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Journal Articles

A Systematic approach for the adequacy analysis of a set of experimental databases: Application in the framework of the ATRIUM activity

Baccou, J.*; Glantz, T.*; Ghione, A.*; Sargentini, L.*; Fillion, P.*; Damblin, G.*; Sueur, R.*; Iooss, B.*; Fang, J.*; Liu, J.*; et al.

Nuclear Engineering and Design, 421, p.113035_1 - 113035_16, 2024/05

Journal Articles

Pressure engineering of van der Waals compound RhI$$_3$$; Bandgap narrowing, metallization, and remarkable enhancement of photoelectric activity

Fang, Y.*; Kong, L.*; Wang, R.*; Zhang, Z.*; Li, Z.*; Wu, Y.*; Bu, K.*; Liu, X.*; Yan, S.*; Hattori, Takanori; et al.

Materials Today Physics (Internet), 34, p.101083_1 - 101083_7, 2023/05

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

The layered van der Waals halides are particularly sensitive to external pressure, suggesting a feasible route to pinpoint their structure with extraordinary behavior. However, a very sensitive pressure response usually lead to a detrimental phase transition and/or lattice distortion, making the approach of materials manipulation in a continuous manner remain challenging. Here, the extremely weak interlayer coupling and high tunability of layered RhI$$_3$$ crystals are observed. A pressure-driven phase transition occurs at a moderate pressure of 5 GPa, interlinking to a change of layer stack mode. Strikingly, such a phase transition does not affect the tendency of quasi-linear bandgap narrowing, and a metallization with an ultra-broad tunability of 1.3 eV redshift is observed at higher pressures. Moreover, the carrier concentration increases by 4 orders of magnitude at 30 GPa, and the photocurrent enhances by 5 orders of magnitude at 7.8 GPa. These findings create new opportunities for exploring, tuning, and understanding the van der Waals halides by harnessing their unusual feature of a layered structure, which is promising for future devices based on materials-by-design that are atomically thin.

Journal Articles

Structure of an aqueous RbCl solution in the gigapascal pressure range by neutron diffraction combined with empirical potential structure refinement modeling

Zhang, W. Q.*; Yamaguchi, Toshio*; Fang, C. H.*; Yoshida, Koji*; Zhou, Y. Q.*; Zhu, F. Y.*; Machida, Shinichi*; Hattori, Takanori; Li, W.*

Journal of Molecular Liquids, 348, p.118080_1 - 118080_11, 2022/02

 Times Cited Count:1 Percentile:37.82(Chemistry, Physical)

The ion hydration and association and hydrogen-bonded water structure in an aqueous 3 mol/kg RbCl solution were investigated at 298 K/0.1 MPa, 298 K/1 GPa, 523 K/1 GPa, and 523 K/4 GPa by neutron diffraction combined with EPSR methods. The second hydration layer of Rb$$^+$$ and Cl$$^-$$ becomes evident under elevated pressure and temperature conditions. The average oxygen coordination number of Rb$$^+$$ (Cl$$^-$$) in the first hydration layer increases from 6.3 (5.9) ambient pressure to 8.9 (9.1) at 4 GPa, while decreasing coordination distance from 0.290 nm (0.322 nm) to 0.288 nm (0.314 nm). The orientation of the water dipole in the first solvation shell of Rb$$^+$$ and a central water molecule is sensitive to pressure, but that in the first solvation shell of Cl$$^-$$ does not change very much. The number of contact-ion pairs Rb$$^+$$-Cl$$^-$$ decreases with elevated temperature and increases with elevated pressure. Water molecules are closely packed, and the tetrahedral hydrogen-bonded network of water molecules no longer exists in extreme conditions.

Journal Articles

A Model intercomparison of atmospheric $$^{137}$$Cs concentrations from the Fukushima Daiichi Nuclear Power Plant accident, phase III; Simulation with an identical source term and meteorological field at 1-km resolution

Sato, Yosuke*; Sekiyama, Tsuyoshi*; Fang, S.*; Kajino, Mizuo*; Qu$'e$rel, A.*; Qu$'e$lo, D.*; Kondo, Hiroaki*; Terada, Hiroaki; Kadowaki, Masanao; Takigawa, Masayuki*; et al.

