Magnetic excitation in the =1/2 Ising-like antiferromagnetic chain CsCoCl in longitudinal magnetic fields studied by high-field ESR measurements

Kimura, Shojiro*; Onishi, Hiroaki; Okunishi, Koichi*; Akaki, Mitsuru*; Narumi, Yasuo*; Hagiwara, Masayuki*; Kindo, Koichi*; Kikuchi, Hikomitsu*

Journal of the Physical Society of Japan, 92(9), p.094701_1 - 094701_9, 2023/09

https://doi.org/10.7566/JPSJ.92.094701

Investigation of the electronic structure of the MgZnY alloy using X-ray photoelectron spectroscopy

Miyazaki, Hidetoshi*; Akatsuka, Tatsuyoshi*; Kimura, Koji*; Egusa, Daisuke*; Sato, Yohei*; Itakura, Mitsuhiro; Takagi, Yasumasa*; Yasui, Akira*; Ozawa, Kenichi*; Mase, Kazuhiko*; et al.

Materials Transactions, 64(6), p.1194 - 1198, 2023/06

https://doi.org/10.2320/matertrans.MT-MD2022019

We investigated the electronic structure of the MgZnY alloy using hard and soft X-ray photoemission spectroscopy and electronic band structure calculations to understand the mechanism of the phase stability of this material. Electronic structure of the MgZnY alloy showed a semi-metallic electronic structure with a pseudo-gap at the Fermi level. The observed electronic structure of the MgZnY alloy suggests that the presence of a pseudogap structure is responsible for phase stability.

Spin excitations of the =1/2 one-dimensional Ising-like antiferromagnet BaCoVO in transverse magnetic fields

Okutani, Akira*; Onishi, Hiroaki; Kimura, Shojiro*; Takeuchi, Tetsuya*; Kida, Takanori*; Mori, Michiyasu; Miyake, Atsushi*; Tokunaga, Masashi*; Kindo, Koichi*; Hagiwara, Masayuki*

Journal of the Physical Society of Japan, 90(4), p.044704_1 - 044704_9, 2021/04

https://doi.org/10.7566/JPSJ.90.044704

Measurement of the angular distribution of -rays after neutron capture by La for a T-violation search

Okudaira, Takuya; Shimizu, Hirohiko*; Kitaguchi, Masaaki*; Hirota, Katsuya*; Haddock, C. C.*; Ito, Ikuya*; Yamamoto, Tomoki*; Endo, Shunsuke*; Ishizaki, Kohei*; Sato, Takumi*; et al.

EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12

https://doi.org/10.1051/epjconf/201921909001

Parity violating effects enhanced by up to 10 times have been observed in several neutron induced compound nuclei. There is a theoretical prediction that time reversal (T) violating effects can also be enhanced in these nuclei implying that T-violation can be searched for by making very sensitive measurements. However, the enhancement factor has not yet been measured in all nuclei. The angular distribution of the (n,) reaction was measured with La by using a germanium detector assembly at J-PARC, and the enhancement factor was obtained. From the result, the measurement time to achieve the most sensitive T-violation search was estimated as 1.4 days, and a 40% polarized La target and a 70% polarized He spin filter whose thickness is 70 atmcm are needed. Therefore high quality He spin filter is developed in JAEA. The measurement result of the (n,) reaction at J-PARC and the development status of the He spin filter will be presented.

Measurements of gamma-ray emission probabilities in the decay of americium-244g

Nakamura, Shoji; Terada, Kazushi*; Kimura, Atsushi; Nakao, Taro*; Iwamoto, Osamu; Harada, Hideo; Uehara, Akihiro*; Takamiya, Koichi*; Fujii, Toshiyuki*

Journal of Nuclear Science and Technology, 56(1), p.123 - 129, 2019/01

https://doi.org/10.1080/00223131.2018.1539353

Accurate data of -ray emission probabilities are frequently needed when one quantitatively determines the amount of isotope by -ray measurements or obtains neutron capture cross-sections using them. Americium-243, one of the most important minor actinides, produces Am after neutron capture. The 744-keV -ray decaying from the ground state of Am has a relatively large -ray emission probability c.a. 66%, however, its uncertainty is as large as 29%. The uncertainty of the -ray emission probability leads to a major factor of the systematic uncertainty on determining an amount of isotope, and therefore the -ray emission probability was measured by using an activation method and an examined level structure of Cm. In this study, the emission probability of 744-keV ray was derived as 66.51.1%, and its uncertainty was improved from 29% to 2%.

