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JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2022

Kokubun, Yuji; Nakada, Akira; Seya, Natsumi; Koike, Yuko; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; Nagai, Shinji; et al.

JAEA-Review 2023-046, 164 Pages, 2024/03

JAEA-Review-2023-046.pdf:4.2MB

The Nuclear Fuel Cycle Engineering Laboratories conducts environmental radiation monitoring around the reprocessing plant in accordance with the "Safety Regulations for Reprocessing Plant of JAEA, Part IV: Environmental Monitoring". This report summarizes the results of environmental radiation monitoring conducted during the period from April 2022 to March 2023 and the results of dose calculations for the surrounding public due to the release of radioactive materials into the atmosphere and ocean. In the results of the above environmental radiation monitoring, many items were affected by radioactive materials emitted from the accident at the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Company, Incorporated (changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016), which occurred in March 2011. Also included as appendices are an overview of the environmental monitoring plan, an overview of measurement methods, measurement results and their changes over time, meteorological statistics results, radioactive waste release status, and an evaluation of the data which deviated of the normal range.

Journal Articles

Evaluation of the remaining spent extraction solvent in vermiculite after leaching tests via PIXE analysis

Arai, Yoichi; Watanabe, So; Hasegawa, Kenta; Okamura, Nobuo; Watanabe, Masayuki; Takeda, Keisuke*; Fukumoto, Hiroki*; Ago, Tomohiro*; Hagura, Naoto*; Tsukahara, Takehiko*

Nuclear Instruments and Methods in Physics Research B, 542, p.206 - 213, 2023/09

 Times Cited Count:1 Percentile:0.02(Instruments & Instrumentation)

Journal Articles

Cost-reduced depletion calculation including short half-life nuclides for nuclear fuel cycle simulation

Okamura, Tomohiro*; Katano, Ryota; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*

Journal of Nuclear Science and Technology, 60(6), p.632 - 641, 2023/06

 Times Cited Count:2 Percentile:50.96(Nuclear Science & Technology)

The Okamura explicit method (OEM) for depletion calculation was developed by modifying the matrix exponential method for dynamic nuclear fuel cycle simulation. The OEM suppressed the divergence of the calculation for short half-life nuclides, even for long time steps. The computational cost of the OEM was small, equivalent to the Euler method, and it maintained sufficient accuracy for the fuel cycle simulation.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2021

Nakada, Akira; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Futagawa, Kazuo; Nemoto, Masashi; Tobita, Keiji; Yamada, Ryohei*; Uchiyama, Rei; Yamashita, Daichi; et al.

JAEA-Review 2022-078, 164 Pages, 2023/03

JAEA-Review-2022-078.pdf:2.64MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2021 to March 2022. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Fact-finding survey on the competencies and literacy of radiological technologists regarding radiation disasters

Arai, Tomohiro*; Murata, Sho*; Watanabe, Yuichi*; Ishihara, Toshihiro*; Fukamizu, Yoshiya*; Takeda, Satoshi*; Ebata, Kiyokadzu*; Watanabe, Yuki; Takashima, Yoshio*; Kaneko, Junichi*

Journal of X-Ray Science and Technology, 31(2), p.237 - 245, 2023/03

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

Radiological technologists have received specialized education about radiation and serve as risk communicators who aim to lessen patients' anxiety about radiation exposure, in addition to performing radiological examinations in routine clinical practice. Also, Radiological technologists across Japan were dispatched to the affected area to conduct an essential procedure-screening the belongings and body surfaces of evacuees for contamination at the nuclear disaster at the Fukushima Daiichi Nuclear Power Plant operated by Tokyo Electric Power Company in March 2011. In this study, we conducted a fact-finding survey on knowledge and awareness of radiation disasters among radiological technologists at National Hospital Organization facilities in Japan to reveal their literacy and competencies regarding radiation disasters. Also, we compared the knowledge and awareness of radiation disasters among Japanese radiological technologists between nuclear power station areas and non-nuclear power station areas and discuss ideal human resource development for radiological technologists to be ready to serve during a radiation disaster.

