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Journal Articles

Development of engineering scale extraction chromatography separation system, 2; Spray drying granulation of silica support for adsorbent

Hasegawa, Kenta; Goto, Ichiro*; Miyazaki, Yasunori; Ambai, Hiromu; Watanabe, So; Watanabe, Masayuki; Sano, Yuichi; Takeuchi, Masayuki

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 5 Pages, 2023/05

Journal Articles

Grain orientation dependence of deformation microstructure evolution and mechanical properties in face-centered cubic high/medium entropy alloys

Yoshida, Shuhei*; Fu, R.*; Gong, W.; Ikeuchi, Takuto*; Bai, Y.*; Feng, Z.*; Wu, G.*; Shibata, Akinobu*; Hansen, N.*; Huang, X.*; et al.

IOP Conference Series; Materials Science and Engineering, 1249, p.012027_1 - 012027_6, 2022/08

 Times Cited Count:0 Percentile:0.83(Metallurgy & Metallurgical Engineering)

Journal Articles

The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; Nishio, Katsuhisa; Lugaro, M.*; Li, Z. H.*; Makii, Hiroyuki; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; Hirose, Kentaro; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

 Times Cited Count:1 Percentile:8.87(Astronomy & Astrophysics)

Journal Articles

Formation of $$alpha$$ clusters in dilute neutron-rich matter

Tanaka, Junki*; Yang, Z.*; Typel, S.*; Adachi, Satoshi*; Bai, S.*; van Beek, P.*; Beaumel, D.*; Fujikawa, Yuki*; Han, J.*; Heil, S.*; et al.

Science, 371(6526), p.260 - 264, 2021/01

 Times Cited Count:48 Percentile:99.12(Multidisciplinary Sciences)

By employing quasi-free $$alpha$$-cluster-knockout reactions, we obtained direct experimental evidence for the formation of $$alpha$$ clusters at the surface of neutron-rich tin isotopes. The observed monotonous decrease of the reaction cross sections with increasing mass number, in excellent agreement with the theoretical prediction, implies a tight interplay between $$alpha$$-cluster formation and the neutron skin.

Journal Articles

Effect of seawater components on corrosion behavior of SUS316L in nitric acid solution containing metal ions

Ambai, Hiromu; Nishizuka, Yusuke*; Sano, Yuichi; Uchida, Naoki; Iijima, Shizuka; Shiwaku, Hideaki; Yaita, Tsuyoshi

Journal of Nuclear Science and Technology, 56(2), p.193 - 200, 2019/02

 Times Cited Count:1 Percentile:11.15(Nuclear Science & Technology)

During the accident that occurred at the Fukushima Daiichi Nuclear Power Plant, a large volume of seawater was introduced as coolant into the storage pools for spent nuclear fuel. If this fuel is reprocessed, some components of seawater will be mixed with the nitric acid solution containing metal ions in the reprocessing process where stainless steels are used as structural material. In this study, we investigated the effect of seawater components in high active liquid waste (HAW) containing nitric acid and metal ions as fission products on the corrosion behavior of SUS316L stainless steel. Corrosion tests were conducted in surrogate HAW containing artificial seawater (ASW). Intergranular corrosion was observed in the HAW with ASW, where Ru increased the corrosion potential to the transpassive region. An increase in the amount of ASW led to a decrease in the corrosion rate and suppression of intergranular corrosion. Interactions between Ru ions and seawater components, such as chloride ions, were indicated by the results of extended Xray absorption fine structure spectroscopy and cyclic voltammetry analyses of the solution containing ASW and HAW.