Atmospheric Environment; X (Internet), 7, p.100086_1 - 100086_12, 2020/10

The third model intercomparison project for investigating the atmospheric behavior of $$^{137}$$Cs emitted during the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident (FDNPP-MIP) was conducted. A finer horizontal grid spacing (1 km) was used than in the previous FDNPP-MIP. Nine of the models used in the previous FDNPP-MIP were also used, and all models used identical source terms and meteorological fields. Our analyses indicated that most of the observed high atmospheric $$^{137}$$Cs concentrations were well simulated, and the good performance of some models improved the performance of the multi-model ensemble. The analyses also confirmed that the use of a finer grid resolution resulted in the meteorological field near FDNPP being better reproduced. The good representation of the wind field resulted in the reasonable simulation of the narrow distribution of high deposition amount to the northwest of FDNPP and the reduction of the overestimation over the area to the south of FDNPP. In contrast, the performance of the models in simulating plumes observed over the Nakadori area, the northern part of Gunma, and the Tokyo metropolitan area was slightly worse.

Journal Articles

Analysis of voltage droop on J-PARC klystron high voltage power supply

Fuwa, Yasuhiro; Ono, Ayato; Takayanagi, Tomohiro; Shinozaki, Shinichi; Mizobata, Satoshi*; Fang, Z.*

Proceedings of 17th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.780 - 782, 2020/09

In the J-PARC linac, High Voltage DC power supplies (HVDC) to drive klystrons. These HVDCs are modulating-anode power supplies with a rated voltage of 110 kV and are operated by connecting up to four klystrons to a single HVDC. Since multiple klystrons are driven by a single HVDC, a voltage droop in the capacitor bank of the HVDC occurs in the beam pulse. This effect causes a decrease in the output power of the klystron. Half of the existing HVDC in J-PARC were installed at the J-PARC construction, and the other half were installed at the LINAC 400 MeV upgrade, and the capacitors show signs of age-related degradation. In the near future, the capacitors will be necessary to be replaced partially or completely. On the replacement of the capacitors, it will be necessary to re-evaluate the operating behavior of the HVDC when the capacitor bank configuration is changed. In this presentation, we evaluated the effect of the voltage droop on the klystron with the present configuration and the effect of changing the capacitor bank configuration with numerical and experimental results, and we discussed the countermeasure for the stable beam operation.

Journal Articles

Upgrade of the 3-MeV linac for testing of accelerator components at J-PARC

Kondo, Yasuhiro; Hirano, Koichiro; Ito, Takashi; Kikuzawa, Nobuhiro; Kitamura, Ryo; Morishita, Takatoshi; Oguri, Hidetomo; Okoshi, Kiyonori; Shinozaki, Shinichi; Shinto, Katsuhiro; et al.

Journal of Physics; Conference Series, 1350, p.012077_1 - 012077_7, 2019/12

 Times Cited Count:1 Percentile:52.4

We have upgraded a 3-MeV linac at J-PARC. The ion source is same as the J-PARC linac's, and the old 30-mA RFQ is replaced by a spare 50-mA RFQ, therefore, the beam energy is 3 MeV and the nominal beam current is 50 mA. The main purpose of this system is to test the spare RFQ, but also used for testing of various components required in order to keep the stable operation of the J-PARC accelerator. The accelerator has been already commissioned, and measurement programs have been started. In this paper, present status of this 3-MeV linac is presented.

Journal Articles

Performance test of J-PARC 324 MHz klystrons

Fuwa, Yasuhiro; Shinozaki, Shinichi; Chishiro, Etsuji; Hirane, Tatsuya; Fang, Z.*; Fukui, Yuji*; Futatsukawa, Kenta*; Mizobata, Satoshi*; Iwama, Yuhei*; Sato, Yoshikatsu*; et al.

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.611 - 613, 2019/10

In the J-PARC linac, a proton accelerator is operated using 45 units of 324 MHz and 972 MHz klystrons. In the future stabilization and advancement of the accelerator, it is important to acquire the klystron output characteristics near the maximum output accurately. In order to understand this characteristics, measurement of the characteristics of the replaced klystron for some reason such as discharge, as well as the new klystron. However, such measurements have not been performed because of the risk of damage including peripheral equipment due to discharge and the temporal interference with the operation of the accelerator. Therefore, we set up a klystron test stand in the linac building and measured the high-voltage characteristics and input/output characteristics of the klystron under various operating parameters. By using this measurement result, the characteristics of klystron can be obtained before installation, and it becomes possible to determine the optimum operation parameters and make effective plan of klystron replacements. In addition, basic data for predicting the degradation tendency of klystron was acquired by comparing the characteristics of the used and used klystron.