JAEA Reports

User manual of NMB4.0

Okamura, Tomohiro*; Nishihara, Kenji; Katano, Ryota; Oizumi, Akito; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*

JAEA-Data/Code 2021-016, 43 Pages, 2022/03

JAEA-Data-Code-2021-016.pdf:3.06MB

The quantitative prediction and analysis of the future nuclear energy utilization scenarios are required in order to establish the advanced nuclear fuel cycle. However, the nuclear fuel cycle consists of various processes from front- to back-end, and it is difficult to analyze the scenarios due to the complexity of modeling and the variety of scenarios. Japan Atomic Energy Agency and Tokyo Institute of Technology have jointly developed the NMB code as a tool for integrated analysis of mass balance from natural uranium needs to radionuclide migration of geological disposal. This user manual describes how to create a database and scenario input for the NMB version 4.0.

Journal Articles

Applicability of equivalent linear analysis to reinforced concrete shear walls; 3D FEM simulation of experiment results of seismic wall ultimate behavior

Ichihara, Yoshitaka*; Nakamura, Naohiro*; Moritani, Hiroshi*; Horiguchi, Tomohiro*; Choi, B.

Nihon Genshiryoku Gakkai Wabun Rombunshi, 21(1), p.1 - 14, 2022/03

In this study, we aim to approximately evaluate the effect of nonlinearity of reinforced concrete structures through seismic response analysis using the equivalent linear analysis method. A simulation analysis was performed for the ultimate response test of the shear wall of the reactor building used in an international competition by OECD/NEA in 1996. The equivalent stiffness and damping of the shear wall were obtained from the trilinear skeleton curves proposed by the Japan Electric Association and the hysteresis curves proposed by Cheng et al. The dominant frequency, maximum acceleration response, maximum displacement response, inertia force-displacement relationship, and acceleration response spectra of the top slab could be simulated well up to a shear strain of approximately $$gamma$$=2.0$$times$$10$$^{-3}$$. The equivalent linear analysis used herein underestimates the maximum displacement response at the time of ultimate fracture of approximately $$gamma$$=4.0$$times$$10$$^{-3}$$. Moreover, the maximum shear strain of the shear wall could not capture the locally occurring shear strain compared with that of the nonlinear analysis. Therefore, when employing this method to evaluate the maximum shear strain and test results, including those during the sudden increase in displacement immediately before the fracture, sufficient attention must be paid to its applicability.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2020

Nakada, Akira; Nakano, Masanao; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Nemoto, Masashi; Tobita, Keiji; Futagawa, Kazuo; Yamada, Ryohei; Uchiyama, Rei; et al.

JAEA-Review 2021-062, 163 Pages, 2022/02

JAEA-Review-2021-062.pdf:2.87MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2020 to March 2021. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

NMB4.0: Development of integrated nuclear fuel cycle simulation code

Okamura, Tomohiro*; Katano, Ryota; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*

Bulletin of the Laboratory for Advanced Nuclear Energy, 6, p.29 - 30, 2022/02

Takeshita Laboratory, Tokyo Institute of Technology, has been developing Nuclear Material Balance code version 4.0 (NMB4.0) in collaboration with Japan Atomic Energy Agency (JAEA). This report summarized the outline and functions of NMB4.0.

Journal Articles

NMB4.0: Development of integrated nuclear fuel cycle simulator from the front to back-end

Okamura, Tomohiro*; Katano, Ryota; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*

EPJ Nuclear Sciences & Technologies (Internet), 7, p.19_1 - 19_13, 2021/11

Nuclear Material Balance code version 4.0 (NMB4.0) has been developed through collaborative R&D between Tokyo Institute of Technology and JAEA. Conventional nuclear fuel cycle simulation codes mainly analyze actinides and are specialized for front-end mass balance analysis. However, quantitative back-end simulation has recently become necessary for considering R&D strategies and sustainable nuclear energy utilization. Therefore, NMB4.0 was developed to realize the integrated nuclear fuel cycle simulation from front- to back-end. There are three technical features in NMB4.0: 179 nuclides are tracked, more than any other code, throughout the nuclear fuel cycle; the Okamura explicit method is implemented, which contributes to reducing the numerical cost while maintaining the accuracy of depletion calculations on nuclides with a shorter half-life; and flexibility of back-end simulation is achieved. The main objective of this paper is to show the newly developed functions, made for integrated back-end simulation, and verify NMB4.0 through a benchmark study to show the computational performance.

