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He, X.*; Kagi, Hiroyuki*; Komatsu, Kazuki*; Iizuka, Riko*; Okajima, Hajime*; Hattori, Takanori; Sano, Asami; Machida, Shinichi*; Abe, Jun*; Goto, Hirotada*; et al.
Journal of Molecular Structure, 1310, p.138271_1 - 138271_8, 2024/08
High-pressure responses of the O-DF hydrogen bonds in deuterated magnesium hydroxyfluoride were investigated using neutron powder diffraction and Raman spectroscopy. The Rietveld analysis at ambient conditions revealed a chemical formula of Mg(OD)F and hydroxyl group/fluorine disorder (OD/F disorder) in the crystal structure, which gave rise to two hydrogen-bonding configurations. The Rietveld analysis showed the hydrogen-bonding geometries remains up to 9.8 GPa, indicating no pressure-induced strengthening of hydrogen bonds. The Raman spectra at ambient conditions showed three hydroxyl stretching bands at 2613, 2694, and 2718 cm. The high frequencies of the O-D stretching modes indicated that the hydroxyls should be involved in weak or none hydrogen-bonding interactions. Up to 20.2 GPa, the mode initially centered at 2694 cm displayed a pressure-induced blue shift, revealing no strengthening of hydrogen bonds under compression. We discuss the existence of hydrogen bonds and the causes of the blue-shifting hydroxyls at ambient and at high pressures.
Nakano, Hiroko; Fujinami, Kyoko; Yamaura, Takayuki; Kawakami, Jun; Hanakawa, Hiroki
JAEA-Review 2023-036, 33 Pages, 2024/03
A practical training course using the JMTR (Japan Materials Testing Reactor) and other research infrastructures was held from November 29 to December 2 in 2021 for Asian young researchers and engineers. This course was adopted as International Youth Exchange Program in Science (SAKURA SCIENCE Exchange Program) which is the project of the Japan Science and Technology Agency, and this course aims to enlarge the number of high-level nuclear researchers/engineers in Asian countries which are planning to introduce a nuclear power plant, and to promote the use of facilities in future. In this year, from the viewpoint of preventing the spread of COVID-19 infection, it was decided to hold the event online. 53 young researchers and engineers joined the course from 6 countries. In FY2022, training programs with invitations were held due to the easing of restrictions on entry into Japan from overseas. 7 young researchers and engineers from4 Asian countries participated in the training from February 1 to 10, 2023.The common curriculum in the training course of FY2021 and FY2022 included lectures on nuclear energy, irradiation testing, safety management, JMTR decommissioning plan, etc. In the online session, conducted in FY2021, information exchange on the energy situation in each country was conducted. On-site training conducted in FY2022, included practical training on operation using simulations, environmental monitoring, etc. and facility tours of the JMTR, etc. Many participants could join the online training course, they created a diversity of expertise and made lively discussions during the information exchange. On-site training, while limited in number of participants, provided a good opportunity for personnel exchange through practical training and face-face communication. It is desirable to hold on-site training as long as circumstances permit. This report summarizes the training conducted in FY2021 and FY2022.
Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.
Nature, 620(7976), p.965 - 970, 2023/08
Times Cited Count:5 Percentile:92.64(Multidisciplinary Sciences)no abstracts in English
Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.
Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08
Times Cited Count:2 Percentile:68.16(Astronomy & Astrophysics)Detailed -ray spectroscopy of the exotic neon isotope Ne has been performed using the one-neutron removal reaction from Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.
Kamiya, Junichiro; Takano, Kazuhiro*; Wada, Kaoru; Yanagibashi, Toru*
e-Journal of Surface Science and Nanotechnology (Internet), 21(3), p.144 - 153, 2023/06
no abstracts in English
Katabuchi, Tatsuya*; Iwamoto, Osamu; Hori, Junichi*; Kimura, Atsushi; Iwamoto, Nobuyuki; Nakamura, Shoji; Rovira Leveroni, G.; Endo, Shunsuke; Shibahara, Yuji*; Terada, Kazushi*; et al.
