke*; Kuramoto, Takayuki*; Nomura, Naoki*; Hagiwara, Hiroki; Dohi, Terumi; et al.
no journal, ,
no abstracts in English
Otosaka, Shigeyoshi*; Aono, Tatsuo*; Fukuda, Miho*; Kambayashi, Shota*; Misono, Toshiharu; Dohi, Terumi; Tsuruta, Tadahiko; Suzuki, Takashi; Takahashi, Yoshio*; Sugihara, Naoko*; et al.
no journal, ,
While the amount of cesium-137 (Cs: half-life 30.1 years) accumulated on the seabed due to the accident of the Fukushima Daiichi Nuclear Power Plant (0.1-0.2 PBq) is only about 1 to 2% of the total amount of Cs transported to the ocean, it has been reported that it will remain for a long time in the coastal areas. On the other hand, long-term migration process of the sedimentary radiocesium and the impact on the ecosystem near the seafloor remain unknown. In this presentation, we will give an overview of the distribution and behavior of Cs, especially on the seafloor along the coast of Fukushima, and report the latest results on the processes I the seafloor that should be considered on decadal timescale.
Aono, Tatsuo*; Nishikawa, Jun*; Otosaka, Shigeyoshi*; Takata, Hyoe*; Misono, Toshiharu; Nakanishi, Takahiro; Miura, Hikaru*; Kambayashi, Shota*; Fukuda, Miho*; Sakurada, Masanobu*; et al.
no journal, ,
From 2016 to 2020, the Tohoku Marine Ecosystem Research Vessel Shinsei-maru conducted four research cruises on the dynamics and bioavailability of radionuclides around off Fukushima. Seawater, sediments and organisms were collected mainly around off the Fukushima Daiichi Nuclear Power Plant (FDNPS). The purpose of those cruises is to observe the flux of radionuclides released into the ocean by the FDNPS accident and to understand the bioavailability of radionuclides. In order to understand the contaminated levels of the marine environment, the concentration of radioactive cesium (Cs) in seawater and sediments around off Fukushima was investigated. As a result, the concentration range of dissolved Cs-137 in the surface seawater near the FDNPS from 2016 to 2018 was 10-23 mBq/L, but decreased to 7 mBq/L in 2020. In terms of points, the concentrations of dissolved Cs-137 tended to decrease with time. On the other hand, in sediments, the Cs-137 concentrations were higher in the surface layer (0-2 cm) than the deep layer from 2016 to 2017 and tended to decrease with depth, but after 2018, subsurface vertical maximum of Cs-137 concentrations was observed at some stations. Although these concentrations tended to increase in the subsurface layer, the concentrations in the sediment also tended to decrease with time. In this presentation, we report on the concentration variation of Cs-137 and their characteristics in seawater and sediments around off Fukushima.
Aono, Tatsuo*; Nishikawa, Jun*; Otosaka, Shigeyoshi*; Takata, Hyoe*; Misono, Toshiharu; Nakanishi, Takahiro; Miura, Hikaru*; Fukuda, Miho*; Kambayashi, Shota*; Sakurada, Masanobu*; et al.
no journal, ,
From 2016 to 2020, four research voyages were conducted to investigate the dynamics of radioactive materials in the waters around Fukushima. Seawater and sediment samples were collected in the waters off the Fukushima Daiichi Nuclear Power Plant (FDNPS). The concentration of radioactive cesium (Cs) in seawater and sediment off the coast of Fukushima was surveyed to understand the status of the marine environment. As a result, no significant changes were observed in both seawater and sediment from 2016 to 2020.
Sato, Rina; Yoshimura, Kazuya; Sanada, Yukihisa; Yajima, Kazuaki*; Aono, Tatsuo*
no journal, ,
no abstracts in English
Takata, Hyoe*; Otsuki, Azusa*; Sato, Shun*; Otosaka, Shigeyoshi*; Toda, Ryoji*; Nishikawa, Jun*; Kenmochi, Hideyuki*; Ishikura, Mei*; Yamada, Momoka*; Shinkai, Yusuke*; et al.
no journal, ,
Research cruises were conducted by the Shinsei Maru from October 7 to October 17, 2021, and from October 2 to 13, 2022, in the coastal waters off Fukushima Prefecture. Those cruises aimed to monitor radionuclide distribution and to clarify the dynamics of radionuclides in the coastal water and the environmental response of ecosystems after the Fukushima Daiichi Nuclear Power Plant accident in March 2011.
Aono, Tatsuo*; Fukuda, Miho*; Sakurada, Masanobu*; Takahashi, Hiroyuki*; Yamazaki, Shinnosuke*; Kambayashi, Shota*; Misono, Toshiharu; Nakanishi, Takahiro; Miura, Hikaru*; Nishikawa, Jun*; et al.
no journal, ,
From 2016 to 2020, R/V Shinsei-maru of JAMSTEC conducted four research cruises on the dynamics and bioavailability of radionuclides around off Fukushima. Seawater, sediments and organisms were collected mainly around off the Fukushima Daiichi Nuclear Power Plant (FDNPS). The purpose of those cruises is to observe the flux of radionuclides released into the ocean by the FDNPS accident and to understand the bioavailability of radionuclides. In order to understand the contaminated levels of the marine environment, the concentration of radiocaesium (Cs) in seawater and sediments around off Fukushima was investigated.
