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Journal Articles

Measurement of spent nuclear fuel burn-up using a new H$$(n,gamma)$$ method

Nauchi, Yasushi*; Sato, Shunsuke*; Hayakawa, Takehito*; Kimura, Yasuhiko; Suyama, Kenya; Kashima, Takao*; Futakami, Kazuhiro*

Nuclear Instruments and Methods in Physics Research A, 1050, p.168109_1 - 168109_9, 2023/05

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

Measurement of neutrons from spent nuclear fuel is performed in this study using the H$$(n,gamma)$$ method, which detects 2.223 MeV $$gamma$$ rays from neutron capture reaction of hydrogen using a highly pure germanium (HPGe) detector. The detection of the 2.223 MeV $$gamma$$ ray is affected by intense $$gamma$$ ray emission from fission products (FPs) because the emission rate of $$gamma$$ rays from the FP is seven orders of magnitude higher than the emission rate of neutrons. To shield the intense $$gamma$$ ray from the FP, the HPGe detector is placed off the axis of a collimator, whereas a polyethylene block is placed on the axis. In this geometry, the detector is shielded from the intense $$gamma$$ rays from the FP, but the detector can measure 2.223 MeV $$gamma$$ rays from the H$$(n,gamma)$$ reactions in the polyethylene block. The measured count rate of the 2.223 MeV $$gamma$$ rays is consistent with the expected rate within the statistical error, which is calculated based on the nuclide composition, which is primary $$^{244}$$Cm, estimated via depletion and decay calculations. Accordingly, the H$$(n,gamma)$$ method is considered feasible to quantify the number of neutron leakage from spent nuclear fuel assembly, which is applicable to certify burn up of the assembly.

Journal Articles

Absolute quantification of $$^{137}$$Cs activity in spent nuclear fuel with calculated detector response function

Sato, Shunsuke*; Nauchi, Yasushi*; Hayakawa, Takehito*; Kimura, Yasuhiko; Kashima, Takao*; Futakami, Kazuhiro*; Suyama, Kenya

Journal of Nuclear Science and Technology, 60(6), p.615 - 623, 2022/06

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A new non-destructive method for evaluating $$^{137}$$Cs activity in spent nuclear fuels was proposed and experimentally demonstrated for physical measurements in burnup credit implementation. $$^{137}$$Cs activities were quantified using gamma ray measurements and numerical detector response simulations without reference fuels, in which $$^{137}$$Cs activities are well known. Fuel samples were obtained from a lead use assembly (LUA) irradiated in a commercial pressurized water reactor (PWR) up to 53 GWd/t. Gamma rays emitted from the samples were measured using a bismuth germinate (BGO) scintillation detector through a collimator attached to a hot cell. The detection efficiency of gamma rays with the detector was calculated using the PHITS particle transport calculation code considering the measurement geometry. The relative activities of $$^{134}$$Cs, $$^{137}$$Cs, and $$^{154}$$Eu in the sample were measured with a high-purity germanium (HPGe) detector for more accurate simulations of the detector response for the samples. The absolute efficiency of the detector was calibrated by measuring a standard gamma ray source in another geometry. $$^{137}$$Cs activity in the fuel samples was quantified using the measured count rate and detection efficiency. The quantified $$^{137}$$Cs activities agreed well with those estimated using the MVP-BURN depletion calculation code.

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