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JAEA Reports

Radiation monitoring via manned helicopter around the nuclear power station in the fiscal year 2022 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.

JAEA-Technology 2023-027, 146 Pages, 2024/03

JAEA-Technology-2023-027.pdf:18.12MB

By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been applied as a method to quickly and extensively measure the distribution of radiation. Japan Atomic Energy Agency (JAEA) has continuously conducted ARM via manned helicopter around FDNPS. In this report, we summarize the results of the ARM around FDNPS in the fiscal year 2022, evaluate the changes of ambient dose rates and other parameters based on the comparison to the past ARM results, and discuss the causes of such changes. In order to contribute to improve the accuracy of ambient dose rate conversion, we analyzed the ARM data taking into account undulating topography, and evaluated the effect of this method. Furthermore, the effect of radon progenies in the air on the ARM was evaluated by applying the discrimination method to the measurement results.

JAEA Reports

Background radiation monitoring via manned helicopter and development of technology for radiation monitoring via unmanned airplane for application of nuclear emergency response technique in the fiscal year 2022 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.

JAEA-Technology 2023-026, 161 Pages, 2024/03

JAEA-Technology-2023-026.pdf:14.66MB

By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been utilized as a method to quickly and extensively measure radiation distribution surrounding FDNPS. In order to utilize ARM and to promptly provide the results during a nuclear emergency, information on background radiation levels, topographical features, and controlled airspace surrounding nationwide nuclear facilities have been prepared in advance. In the fiscal year 2022, we conducted ARM around the Mihama Nuclear Power Station of Kansai Electric Power Company (KEPCO), the Tsuruga Power Station of Japan Atomic Power Company (JAPC), and the Ikata Power Station of Shikoku Electric Power Company (YONDEN), and prepared information on background radiation doses and controlled airspace. In addition, we have developed an aerial radiation detection system via unmanned airplane, which is expected to be an alternative to ARM, during a nuclear emergency. This report summarizes the results and technical issues identified.

JAEA Reports

Analysis of deposits inside the reactor at Fukushima Daiichi Nuclear Power Station in JFY2021; The Subsidy program of "Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris)" starting FY2021

Ikeuchi, Hirotomo; Sasaki, Shinji; Onishi, Takashi; Nakayoshi, Akira; Arai, Yoichi; Sato, Takumi; Ohgi, Hiroshi; Sekio, Yoshihiro; Yamaguchi, Yukako; Morishita, Kazuki; et al.

JAEA-Data/Code 2023-005, 418 Pages, 2023/12

JAEA-Data-Code-2023-005-01.pdf:24.59MB
JAEA-Data-Code-2023-005-02.pdf:32.18MB

For safe and steady decommissioning of Tokyo Electric Power Company Holdings' Fukushima Daiichi Nuclear Power Station (1F), information concerning composition and physical/chemical properties of fuel debris generated in the reactors should be estimated and provided to other projects conducting the decommissioning work including the retrieval of fuel debris and the subsequent storage. For this purpose, in FY2021, samples of contaminants (the wiped smear samples and the deposits) obtained through the internal investigation of the 1F Unit 2 were analyzed to clarify the components and to characterize the micro-particles containing uranium originated from fuel (U-bearing particles) in detail. This report summarized the results of analyses performed in FY2021, including the microscopic analysis by SEM and TEM, radiation analysis, and elemental analysis by ICP-MS, as a database for evaluating the main features of each sample and the probable formation mechanism of the U-bearing particles.

Journal Articles

Decontamination and solidification treatment on spent liquid scintillation cocktail

Watanabe, So; Takahatake, Yoko; Ogi, Hiromichi*; Osugi, Takeshi; Taniguchi, Takumi; Sato, Junya; Arai, Tsuyoshi*; Kajinami, Akihiko*

Journal of Nuclear Materials, 585, p.154610_1 - 154610_6, 2023/11

 Times Cited Count:0 Percentile:0.01

Journal Articles

Application of the Y separation method using DGA resin for the measurement of $$^{90}$$Sr in human teeth and marine fish bones

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Terashima, Motoki

KEK Proceedings 2023-2, p.155 - 160, 2023/11

In this presentation, we report the results of the application of the Y-separation method using DGA resin to the determination of $$^{90}$$Sr in human teeth and seawater fish bones.