Journal Articles

Corrosion behaviour of FeCrAl-ODS steels in nitric acid solutions with several temperatures

Takahatake, Yoko; Ambai, Hiromu; Sano, Yuichi; Takeuchi, Masayuki; Koizumi, Kenji; Sakamoto, Kan*; Yamashita, Shinichiro

Proceedings of Annual Topical Meeting on Reactor Fuel Performance (TopFuel 2018) (Internet), 9 Pages, 2018/10

The corrosion behaviour of FeCrAl-ODS steels for the accident tolerant fuel cladding of LWRs were investigated in nitric acid solutions for the reprocessing process of spent fuels. The corrosion tests were carried out at 60$$^{circ}$$C, 80$$^{circ}$$C and the boiling point of the solutions, and the specimens were then analysed by XPS. The corrosion remarkably progressed at the boiling point, and the highest corrosion rate was 0.22 mm/y. In the oxide film, the atomic concentration of Fe was lower, than that in the base material, and those of Cr and Al were higher. The results show that the corrosion of FeCrAl-ODS steels in hot nitric acid solution is not severe because of the high corrosion resistance of the oxide film formed on the material; hence, the corrosion resistance of the new cladding materials in the dissolution process of spent fuel is acceptable for reprocessing operations.

Journal Articles

Effect of chloride ion on corrosion behavior of SUS316L-grade stainless steel in nitric acid solutions containing seawater components under $$gamma$$-ray irradiation

Sano, Yuichi; Ambai, Hiromu; Takeuchi, Masayuki; Iijima, Shizuka; Uchida, Naoki

Journal of Nuclear Materials, 493, p.200 - 206, 2017/09

 Times Cited Count:7 Percentile:56.89(Materials Science, Multidisciplinary)

Concerning the Fukushima Daiichi Nuclear Power Plant accident, we investigated the effect of chloride ion on the corrosion behavior of SUS316L stainless steel, which is a typical material for the equipment used in reprocessing, in HNO$$_{3}$$ solution containing seawater components, including under the $$gamma$$-ray irradiation condition. Electrochemical and immersion tests were carried out using a mixture of HNO$$_{3}$$ and artificial seawater (ASW). In the HNO$$_{3}$$ solution containing high amounts of ASW, the cathodic current densities increased and uniform corrosion progressed. This might be caused by strong oxidants, such as Cl$$_{2}$$ and NOCl, generated in the reaction between HNO$$_{3}$$ and Cl$$^{-}$$ ions. The corrosion rate decreased with the immersion time at low concentrations of HNO$$_{3}$$, while it increased at high concentrations. Under the $$gamma$$-ray irradiation condition, the corrosion rate decreased due to the suppression of the cathodic reactions by the reaction between the above oxidants and HNO$$_{2}$$ generated by radiolysis.

Journal Articles

Effect of sulfate ion on corrosion behavior of SUS316L in high active liquid waste

Ambai, Hiromu; Sano, Yuichi; Nishizuka, Yusuke*; Iijima, Shizuka; Uchida, Naoki

Zairyo To Kankyo, 66(5), p.169 - 172, 2017/05

We study the effect of sulfate ion which is one component of seawater or concrete on the corrosion behavior in high active liquid waste tank environment. The corrosion tests were conducted using SUS316L and surrogate high active liquid waste containing some metal ions and nitric acid. The results showed that sulfate ion inhibited the corrosion rates. The XPS results indicated the attachment of sulfate ion to material surfaces suppressed the anode reaction.

Journal Articles

Effect of seawater on corrosion of SUS316L in HAW under $$gamma$$-ray irradiation

Ambai, Hiromu; Nishizuka, Yusuke*; Sano, Yuichi; Uchida, Naoki; Iijima, Shizuka

QST-M-2; QST Takasaki Annual Report 2015, P. 90, 2017/03

The spent fuel stored in the storage pools at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company Holdings, Inc. is exposed with the environment containing seawater components, owing to the injection of seawater into the storage pools. Therefore, during reprocessing, it is expected that the spent fuel will be contaminated with seawater components, and the influence of seawater on reprocessing needs to be investigated. We conducted the corrosion tests of the HAW storage tanks under $$gamma$$-ray irradiation, and revealed that no significant effect of seawater components was emerged.