Journal Articles

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

 Times Cited Count:3 Percentile:14.19(Chemistry, Multidisciplinary)

The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 $$^circ$$C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$. From the obtained experimental results, thermochemical data for DbOCl$$_3$$ were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.

JAEA Reports

Selection of nuclides for mass-balance analysis of fission products

Okamura, Tomohiro*; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Takeshita, Kenji*

JAEA-Data/Code 2020-023, 32 Pages, 2021/03

JAEA-Data-Code-2020-023.pdf:1.67MB

Nuclear Material Balance code (NMB code) have been developed in Japan Atomic Energy Agency. The NMB code will be updated with the function of mass balance analysis at the backend process such as reprocessing, vitrification and geological disposal. In order to perform its analysis with high accuracy, it is necessary to expand the number of FP nuclides calculated in the NMB code. In this study, depletion calculation by ORIGEN code was performed under 3 different burn-up conditions such as spent uranium fuel from light water reactor, and nuclides were selected from 5 evaluation indexes such as mass and heat generation. In addition, the FP nuclides required to configure a simple burnup chain with the same calculation accuracy as ORIGEN in the NMB code was selected. As the result, two lists with different number of nuclides, such as "Detailed list" and a "Simplified list", were created.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:44 Percentile:97.1(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2019

Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Seya, Natsumi; Nishimura, Shusaku; Hosomi, Kenji; Nagaoka, Mika; Yokoyama, Hiroya; Matsubara, Natsumi; et al.

JAEA-Review 2020-069, 163 Pages, 2021/02

JAEA-Review-2020-069.pdf:4.78MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2019 to March 2020. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

Journal Articles

Development of mass balance analysis code for various waste management scenario

Okamura, Tomohiro*; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Takeshita, Kenji*

Bulletin of the Laboratory for Advanced Nuclear Energy, 5, P. 31, 2021/02

The Takeshita Laboratory at Tokyo Institute of Technology has started to develop a Nuclear Material Balance code (NMB code) in collaboration with Japan Atomic Energy Agency. This report summarized the results of the joint research conducted in 2019.

Journal Articles

Grain-boundary phosphorus segregation in highly neutron-irradiated reactor pressure vessel steels and its effect on irradiation embrittlement

Hata, Kuniki; Takamizawa, Hisashi; Hojo, Tomohiro*; Ebihara, Kenichi; Nishiyama, Yutaka; Nagai, Yasuyoshi*

Journal of Nuclear Materials, 543, p.152564_1 - 152564_10, 2021/01

 Times Cited Count:12 Percentile:90.3(Materials Science, Multidisciplinary)

Reactor pressure vessel (RPV) steels for pressurized water reactors (PWRs) with bulk P contents ranging from 0.007 to 0.012wt.% were subjected to neutron irradiation at fluences ranging from 0.3 to 1.2$$times$$10$$^{20}$$ n/cm$$^{2}$$ (E $$>$$ 1 MeV) in PWRs or a materials testing reactor (MTR). Grain-boundary P segregation was analyzed using Auger electron spectroscopy (AES) on intergranular facets and found to increase with increasing neutron fluence. A rate theory model was also used to simulate the increase in grain-boundary P segregation for RPV steels with a bulk P content up to 0.020wt.%. The increase in grain-boundary P segregation in RPV steel with a bulk P content of 0.015wt.% (the maximum P concentration found in RPV steels used in Japanese nuclear power plants intended for restart) was estimated to be less than 0.1 in monolayer coverage at 1.0$$times$$10$$^{20}$$ n/cm$$^{2}$$ (E $$>$$ 1 MeV). A comparison of the PWR data with the MTR data showed that neutron flux had no effect upon grain-boundary P segregation. The effects of grain-boundary P segregation upon changes in irradiation hardening and ductile-brittle transition temperature (DBTT) shifts were also discussed. A linear relationship between irradiation hardening and the DBTT shift with a slope of 0.63 obtained for RPV steels with a bulk P content up to 0.026wt.%, which is higher than that of most U.S. A533B steels. It is concluded that the intergranular embrittlement is unlikely to occur for RPV steels irradiated in PWRs.