Journal Articles

JAEA's action on medical RI production using research reactor

Arai, Masaji; Maeda, Shigetaka

Rinsho Hoshasen, 68(10), p.963 - 970, 2023/10

Ac-225 is attracting attention as an alpha-emitting medical radioisotope. Since its demand is expected to increase, domestic production of Ac-225 is required from the viewpoint of Japan's medical research and economic security. To establish the technical bases for the Ac-225 production, JAEA has evaluated the radioactivity that can be produced in the experimental fast reactor Joyo and designed the concept that upgrades the existing facilities for transporting the irradiated target from Joyo to a neighboring PIE facility rapidly. Efficient Actinium-225 Separation from Ra-226 irradiated in a fast reactor was studied. This study has revealed that Joyo can sufficiently produce Ac-225 as a raw material for pharmaceuticals.

Journal Articles

Evaluation of the remaining spent extraction solvent in vermiculite after leaching tests via PIXE analysis

Arai, Yoichi; Watanabe, So; Hasegawa, Kenta; Okamura, Nobuo; Watanabe, Masayuki; Takeda, Keisuke*; Fukumoto, Hiroki*; Ago, Tomohiro*; Hagura, Naoto*; Tsukahara, Takehiko*

Nuclear Instruments and Methods in Physics Research B, 542, p.206 - 213, 2023/09

Journal Articles

Kinetic mass transfer behavior of Eu(III) in nitrilotriacetamide-impregnated polymer-coated silica particles

Miyagawa, Akihisa*; Hayashi, Naoki*; Kuzure, Yoshiaki*; Takahashi, Takumi*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Miyazaki, Yasunori; Hasegawa, Kenta; Sano, Yuichi; et al.

Bulletin of the Chemical Society of Japan, 96(7), p.671 - 676, 2023/07

We investigated the distribution mechanism of Eu(III) in a single polymer-coated silica particle including nitrilotriacetamide (NTA) extractants known as HONTA and TOD2EHNTA. The present study provides a valuable approach for the evaluation and enhancement of the functionality of "single extractant-impregnated polymer-coated silica particle".

Journal Articles

Establishing an evaluation method for the aging phenomenon by physical force in fuel debris

Suzuki, Seiya; Arai, Yoichi; Okamura, Nobuo; Watanabe, Masayuki

Journal of Nuclear Science and Technology, 60(7), p.839 - 848, 2023/07

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The fuel debris, consisting of nuclear fuel materials and reactor structural materials, generated in the accident of Fukushima Daiichi Nuclear Power Plant can become deteriorated like rocks under the changes of environmental temperature. Although the fuel debris have been cooled by water for 10 years, they are affected by seasonal and/or day-and-night temperature changes. Therefore, in evaluating the aging behavior of the fuel debris, it is essential to consider the changes in environmental temperature. Assuming that the fuel debris are deteriorated, radioactive substances that have recently undergone micronization could be eluted into the cooling water, and such condition may affect defueling methods. We focused on the effect of repeated changes in environmental temperature on the occurrence of cracks, and an accelerated test using simulated fuel debris was carried out. The length of the crack increases with increasing number of heat cycle; therefore, the fuel debris become brittle by stress caused by thermal expansion and contraction. In conclusion, it was confirmed that the mechanical deterioration of the fuel debris is similar to that of rocks or minerals, and it became possible to predict changes in the length of the crack in the simulated fuel debris and environmental model.

Journal Articles

Improvement in the elution performance of an N,N,N',N-tetraoctyl diglycolamide impregnated extraction chromatography adsorbent using neodymium via micro-particle-induced X-ray emission analysis

Takahatake, Yoko; Watanabe, So; Arai, Tsuyoshi*; Sato, Takahiro*; Shibata, Atsuhiro

Applied Radiation and Isotopes, 196, p.110783_1 - 110783_5, 2023/06

 Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)

JAEA Reports

Cleaning of the inner surface for Separated-type Drift Tube Linac with Dilute Hydrochloric Acid

Arai, Sora; Kosaka, Satoshi*; Nemoto, Yasuo*; Kitamura, Ryo

JAEA-Technology 2023-009, 18 Pages, 2023/05

JAEA-Technology-2023-009.pdf:1.89MB

The linac located at the head of the J-PARC accelerators and required to provide the stable and high-quality beam. One of the accelerating cavities in the linac is the Separated-type Drift Tube Linac (SDTL). It is important to appropriately apply the RF power into the cavity for the stable operation. However, after the recovery from the Great East Japan Earthquake, the RF power could not be applied into the cavities for several SDTL cavities because the voltage standing wave ratio increased around the designed operating power. The investigation revealed that the inner surface of the cavity was exposed to high humidity and the backflow of oil from the rotary pump for a long period of time after the earthquake. It was suggested that the residue on the inner surface caused the multipactor resulted in the failure when the power was applied. The residue was wiped out with organic solvents and acids, resulted in solving the failure. This report describes the method and results of the cleaning for the cavity in 2021.

