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Journal Articles

Effect of magnetism on lattice dynamics in SrFe$$_2$$As$$_2$$ using high-resolution inelastic X-ray scattering

Murai, Naoki*; Fukuda, Tatsuo; Kobayashi, Tatsuya*; Nakajima, Masamichi*; Uchiyama, Hiroshi*; Ishikawa, Daisuke*; Tsutsui, Satoshi*; Nakamura, Hiroki; Machida, Masahiko; Miyasaka, Shigeki*; et al.

Physical Review B, 93(2), p.020301_1 - 020301_5, 2016/01

 Times Cited Count:7 Percentile:34.12(Materials Science, Multidisciplinary)

JAEA Reports

Research on engineering technology in the full-scale demonstration of EBS and operation technology for HLW disposal; Research report in 2012 (Joint research)

Nakatsuka, Noboru; Sato, Haruo; Tanai, Kenji; Nakayama, Masashi; Sawada, Sumiyuki*; Asano, Hidekazu*; Saito, Masahiko*; Yoshino, Osamu*; Tsukahara, Shigeki*; Hishioka, Sosuke*; et al.

JAEA-Research 2013-034, 70 Pages, 2014/01

JAEA-Research-2013-034.pdf:9.11MB

Japan Atomic Energy Agency (JAEA) and Radioactive Waste Management Funding and Research Center (RWMC) concluded the letter of cooperation agreement on the research and development of radioactive waste disposal in April, 2005, and have been carrying out the collaboration work based on the agreement. JAEA have been carrying out the Horonobe Underground Research Laboratory (URL) Project which is intended for a sedimentary rock in the Horonobe town, Hokkaido, since 2001. In the project, geoscientific research and research and development on geological disposal technology are being promoted. Meanwhile, the government (the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry) has been promoting construction of equipments for the full-scale demonstration of engineered barrier system and operation technology for high-level radioactive waste (HLW) disposal since 2008, to enhance public's understanding to the geological disposal of HLW, e.g. using underground facility. RWMC received an order of the project in fiscal year 2012 (2011/2012) continuing since fiscal year 2008 (2008/2009). Since topics in this project are included in the Horonobe URL Project, JAEA carried out this project as collaboration work continuing in fiscal year 2008. This report summarizes the results of engineering technology carried out in this collaboration work in fiscal year 2012. In fiscal year 2012, part of the equipments for emplacement of buffer material was produced and visualization test for water penetration in buffer material were carried out.

Journal Articles

${it Arabidopsis sos1}$ mutant in a salt-tolerant accession revealed an importance of salt acclimation ability in plant salt tolerance

Ariga, Hirotake*; Katori, Taku*; Yoshihara, Ryohei*; Hase, Yoshihiro; Nozawa, Shigeki; Narumi, Issei; Iuchi, Satoshi*; Kobayashi, Masatomo*; Tezuka, Kenji*; Sakata, Yoichi*; et al.

Plant Signaling & Behavior (Internet), 8(7), p.e24779_1 - e24779_5, 2013/07

Based on analysis of the salinity tolerance among 354 ${it Arabidopsis thaliana}$ accessions, some accessions showed greater salt shock tolerance compared with a reference accession, Col-0 on a typical assay with drastic change in NaCl concentration from 0 mM to 225 mM. On the other hand, several accessions including Zu-0 exhibited marked acquired salt tolerance, which is induced after exposure to moderate salt stress (salt acclimation ability). It is likely that Arabidopsis plants have at least two types of tolerance abilities, salt shock tolerance and salt acclimation. To dissect the salt tolerance mechanisms of the salt tolerant accessions, we isolated a salt-sensitive mutant from ion beam-mutagenized Zu-0 seedlings. The mutant showed severe growth inhibition under salt shock stress due to a single base deletion in SOS1 gene as well-known salt shock tolerance gene, even more salt sensitive than Col-0. Nevertheless, the mutant was able to survive on the salt acclimation with 100 mM NaCl for 7 days followed with 750 mM sorbitol for 20 days (salt acclimation assay) as well as the Zu-0 wild type, whereas Col-0 showed apparent chlorosis under the condition. We propose that a gene for salt acclimation ability is different from a gene for salt shock tolerance and plays an important role in acquisition for marked salt- or osmotic tolerance.