Journal Articles

Role of advection in atmospheric ammonia; A Case study at a Japanese lake basin influenced by agricultural ammonia sources

Kubota, Tomohiro; Kuroda, Hisao*; Watanabe, Mirai*; Takahashi, Akiko*; Nakazato, Ryoji*; Tarui, Mika*; Matsumoto, Shunichi*; Nakagawa, Keita*; Numata, Yasuko*; Ouchi, Takao*; et al.

Atmospheric Environment, 243, p.117856_1 - 117856_9, 2020/12

 Times Cited Count:3 Percentile:15.1(Environmental Sciences)

The dry and wet depositions of atmospheric ammonia (NH$$_{3}$$) is one of the important pathways of nitrogen loads to aquatic ecosystems. Crop and livestock agriculture, one of the largest emitters of NH$$_{3}$$ in Asian countries, are known to cause high spatial and seasonal variation of NH$$_{3}$$ and influence the surrounding lake basin areas via its dry and wet deposition. However, the spatial characteristics of the NH$$_{3}$$ concentration in basin scale are not completely understood for regulation in NH$$_{3}$$ emission. Here we aim to clarify dominant factors of spatial and seasonal variations of the NH$$_{3}$$ concentration in a eutrophic lake basin surrounded by agricultural areas in Japan. Passive sampling over various land use categories in the basin was conducted at 36 sites in total from October 2018 to January 2020. Interestingly, the observed NH$$_{3}$$ concentration near the livestock houses were higher in winter than summer, which was inconsistent with knowledge of seasonal changes of current NH$$_{3}$$ emission inventory based on temperature-driven volatilization process. Comparing monthly NH$$_{3}$$ concentrations with various meteorological factors, we suggested the importance of seasonal advection of NH$$_{3}$$ from high emission sources to which has been rarely paid attention by the previous past studies. As for this, should be considered for lake ecosystem management since deposition of NH$$_{3}$$ is known to be closely related to the ecological processes such as phytoplankton blooming.

Journal Articles

Fabrication of a novel magnetic topological heterostructure and temperature evolution of its massive Dirac cone

Hirahara, Toru*; Otrokov, M. M.*; Sasaki, Taisuke*; Sumida, Kazuki*; Tomohiro, Yuta*; Kusaka, Shotaro*; Okuyama, Yuma*; Ichinokura, Satoru*; Kobayashi, Masaki*; Takeda, Yukiharu; et al.

Nature Communications (Internet), 11, p.4821_1 - 4821_8, 2020/09

 Times Cited Count:42 Percentile:93.06(Multidisciplinary Sciences)

Journal Articles

How different is the core of $$^{25}$$F from $$^{24}$$O$$_{g.s.}$$ ?

Tang, T. L.*; Uesaka, Tomohiro*; Kawase, Shoichiro; Beaumel, D.*; Dozono, Masanori*; Fujii, Toshihiko*; Fukuda, Naoki*; Fukunaga, Taku*; Galindo-Uribarri, A.*; Hwang, S. H.*; et al.

Physical Review Letters, 124(21), p.212502_1 - 212502_6, 2020/05

 Times Cited Count:14 Percentile:73.46(Physics, Multidisciplinary)

The structure of a neutron-rich $$^{25}$$F nucleus is investigated by a quasifree ($$p,2p$$) knockout reaction. The sum of spectroscopic factors of $$pi 0d_{5/2}$$ orbital is found to be 1.0 $$pm$$ 0.3. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus, and the core consists of $$sim$$35% $$^{24}$$O$$_{rm g.s.}$$, and $$sim$$65% excited $$^{24}$$O. The result shows that the $$^{24}$$O core of $$^{25}$$F nucleus significantly differs from a free $$^{24}$$O nucleus. The result may infer that the addition of the $$0d_{5/2}$$ proton considerably changes the neutron structure in $$^{25}$$F from that in $$^{24}$$O, which could be a possible mechanism responsible for the oxygen dripline anomaly.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2018

Nakano, Masanao; Fujii, Tomoko; Nemoto, Masashi; Tobita, Keiji; Kono, Takahiko; Hosomi, Kenji; Nishimura, Shusaku; Matsubara, Natsumi; Maehara, Yushi; Narita, Ryosuke; et al.

JAEA-Review 2019-048, 165 Pages, 2020/03

JAEA-Review-2019-048.pdf:2.69MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2018 to March 2019. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.

144 (Records 1-20 displayed on this page)