Journal Articles

Pressure-induced Diels-Alder reactions in C$$_{6}$$H$$_{6}$$ - C$$_{6}$$F$$_{6}$$ cocrystal towards graphane structure

Wang, Y.*; Dong, X.*; Tang, X.*; Zheng, H.*; Li, K.*; Lin, X.*; Fang, L.*; Sun, G.*; Chen, X.*; Xie, L.*; et al.

Angewandte Chemie; International Edition, 58(5), p.1468 - 1473, 2019/01

 Times Cited Count:29 Percentile:79.84(Chemistry, Multidisciplinary)

Pressure-induced polymerization (PIP) of aromatics is a novel method to construct sp$$^{3}$$-carbon frameworks, and nanothreads with diamond-like structures were synthesized by compressing benzene and its derivatives. Here by compressing benzene-hexafluorobenzene cocrystal(CHCF), we identified H-F-substituted graphane with a layered structure in the PIP product. Based on the crystal structure determined from the in situ neutron diffraction and the intermediate products identified by the gas chromatography-mass spectrum, we found that at 20 GPa CHCF forms tilted columns with benzene and hexafluorobenzene stacked alternatively, which leads to a [4+2] polymer, and then transfers to short-range ordered hydrogenated-fluorinated graphane. The reaction process contains [4+2] Diels-Alder, retro-Diels-Alder, and 1-1' coupling, and the former is the key reaction in the PIP. Our studies confirmed the elemental reactions of the CHCF for the first time, which provides a novel insight into the PIP of aromatics.

Journal Articles

Model intercomparison of atmospheric $$^{137}$$Cs from the Fukushima Daiichi Nuclear Power Plant accident; Simulations based on identical input data

Sato, Yosuke*; Takigawa, Masayuki*; Sekiyama, Tsuyoshi*; Kajino, Mizuo*; Terada, Hiroaki; Nagai, Haruyasu; Kondo, Hiroaki*; Uchida, Junya*; Goto, Daisuke*; Qu$'e$lo, D.*; et al.

Journal of Geophysical Research; Atmospheres, 123(20), p.11748 - 11765, 2018/10

 Times Cited Count:39 Percentile:85.11(Meteorology & Atmospheric Sciences)

A model intercomparison of the atmospheric dispersion of $$^{137}$$Cs emitted following the Fukushima Daiichi Nuclear Power Plant accident was conducted by 12 models to understand the behavior of $$^{137}$$Cs in the atmosphere. The same meteorological data, horizontal grid resolution, and an emission inventory were applied to all the models to focus on the model variability originating from the processes included in each model. The multi-model ensemble captured 40% of the observed $$^{137}$$Cs events, and the figure-of-merit in space for the total deposition of $$^{137}$$Cs exceeded 80. Our analyses indicated that the meteorological data were most critical for reproducing the $$^{137}$$Cs events. The results also revealed that the differences among the models were originated from the deposition and diffusion processes when the meteorological field was simulated well. However, the models with strong diffusion tended to overestimate the $$^{137}$$Cs concentrations.

Journal Articles

Status of the J-PARC Linac LLRF system

Futatsukawa, Kenta*; Fang, Z.*; Fukui, Yuji*; Shinozaki, Shinichi; Mizobata, Satoshi; Sato, Yoshikatsu*

Proceedings of 14th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.486 - 489, 2017/12

In the J-PARC linac, the LLRF systems consist of twenty-four 324-MHz systems and twenty-five 972-MHz systems for ACS cavities. The 324-MHz LLRF systems, which were installed in the stations of RFQ, DTLs, and SDTLs, have been used since the beginning of the J-PARC and are more than ten years into the development. Realistically speaking, the incensement of the failure frequency for these systems is expected. Additionally, it is difficult to maintain those for some discontinued boards of a digital feedback (DFB) and a digital feedforward (DFF) at cPCI, and the older OS and developing environment of software. Therefore, we are starting to study the new LLRF system of the next generation. In the present, we are exploring several possibilities of a new way and investigating each advantage and disadvantage. The project and the status of the development for the new system in the J-PARC linac LLRF are introduced.