JAEA Reports

How to confirm the polarity of the DTQ in the J-PARC DTL

Kosaka, Satoshi*; Arai, Sora; Nemoto, Yasuo*; Kitamura, Ryo

JAEA-Technology 2023-003, 34 Pages, 2023/05

JAEA-Technology-2023-003.pdf:3.79MB

The negative hydrogen (H$$^{-}$$) ion beam is accelerated with a peak current of 50 mA in the J-PARC linac. The linac consists of the H- ion source and four kinds of accelerating cavities; a radio-frequency quadrupole linac (RFQ), a drift-tube linac (DTL), a separated-DTL (SDTL), and an annular-ring coupled structure linac (ACS). The accelerating electric field exists between the drift-tubes in the tank of the DTL. The quadrupole magnet for the beam focusing (DTQ) is installed in the drift-tube. The DTQ at J-PARC employs electromagnets to generate the magnetic field. It is important to set correctly the polarity of the magnetic field of the DTQ for tuning the beam. In this paper, we report the method of confirming the magnetic field polarity of DTQ, that is, the current wiring polarity by measuring DC current using a clamp meter on the power supply side and visually confirming the cable wiring connection on the electromagnet side.

Journal Articles

Study on the uptake of $$^{90}$$Sr and $$^{137}$$Cs into wild animals after the Fukushima Daiichi Nuclear Power Plant accident using hard tissue as an indicator

Koarai, Kazuma

Hosha Kagaku, (47), p.24 - 27, 2023/03

Ca-based tissues, such as teeth and bones, are called hard tissues. Sr is incorporated into the tooth during calcification. Once incorporated, it remains until the tooth falls out. Therefore, $$^{90}$$Sr in teeth recorded $$^{90}$$Sr contamination by the 1F accident in the environment during the formation period. The article presents current research findings.

Journal Articles

Fact-finding survey on the competencies and literacy of radiological technologists regarding radiation disasters

Arai, Tomohiro*; Murata, Sho*; Watanabe, Yuichi*; Ishihara, Toshihiro*; Fukamizu, Yoshiya*; Takeda, Satoshi*; Ebata, Kiyokadzu*; Watanabe, Yuki; Takashima, Yoshio*; Kaneko, Junichi*

Journal of X-Ray Science and Technology, 31(2), p.237 - 245, 2023/03

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

Radiological technologists have received specialized education about radiation and serve as risk communicators who aim to lessen patients' anxiety about radiation exposure, in addition to performing radiological examinations in routine clinical practice. Also, Radiological technologists across Japan were dispatched to the affected area to conduct an essential procedure-screening the belongings and body surfaces of evacuees for contamination at the nuclear disaster at the Fukushima Daiichi Nuclear Power Plant operated by Tokyo Electric Power Company in March 2011. In this study, we conducted a fact-finding survey on knowledge and awareness of radiation disasters among radiological technologists at National Hospital Organization facilities in Japan to reveal their literacy and competencies regarding radiation disasters. Also, we compared the knowledge and awareness of radiation disasters among Japanese radiological technologists between nuclear power station areas and non-nuclear power station areas and discuss ideal human resource development for radiological technologists to be ready to serve during a radiation disaster.

Journal Articles

Investigation of adsorption mechanism of Mo(VI) by baker's yeast and applicability to the uranium liquid waste treatment process

Arai, Yoichi; Hasegawa, Kenta; Watanabe, So; Watanabe, Masayuki; Minowa, Kazuki*; Matsuura, Haruaki*; Hagura, Naoto*; Katsuki, Kenta*; Arai, Tsuyoshi*; Konishi, Yasuhiro*

Journal of Radioanalytical and Nuclear Chemistry, 9 Pages, 2023/00

Journal Articles

Design of MA(III)/Ln(III) separation process of extraction chromatography technology

Akuzawa, Tadashi*; Kim, S.-Y.*; Kubota, Masahiko*; Wu, H.*; Watanabe, So; Sano, Yuichi; Takeuchi, Masayuki; Arai, Tsuyoshi*

Journal of Radioanalytical and Nuclear Chemistry, 331(12), p.5851 - 5858, 2022/12

 Times Cited Count:0 Percentile:33.72(Chemistry, Analytical)

Journal Articles

Mass-spectrometric determination of iodine-129 using O$$_{2}$$-CO$$_{2}$$ mixed-gas reaction in inductively coupled plasma tandem quadrupole mass spectrometry

Matsueda, Makoto; Aoki, Jo; Koarai, Kazuma; Terashima, Motoki; Takagai, Yoshitaka*