Journal Articles

Probing carbon edge exposure of iron phthalocyanine-based oxygen reduction catalysts by soft X-ray absorption spectroscopy

Niwa, Hideharu*; Saito, Makoto*; Kobayashi, Masaki*; Harada, Yoshihisa*; Oshima, Masaharu*; Moriya, Shogo*; Matsubayashi, Katsuyuki*; Nabae, Yuta*; Kuroki, Shigeki*; Ikeda, Takashi; et al.

Journal of Power Sources, 223, p.30 - 35, 2013/02

 Times Cited Count:18 Percentile:50.94(Chemistry, Physical)

To design non-platinum, inexpensive, but high performance carbon-based cathode catalysts for polymer electrolyte fuel cells, it is important to elucidate the active site for oxygen reduction reaction (ORR). However, it is difficult to directly identify the active site by applying conventional structural or electronic probes to such complex systems. Here, we used C 1${it s}$ X-ray absorption spectroscopy (XAS) to observe electronic structure of carbon in iron phthalocyanine-based catalysts, and found a signature of edge exposure below the $$pi^{ast}$$ edge, whose intensity is well correlated with the ORR activity. These results demonstrate that C 1${it s}$ XAS can be used to characterize the ORR activity of carbon-based cathode catalysts in terms of the edge exposure.

Journal Articles

Study on the oxygen adsorption property of nitrogen-containing metal-free carbon-based cathode catalysts for oxygen reduction reaction

Kiuchi, Hisao*; Niwa, Hideharu*; Kobayashi, Masaki*; Harada, Yoshihisa*; Oshima, Masaharu*; Chokai, Masayuki*; Nabae, Yuta*; Kuroki, Shigeki*; Kakimoto, Masaaki*; Ikeda, Takashi; et al.

Electrochimica Acta, 82(1), p.291 - 295, 2012/10

 Times Cited Count:14 Percentile:34.42(Electrochemistry)

We study the characteristics of oxygen adsorption on metal-free carbon-based cathode catalysts derived from nitrogen-containing polyamide (PA) and nitrogen-free phenolic resin (PhRs). Electrochemical analysis and Raman spectroscopy showed higher 2-electron oxygen reduction reaction (ORR) activity and more defect sites in PA than PhRs. The increase in the amount of adsorbed oxygen in PA was also identified by oxygen adsorption isotherms. ${it In-situ}$ X-ray photoelectron spectroscopy reveals that graphite-like nitrogen contributes to oxygen adsorption and C=O components are dominant in PA. These experimental results indicate that the adsorbed C=O components near the graphite-like nitrogen can be assigned as active sites for 2-electron ORR.

Journal Articles

Numerical experiments on dispersion of radionuclides in the ocean released from the Fukushima Daiichi Nuclear Power Plant

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; In, Teiji*; Ishikawa, Yoichi*; Nakayama, Tomoharu*; Shima, Shigeki*; Awaji, Toshiyuki*

Reports of Research Institute for Applied Mechanics, Kyushu University, (143), p.111 - 117, 2012/09

Because of the Fukushima Dai-ichi Nuclear Power Plant disaster, some radionuclides were released into the ocean from the Fukushima Dai-ichi Nuclear Power Plant. In response to this situation, numerical experiments were carried out at Japan Atomic Energy Agency using an oceanic dispersion model and an ocean general circulation model to estimate an effect of the radionuclides on marine environment. It was suggested that the radionuclides deposited from the atmosphere mainly in the middle of March after the disaster spread over a comparatively wide area of the Pacific Ocean east of Japan. On the other hand the radionuclides directly released into the ocean from the Fukushima Dai-ichi Nuclear Power Plant were carried along the coast and then spread along the Kuroshio extension.