EPJ Web of Conferences, 281, p.00014_1 - 00014_4, 2023/03
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Meigo, Shinichiro; Jameson, R. A.*
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.499 - 502, 2023/01
The Japan Atomic Energy Agency (JAEA) is designing a 30-MW proton linear accelerator (linac) for the accelerator-driven subcritical system (ADS). The Radio Frequency Quadrupole (RFQ) is an essential component for the performance of high-intensity linac, especially in ADS, where stringent reliability is demanded. The present RFQ will capture a 20 mA proton beam and accelerate from the energy of 35 keV to 2.5 MeV, where the space-charge effects are severe. The present RFQ's design employs the equipartitioning (EP) beam scheme to control the emittance growth and compactness. As a result, the beam halo formation was minimized and allowed to optimize the superconducting linac downstream part. A remarkable feature of this RFQ is the low Kilpatrick factor of 1.2 adopted to achieve high stability by reducing the probability of surface sparking on the vane. This work presents and discusses the results of this RFQ design.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Meigo, Shinichiro
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.179 - 183, 2023/01
The Japan Atomic Energy Agency accelerator-driven subcritical system (JAEA-ADS) pursues the reduction of nuclear waste by transmuting minor actinides. JAEA-ADS project drives a 30-MW proton beam to a lead-bismuth eutectic (LBE) spallation target to produce neutrons for a subcritical core reactor. To this end, the JAEA-ADS beam transport (BT) must provide a suitable beam profile and stable beam power to the beam window of the spallation target to avoid high-thermal stress in the components, such as the beam window. The beam transport was optimized by tracking a large number of macroparticles to mitigate the beam loss, performance with high stability in the presence of errors, and fulfill the length requirement on the transport. This work presents beam transport design and beam dynamics research for the JAEA-ADS project.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Meigo, Shinichiro
Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.286 - 290, 2023/01
Japan Atomic Energy Agency (JAEA) is designing a 30-MW proton linear accelerator (linac) as one of the fundamental components for its accelerator-driven subcritical system (ADS) project. ADS accelerators demand extremely high reliability and availability to avoid thermal stress in the subcritical reactor structures. Thus, reliability and availability assessments of the accelerator are mandatory to detect weakness in the lattice designed and evaluate redundancy configurations to fulfill the demanded operation. This study applied the Reliability Block Diagrams (RBD) method to calculate the Medium Time Between Failures (MTBF) for different linac configurations: all the linac's elements in a series configuration and a combination of hot-standby for the low-energy section of the linac and k-out-n redundancy for the high-energy part. The estimation considered the detailed arrangement of the cavities and magnets that compose the linac lattice. In this report, we describe the reliability model of the JAEA-ADS linac, report the MTBF results, and point out the potential route toward operating with the required availability.
Yee-Rendon, B.; Meigo, Shinichiro; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Iwamoto, Hiroki; Sugawara, Takanori; Nishihara, Kenji
Journal of Instrumentation (Internet), 17(10), p.P10005_1 - P10005_21, 2022/10
Times Cited Count:0 Percentile:0(Instruments & Instrumentation)To reduce the hazard of minor actinides in nuclear waste, JAEA proposed an accelerator-driven subcritical system (JAEA-ADS). The JAEA-ADS drives a subcritical reactor 800-MWth by 30-MW proton linac delivering the beam to the spallation neutron target inside the reactor. The beam transport to the target (BTT) is required for high-beam power stability and low peak density to ensure the integrity of the beam window. Additionally, the design should have compatible with the reactor design for the maintenance and replacement of the fuel and the beam window. A robust-compact BTT design was developed through massive multiparticle simulations. The beam optics was optimized to guarantee beam window feasibility requirements by providing a low peak density of less than 0.3 A/mm. Beam stability was evaluated and improved by simultaneously applying the linac's input beam and element errors. The input beam errors to the reactor were based on the beam degradation obtained by implementing fast fault compensation in the linac. Those results show that the BTT fulfills the requirements for JAEA-ADS.
