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SrMnO
(R = Gd, Tb and Dy)Yoshii, Kenji; Hiramitsu, Yusuke*; Okajima, Yuka*; Yoneda, Yasuhiro; Nishihata, Yasuo; Mizuki, Junichiro; Nakamura, Akio; Shimojo, Yutaka; Ishii, Yoshinobu*; Morii, Yukio; et al.
Materials Research Bulletin, 45(11), p.1574 - 1580, 2010/10
Times Cited Count：12 Percentile：37.13(Materials Science, Multidisciplinary)Magnetic and dielectric properties of perovskite manganites RSrMnO (R = Gd, Tb and Dy) have been investigated. DC and AC magnetic measurements showed short-range glassy magnetic ordering at Tg about 40 K. Such ordering was observed by neutron diffraction and is ascribable to the size mismatch of R
and Sr settled randomly at the same crystallographic site. Dielectric constants for each material were about 1000-10000 between about 50 K and 300 K and showed broad maximums above Tg. Dielectric dispersion showed poor coherency of the motion of polar regions, plausibly because of the size-mismatch effect; both the magnetic and dielectric properties of this system are governed by the randomness at the R/Sr site. The tan
and EXAFS data suggest that the dielectric response is rooted in a transfer of the Mn-3d electrons.
CaMnO (R=Eu-Lu)Yoshii, Kenji; Hiramitsu, Yusuke*; Yoneda, Yasuhiro; Okajima, Yuka; Nishihata, Yasuo; Mizuki, Junichiro; Ikeda, Naoshi*
Ferroelectrics, 379(1), p.183 - 190, 2009/05
Times Cited Count：9 Percentile：39.74(Materials Science, Multidisciplinary)The magnetic and dielectric properties of perovskite manganites RCaMnO (R=Eu-Lu) have been investigated. Their dielectric constants were about 1000 at around room temperature. Inflections or peaks of temperature dependences of the dielectric constants were observed at around the charge-ordering temperatures determined from the magnetic measurements. Analyses of tan and EXAFS spectra suggested that the dielectric properties of this system are due to a spatial arrangement and transfer of the Mn-3d electrons. The observation of a two-peak structure of tan indicates that dielectric measurement can be used to observe homogeneity or in homogeneity of sample, as mentioned in our previous paper.
CaMnOHiramitsu, Yusuke*; Yoshii, Kenji; Yoneda, Yasuhiro; Mizuki, Junichiro; Nakamura, Akio; Shimojo, Yutaka; Ishii, Yoshinobu*; Morii, Yukio; Ikeda, Naoshi*
Japanese Journal of Applied Physics, Part 1, 46(10B), p.7171 - 7174, 2007/10
Times Cited Count：16 Percentile：53.11(Physics, Applied)Magnetic and dielectric properties of a perivskite manganite TbCaMnO were investigated. Magnetic measurements showed three characteristic temperatures, originating from charge ordering (300 K), antiferromagnetic ordering (120 K) and a transition to a glassy state (50 K). The coexistence of the charge and antiferromagnetic ordering was consistent with the result of powder neutron diffraction. AC dielectric measurements showed large dielectric constants of about 5000 at around room temperature. A temperature dependence of the dielectric constant changed just below the charge-ordering temperature. From the analysis of tan;, the activation energy for a domain-boundary motion was calculated to be about 0.09 eV. These results strongly suggest that the dielectric properties of this material are governed by the ordering and transfer of the Mn-3d charges.
CaMnO (R: rare earths)Yoshii, Kenji; Hiramitsu, Yusuke*; Okajima, Yuka; Yoneda, Yasuhiro; Nishihata, Yasuo; Mizuki, Junichiro; Ikeda, Naoshi*
no journal, ,
no abstracts in English