Analytical Sciences, 38(11), p.1371 - 1376, 2022/11

 Times Cited Count:1 Percentile:17.04(Chemistry, Analytical)

The $$^{129}$$I analysis using ICP-MS is challenging caused by xenon-129 ($$^{129}$$Xe) and $$^{127}$$IH$$_{2}$$ generated from excess stable isotope $$^{127}$$I. In this study, mass discrimination between iodine-129 ($$^{129}$$I) and interfering substances was achieved by inductively coupled plasma-tandem quadrupole mass spectrometry (ICP-MS/MS) with a dynamic reaction cell introduced a mixture gas of O$$_{2}$$ and CO$$_{2}$$. As a result, the ratio of (background noise intensity at m/z 129)/$$^{127}$$I was 3.8 $$times$$ 10$$^{-10}$$ and 10 mBq/L of $$^{129}$$I was analyzed without chemical separation in the presence of 100 mg/L stable $$^{127}$$I. Spiked tests with actual rainwater were performed, and obtained values were agreed with the spiked amounts.

Journal Articles

Development of an analytical method for $$^{90}$$Sr with ICP-MS/MS using O$$_{2}$$ and NH$$_{3}$$ mixed gas reaction

Koarai, Kazuma; Matsueda, Makoto; Terashima, Motoki

KEK Proceedings 2022-2, p.102 - 107, 2022/11

Analytical methods with inductively coupled plasm mass spectrometry (ICP-MS) have been developed for the determination of $$^{90}$$Sr in environmental samples; however, the sensitivity of the ICP-MS methods and removal of interferences are insufficient to measure trace amount of $$^{90}$$Sr in the environmental samples. In this study, we developed an analytical method for $$^{90}$$Sr with ICP-DRC-MS/MS using oxygen and ammonia mixed gas reaction. This analytical method could be applied for measurement of $$^{90}$$Sr in reference soil.

Journal Articles

Oxygen reduction activity and interfacial structures of La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ at initial electrochemical process in an alkaline solution

Matsuzaki, Akira*; Hirayama, Masaaki*; Oguchi, Shoya*; Komo, Mamoru*; Ikezawa, Atsunori*; Suzuki, Kota*; Tamura, Kazuhisa; Arai, Hajime*; Kanno, Ryoji*

Electrochemistry (Internet), 90(10), p.107001_1 - 107001_8, 2022/10

 Times Cited Count:0 Percentile:0.01(Electrochemistry)

Oxygen reduction and evolution reactions (ORR and OER) of perovskite-type La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ were characterized using two-dimensional model electrodes with different reaction planes. Synthesized by pulsed laser deposition, these thin and flat electrodes can reveal the reaction plane dependence of the ORR activity. From steady-state polarization measurements in KOH (aq.), the ORR activity was the highest on the (001) film during the first ORR/OER cycle, and it decreased significantly during the second cycle. In-situ synchrotron X-ray diffraction clarified crystal structure changes in the bulk and surface regions of La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$, and these changes are associated with forming oxygen defects during the initial electrochemical process. Furthermore, the La$$_{0.8}$$Sr$$_{0.2}$$CoO$$_{3}$$ surface partially decomposed upon reacting. Therefore, the interfacial structures formed in the electrochemical reaction field is important for enhancing ORR and OER activities.

Journal Articles

Using CO$$_{2}$$ Reactions to Achieve Mass-spectrometric Discrimination in Simultaneous Plutonium-isotope Speciation with Inductively Coupled Plasma-Tandem Mass Spectrometry

Matsueda, Makoto; Kawakami, Tomohiko*; Koarai, Kazuma; Terashima, Motoki; Fujiwara, Kenso; Iijima, Kazuki; Furukawa, Makoto*; Takagai, Yoshitaka*

Chemistry Letters, 51(7), p.678 - 682, 2022/07

 Times Cited Count:2 Percentile:63.98(Chemistry, Multidisciplinary)

New methodology for a simultaneous isotope speciation of various Pu isotopes without complicated isobaric interferences is developed by using inductively coupled plasma-mass spectrometry (ICP-MS). In analyzing ICP tandem MS (ICP-MS/MS), CO$$_{2}$$ gas reactions in a dynamic reaction cell (DRC) almost eliminated the background noise intensity produced by isobaric interference from isotopes originating from actinides such as Am, Cm, and U at the locations (m/z) of significant Pu isotopes ($$^{239}$$Pu, $$^{240}$$Pu, $$^{241}$$Pu, $$^{242}$$Pu, $$^{244}$$Pu).

1464 (Records 1-20 displayed on this page)