Journal Articles

Preliminary numerical experiments on Oceanic dispersion of $$^{131}$$I and $$^{137}$$Cs discharged into the ocean because of the Fukushima Daiichi Nuclear Power Plant disaster

Kawamura, Hideyuki; Kobayashi, Takuya; Furuno, Akiko; In, Teiji*; Ishikawa, Yoichi*; Nakayama, Tomoharu*; Shima, Shigeki*; Awaji, Toshiyuki*

Journal of Nuclear Science and Technology, 48(11), p.1349 - 1356, 2011/11

AA2011-0314.pdf:0.68MB

 Times Cited Count:180 Percentile:99.79(Nuclear Science & Technology)

Numerical experiments were carried out to predict the spreading of $$^{131}$$I and $$^{137}$$Cs released into the ocean due to the Fukushima Daiichi Nuclear Power Plant incident. Results in the numerical experiments were in good agreement with the concentrations of $$^{131}$$I and $$^{137}$$Cs in the monitoring data. It was suggested that the high $$^{131}$$I concentration detected in the young lancefish caught off Kitaibaraki city was due to the deposition from the atmosphere. The numerical experiments suggest that the deposition of radionuclides released into the atmosphere in the middle March largely effected the concentrations of radionuclides east of Japan in the Pacific Ocean.

Journal Articles

A Study of released radionuclide in the coastal area from a discharge pipe of nuclear fuel reprocessing plant in Rokkasho, Aomori, Japan

Kobayashi, Takuya; In, Teiji*; Ishikawa, Yoichi*; Kawamura, Hideyuki; Nakayama, Tomoharu*; Shima, Shigeki*; Awaji, Toshiyuki*; Togawa, Orihiko

Progress in Nuclear Science and Technology (Internet), 2, p.682 - 687, 2011/10

When the reprocessing plant is in routine operation, radionuclides are released to the coastal ocean as scheduled. Released radionuclides migrate in the ocean by physical, chemical and biological processes. Thus, for environmental safety, it is important to understand the migration behavior due to routine releases of radionuclides to the coastal ocean from the reprocessing plant. A numerical simulation model system that consists of an ocean general circulation model and a particle random-walk model to describe the radionuclide migration behavior in Rokkasho coastal region has been developed. The particle random-walk model, SEA-GEARN, calculates the radionuclides migration in the ocean. The system has been applied to simulate the nowcast of Rokkasho coastal region in 2007 and hypothetical radionuclide release has been carried out.

Journal Articles

Effect of ion beam irradiation for ${it Asclepias}$ species

Kobayashi, Nobuo*; Sasaki, Shinichiro*; Tasaki, Keisuke*; Nakatsuka, Akira*; Nozawa, Shigeki; Hase, Yoshihiro; Narumi, Issei

JAEA-Review 2010-065, JAEA Takasaki Annual Report 2009, P. 67, 2011/01

Journal Articles

Recent progress in the energy recovery linac project in Japan

Sakanaka, Shogo*; Akemoto, Mitsuo*; Aoto, Tomohiro*; Arakawa, Dai*; Asaoka, Seiji*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; et al.

Proceedings of 1st International Particle Accelerator Conference (IPAC '10) (Internet), p.2338 - 2340, 2010/05

Future synchrotron light source using a 5-GeV energy recovery linac (ERL) is under proposal by our Japanese collaboration team, and we are conducting R&D efforts for that. We are developing high-brightness DC photocathode guns, two types of cryomodules for both injector and main superconducting (SC) linacs, and 1.3 GHz high CW-power RF sources. We are also constructing the Compact ERL (cERL) for demonstrating the recirculation of low-emittance, high-current beams using above-mentioned critical technologies.

