Temperature dependence of positron annihilation lifetime in near-surface and bulk of room-temperature ionic liquid observed by a slow positron beam

Hirade, Tetsuya; Michishio, Koji*; Kobayashi, Yoshinori*; Oshima, Nagayasu*

Chemical Physics Letters, 795, p.139507_1 - 139507_4, 2022/05

https://doi.org/10.1016/j.cplett.2022.139507

We obtained the temperature dependence up to 150C of the triplet positronium (-Ps) lifetime in N,N,N-Trimethyl-N-propylammonium bis(trifluoromethanesulfonyl)imide (TMPA-TFSI) by the vertical slow positron beamline installed at AIST. Positrons penetrate into the liquid surface of TMPA-TFSI with the positron energies of 2 keV and 12 keV to investigate at the near-surface and the balk. The surface structure was visible at 150C, 120C above the melting temperature. The -Ps lifetime became shorter at higher temperatures for both positron energies. Similar temperature dependence had appeared just in water as the result of the reaction of -Ps and radiolysis products such as the OH radicals. The temperature dependence observed for TMPA-TFSI suggested that the chemical reaction of -Ps occurred.

Upgrade history and present status of the general control system for the Materials and Life Science Experimental Facility at J-PARC

Sakai, Kenji; Oi, Motoki; Haga, Katsuhiro; Kai, Tetsuya; Nakatani, Takeshi; Kobayashi, Yasuo*; Watanabe, Akihiko*

JPS Conference Proceedings (Internet), 33, p.011151_1 - 011151_6, 2021/03

https://doi.org/10.7566/JPSCP.33.011151

For safely and efficiently operating a spallation neutron source and a muon target, a general control system (GCS) operates within Materials and Life Science Experimental Facility (MLF), GCS administers operation processes and interlocks of many instruments for various operation statuses. It consists of several subsystems such as an integral control system (ICS), interlock systems (ILS), shared servers, network system, and timing distribution system (TDS). Although GCS is an independent system that controls the target stations, it works closely with the control systems of other facilities in J-PARC. Since the first beam injection in 2008, GCS has operated stably without any serious troubles after modification based on commissioning for operation and control. Then, significant improvements in GCS such as upgrade of ICS by changing its framework software and function enhancement of ILS were proceeded until 2015, in considering sustainable long-term operation and maintenance. In recent years, many instruments in GCS have replaced due to end of production and support of them. In this way, many modifications have been proceeded in the entire GCS after start of beam operation. Under these situation, it is important to comprehend upgrade history and present status of GCS in order to decide its upgrade plan for the coming ten years. This report will mention upgrade history, present status and future agenda of GCS.

Temperature dependence of ortho-positronium annihilation in room temperature ionic liquids

Hirade, Tetsuya; Michishio, Koji*; Kobayashi, Yoshinori*; Oshima, Nagayasu*

Acta Physica Polonica A, 137(2), p.109 - 112, 2020/02

https://doi.org/10.12693/APhysPolA.137.109

Recently, it was reported that the positronium (Ps) bubble in Room Temperature Ionic Liquids (RTILs) showed some phenomena that were very different from them observed in other molecular liquids. Now the reason of these interesting phenomena is being understood. The structure caused by the ionic interaction between anions and cations can exist even at the higher temperatures than the melting temperatures. It was the reason why the oscillation of Ps bubble was observed at the temperatures near the melting temperatures in RTILs. The temperature dependence of the Ps bubble size estimated by the triplet Ps (-Ps) pick-off annihilation lifetime indicated that there was a nano-meter structure remained by ionic interactions even at high temperatures. The -Ps pick-off annihilation lifetime will be a strong tool to study nano-structure in RTILs.

Applicability confirmation test of optimum decay heat evaluation method for HTGR with HTTR (Non-nuclear heating test); Validation of residual heat evaluation model

Honda, Yuki; Inaba, Yoshitomo; Nakagawa, Shigeaki; Yamazaki, Kazunori; Kobayashi, Shoichi; Aono, Tetsuya; Shibata, Taiju; Ishitsuka, Etsuo

JAEA-Technology 2017-013, 20 Pages, 2017/06

JAEA-Technology-2017-013.pdf:2.52MB

Decay heat is one of an important factor for a safety evaluation of depressurized loss-of-forced cooling accident, a representative high consequence accident, in high temperature gas-cooled reactor (HTGR). Traditionally, a conservative decay heat curve is used for safety analysis according to the regulatory standards. On the other hand, there is growing interest in obtaining test data related to decay heat for the use of uncertainty analysis. However, such data has not been obtained for prismatic-type HTGR. Therefore, we have launched a test program to obtain the decay heat data from the HTTR. As an initial step, an applicability confirmation test of decay heat evaluation method for HTGR was conducted in February 2017 without non-nuclear heating condition. This report introduces an estimation method for the decay heat based on test data using HTTR and shows the results of validation of the reactor residual heat evaluation method which will be used to obtain the decay heat data based on test data.

