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Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2023-027, 126 Pages, 2024/03
JAEA-Review-2023-027.pdf:5.51MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Study on rational treatment/disposal of contaminated concrete waste considering leaching alteration" conducted from FY2020 to FY2022. The present study aims to understand migration behaviors of radionuclides in relation to the properties of concrete altered by leaching, to develop migration model of radionuclides, and to evaluate waste management scenarios, focusing on underground concrete structures in contact with contaminated water.
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2022-050, 116 Pages, 2023/01
JAEA-Review-2022-050.pdf:11.41MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Safe, efficient cementation of challenging radioactive wastes using alkali activated materials with high-flowability and high-anion retention capacity" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. The present study aims to explore alkali activated materials with high anionic nuclide retention and flowability and their recipes for safe storage and disposal of iron flocculant from the water treatment facility at 1F, and to propose a design of a solidification device that is feasible as an actual plant. In order to achieve these objectives, the following five items were carried out in this study.
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2022-038, 102 Pages, 2023/01
JAEA-Review-2022-038.pdf:4.76MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Study on rational treatment/disposal of contaminated concrete waste considering leaching alteration" conducted in FY2021. The present study aims to understand migration behaviors of radionuclides in relation to the properties of concrete altered by leaching, to develop a model to predict concentration profiles, and to analyze waste management scenarios, with a focus on underground concrete structures in contact with contaminated water. Migration behaviors depend on radionuclides and their chemical species. Sorption of I
is less significant on C-S-H and C-A-S-H than on hardened cement paste with two orders of magnitude smaller distribution coefficient 
, while of U was the same …
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2021-070, 98 Pages, 2022/03
JAEA-Review-2021-070.pdf:4.75MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Study on rational treatment/disposal of contaminated concrete waste considering leaching alteration" conducted in FY2020. The present study aims to understand migration behaviors of radionuclides in relation to the properties of concrete materials altered due to leaching, to develop a model to simulate the migration behaviors based on the experimental findings, and to analyze waste management scenarios for radioactive concrete. The focus of the study is the underground concrete structures of Fukushima Daiichi Nuclear Power Station, which is in contact with contaminated water.
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2021-036, 95 Pages, 2021/12
JAEA-Review-2021-036.pdf:5.13MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Safe, efficient cementation of challenging radioactive wastes using alkali activated materials with high-flowability and high-anion retention capacity" conducted in FY2020. For safe storage and disposal of iron sludge generated from contaminated water treatment, the present study aims to 1) explore alkali activated materials (AAM) with high-flowability and high-anion retention capacity and its recipe, 2) try mock-up manufacture and evaluation for one-tenth the size of real waste and propose the concept of the manufacturing equipment for a real plant, 3) show potential of AAM as the material for the solidification of waste with various physicochemical properties and radioactive nuclide compositions from the result ...
Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*
JAEA-Review 2020-054, 72 Pages, 2021/01
JAEA-Review-2020-054.pdf:5.62MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Safe, efficient cementation of challenging radioactive wastes using alkali activated materials with high-flowability and high-anion retention capacity". The purpose of this study is to find safe, efficient cementation of challenging radioactive wastes using alkali activated materials with high-flowability and high-anion retention capacity, and to propose the concept of a manufacturing apparatus that is established as an actual plant. As a result of study in this year, it was revealed that the K-based alkali activated material has high-flowability and quick curing, and that high-iodine retention capacity is achieved by incorporating silver ions during manufacturing of solidified waste.
Hokkaido University*
JNC TJ8400 99-033, 44 Pages, 1999/02
As a basic research for geological disposal of high-level radioactive wastes, long-term durability of clay buffer materials was studied from the viewpoint of performance of clay as barrier, which would be changed when exchangeable cations (Na
ions) of Na-montmorillonite were replaced with Ca
ions. The apparent diffusion coefficients of Cs ions were determined as functions of the diffusion temperature and the ionic equivalent fraction of Ca ions. The apparent diffusion coefficients were almost constant at higher temperatures, 323 and 313 K, while they decreased with increasing ionic equivalent fraction at lower temperatures, 298 and 288 K. The activation energy increased from 34 kJ mol
to 38 kJ mol as the ionic equivalent fraction increased from zero to 0.75, after which it increased steeply and reached 49 kJ mol at the ionic equivalent fractions of 0.94 and 1.0. These findings cannot be explained by the pore water or surface diffusion model. Interlayer diffusion is suggested as the most probable explanation for the diffusion of Cs ions. Corrosion experiments were carried out using neutron-activated iron foils and bentonite specimens with different drying periods to evaluate the effects of oxidation of pyrite on the corrosion rates of iron and the apparent diffusion coefficients of the corrosion products in bentonite. There was a decrease in the quantity of pyrite in the bentonite during drying, together with a decrease in pH, and an increase in SO
concentration in bentonite-water suspension. These results indicate that the oxidation of pyrite proceeded gradually during the drying process. It was found that the average corrosion rate of iron and the apparent diffusion coefficients of iron corrosion products in the compacted bentonite increased with the drying period. It is likely that the decrease of pH caused by the oxidation of pyrite affects the corrosion rates and the apparent diffusion coefficient.