Watabe, Tadashi*; Liu, Y.*; Kaneda, Kazuko*; Sato, Tatsuhiko; Shirakami, Yoshifumi*; Oe, Kazuhiro*; Toyoshima, Atsushi*; Shimosegawa, Eku*; Wang, Y.*; Haba, Hiromitsu*; et al.
International Journal of Molecular Sciences (Internet), 23(16), p.9434_1 - 9434_11, 2022/08
Times Cited Count:7 Percentile:78.48(Biochemistry & Molecular Biology)In this study, we compare the therapeutic effect between [At]NaAt and [I]NaI. In vitro analysis of double-stranded DNA break (DSB) and colony formation assay were performed using K1-NIS cells. [At]NaAt induced higher numbers of DSBs and had a reduced colony formation than [I]NaI. In K1-NIS mice, dose-dependent therapeutic effects were observed in both [At]NaAt and [I]NaI. The superior therapeutic effect of [At]NaAt suggests the promising clinical applicability of targeted alpha therapy using [At]NaAt in patients with differentiated thyroid cancer refractory to standard [I]NaI treatment.
Yee-Rendon, B.; Kondo, Yasuhiro; Tamura, Jun; Nakano, Keita; Maekawa, Fujio; Meigo, Shinichiro
Physical Review Accelerators and Beams (Internet), 25(8), p.080101_1 - 080101_17, 2022/08
Times Cited Count:2 Percentile:52.69(Physics, Nuclear)High reliability and availability are primary goals for the operation of particle accelerators, especially for accelerator-driven subcritical systems (ADS). ADSs employ high-power beams for the transmutation of minor actinide; as a result, the amount and the radiotoxicity of the nuclear waste are considerably reduced. To this end, the Japan Atomic Energy Agency is designing a 30-MW continuous wave (cw) super-conducting proton linear accelerator (linac) that supplies neutrons to an 800-MW subcritical reactor by a spallation process. The major challenge for an ADS linac is the strict control of the beam trip duration and its frequency to avoid thermal stress in the subcritical reactor structures. The maximum allowed beam trips for failures longer than a few seconds are estimated to be far below the rate achieved in current accelerators. Thus, we implemented a combination of hot standby and local compensation that enables a fast beam recovery. This work comprehensively investigated the tolerance of our linac lattice for the local compensations for failures in superconducting cavities and magnets. This scheme includes simultaneous compensation of multiple cavities in independent and same cryomodules that significantly enhance the reliability of the linac. The returned schemes present acceptable beam performance to guarantee the integrity of the linac and the beam transport to the target; moreover, they satisfy the beam stability in the beam window. In addition, the readjusted elements are subjected to moderate stress to ensure a sustainable operation. This manuscript reports the beam dynamics results toward fulfilling the high reliability demanded by an ADS linac.
Fujita, Yoshitaka; Seki, Misaki; Ngo, M. C.*; Do, T. M. D.*; Hu, X.*; Yang, Y.*; Takeuchi, Tomoaki; Nakano, Hiroko; Fujihara, Yasuyuki*; Yoshinaga, Hisao*; et al.
KURNS Progress Report 2021, P. 118, 2022/07
no abstracts in English
Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.
Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07
This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.
Rovira Leveroni, G.; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Iwamoto, Osamu; Iwamoto, Nobuyuki; Katabuchi, Tatsuya*; Kodama, Yu*; Nakano, Hideto*; Sato, Yaoki*; et al.