Journal Articles

Corrosion behavior of SUS316L in nitric acid solution containing seawater components

Sano, Yuichi; Ambai, Hiromu; Takeuchi, Masayuki; Iijima, Shizuka; Uchida, Naoki

Proceedings of European Corrosion Congress 2016 (EUROCORR 2016) (USB Flash Drive), 10 Pages, 2016/09

During the Fukushima Daiichi Nuclear Power Plant accident, significant volume of seawater was injected into the storage pool for spent nuclear fuel as the coolant. In this study, we investigated the effect of seawater components on the corrosion behavior of SUS316L stainless steel in HNO$$_{3}$$ solution. Electrochemical and immersion tests were carried out using a mixture of HNO$$_{3}$$ and artificial seawater (ASW). In the HNO$$_{3}$$ solution containing high amounts of ASW, the cathodic current densities increased and uniform corrosion progressed. This might be caused by strong oxidants, such as Cl$$_{2}$$ and NOCl, generated in the reaction between HNO$$_{3}$$ and Cl$$^{-}$$ ions. In addition, pitting corrosion occurred simultaneously at low HNO$$_{3}$$ concentrations. The corrosion rate decreased with the immersion time at low concentrations of HNO$$_{3}$$, while it increased at high concentrations. It is assumed that the cathodic reactions proceed slowly and the anodic reactions are gradually prevented by the growth of an oxide film on the surface of the coupon in low-concentration HNO$$_{3}$$. On the other hand, high-concentration HNO$$_{3}$$ triggers a vigorous cathodic reaction, which disturbs the growth of the oxide film and activates the anodic reactions. This competition between the cathodic and anodic reactions causes a change in the corrosion rates with the immersion time in a mixture of HNO$$_{3}$$ and ASW.

Journal Articles

Examination of the surrogate ratio method for the determination of the $$^{93}$$Zr(n,$$gamma$$)$$^{94}$$Zr cross section with $$^{90,92}$$Zr($$^{18}$$O,$$^{16}$$O)$$^{92,94}$$Zr reactions

Yan, S. Q.*; Li, Z. H.*; Wang, Y. B.*; Nishio, Katsuhisa; Makii, Hiroyuki; Su, J.*; Li, Y. J.*; Nishinaka, Ichiro; Hirose, Kentaro; Han, Y. L.*; et al.

Physical Review C, 94(1), p.015804_1 - 015804_5, 2016/07

 Times Cited Count:6 Percentile:44.49(Physics, Nuclear)

JAEA Reports

Countercurrent extraction/stripping experiments using TDdDGA solvent extractant in a centrifugal contactors system

Kibe, Satoshi; Fujisaku, Kazuhiko*; Ambai, Hiromu; Sakamoto, Atsushi; Sano, Yuichi; Takeuchi, Masayuki; Suzuki, Hideya; Tsubata, Yasuhiro; Matsumura, Tatsuro

JAEA-Research 2015-021, 40 Pages, 2016/02

JAEA-Research-2015-021.pdf:2.3MB

The flowsheet with TDdDGA extractant has been being developed for recovering MA from PUREX raffinate. In the previous study, the yields of MA and other elements in countercurrent extraction/stripping experiments using mixer-settlers were not enough for the target and it would be due to the insufficient phase (aqueous/organic) separation. In this study, we carried out countercurrent experiments with surrogate PUREX raffinate using centrifugal contactors which had superior phase separation ability, and evaluated the extraction/stripping behavior of each element. During the operation, abnormal fluid behavior, such as overflow and entrainment, was not observed, and sufficient phase separation was achieved by centrifugal contactors. Extraction behavior of lanthanides was similar to that in mixer-settlers, but their stripping efficiencies decreased. This would be due to shorter residence time in mixing zone.

Journal Articles

Signature splitting inversion and backbending in $$^{80}$$Rb

He, C.*; Shen, S.*; Wen, S.*; Zhu, L.*; Wu, X.*; Li, G.*; Zhao, Y.*; Yan, Y.*; Bai, Z.*; Wu, Y.*; et al.

Physical Review C, 87(3), p.034320_1 - 034320_10, 2013/03

 Times Cited Count:6 Percentile:43.66(Physics, Nuclear)

Journal Articles

Identified charged hadron production in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06

 Times Cited Count:184 Percentile:99.44(Physics, Nuclear)

Transverse momentum distributions and yields for $$pi^{pm}, K^{pm}, p$$, and $$bar{p}$$ in $$p + p$$ collisions at $$sqrt{s}$$ = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different $$sqrt{s}$$ collisions. We also present the scaling properties such as $$m_T$$ and $$x_T$$ scaling and discuss the mechanism of the particle production in $$p + p$$ collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.