Study of beam loading compensation with comb-like structure at J-PARC linac

Futatsukawa, Kenta*; Kobayashi, Tetsuya*; Sato, Yoshikatsu; Shinozaki, Shinichi; Fang, Z.*; Fukui, Yuji*; Mizobata, Satoshi; Michizono, Shinichiro*

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.327 - 331, 2016/11

In the J-PARC linac, an intermediate-pulse with the comb-like structure is shaped by kicking an unwanted beam by the chopper cavity. Therefore, the cavities lying downstream of the RF-chopper have the beam loading with this beam shape. The present feedforward system which assumes the averaged beam current and not the comb-like beam was operated in the present LLRF, because the beam current in the linac was lower than the design value. However, it has been difficult that the required precision for the RF system is satisfied with increasing beam current. Thus, we performed the beam study of the beam loading compensation with the same shapes as the intermediate-pulses. The positive results for the cavities of SDTL and DTL with high Q values were obtained compared to the present system. On the other hand, when this compensation system was used in the case of ACS cavities, the neighbor modes were excited by the input RF. We have to improve the FF system for the operation against the real beam.

The Role of nitric oxide in radiation-induced bystander cell-killing effect

Yokota, Yuichiro; Funayama, Tomoo; Ikeda, Hiroko; Sakashita, Tetsuya; Suzuki, Michiyo; Kobayashi, Yasuhiko

JAEA-Review 2015-022, JAEA Takasaki Annual Report 2014, P. 67, 2016/02

https://doi.org/10.11484/jaea-review-2015-022

The role of nitric oxide (NO) in bystander effect was investigated. Human fibroblasts were irradiated with -rays (LET: 0.2 keV/m) or carbon-ion beam (108 keV/m), and then, co-cultured with the non-irradiated cells. After 24 h culture, the survival rates of non-irradiated cells and the concentrations of nitrate, an oxide of NO, in the medium were measured. The survival rates of non-irradiated cells decreased in dose-dependent and radiation quality-independent manners. Negative relationships between survival rates and nitrite concentrations existed, indicating the amounts of produced NO are an important determinant of bystander effects. Next, a reagent producing two molecules of NO in a half-life of 100 min was added in the culture medium. After incubation of 24 h the survival rates of treated cells did not decrease, suggesting NO produced intracellularly has an important role to lead the bystander effect but is not the signal molecule for intercellular communication.

Reconsideration of the period of volcanic activity of Kuroshima Island, and summary of K-Ar age of the volcanic rocks of Nansei shoto off Kyushu

Fukuda, Tetsuya*; Tanase, Atsushi*; Umeda, Koji; Kobayashi, Tetsuo*

Gekkan Chikyu, 37(5), p.197 - 203, 2015/05

no abstracts in English

Effect of ionizing radiation upon dehydrated Pv11 cultured cells originated from the sleeping chironomid

Watanabe, Kazuyo*; Akitsuki, Takashi*; Shimura, Sachiko*; Gusev, O.*; Cornette, R.*; Kikawada, Takahiro*; Sakashita, Tetsuya; Funayama, Tomoo; Kobayashi, Yasuhiko; Okuda, Takashi*

JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 87, 2015/03

https://doi.org/10.11484/jaea-review-2014-050

The Sleeping Chironomid, can stand complete desiccation (anhydrobiosis) and also shows radio-resistance. Recently, we have generated cultured cell (Pv11) originated from embryo which can also stand complete dehydration. In this study, we examine the tolerance of cultured cell Pv11 against ionbeam irradiation.

Bystander effect mediated by nitric oxide depends on irradiation dose but not on radiation quality

Yokota, Yuichiro; Funayama, Tomoo; Ikeda, Hiroko; Sakashita, Tetsuya; Suzuki, Michiyo; Kobayashi, Yasuhiko

JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 75, 2015/03

https://doi.org/10.11484/jaea-review-2014-050

We investigated the bystander effect induced by -rays or carbon ions and analyzed the role of nitric oxide (NO) in the effect. Normal human fibroblasts were used. Cells inoculated on a porous membrane were irradiated with varying doses of -rays or carbon ions. Irradiated cells were then non-contact co-cultured with non-irradiated cells for 24 h. After co-culture, the survival rates of non-irradiated bystander cells co-cultured with irradiated cells decreased with increasing dose and bottomed out at 0.5 Gy or higher doses. This indicates that the bystander effect is dependent on irradiation dose but independent of radiation quality. Next, a specific NO scavenger c-PTIO was added to the culture medium during irradiation and co-culture. This treatment prevented the reduction in survival rates of bystander cells, clearly indicating that NO has an important role in the bystander effect.

Mechanisms for the induction of radioadaptive response by radiation-induced bystander response

Matsumoto, Hideki*; Tomita, Masanori*; Otsuka, Kensuke*; Hatashita, Masanori*; Maeda, Munetoshi*; Funayama, Tomoo; Yokota, Yuichiro; Suzuki, Michiyo; Sakashita, Tetsuya; Ikeda, Hiroko; et al.

JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 76, 2015/03

https://doi.org/10.11484/jaea-review-2014-050

The objective of this project is to elucidate molecular mechanisms for the induction of radioadaptive response through radiation-induced bystander responses induced by irradiation with heavy ion microbeams in JAEA. We found that the adaptive response was induced by Ar (520 MeV Ar) microbeam-irradiation of a limited number of cells, followed by the broad beam-irradiation and that the adaptive response was almost completely suppressed by the addition of carboxy-PTIO, as a nitric oxide (NO) scavenger. In addition, we found several genes induced specifically and preferentially when radioadaptive response could be induced. We confirmed that expression was specifically induced only when radioadaptive response could be induced. Our findings strongly suggested that radioadaptive response can be induced by NO-mediated bystander responses evoked by irradiation with heavy ion microbeams.