Journal of Nuclear Science and Technology, 59(5), p.647 - 655, 2022/05
Times Cited Count:1 Percentile:16.35(Nuclear Science & Technology)Kamiya, Junichiro; Takano, Kazuhiro*; Yuza, Hiromu*; Wada, Kaoru
e-Journal of Surface Science and Nanotechnology (Internet), 20(2), p.107 - 118, 2022/05
no abstracts in English
Rovira Leveroni, G.; Iwamoto, Osamu; Kimura, Atsushi; Nakamura, Shoji; Iwamoto, Nobuyuki; Endo, Shunsuke; Katabuchi, Tatsuya*; Terada, Kazushi*; Kodama, Yu*; Nakano, Hideto*; et al.
JAEA-Conf 2021-001, p.156 - 161, 2022/03
Murase, Satoshi*; Yoshikawa, Yumi*; Fujiwara, Kosuke*; Fukada, Yukimasa*; Teranishi, Takashi*; Kano, Jun*; Fujii, Tatsuo*; Inada, Yasuhiro*; Katayama, Misaki*; Yoshii, Kenji; et al.
Journal of Physics and Chemistry of Solids, 162, p.110468_1 - 110468_6, 2022/03
Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)We report a trial of the valence control for mixed valence iron triangular oxide YbFeO in order to develop an effective technique to control the frustration of charges in strongly correlated electron systems. The electro-chemical doping of Li into YbFeO was examined on the cell type sample similar to the Li-ion secondary battery cell. Systematic change of the lattice constant, Fe-Fe and Fe-Yb distance were observed with Li doping. Maximum value of the doping was over 300 mAh/g. An EXAFS experiment indicated that Li positioned between Yb octahedron layer (U-layer) and Fe-bipyramidal layer (W-layer). However, detailed change of iron valence state of YbFeO was not clearly observed because of the superimpose of the signal from iron metal nano particles in XANES observation. The results indicate that the electrochemical method might be one of the potential technique to control the frustration of charges in YbFeO.
Nakada, Akira; Nakano, Masanao; Kanai, Katsuta; Seya, Natsumi; Nishimura, Shusaku; Nemoto, Masashi; Tobita, Keiji; Futagawa, Kazuo; Yamada, Ryohei; Uchiyama, Rei; et al.
JAEA-Review 2021-062, 163 Pages, 2022/02
Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2020 to March 2021. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Station of Tokyo Electric Power Co., Inc. (the trade name was changed to Tokyo Electric Power Company Holdings, Inc. on April 1, 2016) in March 2011. Appendices present comprehensive information, such as monitoring programs, monitoring methods, monitoring results and their trends, meteorological data and discharged radioactive wastes. In addition, the data which were influenced by the accidental release and exceeded the normal range of fluctuation in the monitoring, were evaluated.
Takano, Kazuhiro; Kotoku, Hirofumi*; Kobayashi, Fuminori*; Miyao, Tomoaki*; Moriya, Katsuhiro; Kamiya, Junichiro
JAEA-Technology 2021-017, 35 Pages, 2021/11
In J-PARC LINAC, the vacuum system of L3BT, which is a beam transport line connecting LINAC and 3GeV synchrotron, uses a turbo molecular pump and roots pump for rough exhaust and an ion pump for main exhaust. In addition, beam dumps are connected to the end of the L3BT at 0 degree, 30 degree, 90 degree, and 100 degree positions via vacuum partition windows. The roots pumps are used as the exhaust system for each beam dump. The roots pump controllers have been installed away from the pump in the accelerator tunnel to avoid radiation damages. Besides, the special controllers, which have no inverter circuit inside, have been used to reduce the electrical noise on the beam loss monitors nearby. However, using the special controller without inverters, several problems have occurred such as the instability or wide variability of the pumping speed. To solve such problems, the roots pump controller with the inverter circuit must be used after reducing the electrical noise. In this report, some countermeasures to reduce the electrical noise from the inverters were investigated. The noise reduction circuit was successfully optimized to the level where the beam loss monitors works unaffected.