Measurements of neutron total and capture cross sections of Am with ANNRI at J-PARC

Terada, Kazushi*; Kimura, Atsushi; Nakao, Taro*; Nakamura, Shoji; Mizuyama, Kazuhito*; Iwamoto, Nobuyuki; Iwamoto, Osamu; Harada, Hideo; Katabuchi, Tatsuya*; Igashira, Masayuki*; et al.

Journal of Nuclear Science and Technology, 55(10), p.1198 - 1211, 2018/10

AA2017-0628.pdf:2.06MB

https://doi.org/10.1080/00223131.2018.1485519

Application of modified REFIT code for J-PARC/MLF to evaluation of neutron capture cross section on Gd

Mizuyama, Kazuhito; Iwamoto, Nobuyuki; Iwamoto, Osamu; Hasemi, Hiroyuki*; Kino, Koichi*; Kimura, Atsushi; Kiyanagi, Yoshiaki*

EPJ Web of Conferences, 146, p.11042_1 - 11042_4, 2017/09

https://doi.org/10.1051/epjconf/201714611042

Gadolinium has been used as neutron-absorbing material in a thermal reactor since have large thermal neutron capture cross sections. Nevertheless, there is a discrepancy between RPI data and JENDL-4.0 data for Gd. The criticality in the reactor is very sensitive to the capture cross section. The RPI data made the criticality of Gd-loaded thermal systems in ICSBEP overestimated. Recently, the neutron capture cross sections of Gd were measured by the neutron time-of-flight (TOF) method using the Accurate Neutron-Nucleus Reaction measurement Instrument (ANNRI) in the J-PARC/MLF. The pulsed neutron beam from the Japan Spallation Neutron Source (JSNS) was used with a double-bunch structure in this measurement, since the incident proton beam is normally delivered in a double-bunch scheme in the J-PARC. In addition to this, it is necessary to take into account the energy resolution of the pulsed neutron beam at the JSNS for the accurate derivation of resolved resonance parameters. In this study, using the least-squares multilevel R-matrix code REFIT modified to include the double bunch structure and the resolution function for the ANNRI, we fitted the calculated capture cross sections of Gd to the experimental data at the ANNRI. We derived the resonance parameters for some low-lying resonances of the two Gd isotopes.

Magnetic structure and dispersion relation of the =1/2 quasi-one-dimensional Ising-like antiferromagnet BaCoVO in a transverse magnetic field

Matsuda, Masaaki*; Onishi, Hiroaki; Okutani, Akira*; Ma, J.*; Agrawal, H.*; Hong, T.*; Pajerowski, D. M.*; Copley, J. R. D.*; Okunishi, Koichi*; Mori, Michiyasu; et al.

Physical Review B, 96(2), p.024439_1 - 024439_8, 2017/07

https://doi.org/10.1103/PhysRevB.96.024439

Measurements of -ray emission probabilities of Am and Np

Terada, Kazushi; Nakamura, Shoji; Nakao, Taro; Kimura, Atsushi; Iwamoto, Osamu; Harada, Hideo; Takamiya, Koichi*; Hori, Junichi*

Journal of Nuclear Science and Technology, 53(11), p.1881 - 1888, 2016/11

https://doi.org/10.1080/00223131.2016.1174167

-ray emission probabilities of Am and Np have been precisely measured with - and -ray spectroscopic methods. The activities of Am samples were determined by measuring alpha particles using a Si semiconductor detector. -rays emitted from the samples were measured with a planar type High-Purity Germanium (HPGe) detector. An efficiency curve of the Ge detector was derived with uncertainties of 0.7% from 50 to 1332 keV and 1.3% below 50 keV by combining measured efficiencies and Monte Carlo simulation. The -ray emission probabilities for the major -rays of these nuclides were determined with uncertainties less than 1.2%.

Search for neutron resonances of Pd

Nakamura, Shoji; Kimura, Atsushi; Toh, Yosuke; Harada, Hideo; Katabuchi, Tatsuya*; Mizumoto, Motoharu*; Igashira, Masayuki*; Hori, Junichi*; Kino, Koichi*

JAEA-Conf 2015-003, p.113 - 118, 2016/03

https://doi.org/10.11484/jaea-conf-2015-003

Experiments were carried out with the Ge detector of ANNRI to confirm whether or not the weak resonances were surely due to Pd. The prompt rays due to capture reaction of Pd were clearly observed at the -ray energy at 115 kev and around 300 keV. When a TOF spectrum was extracted by gating at the prompt ray around 300 keV, the small resonance peaks were revealed at the neutron energy of 146 and 156 eV.