Journal Articles

Azimuthal correlations of electrons from heavy-flavor decay with hadrons in $$p+p$$ and Au+Au collisions at $$sqrt{s_{NN}}$$ = 200 GeV

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.

Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04

 Times Cited Count:8 Percentile:49.7(Physics, Nuclear)

Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled $$p+p$$ collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to $$p+p$$ collisions.

Journal Articles

Measurement of neutral mesons in $$p$$ + $$p$$ collisions at $$sqrt{s}$$ = 200 GeV and scaling properties of hadron production

Adare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Y.*; Al-Bataineh, H.*; Alexander, J.*; Aoki, K.*; Aphecetche, L.*; Armendariz, R.*; et al.

Physical Review D, 83(5), p.052004_1 - 052004_26, 2011/03

 Times Cited Count:175 Percentile:98.48(Astronomy & Astrophysics)

The PHENIX experiment at RHIC has measured the invariant differential cross section for production of $$K^0_s$$, $$omega$$, $$eta'$$ and $$phi$$ mesons in $$p + p$$ collisions at $$sqrt{s}$$ = 200 GeV. The spectral shapes of all hadron transverse momentum distributions are well described by a Tsallis distribution functional form with only two parameters, $$n$$ and $$T$$, determining the high $$p_T$$ and characterizing the low $$p_T$$ regions for the spectra, respectively. The integrated invariant cross sections calculated from the fitted distributions are found to be consistent with existing measurements and with statistical model predictions.

Oral presentation

Corrosion resistance of tank material for flock storage, 2; Corrosion behavior in fluid flow condition by air agitation

Ambai, Hiromu; Sano, Yuichi; Takeuchi, Masayuki; Sakauchi, Nobuyuki; Hoshi, Masayuki; Ogino, Hideki; Koizumi, Kenji

no journal, , 

We studied the corrosion behavior of the tank material SS400 for flock storage in fluid flow condition by air agitation. Fluid flow increased the corrosion rate and this effect was reduced by the presence of the flock. Decreasing of flow rate and change of air to inactive gas are effective in corrosion prevention measures.

Oral presentation

Corrosion resistance of tank material for flock storage

Ambai, Hiromu; Sano, Yuichi; Takeuchi, Masayuki; Koma, Yoshikazu

no journal, , 

We studied the corrosion behavior of the tank material SS400 for flock storage in fluid flow condition by air agitation. Fluid flow increased the corrosion rate and this effect was reduced by the presence of the flock. Decreasing of flow rate and change of air to inactive gas are effective in corrosion prevention measures.

Oral presentation

Effect of seawater on corrosion of materials used in reprocessing process, 3; Corrosion of storage tank for high level liquid waste

Ambai, Hiromu; Nishizuka, Yusuke; Sano, Yuichi; Uchida, Naoki; Taguchi, Katsuya; Takeuchi, Masayuki

no journal, , 

As part of the investigation of reprocessing the spent nuclear fuels which are stored in the spent fuel pools of Fukushima Daiichi Nuclear Power Plant, we studied the influence of seawater components on the corrosion of storage tank for high level liquid waste. From the results of our corrosion experiments by using simulated high level liquid waste, the corrosion is inhibited by seawater components.

Oral presentation

Effect of seawater on corrosion of materials used in reprocessing process, 4; Corrosion of storage tank for high level liquid waste

Ambai, Hiromu; Nishizuka, Yusuke; Sano, Yuichi; Uchida, Naoki; Iijima, Shizuka

no journal, , 

As a part of studies about reprocessing of the spent nuclear fuels in the storage pool at the Fukushima Daiichi Nuclear Power Plant, we investigated the effect of seawater components in high activity liquid waste on the corrosion. The corrosion tests with $$gamma$$ ray irradiation showed that sea water components didn't make significant difference in the corrosion.

28 (Records 1-20 displayed on this page)