JAEA Reports

Improvement of the marine radionuclides prediction code in the off Shimokita Region

Kobayashi, Takuya; Togawa, Orihiko; Ito, Toshimichi; Otosaka, Shigeyoshi; Kawamura, Hideyuki; Hayashi, Keisuke*; Shima, Shigeki*; Nakayama, Tomoharu*; In, Teiji*

JAEA-Research 2009-040, 63 Pages, 2009/12

JAEA-Research-2009-040.pdf:12.19MB

A spent nuclear fuel reprocessing plant has the possibility of routine releases of liquid radioactive wastes from a discharge pipe to the off Shimokita region during its operations. Thus, for environmental safety, it is important to assess the migration processes of released radionuclides from the plant. Therefore, an ocean circulation prediction code and an oceanic radionuclides migration prediction code, which were developed by Japan Atomic Energy Agency, has been improved to describe the migration behavior of radionuclides in the off Shimokita region. Parameters on characteristics and dynamics of particulate materials in seawater have also been obtained in the study area for the adjustment and verification of the oceanic radionuclides migration prediction code. This report summarizes the primary results of the study which was carried out at the off Shimokita region from FY2003 to 2008.

Journal Articles

Mutation induction in ${it Asclepias}$ using ion beam irradiation

Kobayashi, Nobuo*; Kano, Sayaka*; Sasaki, Shinichiro*; Tasaki, Keisuke*; Nakatsuka, Akira*; Nozawa, Shigeki; Hase, Yoshihiro; Narumi, Issei

JAEA-Review 2009-041, JAEA Takasaki Annual Report 2008, P. 77, 2009/12

Journal Articles

Halo structure of the island of inversion nucleus $$^{31}$$Ne

Nakamura, Takashi*; Kobayashi, Nobuyuki*; Kondo, Yosuke*; Sato, Yoshiteru*; Aoi, Nori*; Baba, Hidetada*; Deguchi, Shigeki*; Fukuda, Naoki*; Gibelin, J.*; Inabe, Naoto*; et al.

Physical Review Letters, 103(26), p.262501_1 - 262501_4, 2009/12

 Times Cited Count:198 Percentile:97.53(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Development of a system for the prediction of radionuclide migration in the off Shimokita region and its case study

Kobayashi, Takuya; In, Teiji*; Ishikawa, Yoichi*; Matsuura, Yasutaka*; Shima, Shigeki*; Nakayama, Tomoharu*; Awaji, Toshiyuki*; Kawamura, Hideyuki; Togawa, Orihiko

Nihon Genshiryoku Gakkai Wabun Rombunshi, 7(2), p.112 - 126, 2008/06

The radionuclides migration forecasting system in the off Shimokita region has been developed to predict the routine and accidental releases of liquid radioactive wastes during the operations of a spent nuclear fuel reprocessing plant in Aomori prefecture, Japan. The results obtained from the case studies are as follows; (1) The ocean general circulation model by using the techniques of data assimilation and nesting reproduced well the flow pattern of a coastal area. (2) The estimated internal dose due to ingestion of marine products from hypothetical release of $$^{3}$$H was 0.45 $$mu$$Sv/y. (3) The results of hypothetical release of $$^{137}$$Cs showed that about four percent of the whole deposited on the seabed after a 60-day calculation. The concentration of $$^{137}$$Cs of hypothetical release from the off Shimokita region is the same or less than that of global fallout measured at the same area.

Journal Articles

Progress in R&D efforts on the energy recovery linac in Japan

Sakanaka, Shogo*; Ago, Tomonori*; Enomoto, Atsushi*; Fukuda, Shigeki*; Furukawa, Kazuro*; Furuya, Takaaki*; Haga, Kaiichi*; Harada, Kentaro*; Hiramatsu, Shigenori*; Honda, Toru*; et al.

Proceedings of 11th European Particle Accelerator Conference (EPAC '08) (CD-ROM), p.205 - 207, 2008/06

Future synchrotron light sources based on the energy-recovery linacs (ERLs) are expected to be capable of producing super-brilliant and/or ultra-short pulses of synchrotron radiation. Our Japanese collaboration team is making efforts for realizing an ERL-based hard X-ray source. We report recent progress in our R&D efforts.