Journal Articles

A 3 MeV linac for development of accelerator components at J-PARC

Kondo, Yasuhiro; Asano, Hiroyuki*; Chishiro, Etsuji; Hirano, Koichiro; Ishiyama, Tatsuya; Ito, Takashi; Kawane, Yusuke; Kikuzawa, Nobuhiro; Meigo, Shinichiro; Miura, Akihiko; et al.

Proceedings of 28th International Linear Accelerator Conference (LINAC 2016) (Internet), p.298 - 300, 2017/05

We have constructed a linac for development of various accelerator components at J-PARC. The ion source is same as the J-PARC linac's, and the RFQ is a used one in the J-PARC linac. The beam energy is 3 MeV and nominal beam current is 30 mA. The accelerator has been already commissioned, and the first development program, laser-charge-exchange experiment for the transmutation experimental facility, has been started. In this paper, present status of this 3-MeV linac is presented.

Journal Articles

Type II shell evolution in $$A=70$$ isobars from the $$N geq 40$$ island of inversion

Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; Tsunoda, Yusuke*; Otsuka, T.*; Nishimura, Shunji*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; et al.

Physics Letters B, 765, p.328 - 333, 2017/02

 Times Cited Count:31 Percentile:92.19(Astronomy & Astrophysics)

Journal Articles

Study of beam loading compensation with comb-like structure at J-PARC linac

Futatsukawa, Kenta*; Kobayashi, Tetsuya*; Sato, Yoshikatsu; Shinozaki, Shinichi; Fang, Z.*; Fukui, Yuji*; Mizobata, Satoshi; Michizono, Shinichiro*

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.327 - 331, 2016/11

In the J-PARC linac, an intermediate-pulse with the comb-like structure is shaped by kicking an unwanted beam by the chopper cavity. Therefore, the cavities lying downstream of the RF-chopper have the beam loading with this beam shape. The present feedforward system which assumes the averaged beam current and not the comb-like beam was operated in the present LLRF, because the beam current in the linac was lower than the design value. However, it has been difficult that the required precision for the RF system is satisfied with increasing beam current. Thus, we performed the beam study of the beam loading compensation with the same shapes as the intermediate-pulses. The positive results for the cavities of SDTL and DTL with high Q values were obtained compared to the present system. On the other hand, when this compensation system was used in the case of ACS cavities, the neighbor modes were excited by the input RF. We have to improve the FF system for the operation against the real beam.

Journal Articles

Development of beam scrapers using a 3-Mev linac at J-PARC

Hirano, Koichiro; Asano, Hiroyuki; Ishiyama, Tatsuya; Ito, Takashi; Okoshi, Kiyonori; Oguri, Hidetomo; Kondo, Yasuhiro; Kawane, Yusuke; Kikuzawa, Nobuhiro; Sato, Yoshikatsu; et al.

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.310 - 313, 2016/11

We have used a beam scraper with the incident angle of 65deg to reduce the beam power deposition density in the MEBT between a 324 MHz RFQ and a 50-MeV DTL of the J-PARC linac. The 65$$^{circ}$$ scraper was irradiated by the H$$^{-}$$ beam up to particle number of 1.47E22. We observed a lot of surface projections with several hundred micrometers high in the beam irradiation damage on the scraper by using the laser microscope. In order to study the limits of scrapers, we constructed a new 3 MeV linac at J-PARC. We will conduct the scraper irradiation test at the end of this year.

Journal Articles

Beam commissioning of the linac for iBNCT

Naito, Fujio*; Anami, Shozo*; Ikegami, Kiyoshi*; Uota, Masahiko*; Ouchi, Toshikatsu*; Onishi, Takahiro*; Oba, Toshiyuki*; Obina, Takashi*; Kawamura, Masato*; Kumada, Hiroaki*; et al.

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1244 - 1246, 2016/11

The proton linac installed in the Ibaraki Neutron Medical Research Center is used for production of the intense neutron flux for the Boron Neutron Capture Therapy (BNCT). The linac consists of the 3-MeV RFQ and the 8-MeV DTL. Design average beam current is 10mA. Target is made of Beryllium. First neutron production from the Beryllium target was observed at the end of 2015 with the low intensity beam as a demonstration. After the observation of neutron production, a lot of improvement s was carried out in order to increase the proton beam intensity for the real beam commissioning. The beam commissioning has been started on May 2016. The status of the commissioning is summarized in this report.