Journal Articles

The Oceanic forecasting system near the Shimokita Peninsula, Japan

In, Teiji*; Nakayama, Tomoharu*; Matsuura, Yasutaka*; Shima, Shigeki*; Ishikawa, Yoichi*; Awaji, Toshiyuki*; Kobayashi, Takuya; Kawamura, Hideyuki; Togawa, Orihiko; Toyoda, Takahiro*

Proceedings of International Symposium on Environmental Modeling and Radioecology, p.58 - 64, 2007/03

The northwestern part of the Pacific Ocean off the Shimokita Peninsula assumes a complex water mass structure. It is necessary to accurately reproduce the striking circulation patterns and the complicated water mass structures in this area with an ocean general circulation model. We have planned to make use of a one-way nesting method. To initialize the forecast system, we use a 4-dimensional variational method of data assimilation. The assimilated data consist of hydrographic observations collected through the Global Temperature-Salinity Profile Program, sea surface temperature and sea surface height data observed by satellites. A forecast experiment on the basis of oceanographic observations made in 2003 illustrates the good performance of our system. We shall focus, in particular, on the shift from the coastal mode to the gyre mode and vice versa.

Journal Articles

Status of 324 MHz RF test stand at the J-PARC linac

Yamazaki, Masayoshi; Chishiro, Etsuji; Kobayashi, Tetsuya; Hori, Toshihiko; Suzuki, Hiroyuki; Hasegawa, Kazuo; Anami, Shozo*; Kawamura, Masato*; Fukui, Yuji*; Nammo, Kesao*; et al.

Proceedings of 3rd Annual Meeting of Particle Accelerator Society of Japan and 31st Linear Accelerator Meeting in Japan (CD-ROM), p.391 - 393, 2006/00

no abstracts in English

Journal Articles

Development of the ocean forecasting system for Shimokita region

In, Teiji*; Shima, Shigeki*; Nakayama, Tomoharu*; Ishikawa, Yoichi*; Togawa, Orihiko; Kobayashi, Takuya; Kawamura, Hideyuki

Gekkan Kaiyo, 37(9), p.674 - 680, 2005/09

no abstracts in English

Journal Articles

Status of RF system for the J-PARC linac

Chishiro, Etsuji; Hori, Toshihiko*; Kobayashi, Tetsuya; Suzuki, Hiroyuki*; Suganuma, Kazuaki; Yamazaki, Masayoshi*; Anami, Shozo*; Fang, Z.*; Fukuda, Shigeki*; Fukui, Yuji*; et al.

Proceedings of 2nd Annual Meeting of Particle Accelerator Society of Japan and 30th Linear Accelerator Meeting in Japan, p.236 - 238, 2005/07

no abstracts in English

JAEA Reports

Development of the JNC Geological Disposal Technical Information Integration System Subjected for Repository Design and Safety Assessment -Document on Present State of Affairs-

Ishihara, Yoshinao*; Ito, Takashi*; Kobayashi, Shigeki*; Neyama, Atsushi*

JNC TJ8440 2004-005, 137 Pages, 2004/02

JNC-TJ8440-2004-005.pdf:2.42MB

On this work, system manufacture about disposal technology and safety assessment field was performed towards construction of the JNC Geological Disposal Technical Information Integration System which systematized three fields of technical information acquired in investigation (site characteristic investigation) of geology environmental conditions, disposal technology (design of deep repository), and performance/safety assessment.The technical information database managed focusing on the technical information concerning individual research of an examination, analysis, etc. and the parameter set database managed focusing on the set up data set used in case of comprehensive evaluation are examined.In order to support and promote share and use of the technical information registered and managed by the database, utility functions, such as a technical information registration function, technical information search / browse function, analysis support function, and visualization function, are considered, and the system realized in these functions is built.The built system is installed in the server of JNC, and the functional check examination is carried out.

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