Journal Articles

Low-lying excitations in $$^{72}$$Ni

Morales, A. I.*; Benzoni, G.*; Watanabe, H.*; Nishimura, Shunji*; Browne, F.*; Daido, R.*; Doornenbal, P.*; Fang, Y.*; Lorusso, G.*; Patel, Z.*; et al.

Physical Review C, 93(3), p.034328_1 - 034328_14, 2016/03

 Times Cited Count:25 Percentile:85.51(Physics, Nuclear)

Journal Articles

Decay properties of $$^{68,69,70}$$Mn; Probing collectivity up to N=44 in Fe isotopic chain

Benzoni, G.*; Morales, A. I.*; Watanabe, H.*; Nishimura, Shunji*; Coraggio, L.*; Itaco, N.*; Gargano, A.*; Browne, F.*; Daido, R.*; Doornenbal, P.*; et al.

Physics Letters B, 751, p.107 - 112, 2015/12

 Times Cited Count:20 Percentile:78.31(Astronomy & Astrophysics)

Journal Articles

Development of phase rotation system for RF-chopper at J-PARC Linac

Futatsukawa, Kenta*; Kobayashi, Tetsuya*; Sato, Fumiaki; Shinozaki, Shinichi; Chishiro, Etsuji; Hirano, Koichiro; Fang, Z.*; Fukui, Yuji*; Hori, Toshihiko; Michizono, Shinichiro*

Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1317 - 1320, 2015/09

In the J-PARC linac, an RF deflector installed in 3-MeV Medium Energy Beam Transport (MEBT1) is used to kick the unnecessary beam and the intermediate-pulse like a comb is created. The kicked beam leads to a scraper downstream the RF deflector and lose all kinetic energy. When the beam current increases to 50 mA of the design value, the heat load of a scraper to irradiate the kicked beam increases and its surface is predicted to be damaged. Therefore, we are preparing the tandem scrapers to reduce the damage. The half of the kicked beam leads to a scraper and the residual is to the other. The chopping operation is achieved by rotating the phase of the RF deflector in the periodic cycles by the LLRF system. We will introduce the phase rotation system and the test results.

Journal Articles

Development of RF chopper system at J-PARC Linac, 2

Hirano, Koichiro; Kondo, Yasuhiro; Kawane, Yusuke; Shinozaki, Shinichi; Miura, Akihiko; Morishita, Takatoshi; Sawabe, Yuki; Sugimura, Takashi*; Naito, Fujio*; Fang, Z.*; et al.

Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.944 - 947, 2015/09

Two RF-deflecting cavities as a chopper and a beam scraper have been used in the MEBT1 between a 324 MHz RFQ and a 50-MeV DTL of the J-PARC Linac. We replaced with a newly fabricated RF chopper to decrease beam loss for the operation with 50 mA. We installed two new scrapers to absorb the higher power of the deflected beam by the RF chopper. This paper describes the RF chopper system and beam irradiation test results of the scraper.

Journal Articles

Beam test of a new radio frequency quadrupole linac for the Japan Proton Accelerator Research Complex

Kondo, Yasuhiro; Morishita, Takatoshi; Yamazaki, Saishun; Hori, Toshihiko; Sawabe, Yuki; Chishiro, Etsuji; Fukuda, Shimpei; Hasegawa, Kazuo; Hirano, Koichiro; Kikuzawa, Nobuhiro; et al.

Physical Review Special Topics; Accelerators and Beams, 17(12), p.120101_1 - 120101_8, 2014/12

 Times Cited Count:6 Percentile:43.07(Physics, Nuclear)

We performed a beam test of a new radio frequency quadrupole linac (RFQ III) for the beam current upgrade of the Japan Proton Accelerator Research Complex. First, the conditioning of RFQ III was conducted, and after 20 h of conditioning, RFQ III became very stable with a nominal peak power and duty factor of 400 kW and 1.5%, respectively. An off-line beam test was subsequently conducted before installation in the accelerator tunnel. The transmission, transverse emittance, and energy spread of the 50-mA negative hydrogen beam from RFQ III were measured and compared with simulation results. The experiment and simulation results showed good agreement; therefore, we conclude that the performance of RFQ III conforms to its design.

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